• Title/Summary/Keyword: Thorium Cycle

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Comparison of proliferation resistance among natural uranium, thorium-uranium, and thorium-plutonium fuels used in CANada Deuterium Uranium in deep geological repository by combining multiattribute utility analysis with transport model

  • Nagasaki, Shinya;Wang, Xiaopan;Buijs, Adriaan
    • Nuclear Engineering and Technology
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    • v.50 no.5
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    • pp.794-800
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    • 2018
  • The proliferation resistance (PR) of Th/U and Th/Pu fuels used in CANada Deuterium Uranium for the deep geological repository was assessed by combining the multiattribute utility analysis proposed by Chirayath et al., 2015 with the transport model of radionuclides in the repository and comparing with that of the used natural U fuel case. It was found that there was no significant advantage for Th/U and Th/Pu fuels from the viewpoint of the PR in the repository. It was also found that the PR values for used nuclear fuels in the repository of Th/U, Th/Pu, and natural U was comparable with those for enrichment and reprocessing facilities in the pressurized water reactor (PWR) nuclear fuel cycle. On the other hand, the PR values considering the transport of radionuclides in the repository were found to be slightly smaller than those without their transport after the used nuclear fuels started dissolving after 1,000 years.

Computational study of protactinium incorporation effects in Th and Th compounds

  • Daroca, D. Perez;Llois, A.M.;Mosca, H.O.
    • Nuclear Engineering and Technology
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    • v.52 no.10
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    • pp.2285-2289
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    • 2020
  • Protactinium contamination is a mayor issue in the thorium fuel cycle. We investigate, in this work, the consequences of Pa incorporation in vacancy defects and interstitials in Th, ThC and ThN. We calculate charge transfers and lattice distortions due to these incorporations as well as migration paths and energies involved in the diffusion of Pa.

Effect of process parameters on the recovery of thorium tetrafluoride prepared by hydrofluorination of thorium oxide, and their optimization

  • Kumar, Raj;Gupta, Sonal;Wajhal, Sourabh;Satpati, S.K.;Sahu, M.L.
    • Nuclear Engineering and Technology
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    • v.54 no.5
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    • pp.1560-1569
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    • 2022
  • Liquid fueled molten salt reactors (MSRs) have seen renewed interest because of their inherent safety features, higher thermal efficiency and potential for efficient thorium utilisation for power generation. Thorium fluoride is one of the salts used in liquid fueled MSRs employing Th-U cycle. In the present study, ThF4 was prepared by hydro-fluorination of ThO2 using anhydrous HF gas. Process parameters viz. bed depth, hydrofluorination time and hydrofluorination temperature, were optimized for the preparation of ThF4 in a static bed reactor setup. The products were characterized with X-Ray diffraction and experimental conditions for complete conversion to ThF4 were established which also corroborated with the yield values. Hydrofluorination of ThO2 at 450 ℃ for half an hour at a bed depth of 6 mm gave the best result, with a yield of about 99.36% ThF4. No unconverted oxide or any other impurity was observed. Rietveld refinement was performed on the XRD data of this ThF4, and Chi2 value of 3.54 indicated good agreement between observed and calculated profiles.

Burnup analysis for HTR-10 reactor core loaded with uranium and thorium oxide

  • Alzamly, Mohamed A.;Aziz, Moustafa;Badawi, Alya A.;Gabal, Hanaa Abou;Gadallah, Abdel Rraouf A.
    • Nuclear Engineering and Technology
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    • v.52 no.4
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    • pp.674-680
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    • 2020
  • We used MCNP6 computer code to model HTR-10 core reactor. We used two types of fuel; UO2 and (Th+Pu)O2 mixture. We determined the critical height at which the reactor approached criticality in both two cases. The neutronic and burnup parameters were investigated. The results indicated that the core fueled with mixed (Th+Pu)O2, achieved about 24% higher fuel cycle length than the UO2 case. It also enhanced safeguard security by burning Pu isotopes. The results were compared with previously published papers and good agreements were found.

A Feasibility of Once-Through Thorium Fuel Cycle for PWR (가압경수로에서 비순환 토륨 핵연료 주기의 적용 타당성)

  • 우일탁;김명현
    • Proceedings of the Korea Society for Energy Engineering kosee Conference
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    • 1999.11a
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    • pp.131-136
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    • 1999
  • 토륨은 자연계에서 유일한 동위원소인 Th-232로 존재하며 반감기는 1.4$\times$$10^{10}$년으로 U-238의 4.5$\times$$10^{9}$년에 비하여 약 3배 길고 매장량도 약 3배 많은 것으로 알려져 있다. 토륨은 원자력 초기 개발단계인 1950년대부터 우라늄에 관한 연구와 함께 시작되었지만, 70년대 중반 이후로는 토륨 핵연료 재처리의 어려움과 여러 정치적 이유로 이에 관한 연구가 거의 중단되었다.(중략)

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Facility to study neutronic properties of a hybrid thorium reactor with a source of thermonuclear neutrons based on a magnetic trap

  • Arzhannikov, Andrey V.;Shmakov, Vladimir M.;Modestov, Dmitry G.;Bedenko, Sergey V.;Prikhodko, Vadim V.;Lutsik, Igor O.;Shamanin, Igor V.
    • Nuclear Engineering and Technology
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    • v.52 no.11
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    • pp.2460-2470
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    • 2020
  • To study the thermophysical and neutronic properties of thorium-plutonium fuel, a conceptual design of a hybrid facility consisting of a subcritical Th-Pu reactor core and a source of additional D-D neutrons that places on the axis of the core is proposed. The source of such neutrons is a column of high-temperature plasma held in a long magnetic trap for D-D fusionreactions. This article presents computer simulation results of generation of thermonuclear neutrons in the plasma, facility neutronic properties and the evolution of a fuel nuclide composition in the reactor core. Simulations were performed for an axis-symmetric radially profiled reactor core consisting of zones with various nuclear fuel composition. Such reactor core containing a continuously operating stationary D-D neutron source with a yield intensity of Y = 2 × 1016 neutrons per second can operate as a nuclear hybrid system at its effective coefficient of neutron multiplication 0.95-0.99. Options are proposed for optimizing plasma parameters to increase the neutron yield in order to compensate the effective multiplication factor decreasing and plant power in a long operating cycle (3000-day duration). The obtained simulation results demonstrate the possibility of organizing the stable operation of the proposed hybrid 'fusion-fission' facility.

Searching for the viability of using thorium-based accident-tolerant fuel for VVER-1200

  • Mohamed Y.M. Mohsen;Mohamed A.E. Abdel-Rahman;Ahmed Omar;Nassar Alnassar;A. Abdelghafar Galahom
    • Nuclear Engineering and Technology
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    • v.56 no.1
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    • pp.167-179
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    • 2024
  • This study explores the feasibility of employing (U, Th)-based accident tolerant fuels (ATFs), specifically (0.8UO2, 0.2ThO2), (0.8UN, 0.2ThN), and (0.8UC, 0.2ThC). The investigation assesses the overall performance of these proposed fuel materials in comparison to the conventional UO2, focusing on deep neutronic and thermal-hydraulic (Th) analyses. Neutronic analysis utilized the MCNPX code, while COMSOL Multiphysics was employed for thermal-hydraulic analysis. The primary objective of this research is to overcome the limitations associated with traditional UO2 fuel by exploring alternative fuel materials that offer advantages in terms of abundance and potential improvements in performance and safety. Given the limited abundance of UO2, long-term sustainable nuclear energy production faces challenges. From a neutronic standpoint, the U-Th based fuels demonstrated remarkable fuel cycle lengths, except (0.8UN, 0.2ThN), which exhibited the minimum fuel cycle length and, consequently, the lowest fuel burn-up. Regarding thermal-hydraulic performance, (0.8UN, 0.2ThN) exhibited outstanding performance with significant margins against fuel melting compared to the other materials. Overall, when considering the integrated performance, the most favourable results were obtained with the use of the (0.8UC, 0.2ThC) fuel configurations. This study contributes valuable insights into the potential benefits of (U, Th)-based ATFs as a promising avenue for enhanced nuclear fuel performance.

DEVELOPMENT OF LEAD SLOWING DOWN SPECTROMETER FOR ISOTOPIC FISSILE ASSAY

  • Lee, YongDeok;Park, Chang Je;Ahn, Sang Joon;Kim, Ho-Dong
    • Nuclear Engineering and Technology
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    • v.46 no.6
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    • pp.837-846
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    • 2014
  • A lead slowing down spectrometer (LSDS) is under development for analysis of isotopic fissile material contents in pyro-processed material, or spent fuel. Many current commercial fissile assay technologies have a limitation in accurate and direct assay of fissile content. However, LSDS is very sensitive in distinguishing fissile fission signals from each isotope. A neutron spectrum analysis was conducted in the spectrometer and the energy resolution was investigated from 0.1eV to 100keV. The spectrum was well shaped in the slowing down energy. The resolution was enough to obtain each fissile from 0.2eV to 1keV. The detector existence in the lead will disturb the source neutron spectrum. It causes a change in resolution and peak amplitude. The intense source neutron production was designed for ~E12 n's/sec to overcome spent fuel background. The detection sensitivity of U238 and Th232 fission chamber was investigated. The first and second layer detectors increase detection efficiency. Thorium also has a threshold property to detect the fast fission neutrons from fissile fission. However, the detection of Th232 is about 76% of that of U238. A linear detection model was set up over the slowing down neutron energy to obtain each fissile material content. The isotopic fissile assay using LSDS is applicable for the optimum design of spent fuel storage to maximize burnup credit and quality assurance of the recycled nuclear material for safety and economics. LSDS technology will contribute to the transparency and credibility of pyro-process using spent fuel, as internationally demanded.