• Title/Summary/Keyword: Neutron capture

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Study on the Isomeric Ratio by Thermal Neutron Activation

  • Bak, Hae-Ill
    • Nuclear Engineering and Technology
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    • v.6 no.2
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    • pp.89-96
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    • 1974
  • The cross-section ratios of the nuclear isomeric pairs $^{80}$ B $r^{m, g}$, sup 81/S $e^{m, g}$, $^{104}$ R $h^{m, g}$, $^{116}$ I $n^{m, g}$ and $^{134}$ C $s^{m, g}$ through the radiative thermal neutron capture process have been studied. The experimental values of these ratios obtained by the activation method have been compared with the calculated ones deduced from the modified Huizenga-Vandenbosch method. Agreement between these values within 30% could be attained by controlling the spin cut-off parameter and gamma-ray multiplicity.

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Comprehensive validation of silicon cross sections

  • Czakoj, Tomas;Kostal, Michal;Simon, Jan;Soltes, Jaroslav;Marecek, Martin;Capote, Roberto
    • Nuclear Engineering and Technology
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    • v.52 no.12
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    • pp.2717-2724
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    • 2020
  • Silicon, especially silicon in the form of SiO2, is a major component of rocks. Final spent fuel storages, which are being designed, are located in suitable rock formations in the Earth's crust. Reduction of the uncertainty of silicon neutron scattering and capture is needed; improved silicon evaluations have been recently produced by the ORNL/IAEA collaboration within the INDEN project. This paper deals with the nuclear data validation of that evaluation performed at the LR-0 reactor by means of critical experiments and measurement of reaction rates. Large amounts of silicon were used both as pure crystalline silicon and SiO2 sand. The critical moderator level was measured for various core configurations. Reaction rates were determined in the largest core configuration. Simulations of the experimental setup were performed using the MCNP6.2 code. The obtained results show the improvement in silicon cross-sections in the INDEN evaluations compared to existing evaluations in major libraries. The new Thermal Scattering Law for SiO2 published in ENDF/B-VIII.0 additionally reduces the discrepancy between calculation and experiments. However, an unphysical peak is visible in the neutron spectrum in SiO2 obtained by calculation with the new Thermal Scattering Law.

Identification of Pb-Zn ore under the condition of low count rate detection of slim hole based on PGNAA technology

  • Haolong Huang;Pingkun Cai;Wenbao Jia;Yan Zhang
    • Nuclear Engineering and Technology
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    • v.55 no.5
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    • pp.1708-1717
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    • 2023
  • The grade analysis of lead-zinc ore is the basis for the optimal development and utilization of deposits. In this study, a method combining Prompt Gamma Neutron Activation Analysis (PGNAA) technology and machine learning is proposed for lead-zinc mine borehole logging, which can identify lead-zinc ores of different grades and gangue in the formation, providing real-time grade information qualitatively and semi-quantitatively. Firstly, Monte Carlo simulation is used to obtain a gamma-ray spectrum data set for training and testing machine learning classification algorithms. These spectra are broadened, normalized and separated into inelastic scattering and capture spectra, and then used to fit different classifier models. When the comprehensive grade boundary of high- and low-grade ores is set to 5%, the evaluation metrics calculated by the 5-fold cross-validation show that the SVM (Support Vector Machine), KNN (K-Nearest Neighbor), GNB (Gaussian Naive Bayes) and RF (Random Forest) models can effectively distinguish lead-zinc ore from gangue. At the same time, the GNB model has achieved the optimal accuracy of 91.45% when identifying high- and low-grade ores, and the F1 score for both types of ores is greater than 0.9.

An approach to minimize reactivity penalty of Gd2O3 burnable absorber at the early stage of fuel burnup in Pressurized Water Reactor

  • Nabila, Umme Mahbuba;Sahadath, Md. Hossain;Hossain, Md. Towhid;Reza, Farshid
    • Nuclear Engineering and Technology
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    • v.54 no.9
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    • pp.3516-3525
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    • 2022
  • The high capture cross-section (𝜎c) of Gadolinium (Gd-155 and Gd-157) causes reactivity penalty and swing at the initial stage of fuel burnup in Pressurized Water Reactor (PWR). The present study is concerned with the feasibility of the combination of mixed burnable poison with both low and high 𝜎c as an approach to minimize these effects. Two considered reference designs are fuel assemblies with 24 IBA rods of Gd2O3 and Er2O3 respectively. Models comprise nuclear fuel with a homogeneous mixture of Er2O3, AmO2, SmO2, and HfO2 with Gd2O3 as well as the coating of PaO2 and ZrB2 on the Gd2O3 pellet's outer surface. The infinite multiplication factor was determined and reactivity was calculated considering 3% neutron leakage rate. All models except Er2O3 and SmO2 showed expected results namely higher values of these parameters than the reference design of Gd2O3 at the early burnup period. The highest value was found for the model of PaO2 and Gd2O3 followed by ZrB2 and HfO2. The cycle burnup, discharge burnup, and cycle length for three batch refueling were calculated using Linear Reactivity Model (LRM). The pin power distribution, energy-dependent neutron flux and Fuel Temperature Coefficient (FTC) were also studied. An optimization of model 1 was carried out to investigate effects of different isotopic compositions of Gd2O3 and absorber coating thickness.

Chemical and Kinematic Properties of the Galactic Halo System

  • Jung, Jaehun;Lee, Young Sun;Kim, Young Kwang
    • The Bulletin of The Korean Astronomical Society
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    • v.42 no.2
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    • pp.80.2-80.2
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    • 2017
  • We present chemical and kinematic properties of the Milky Way's halo system investigated by carbon-enhanced metal-poor (CEMP) stars identified from the Sloan Digital Sky Survey. We first map out fractions of CEMP-no stars (those having no over-abundances of neutron-capture elements) and CEMP-s stars (those with over-enhancements of the s-process elements) in the inner- and outer-halo populations, separated by their spatial distribution of carbonicity ([C/Fe]). Among CEMP stars, the CEMP-no and CEMP-s objects are classified by different levels of absolute carbon abundances, A(C). We investigate characteristics of rotation velocity and orbital eccentric for these subclasses for each halo population. Any distinct kinematic features identified between the two categories in each halo region provide important clues on the origin of the dichotomy of the Galactic halo.

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미임계 증배 집합체를 이용한 BNCT용 열외중성자빔의 설계

  • 한치영;김도헌;김종경
    • Proceedings of the Korean Nuclear Society Conference
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    • 1998.05b
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    • pp.746-751
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    • 1998
  • 붕소 중성자 포획 요법(BNCT, Boron Neutron Capture Therapy)용 열외중성자빔의 개발을 위하여 방사성 동위원소인 Cf-252를 중성자 선원으로 사용하였으며 상대적으로 낮은 중성자속을 높이기 위하여 미임계 증배 집합체를 이용하였다. 이전에 계시된 미임계 증배 집합체는 높은 핵연료 농축도를 필요로 하는 단점이 있어 본 연구에서는 이를 감소시키기 위한 몇 가지 설계안을 제시하였다. 중성자빔 설계를 위하여 몬테칼로 방법을 이용한 전산코드인 MCNP를 이용, 타원형두뇌 팬텀 내에서 AD, AR ADDR및 각각의 선량성분 등을 계산함으로써 설계된 중성자빔의 특성분석을 수행하였다. 새롭게 개선되어 제시된 중성자빔의 설계는 상대적으로 낮은 핵연료 농측도를 보이면서 기존의 결과와 유사한 결과를 보여주고 있으며 특히 두뇌 팬텀 내에서의 선량률은 기존에 비해 매우 높은 값을 보임으로써 짧은 시간에 효과적으로 뇌종양을 치료할 수 있는 이 점이 있다.

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Dichotomy of the Galactic Halo as Revealed by Carbon-Enhanced Metal-Poor Giants

  • Jung, Jaehun;Lee, Young Sun;Kim, Young Kwang
    • The Bulletin of The Korean Astronomical Society
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    • v.43 no.1
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    • pp.66.3-67
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    • 2018
  • We present distinct chemical and kinematic properties associated with the inner and outer halos of the Milky Way, as identified by metal-poor stars from the Sloan Digital Sky Survey. In particular, using carbon-enhance metal-poor (CEMP) giants, we first map out the fractions of CEMP-no stars (without strongly enhanced neutron-capture elements) and CEMP-s stars (with a large enhancement of s-process elements) in the inner- and outer-halo populations, separated by their spatial distribution of carbonicity ([C/Fe]). The CEMP-no and CEMP-s objects are classified by their different levels of absolute carbon abundances, A(C). We investigate characteristics of rotational velocity and orbital eccentricity for these sub-classes within the halo populations. Distinct kinematic features and fractions between CEMP-no and CEMP-s stars identified in each halo region will provide important clues on the origin of the dichotomy of the Galactic halo.

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Some Improvements of Gamma-ray Measurement for the Determination of the Boron Content (붕소 함량결정을 위한 즉발 감마선 계측법의 개선)

  • Nak Bae Kim;Hae-Ill Bak
    • Nuclear Engineering and Technology
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    • v.16 no.1
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    • pp.18-20
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    • 1984
  • The detection limit of boron has been lowered further in the capture gamma-ray measurement after preconcentration of boron by placing natural lithium brick in front of Ge(Li) detector. The experimental detection limit is found to be 0.30ppm, 0.18ppm, 0.045ppm and 0.090ppm for the samples of aluminum, steel, uranium dioxide and graphite, respectively. An alternate counting technique kas been also used for neglecting the error caused by the fluctuation of neutron flux during counting.

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Hot Atom Chemistry of Aromatic Halides : Scavenger, Temperature and Oxygen Effect (芳香族할라이드의 Hot Atom Chemistry 스캐벤져, 溫度 및 酸素의 效果)

  • Choi, Jae-Ho;Park, Yong-Chan;Son, Mi-Ja
    • Journal of the Korean Chemical Society
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    • v.9 no.2
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    • pp.78-80
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    • 1965
  • The organic yields(i.e., fraction of nuclear events resulting in organic compound formation) of the radioactive neutron capture reactions of the halogens in purified aromatic halides have been determined in the liquid and solid state, in the presence of scavenger, elemental halogen for thermal atoms, and in the presence of oxygen. Among the important results are; (1) organic yields of the halides are due in part to hot processes and in part to thermal processes; (2) temperature (from liquid state to solid state); (3) the organic yield of chlorobenzene is the same in the solid phase as in the liquid phase whereas the yields of the bromo-and iodobenzene are higher in the solid.

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Boronated Porphyrins and Chlorins as Potential Anticancer Drugs

  • Ol'shevskaya, Valentina A.;Zaytsev, Andrey V.;Savchenko, Arina N.;Shtil, Alexander A.;Cheong, Chan-Seong;Kalinin, Valery N.
    • Bulletin of the Korean Chemical Society
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    • v.28 no.11
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    • pp.1910-1916
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    • 2007
  • Analyzed are recent advances in design of novel boronared conjugates of synthetic and natural porphyrins and chlorins. These compounds showed high efficacy as cytotoxic agents for tumor cells in culture and as phototoxins in photodynamic therapy of tumor xenografts. Thus, boronated porphyrins and chlorins emerge as promising class of anticancer agents with potentially multiple advantages: the chemotherapeutic drugs alone and photo- and radiosensitizers in binary treatments.