• Title/Summary/Keyword: $^{137}Cs$ radionuclide

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Sorption and Migration Studies of Fission Products for Ground Waste Disposal

  • Lee, Sang-Hoon;Chun, Kwan-Sik;Yoon, Young-Ku
    • Nuclear Engineering and Technology
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    • v.10 no.3
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    • pp.153-163
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    • 1978
  • The problems of solid waste disposal into the ground in connection with environmental aspects in the vicinity of a site would be very significant, though ground disposal for solid waste is safe and economical method. Studies of the waste-movement and migration of radionuclides (Sr-90 and Cs-137) for the disposal into the ground were performed under laboratory and field conditions. Affinity of the soils for radionuclide solution was higher than that in the acid solution. The sorption of radionuclides by the soils showed a time-dependent reation. The migration rates of radiostrontium and radiocesium were a range of 3.73$\times$10$^{-3}$ to 10.9$\times$10$^{-3}$ cm/day. The nuclides in the soil migrate much more slowly than the water, probably due to its high exchange capacity. The observed distribution of tritium was compared with that calculated by a mathematical model based on diffusivity. This study suggests that the tritiated water can be used to trace the movement of ground water.

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Assessment of radionuclides from coal-fired brick kilns on the outskirts of Dhaka city and the consequent hazards on human health and the environment

  • M.M. Mahfuz Siraz;M.D.A. Rakib;M.S. Alam;Jubair Al Mahmud;Md Bazlar Rashid;Mayeen Uddin Khandaker;Md. Shafiqul Islam;S. Yeasmin
    • Nuclear Engineering and Technology
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    • v.55 no.8
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    • pp.2802-2811
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    • 2023
  • In a first-of-its-kind study, terrestrial radionuclide concentrations were measured in 35 topsoil samples from the outskirts of Dhaka using HPGe gamma-ray spectrometry to assess the radiological consequences of such a vast number of brick kilns on the plant workers, general as well as dwelling environment. The range of activity concentrations of 226Ra, 232Th, and 40K is found at 19 ± 3.04 to 38 ± 4.94, 39 ± 5.85 to 57 ± 7.41, and (430 ± 51.60 to 570 ± 68.40) Bq/kg, respectively. 232Th and 40K concentrations were higher than the global averages. Bottom ash deposition in lowlands, fly ash buildup in soils, and the fallout of micro-particles are all probable causes of the elevated radioactivity levels. 137Cs was found in the sample, which indicates the migration of 137Cs from nuclear accidents or nuclear fallout, or the contamination of feed coal. Although the effective dose received by the general public was below the recommended dose limit but, most estimates of hazard parameters surpass their respective population weighted global averages, indicating that brick kiln workers and nearby residents are not safe due to prolonged exposures to terrestrial radiation. In addition, the soil around sampling sites is found to be unsuitable for agricultural purposes.

Radionuclide identification based on energy-weighted algorithm and machine learning applied to a multi-array plastic scintillator

  • Hyun Cheol Lee ;Bon Tack Koo ;Ju Young Jeon ;Bo-Wi Cheon ;Do Hyeon Yoo ;Heejun Chung;Chul Hee Min
    • Nuclear Engineering and Technology
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    • v.55 no.10
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    • pp.3907-3912
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    • 2023
  • Radiation portal monitors (RPMs) installed at airports and harbors to prevent illicit trafficking of radioactive materials generally use large plastic scintillators. However, their energy resolution is poor and radionuclide identification is nearly unfeasible. In this study, to improve isotope identification, a RPM system based on a multi-array plastic scintillator and convolutional neural network (CNN) was evaluated by measuring the spectra of radioactive sources. A multi-array plastic scintillator comprising an assembly of 14 hexagonal scintillators was fabricated within an area of 50 × 100 cm2. The energy spectra of 137Cs, 60Co, 226Ra, and 4K (KCl) were measured at speeds of 10-30 km/h, respectively, and an energy-weighted algorithm was applied. For the CNN, 700 and 300 spectral images were used as training and testing images, respectively. Compared to the conventional plastic scintillator, the multi-arrayed detector showed a high collection probability of the optical photons generated inside. A Compton maximum peak was observed for four moving radiation sources, and the CNN-based classification results showed that at least 70% was discriminated. Under the speed condition, the spectral fluctuations were higher than those under dwelling condition. However, the machine learning results demonstrated that a considerably high level of nuclide discrimination was possible under source movement conditions.

Contaminative Influence of Beef Due to the Inhalation of Air and the Ingestion of Soil of Livestock from an Acute Release of Radioactive Materials (원자력시설의 사고시 가축의 공기 흡입과 토양 섭취가 육류의 방사능 요염에 미치는 영향)

  • 황원태;김은한;서경석;정효준;한문희
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.2 no.3
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    • pp.181-188
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    • 2004
  • The contaminative influence of beef due to the inhalation of air and the ingestion of soil of livestock, both of which are dealt with as minor contaminative pathways in most radioecological models but may not be neglected, was comprehensively investigated with the improvement of the Korean food chain model DYNACON. As the results, it was found that both pathways can not be neglected at all in the contamination of beef in the case of an accidental release during the non-grazing period of livestock. The ingestion of soil was more influential in the contamination of beef than the inhalation of air over most time following an release. If precipitation is encountered during an accidental release, contaminative influence due to the ingestion of soil was far greater compared with the cases of no precipitation. This fact was more distinct for a long-lived radionuclide $^{l37}Cs$ than a short-lived radionuclide $^{131}I$ (elemental iodine). Compared with the results for milk performed prior to this study, the contaminative pathways due to the inhalation of air and the ingestion of soil were more important in beef because of longer biological half-lives. On the other hand, in the case of an accidental release during the grazing period of livestock, radioactive contamination due to the ingestion of pasture was dominant irrespective of the existence of precipitation during an accidental release. It means that contaminative influence due to the inhalation of air and the ingestion of soil is negligible, like the cases of milk.

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An Analysis of Domestic Experimental Results for Soil-to-Crops Transfer Factors of Radionuclides (주요 핵종의 토양-작물체 전이 계수의 국내 실험 결과에 대한 분석)

  • Jun, In;Choi, Young-Ho;Keum, Dong-Kwon;Kang, Hee-Seok;Lee, Han-Soo;Lee, Chang-Woo
    • Journal of Radiation Protection and Research
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    • v.31 no.4
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    • pp.211-217
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    • 2006
  • For more realistic assessment of Korean food chain radiation doses due to the operation of nuclear facilities, it is required to use domestically produced data for radionuclide transfer parameters in crop plants. This paper analyzed results of last about 10 year's studies on radionuclide transfer parameters in major crop plants by the Korean Atomic Energy Research Institute, comparing with the published international data, and consequently suggested the proper parameters to use. The trends of transfer parameter shows normal distributions if we have a lot of experimental data, but some radionuclides showed enormous variations with the environment of experimental, crops and soils. These transfer factors can be used to assess realistic radiation doses or to predict the doses in crops for normal operation or accidental release. Some kinds of parameter can be produced as conservatives or fragmentary results because soil-to-plant transfer factors were measured through greenhouse experiments which sometimes showed improper field situations. But these parameters mentioned in this paper can be representative of the status of Korean food chain than that of foreign country.

Improvement of a Dynamic Food Chain Model Considering the Influence of Radioactive Contamination of Foods by Rainfall During a Nuclear Emergency (원자력 사고 중 강우에 의한 음식물 오염영향을 고려한 역동학적 섭식경로모델 개선)

  • Hwang, Won-Tae;Kim, Eun-Han;Han, Moon-Hec;Choi, Yong-Ho;Lee, Han-Soo;Lee, Chang-Woo
    • Journal of Radiation Protection and Research
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    • v.27 no.1
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    • pp.21-26
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    • 2002
  • For the consideration of the influence on radioactive contamination of foods due to rain during the release period of radionuclides in a nuclear accident, the previous dynamic food chain model was improved. Wet interception coefficients for the agricultural plants were derived as a function of radionuclide and rainfall amount, and mathematical formula of the model was also re-established. In the results for the same time-integrated radioactive concentrations on the ground, radioactive contamination of foods decreased greatly by rainfall, and it decreased dramatically according to increasing rainfall amount. It means that predictive contamination in foods using the previous dynamic food chain model, in which dry interception to the agricultural plants is only considered, can be overestimated. Among radionuclides considering in this study ($^{137}Cs,\;^{90}Sr,\;^{131}I$), influence of rainfall for food contamination was the most sensitive to $^{131}I$, and the least sensitive to $^{90}Sr$.

A Methodology for Determining the Optimal Durations of the Use of Contaminated Crops As Feedstuffs of Cattle Following a Nuclear Accident (원자력 사고후 가축 사료로서 오염 농작물 이용에 대한 최적기간 결정 방법론)

  • Hwang, Won-Tae;Han, Moon-Hee;Choi, Yong-Ho;Cho, Gyu-Seong
    • Journal of Radiation Protection and Research
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    • v.24 no.2
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    • pp.65-72
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    • 1999
  • A methodology for determining the optimal durations of the use of contaminated crops as feedstuffs of cattle was designed based on the cost-benefit analysis method. The results of application for pigs, an omnivorous cattle, were discussed for the hypothetical deposition of radionuclides on August 15 when a number of crops are fully developed in Korean agricultural conditions. For investigating the relative cost-effectiveness of the use of contaminated crops as feedstuffs, the net benefit was compared with the case of the direct disposal of contaminated crops. The time-dependent radionuclide concentration in crops after the deposition was predicted using a dynamic food chain model DYNACON. The net benefit from the actions was quantitatively evaluated in terms of cost equivalent of doses and monetary costs of implementing the action. It depended on a number of factors such as radionuclides, variety of crops supplied as feedstuffs and duration of the actions. The use of contaminated crops as feedstuffs was more cost effective for $^{90}Sr\;or\;^{131}I$ deposition than for $^{137}Cs$ deposition.

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Improvement on the KFOOD Code for More Realistic Assessment of the Annual Food Chain Radiation Dose Due to Operating Nuclear Facilities (가동중 원자력 시설에 의한 년간 섭식경로 피폭선량 평가의 현실성 제고를 위한 KFOOD 코드의 개선)

  • Park, Yong-Ho;Lee, Chang-Woo;Kim, Jin-Kyu;Lee, Myung-Ho;Lee, Jeong-Ho
    • Nuclear Engineering and Technology
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    • v.25 no.3
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    • pp.437-446
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    • 1993
  • More realistic calculation models for evaluating man's annual intakes of radionuclides released from operating nuclear facilities were established. For the application of these models, the harvest years of food and feed crops consumed in the year of dose assessment and every year's average concentrations of a radionuclide in air and in water for the whole period of real operation had to be taken into account. KFOOD, an existing equilibrium food chain computer code for the Korean dose assessment, was modified according to the models. Sample runs of the modified code on the assumption of a constant release during 10 years' operation were made with three kinds of the input data files enabling the dose assessment in the improved method, the KFOOD method and another existing method, respectively, and the results were compared. Annual committed effective doses to Korean adult by intakes of Mn-54, Co-60, Sr-90, I-131 and Cs-137 calculated in the improved method were about 11, 2, 5, 60 and 3%, respectively, lower than the corresponding KFOOD dose. To the intakes of the radionuclides except Sr-90 evaluated in the improved method, foliar uptake contributed much more than root uptake did but, in the case of Sr-90, the result was opposite.

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Intercomparison Exercise at Harshaw 6600, DVG-02TM, and D-Shuttle Dosimeters for the Individual Monitoring of Ionizing Radiation

  • Kim, Dmitriy Spartakovich;Murayama, Kentaro;Nurtazin, Yernat;Koguchi, Yasuhiro;Kenzhin, Yergazy;Kawamura, Hiroshi
    • Journal of Radiation Protection and Research
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    • v.44 no.2
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    • pp.79-88
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    • 2019
  • Background: The main goal of experiments is to compare various operational and technical characteristics of D-Shuttle semiconductor personal dosimeters of the Japanese company "Chiyoda Technol Corporation" and Harshaw thermoluminescent dosimeters (TLD) manufactured by "Thermo Fisher Scientific" and DTL-02 of the Russian Research and Production Enterprise (RPE) "Doza" by their occupational and calibration exposure at various dose equivalents from 0.5 to 20 mSv of gamma-radiation. Materials and Methods: Besides dosimeters DTL-02, D-Shuttle and Harshaw TLD, there were also used: (1) the primary reference radionuclide source Hopewell Designs IAEA: G10-1-12 with $^{137}Cs$ isotope (an error is not more than 6% and activity is 20 Ci), and (2) the verification device UPGD-2M of RPE "Doza" and installed in the National Center for Expertise and Certification of the Republic of Kazakhstan (Kapchagai, the National Center for Expertise and Certification). Results and Discussion: The main results of researches are the following: (1) TLDs for Harshaw 6600 and DVG-02TM have an approximately equal measurement accuracy of the individual dose equivalents in the range from 0.5 to 20 mSv of gamma-radiation. (2) Advantages of dosimeters for Harshaw 6600 are due to the high measurement productivity and opportunity to indicate the dose on the skin $H_p$(0.07). Advantages of DVG-02TM consist of operation simplicity and lower cost than of Harshaw 6600. (3) D-Shuttles are convenient for use in the current and the operational monitoring of ionizing radiation. Measurement accuracy and 10% linearity of measurements are ensured when D-Shuttle is irradiated with dose equivalents below 1 mSv at the equivalent dose rate not higher than $3mSv{\cdot}hr^{-1}$. This allows using D-Shuttle at a routine technological activity. Conclusion: The obtained results of experiments demonstrate advantages and disadvantages of D-Shuttle semiconductor dosimeters in comparison with two TLD systems of DVG-02TM and Harshaw 6600.

Study on Radioactive Material Management Plan and Environmental Analysis of Water (II) Study of Management System in Water Environment of Japan (물 환경의 방사성 물질 관리 방안과 분석법에 관한 연구 (II) 일본의 물 환경 방사성물질 관리 체계에 대한 고찰)

  • Han, Seong-Gyu;Kim, Jung-Min
    • Journal of radiological science and technology
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    • v.38 no.3
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    • pp.305-313
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    • 2015
  • After Fukushima Daiichi nuclear disaster in 2011, study and maintenance of monitoring systems have been made at home and abroad. As concerns about radioactive contamination of water have increased in Korea, update of maintenance of managing radioactive materials in water is being made mainly by Ministry of Environment. In this study, we analysed current state of monitoring system modification in Japan, the country directly involved and neighboring country. According to the result, Japan modified the legislations first. Then Ministry of Education, Culture, Sports, Science and Technology (MEXT) provides theoretical background of radiological monitoring. And Ministry of the Environment actually watches state of water pollution in public waters and underground water. Finally related agencies like local government are monitoring current state of radioactive contamination in water environment. By region, local monitoring stations share the investigation of the whole country. Also, additional monitoring is running around nuclear facilities. After Fukushima disaster, monitoring for area near Fukushima is added. Among the reference levels, management target value of drinking water and tap water is 10 Bq/kg, and those of public water and underground water are 1 Bq/L. Measuring intervals varied from every hour to once a year, regularly or irregularly depending on the investigation. The main measuring items are air dose rate, gross ${\alpha}$, gross ${\beta}$, ${\gamma}$ radionuclide, Cs-134, Cs-137, Sr-89, Sr-90, I-131, and so on. In comparison, regulations about general public water in Korea need to be modified, while those about area near nuclear facility and drinking water are organized well. In future, therefore, domestic system would be expected to be modified with making reference to the guidelines like WHO's one. As good case of applying international guideline to domestic environment, Japanese system could be a reference when general standard of radioactivity in public water is made in Korea.