New approach to achieve the safety goals in transportation and dry storage of SNF, so called SSEM has been proposed. The main concept of the SSEM is that it simplifies the reviewing processes of each campaign of the transportation or storage of SNF with standard format. This SSEM could be considered as a model case for assuring public that the SNF be managed safely.

Pyroprocessing at KAERI (Korea Atomic Energy Research Institute) consists of pretreatment, electroreduction, electrorefining and electrowinning. SFR (Sodium Fast Reactor) fuel is prepared from the electrowinning process which is composed of LCC (Liquid Cadmium Process) and Cd distillation et al. LCC is an electrochemical process to obtain actinides from spent fuel. In order to recover actinides inert anodes such as carbon material are used, where chlorine gas ($Cl_2$) evolves on the surface of the carbon material. And, stainless steel (SUS) crucible should be installed in large-scale electrowinning system. Therefore, the effect of chlorine on the SUS material needs to be studied. LiCl-KCl-$UCl_3$-$NdCl_3$-$CeCl_3$-$LaCl_3$-$YCl_3$ salt was contained in 2 kinds of electrolytic crucible having an inner diameter of 5cm, made of an insulated alumina and an SUS, respectively. And, three kinds of electrodes such as cathode, anode, reference were used for the electrochemical experiments. Both solid tungsten (W) and LCC were used as cathodes. Cd of 45 g as the cathode material was contained in alumina crucibles for the deposition experiments, where the crucible has an inner diameter of 3 cm. Glassy carbon rod with the diameter of 0.3 cm was employed as an anode, where shroud was not used for the anode. A pyrex tube containing LiCl-KCl-1mol% AgCl and silver (Ag) wire having a diameter of 0.1cm was used as a reference electrode. Electrodeposition experiments were conducted at $500^{\circ}C$ at the current densities of $50{\sim}100mA/cm^2$. In conclusion, Fe ions were produced in the salt during the electrodeposition by the reaction of chlorine evolved from the anode and Fe of the SUS crucible and thereby LCC system using SUS crucible showed very low current efficiencies compared with the system using the insulated alumina crucible. Anode shroud needs to be installed around the glassy carbon not to influence surrounding SUS material.

Electrorefining is a key step in pyroprocessing. The electrorefining process is generally composed of two recovery steps - the deposit of uranium onto a solid cathode and the recovery of the remaining uranium and TRU elements simultaneously by a liquid cadmium cathode. Uranium deposit recovered from the solid cathode is a dendritic powder. It is necessary to separate the adhered salt from the deposits prior to the consolidation of uranium deposit. The adhered salt is composed of lithium, potassium, uranium, and rare earth chlorides. Distillation process was employed for the cathode processing. One of the operation methods is distillation of the salt at low temperature ($900^{\circ}C$), and then melting of the deposit at high temperature to avoid a backward reaction. For the development of the salt distiller, the distillation behavior of the low vapor pressure chlorides should be studied. Rare earth chlorides in the adhered salt of uranium deposits have relatively low vapor pressures compared to the process salt (LiCl-KCl). In this study, the evaporation rates of the lanthanum and neodymium chlorides were measured for the salt separation from electrorefiner uranium deposits in the temperature range of $825{\sim}910^{\circ}C$. The evaporation rate of both chlorides increased with an increasing templerature. The evaporation rate of lanthanum chloride varied from 0.12 to $1.68g/cm^2/h$. Neodymium chloride was more volatile than lanthanum chloride. The evaporation rate of neodymium chloride varied from 0.20 to $4.55g/cm^2/h$. The evaporation rate of both chlorides are more than $1g/cm^2/h$ at $900^{\circ}C$. Even though the evaporation rates of both chlorides were less than that of the process salt, the contents of the lanthanide chlorides were small in the adhered salt. Therefore it can be concluded that $900^{\circ}C$ is suitable for the operation temperature of the salt distiller.

This study, electrolytic behavior of Thulium and Tm-Bi ion system was studied. The electrochemical behavior of Tm was studied in $LiCl-KCl-TmCl_3$ molten salts using electrochemical techniques Cyclic Voltammetry on tungsten electrodes at 773K. During the process of CV and SWV, intermetallic compound were observed Bi-Tm. Further study, in order to determine clarity of diffusion coefficient in this experiment, we will compare result of electrochemistry method and we also need to quantitative research.

In this study, assembling procedure of TRU fuel assembly was reviewed and divided into rod bundle assembling, mating preassemblies and welding, and inspection and non-destructive examination. Based on this assumption, the design criteria of a remote assembler for TRU fuel assembly of PGSFR is defined and predictable technical issues are proposed.

For the safe transportation of SNF and licensing, the integrity of SNF should be evaluated carefully. Researches to obtain the data for SNF cladding properties, i.e. impact toughness, DBTT (hydride behavior) when evaluating transportation of SNF, shall be precisely implemented by simulating the condition of real SNF to the hilt, accordingly.

The spectroscopic reference data for plutonium at different temperatures are necessary information for the chemical speciation and evaluation of thermodynamic data at elevated temperature. This work is the initial step to extend research activities for understanding the plutonium chemistry in aquatic solutions at high temperature. The hydrolysis of Pu(III) and the solubility of Pu(III) hydroxide at the elevated temperature will be discussed.

For the concept design of the device, a tool was made to test the simulated fuel rods and cutting force and the cutting force was measured. When 2-CUT and 3-CUT modules were used, the maximum force in 2-CUT at 12.5 mm/s speed change was $197.5kg_f$ and the maximum force at 3-CUT was $363.2kg_f$. The change of force in 2-CUT rapidly increases from about 1 second, and you can see that there are increase and decrease of the force change from about 5 seconds to 18 seconds, and it was rapidly decreased and the cut was made. The force change in 3-CUT has higher force at about 5 seconds later than 2-CUT at the speed of 12.5 mm/s, and you can see that it has the same tendency afterwards. If you search for the force at adequate speed from this cutting force test, 2-CUT module requires less slitting force than 3-CUT module, and the cutting time for 250 mm at 12.5 mm/s was 21 seconds, which can cut 4 m fuel rod in 5 minutes. But, there are cases of not completely slitting with 2-CUT module, so it is necessary to supplement this in the future through experiments.