• Title/Summary/Keyword: Atmospheric deposition

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Assessing the Impact of Locally Produced Aerosol on the Rainwater Composition at the Gosan Background Site in East Asia

  • Han, Yeongcheol;Huh, Youngsook
    • Asian Journal of Atmospheric Environment
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    • v.8 no.2
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    • pp.69-80
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    • 2014
  • It is often assumed that atmospheric observations at remote sites represent long-range transport of airborne material, and local influences are overlooked. We evaluated the impact of local input on the rainwater composition at Gosan Station, a strategic site for monitoring the continental outflow from Asia. We analyzed a 14-year record of rainwater chemical composition archived by the Korea Meteorological Administration and detected local terrestrial contribution for nitrate, sulfate and ammonium. We also measured the chemical composition of rainwater sampled simultaneously at multiple locations within the premises of the Gosan Station, from which local influence with meter-scale spatial heterogeneity could be discerned. We estimate that the local input accounted for at least ~10% of the wet deposition of nitrogen and ~12% of the wet deposition of sulfur during the 14 years. This highlights the significance of the local influence, which should be carefully assessed when interpreting atmospheric observations at this site.

Measurement of Nitrogen and Sulfur Deposition to Lake Paldang (팔당호로의 질소와 황성분 침적 측정)

  • Ghim Young Sung;Jin Hyoun Cheol
    • Journal of Korean Society for Atmospheric Environment
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    • v.21 no.1
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    • pp.39-48
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    • 2005
  • Nitrogen and sulfur deposition was measured on Lake Pal dang from March 2002 to October 2003. Wet and dry depositions were separately measured using wet- and dry-only samplers, respectively. In order to measure the dry deposition to the water body, a dry deposition sampler composed of three pans filled with pure water, called the deposition water, was used. Since ammonium was generally in excess in ambient air, more than half of ammonium was present in the gaseous form. Ammonium concentration was also generally higher than the sum of major anion concentrations in the deposition water because gaseous species were much easily deposited than the species in fine particles. Nevertheless, the contribution of gaseous ammonia to the deposition of ammonium was not high as well as that of particulate ammonium while the contribution of gaseous nitric acid was much higher than that of particulate nitrate. Annual wet deposition fluxes of nitrogen and sulfur were five and six times higher than their dry deposition fluxes, respectively. Except for ammonium, the dry deposition flux estimated in the present work was a half of the previous results. This was mainly caused by much smaller dry deposition velocities over the water than over the ground.

A Simulation for Dry Depositon Velocity of Air Pollutants over various surfaces. (지표 부근에서의 대기오염물질 건성 침적속도에 관한 모수화)

  • 이화운;박종길
    • Journal of Environmental Science International
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    • v.3 no.4
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    • pp.367-372
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    • 1994
  • A predictive model is demonstrated for gas removal rates from the aklosphere by dw deposition. Typical deposition velocities are complex functions of surface types, atmospheric stabilities, friction velocities, air pollutants, and so on. In this paper we simulated the calculation of dry deposition velocities near the earth surfaces, simultaneously we estimated real dry deposition velocities using the previous simulation. The measurement taken over a deciduous forest by Padro et d.(1988) were used to verify this model. In the comparison of the value of deposition velocity between numerical computation and observation, there are partially overestimations and underestimations between them, but we can speak that they are in a good accordance.

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Effects of the Block Distance of Collecting Plate and Particle Size on the particle Deposition Efficiency in the Two-Stage Electrostatic Precipitator (2단식 전기집진기의 집진판 블록간격 및 입자크기가 입자의 부착효율에 미치는 영향)

  • 박청연
    • Journal of Korean Society for Atmospheric Environment
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    • v.16 no.2
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    • pp.165-178
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    • 2000
  • In this study the effects of block distance have been investigated on the particle deposition efficiency in the collecting cell of two-stage electrostatic precipitator by numerical analysis. Particle trajectories have been changed by the electrostatic and inertial force of particle with the inlet velocity electrostatic number and particle diameter. The total deposition efficiency has a minimum value by the interaction between the effect of particle inertial force and electrostatic force in the collecting cell. The increase of block distance makes the total deposition efficiency decrease under the range of the particle size which has the minimum deposition efficiency. However beyond the range of particle size which has minimum deposition efficiency total deposition efficiency has no trend with the variation of block distance.

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3-D Numerical Prediction Modeling of Air Pollution in Coastal Urban Region -(I) An Effect Prediction for Deposition Phenomenon affecting on Air Quality (연안도시지역에서 대기오염의 3차원 수치예측모델링 -(I) 침적현상이 대기질에 미치는 영향예측)

  • 원경미;이화운
    • Journal of Korean Society for Atmospheric Environment
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    • v.15 no.5
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    • pp.625-638
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    • 1999
  • Air quality modeling for coastal urban region has been composed of a complex system including meteorological, chemical and physical processes and emission characteristics in complex terrain. In this study, we studied about an effect prediction for deposition phenomenon affecting on air quality in Pusan metopolitan metropolitan city. In air quality modeling including ship sources, a situation considered deposition process habe better result than not considered when compared with observed value. Air pollutants emitted into urban air during the daytime nearly removed through urban atmosphere polluted. Also these phenomena correlated concentration variation connent with sea/land breezes and terrain effect. Therefore we conclude that the concentration was low at daytime when deposition flux is high, and deposition effect on industrial complex and Dongrae region is considerable in particular.

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A Study on the Quantitative Analysis of SO$_2$ Dry Deposition in the Northeastern Asia (동북아 지역에서의 SO$_2$ 건성 침적에 관한 정량분석)

  • 홍민선;김순태;이동섭
    • Journal of Korean Society for Atmospheric Environment
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    • v.13 no.3
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    • pp.231-241
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    • 1997
  • A tracer model was applied in the Far East Asia to investigate the dry deposition rates of air pollutants on Korean Peninsula originated from different countries including China and Japan. Wind direction was chosen to predict the maximum deposition rates and SO$_2$ was chosen as a tracer to estimate the source strength. Model simulation shows that inflow, deposition and airborne ratios of China-originated SO$_2$ were 50%, 8% and 30%, respectively, at most. Also it was found that deposition, outbounded and airborne ratios of Korea-originated SO$_2$ were 15~77%, 8~75%, and 3~30%, respectively Model simulation also shows that inflow, deposition and airborne ratios of Kyushu-originated SO$_2$ were, 30~45%, 8~14% and 20~25%, respectively. This study shows that tracer model can be applied on the estimation of air pollutants partitioning in regional scale and that more sophisticated modules and schemes can be developed and applied to better predict the transboundary amounts of air pollutants in this region.

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Addition Effect of the Deposition and Buoyancy Terms in Modeling Turbulence Diffusion of Hazardous Air Pollutants (유해 대기오염물질의 난류확산 수치모의에서 침적한과 부력항 추가에 따른 효과)

  • Won, Gyeong-Mee;Lee, Hwa-Woon;Ji, Hyo-Eun;Kim, Cheol-Hee;Song, Chang-Keun
    • Journal of Korean Society for Atmospheric Environment
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    • v.22 no.1
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    • pp.73-84
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    • 2006
  • Hazardous Air Pollutants (HAPs) are characterized by being relatively heavier and denser than that of ambient air due to the various reasons such as higher molecular weight, low temperature and other complicated chemical transformations (Witlox, 1994). In an effort to investigate transport and diffusion from instantaneous emission of heavy gas, Lagrangian Particle Dispersion Model (LPDM) coupled with the RAMS output was employed. Both deposition process and buoyancy term were added on the atmospheric diffusion equations of LPDM, and the locations and concentrations of dense gas particle released from instantaneous single point source (emitting initially for 10 minutes only) were analyzed. The result overall shows that adding deposition process and buoyancy terms on the diffusion equation of LPDM has very small but detectable effect on the vertical and horizontal distribution of Lagrangian particles that especially transported for a fairly long traveling time. Also the slumping of dense gas can be found to be ignored horizontally compared to the advection by the horizontal wind suggesting that it was essential to couple the Lagrangian particle dispersion model coupled with the RAMS model in order to explain the dispersion of HAPs more accurately. However, during the initial time of instantaneous emission, buoyancy term play an important role on the vertical locations of dense particles for near surface atmosphere and around source area, indicating the importance of densities of HAPs in the beginning stage or short duration for the risk assessment of HAPs or management of heavy vapors during the explosive accidents.

Estimation of Dry Deposition in Urban Area, 2005 (2005년 도시지역의 건성침적량 산정에 관한 연구)

  • Shin S.A.;Han J.S.;Lee S.D.;Choi J.S.
    • Journal of Korean Society for Atmospheric Environment
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    • v.22 no.4
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    • pp.477-486
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    • 2006
  • Dry deposition fluxes for $SO_2$, particulate sulfate, nitrate, ammonium and $HNO_3$ were estimated in urban area for the time period January$\sim$ October 2005. Fluxes were generated using atmospheric concentration data collected both in Acid Deposition and Air Quality Monitoring Networks, and deposition velocities computed by combining land-use data with meteorological information. The resulting annually averaged $SO_2$, $NO_3$, and aerosol deposition velocities were found to be 0.4 cm/s, 4.3 cm/s and 0.1 cm/s, respectively, and thus deposition rates were 4.4 mg/$m^2$. day for $SO_2$, and 5.4 mg/$m^2$ . day for $NHO_3$, and particulate sulfate, ammonium and nitrate recorded 1.0 mg/$m^2$ . day, 0.4 mg/$m^2$ . day and 0.4 mg/$m^2$ day, respectively. Maximum for in seasonal variation of monthly averaged deposition velocities occurred in summer in contrast to $HNO_3$ showing peak in spring. There was no significant variation for aerosol. The dry to total (wet and dry) deposition contributed about 40% for sulfur and 28% for nitrogen species in this study.

A Study on the Atmospheric Deposition of Radionuclides($^137Cs$ and $^210Pb$) on the Korean Peninsula (대기를 통하여 한반도 지표면으로 공급되는 방사성 핵종( $^137Cs$$^210Pb$)에 관한 연구)

  • 이윤구;김석현;홍기훈;이광우
    • Journal of Korean Society for Atmospheric Environment
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    • v.11 no.4
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    • pp.351-359
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    • 1995
  • In order to investigate geochemical behaviors of artificial radionuclide($^{137}$ Cs), the fallout deposition of arificial radioisotope($^{137}$ Cs) was measured from May to October in 1994 at the Korea Ocean Research & Development Institute(KORDI), Ansan, Kyunggido, Korea. And to study radioisotopic behavior and cumulative action in soil, soil samples were collected from Kwang-Leung Forest, Kyunggidom and artificial radioisotope ($^{137}$ Cs) and natural radioisotope($^{210}$ Pb) were identified. The amount of $^{137}$ Cs in atmosphere collected by wet deposition process in May was found to be 4.95 to 11.96mBq m$^{-2}$ whereas the amounts of $^{137}$ Cs by dry deposition process in May and October were found to be 4.0mBq g$^{-1}$ and 3.0mBq g$^{-1}$ , respectively. The amount of $^{137}$ Cs accumulated in soil was measured to be 311mBq cm$^{-2}$ , which contained 83% of the total inputs from atmospheric fallout (374 mBq cm$^{-2}$ ) since 1960s. In addition, the accumulation rate and the annual flux of $^{210}$ Pb into soils were 0.32cm yr$^{-1}$ and 34 mBq cm$^{-2}$ yr$^{-1}$ , respectively. Conclusively, it was found that arificial radioisotopes were mainly from the stratosphere and soil resupension of continental China through the troposphere.

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Measurement of Dry Deposition Flux of Air Pollutants to the Waterbody (수체로의 대기오염물질 건식침적량 측정)

  • 김영성;진현철;김용표
    • Journal of Korean Society for Atmospheric Environment
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    • v.20 no.3
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    • pp.421-426
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    • 2004
  • Dry deposition fluxes of inorganic acidic species to the waterbody were measured by the dry deposition sampler (DDS). DDS was composed of three pans filled with pure water. An average concentration increase during the sampling time, after removing an abnormal value if existed, was considered as the input by deposition. Important operation parameters such as the amount of water used and sampling time were determined through a series of laboratory experiments. The deposition flux measured by DDS was compared with that by the water surface sampler developed by Yi et ai. (1997a,b).