• Title/Summary/Keyword: Biomass burning aerosol

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THE APPLICATION OF THE TOMS AEROSOLS RETRIEVAL ALGORITHM TO GLI MEASUREMENTS

  • Lee Hyun Jin;Kim Jae Hwan;Fukushima Hajime;Ha Kyung-Ja
    • Proceedings of the KSRS Conference
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    • 2005.10a
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    • pp.381-384
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    • 2005
  • We have applied the TOMS aerosols retrieval algorithm to GLI measurements. TOMS has utilized the aerosol index, which is a measure of the change in spectral contrast due to the wavelength-dependent effects of aerosols. We have retrieved the GLI aerosol index, which is made by the pair of 380/400nm, 380/412nm, 380/460nm, and 412/460nm. We have found that the biomass burning aerosols represent the absorbing aerosols. In addition, the pair of 380/460nm has shown the best signal for detecting aerosols in Principal Component Analysis(PCA) and comparison of aerosol optical thickness from AERONET data. The theoretical aerosol index is also shown the best signal in the pair of 380/460nm.

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MODIS-estimated Microphysical Properties of Clouds Developed in the Presence of Biomass Burning Aerosols (MODIS 관측자료를 이용한 러시아 산불 영향 하에 발달한 구름의 미세 물리적 특성 연구)

  • Kim, Shin-Young;Sohn, Byung-Ju
    • Korean Journal of Remote Sensing
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    • v.24 no.4
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    • pp.289-298
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    • 2008
  • An algorithm was developed to retrieve both cloud optical thickness and effective particle radius considered the aerosol effect on clouds. This study apply the algorithm of Nakajima and Nakajima (1995) that is used to retrieve cloud optical thickness and effective particle radius from visible, near infrared satellite spectral measurements. To retrieve cloud properties, Look-up table (LUT) was made under different atmospheric conditions by using a radiative transfer model. Especially the vertical distribution of aerosol is based on a tropospheric aerosol profile in radiative transfer model. In the case study, we selected the extensive forest fire occurred in Russia in May 2003. The aerosol released from this fire may be transported to Korea. Cloud properties obtained from these distinct atmospheric situations are analysed in terms of their possible changes due to the interactions of the clouds with the aerosol particle plumes. Cloud properties over the East sea at this time was retrieved using new algorithm. The algorithm is applied to measurements from the MODerate Resolution Imaging Spectrometer (MODIS) onboard the Terra spacecrafts. As a result, cloud effective particle radius was decreased and cloud optical thickness was increased during aerosol event. Specially, cloud effective particle radius is hardly greater than $20{\mu}m$ when aerosol particles were present over the East Sea. Clouds developing in the aerosol event tend to have more numerous but smaller droplets.

Characteristic of Size-Resolved Water-Soluble Organic Carbon in Atmospheric Aerosol Particles Observed during Daytime and Nighttime in an Urban Area (도시지역 낮.밤 대기에어로졸의 입경 별 수용성 유기탄소의 특성)

  • Park, Seung Shik;Shin, Dong Myung
    • Particle and aerosol research
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    • v.9 no.1
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    • pp.7-21
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    • 2013
  • Twelve-hour size-resolved atmospheric aerosols were measured to determine size distributions of water-soluble organic carbon(WSOC) during daytime and nighttime, and to investigate sources and formation pathways of WSOC in individual particle size classes. Mass, WSOC, ${NO_3}^-$, $K^+$, and $Cl^-$ at day and night showed mostly bimodal size distributions, peaking at the size range of $0.32-0.55{\mu}m$(condensation mode) and $3.1-6.2{\mu}m$(coarse mode), respectively, with a predominant condensation mode and a minor coarse mode. While ${NH_4}^+$ and ${SO_4}^{2-}$ showed unimodal size distributions which peaked between 0.32 and $0.55{\mu}m$. WSOC was enriched into nuclei mode particles(< $0.1{\mu}m$) based on the WSOC-to-mass and WSOC-to-water soluble species ratios. The sources and formation mechanisms of WSOC were inferred in reference to the size distribution characteristics of inorganic species(${SO_4}^{2-}$, ${NO_3}^-$, $K^+$, $Ca^{2+}$, $Na^+$, and $Cl^-$) and carbon monoxide. Nuclei mode WSOC was likely associated with primary combustion sources during daytime and nighttime. Among significant sources contributing to the condensation mode WSOC were homogeneous gas-phase oxidation of VOCs, primary combustion emissions, and fresh(or slightly aged) biomass burning aerosols. The droplet mode WSOC could be attributed to aqueous oxidation of VOCs in clouds, cloud-processed biomass burning aerosols, and small contributions from primary combustion sources. From the correlations between WSOC and soil-related particles, and between WSOC and sea-salt particles, it is suggested that the coarse mode WSOC during daytime is likely to condense on the soil-related particles($K^+$ and $Ca^{2+}$), while the WSOC in the coarse fraction during nighttime is likely associated with the sea-salt particles($Na^+$).

The variation of aerosol optical depth over the polar stations of Korea (남북극 과학기지에서의 에어로졸 광학 깊이 변동성)

  • Koo, Ja-Ho;Choi, Taejin;Cho, Yeseul;Lee, Hana;Kim, Jaemin;Ahn, Dha Hyun;Kim, Jhoon;Lee, Yun Gon
    • Particle and aerosol research
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    • v.13 no.4
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    • pp.141-150
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    • 2017
  • Using the NASA's Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis for aerosol optical depth (AOD) and satellite-observed carbon monoxide (CO) data, we examined the basic pattern of AOD variations over the three polar stations of Korea: Jangbogo and King Sejong stations in the Antarctica, and Dasan station in the Arctic area. AOD values at King Sejong and Dasan station show the maximum peaks in spring, which looks associated with the high amount of atmospheric CO emitted from the natural burning and the biomass burning. Jangbogo station shows the much less AOD compared to other two stations, and seems not strongly affected by the transport of airborne particles generated from mid-latitude regions. All three polar stations show the AOD increasing trend in general, indicating that the polar background air quality becomes polluted.

Particle-size-dependent aging time scale of atmospheric black carbon (입자 크기의 함수로 나타낸 대기 중 블랙카본의 변성시간척도)

  • Park, Sung Hoon
    • Particle and aerosol research
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    • v.5 no.2
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    • pp.45-52
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    • 2009
  • Black carbon, which is a by-product of combustion of fossil fuel and biomass burning, is the component that imposes the largest uncertainty on quantifying aerosol climate effect. The direct, indirect and semi-direct climate effects of black carbon depend on its state of the mixing with other water-soluble aerosol components. The process that transforms hydrophobic externally mixed black carbon particles into hygroscopic internally mixed ones is called "aging". In most climate models, simple parameterizations for the aging time scale are used instead of solving detailed dynamics equations on the aging process due to the computation cost. In this study, a new parameterization for the black carbon aging time scale due to condensation and coagulation is presented as a function of the concentration of hygroscopic atmospheric components and the black carbon particle size. It is shown that the black carbon aging time scale due to condensation of sulfuric acid vapors varies to a large extent depending on the sulfuric acid concentration and the black carbon particle size. This result indicates that the constant aging time scale values suggested in the literature cannot be directly applied to a global scale modeling. The aging time scale due to coagulation with internally mixed aerosol particles shows an even stronger dependency on particle size, which implies that the use of a particle-size-independent aging time scale may lead to a large error when the aging is dominated by coagulation.

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Characterization of fine organic aerosols from biomass burning emissions using FTIR method (분광학적 방법을 이용한 바이오매스 연소 배출 유기 입자의 화학적 특성)

  • Son, Se-Chang;Park, Tae-Eon;Park, Seungshik
    • Particle and aerosol research
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    • v.17 no.4
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    • pp.125-132
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    • 2021
  • Fresh PM2.5 smokes emitted from combustion of four biomass materials (pellet, palm fruit fiber (PFF), PKS, and sawdust) in a laboratory-controlled environment were characterized using an attenuated total reflectance-fourier transform infrared (ATR-FTIR) technique. In smoke samples emitted from combustion of pellets, PFF and PKS, which is being used as boiler fuels for greenhouses in rural areas, the organic carbon/elemental carbon (OC/EC) ratios in PM2.5 were very high (14.0-35.5), whereas in sawdust smoke samples they were significantly low (<4.0) due to the combustion method close to flaming combustion. ATR-FTIR analysis showed that OH(3400-3250 cm-1), CH3(2958-2840 cm-1), CH2(2910 cm-1 and 2850 cm-1), ketone(1726-1697 cm-1), C=C(1607-1606 cm-1 and 1515-1514 cm-1), lignin (1463-1462 cm-1 and 1430-1428 cm-1) and -NO2(1360-1370 cm-1) peaks were identified in all biomass burning (BB) smoke samples. However, additional peaks appeared depending on the type of biomass. Among the four types of biomass materials, an additional peak of the methylene group CH3(2872-2870 cm-1) appeared only in PFF and PKS smoke samples, and a peak of C=O(1685 cm-1) was also confirmed. And in the case of PKS smoke samples, a peak of aromatic C=C(1593 cm-1 and 1476 cm-1) that did not appear in other BB samples was also observed. This indicates that the molecular structure of organic compounds emitted during BB differs depending on the type of biomass materials. The results of this study are expected to provide valuable information to more specifically reveal the effect of BB on PM2.5 collected in the atmospheric environment.

Using Unmanned Aerial Vehicles (UAVs) to Study on the Climate Impacts of the Atmospheric Brown Clouds (무인항공기를 이용한 대기갈색연무의 기후효과 연구)

  • Kim, Sang-Woo;Yoon, Soon-Chang
    • Atmosphere
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    • v.20 no.4
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    • pp.519-530
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    • 2010
  • In this paper we review current research on Atmospheric Brown Clouds (ABCs) with lightweight Unmanned Aerial Vehicles (UAVs) and miniaturized instruments. The UAV technology for in-situ measurements, including aerosol concentration, aerosol size distribution, aerosol absorption, cloud drop size distribution, solar radiation fluxes (visible and broadband), and spectral radiative fluxes, is a leading-edge technology for cost-effective atmospheric sounding, which can fill the gap between the ground measurement and satellite observation. The first experimental observation with UAVs in Korea, Cheju ABC Plume Monsoon Experiment (CAPMEX), conducted during summer 2008 revealed that the Beijing plumes exerted a strong positive influence on the net warming and fossil-fuel-dominated black-carbon plumes were approximately 100% more efficient warming agents than biomass-burning-dominated plumes. Long-term sustainable routine UAV measurements will eventually provide truly three-dimensional data of ABCs, which is necessary for the better understanding of their climate impacts and for the improvement of numerical models for air pollution, weather forecast and climate change.

A Study on the PM2.5 Source Characteristics Affecting the Seoul Area Using a Chemical Mass Balance Receptor Model (수용모델을 이용한 서울지역 미세입자 (PM2.5)에 영향을 미치는 배출원 특성에 관한 연구)

  • Lee Hak Sung;Kang Choong-Min;Kang Byung-Wook;Lee Sang-Kwun
    • Journal of Korean Society for Atmospheric Environment
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    • v.21 no.3
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    • pp.329-341
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    • 2005
  • The purpose of this study is to study the $PM_{2.5}$ source characteristics affecting the Seoul area using a chemical mass balance (CMB) receptor model. This study was also to evaluate the $PM_{2.5}$ source profiles, which were directly measured and developed. Asian Dust Storm usually occurred in the spring, and very high $PM_{2.5}$ concentrations were observed in the fall among the sampling periods. So the ambient data collected in the spring and fall were evaluated. The CMB model results as well as the $PM_{2.5}$ source profiles were validated using the diagnostic categories, such as: source contribution estimate, t-statistic, R-square, Chi-square, and percent of total mass explained. In the spring months, the magnitude of $PM_{2.5}$ mass contributors was in the following order: Chinese aerosol $(31.7\%)>$ secondary aerosols ($22.3\%$: ammonium sulfate $13.4\%$ and ammonium nitrate $8.9\%)>$ vehicles ($16.1\%$: gasoline vehicle $1.4\%$ and diesel vehicles $14.7\%)>$biomass burning $(15.5\%)>$ geological material $(10.5\%)$. In the fall months, the general trend of the $PM_{2.5}$ mass contributors was the following: biomass burning $(31.1\%)>$ vehicles ($26.9\%$: gasoline vehicle $5.1\%$ and diesel vehicles $21.8\%)>$ secondary aerosols ($23.0\%$: ammonium sulfate $9.1\%$ and ammonium nitrate $13.9\%)>$ Chinese aerosol $(10.7\%)$. The results show that the $PM_{2.5}$ mass in the Seoul area was mainly affected by the Chinese area.

Estimation of major sources of Polycyclic Aromatic Hydrocarbons (PAHs) in Seoul by using the receptor models (수용 모델을 이용한 서울시의 PAHs 주요 배출원 추정)

  • Han, Sang Hee;Lee, Ji Yi;Kim, Yong Pyo
    • Particle and aerosol research
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    • v.12 no.2
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    • pp.27-36
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    • 2016
  • The PMF result was compared with the result from the Chemical Mass Balance (CMB) modelling (Lee and Kim, 2007) to estimate major source of PAHs observed at Seoul from August 2002 to December 2003. Five major sources were estimated from PMF and CMB modellings respectively. Among them three major sources (coal combustion for residential, coke oven and biomass burning) were identified at both models.

Spatial Analysis of Major Atmospheric Aerosol Species Using Earth Observing Satellite Data (지구관측 위성자료를 이용한 주요 대기 에어러솔 성분의 공간분포 분석)

  • Lee, Kwon-Ho
    • Journal of the Korean Association of Geographic Information Studies
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    • v.14 no.2
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    • pp.109-127
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    • 2011
  • Atmospheric aerosols, small particles in the atmosphere, are one of the important parameters in climate change and human health. Additionally, accurate estimates of aerosol species are increasingly important in environmental impact assessment studies. Recent advances in global satellite remote sensing provide powerful tool for air quality monitoring. This study explores the potential usage of satellite derived data such as atmospheric aerosols for air quality monitoring as well as climate change study. The objectives of this study is to understand the general features of the global distribution of type dependent aerosols. A detailed spatio-temporal variability of the each different satellite dataset shows the variation of the global zonal average and specific geographical regions where the strong emission sources are located. Especially, significantly large aerosol amounts are observed in Asia and Africa because of the desert dust storm, anthropogenic and biomass burning emissions.