• Title/Summary/Keyword: Optical Properties of Asian Dust

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Chemically Aged Asian Dust Particles Proven by Traditional Spot Test and the Most Advanced micro-PIXE

  • Ma, Chang-Jin;Tohno, Susumu;Kang, Gong-Unn
    • Asian Journal of Atmospheric Environment
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    • v.10 no.2
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    • pp.114-123
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    • 2016
  • A change in chemical compositions of Asian dust (AD) particles can dramatically alter their optical properties, cloud-forming properties, and health effects. The present study was undertaken to evaluate this aging of AD particles by means of two complementary methods (i.e., the traditional spot test and the most advanced micro-PIXE analytical technique) for single particle analysis. Size-classified particles were sampled at the rural peninsula of Korea (Byunsan, 35.37N; 126.27E) during AD event and non-AD period in 2004. Sulfate was principally enriched on the particles in the size range of $7.65-10.85{\mu}m$ collected during AD event. The average number fraction of coarse particles ($>2.05{\mu}m$) containing chloride was 16.2% during AD event. Relatively low particles containing nitrate compared to those containing sulfate and chloride were found in AD event. Micro-PIXE elemental maps indicated that a large number of AD particles were internally mixed with man-made zinc. The highest peaks of EC and OC concentrations were appeared at $0.01-0.43{\mu}m$ particle aerodynamic diameter. High EC concentration in $PM_1$ was might be caused by the Saemangeum Seawall Project that was being conducted during our field measurement.

Study on the Variation of Optical Properties of Asian Dust Plumes according to their Transport Routes and Source Regions using Multi-wavelength Raman LIDAR System (다파장 라만 라이다 시스템을 이용한 발원지 및 이동 경로에 따른 황사의 광학적 특성 변화 연구)

  • Shin, Sung-Kyun;Noh, Youngmin;Lee, Kwonho;Shin, Dongho;Kim, KwanChul;Kim, Young J.
    • Korean Journal of Remote Sensing
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    • v.30 no.2
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    • pp.241-249
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    • 2014
  • The continuous observations for atmospheric aerosol were carried out during 3 years (2009-2011) by using a multi-wavelength Raman lidar at the Gwangju Institute of Science and Technology (GIST), Korea ($35.11^{\circ}N$, $126.54^{\circ}E$). The particle depolarization ratios were retrieved from the observations in order to distinguish the Asian dust layer. The vertical information of Asian dust layers were used as input parameter for the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model for analysis of its backward trajectories. The source regions and transport pathways of the Asian dust layer were identified. The most frequent source region of Asian dust in Korea was Gobi desert during observation period in this study. The statistical analysis on the particle depolarization ratio of Asian dust was conducted according to their transport route in order to retrieve the variation of optical properties of Asian dust during long-range transport. The transport routes were classified into the Asian dust which was transported to observation site directly from the source regions, and the Asian dust which was passed over pollution regions of China. The particle depolarization ratios of Asian dust which were transported via industrial regions of China was ranged 0.07-0.1, whereas, the particle depolarization ratio of Asian dust which was transported directly from the source regions to observation site were comparably higher and ranged 0.11-0.15. It is considered that the pure Asian dust particle from source regions were mixed with pollution particles, which is likely to spherical particle, during transportation so that the values of particle depolarization of Asian dust mixed with pollution was decreased.

A case study of aerosol features of Asian dust, fog, clear sky, and cloud at Anmyeon Island in April 2006 (2006년 4월 안면도에서 발생한 황사, 안개, 청명, 구름 사례에 대한 에어러솔 특성 분석)

  • Goo, Tae-Young;Hong, Gi-Man;Kim, Sang-Beak;Gong, Jong-Ung;Kim, Myoung-Soo
    • Atmosphere
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    • v.18 no.2
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    • pp.97-109
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    • 2008
  • The aerosol characteristics in terms of 4 different cases (Asian dust, fog, clear sky and cloud) which had happened at Anmyeon Island in April 2006 were studied using various measurements such as the Micro Pulse Lidar (MPL), sunphotometer, $\beta$-ray $PM_{10}$ Analyzer, anemoscope and anemometer. In addition, synoptic charts, back trajectory analyses and satellite images were also used to help characterize the aerosol events. The aerosol optical properties were featured by the Aerosol Optical Depth (AOD) and ${\AA}ngstr\ddot{o}m$ exponent which were estimated by the sunphotometer. When Anmyeon Island was dominated by the Asian dust, the AOD was sharply increased as seven times as a yearly average of it (0.35). As compared with a yearly average of the ${\AA}ngstr\ddot{o}m$ exponent of 0.97, the ${\AA}ngstr\ddot{o}m$ exponent of a dust day was significantly low (0.099). In addition, $PM_{10}$ mass concentration showed an extremely high record. The maximum concentration reached $1790.5{\mu}gm^{-3}$ on 8 April 2006. The maximum mass concentration was shown with delay when the wind speed of $0ms^{-1}$ was observed. It was also found that a satellite image of the MODIS-RGB had a good agreement with the results of those measurements. It was shown that the MPL was able to describe effectively the vertical distribution of aerosol for all the cases. In particular, the MPL evidently captured the aerosol layer before the cloud observation. The aerosol layer was similarly described by the AOD. On a clear sky day, the AOD had not only a very low value (0.054) but also a feature of homogeneity.

Analysis of Aerosol Optical Properties for High Particulate Matters and Light Asian Dust in Seoul Using GOCI (GOCI 자료를 이용한 서울 지역 고농도 미세먼지와 옅은 황사 시 에어로졸 광학적 특성 분석)

  • Kim, Deok-Rae;Choi, Won-Jun;Choi, Myungje;Kim, Jiyoung;Cho, Ara;Kim, Sang-Kyun;Kim, Jhoon;Moon, Kyung-Jung
    • Journal of Korean Society for Atmospheric Environment
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    • v.33 no.3
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    • pp.233-240
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    • 2017
  • To distinguish between high particulate matter (HPM) and light Asian dust (LAD) events, aerosol optical properties from GOCI were investigated in Seoul from 2014 to 2016. The poor air quality case caused by fine atmospheric particulate matter (i.e., 80<$PM_{10}$<$400{\mu}g/m^3$) is clearly separated from the case of heavy Asian dust that generally shows the $PM_{10}$ concentration more than $400{\mu}g/m^3$. In this study, we have found eight cases for the poor air quality and divided them into the two events(i.e., HPM and LAD). In case of aerosol optical depth (AOD), there was no big difference between two events. However, Angstrom exponent (AE) for HPM events was greater than 1, while that for LAD events less than 1. As a result of comparing aerosol type, non-absorbing fine mode aerosols were dominant for HPM events, but coarse and absorbing coarse mode aerosols for LAD events. Therefore, AE and aerosol type from GOCI can be used to distinguish between two events effectively.

Optical Properties of Aerosol at Gongju Estimated by Ground-based Measurements Using Sky-radiometer (스카이라디오미터(Sky-radiometer)로 관측된 공주지역 에어로솔의 광학적 특성)

  • Kwak, Chong-Heum;Suh, Myoung-Seok;Kim, Maeng-Ki;Kwak, Seo-Youn;Lee, Tae-Hee
    • Journal of the Korean earth science society
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    • v.26 no.8
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    • pp.790-799
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    • 2005
  • We investigate the optical properties of aerosols over Gongju by an indirect method using the pound measurement, Sky-radiometer. The analysis period is from January to December, 2004. Skyrad. pack.3 is used to estimate the optical properties, such as the aerosol optical thickness (AOT), single scattering albedo (SSA), ${\AA}ngstron$ exponent $({\alpha})$ and size distribution, of aerosols from the ground measured radiance data. And qualify control is applied to minimize the cloud-contaminated data and improve the quality of analysis results. The 12-month average of AOT, ${\alpha}$, and SSA are 0.46, 1.14, and 0.91, respectively. The average volume spectra of aerosols shows a bi-modal distribution, the first peak at fine mode and the second peak at coarse mode. AOT and coarse particles clearly increases while SSA decreases during the Asian dust events. The optical properties of aerosols at Gongju vary with?seasons, but those are not influenced by the wind direction.

Radiative Properties of Greenhouse Gases, Aerosols and Clouds in Korea

  • Moon, Yun-Seob;Bang, So-Young;Oh, Sung-Nam
    • Proceedings of the Korean Environmental Sciences Society Conference
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    • 2003.11a
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    • pp.51-54
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    • 2003
  • We analyzed radiative properties of aerosols, $CO^{2}$ and clouds using Optical Properties of Aerosols and Clouds(OPAC) and the Column Radiation Model (CRM). From OPAC, if the soot component is disregarded, dust-like components depict the highest extinction values in the solar spectral range and the lowest. single scattering albedoes, which are attributable to the presence of large particles. In the dust aerosol, the high absorptivity in the infrared may induce a warming of the lower atmospheric layer in the nighttime. The radiative properties of aerosols, clouds and double $CO^{2}$ using the CRM model at Seoul (37N, 127.4 E) on 3 April 2003 were calculated. The solar zenith angle is 65˚ and the surface albedo is 0.1836 during the clear day. The aerosol optical depth change 0.14 to 1.7, which is derived during Asian dust days in Korea. At this time, abedo by aerosols is considered as 0.3. In cloudy condition, the short wave cloud forcing on both the TOA and the surface is -193.89 $Wm^{-2}$ and -195.03 $Wm^{-2}$, respectively, and the long wave cloud forcing is 19.58 $Wm^{-2}$ and 62.08 $Wm^{-2}$, respectively. As a result, the net radiative cloud forcing is -174.31 $Wm^{-2}$ and -132.95 $Wm^{-2}$, respectively. We calculate also radiative heating rates by double $CO^{2}$ during the clear day. The $CO^{2}$ volumn mixing ratio is 3.55E-4.

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Derivation of aerosol vertical profiles in Seoul based on O4 measurements using UV scanning spectrometer

  • Lee, Hanlim;Hwang, JungBae;Son, Yoonhee
    • Korean Journal of Remote Sensing
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    • v.29 no.3
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    • pp.325-329
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    • 2013
  • This present study describes an application of UV scanning spectrometer $O_4$ data for retrieval of aerosol vertical profiles in Seoul during the measurement period that includes two Asian dust event days. The results show large variations of aerosol load in vertical and temporal scales. Large variations in aerosol were observed at 1 km in height during the daytime in the measurement period when the Asian dust events took place. The aerosol load, however, was found to be largest at the surface compared to those retrieved at the higher atmospheric layers. The results also clearly identified the diurnal patterns of aerosol vertical distributions. The aerosol load was high in the morning and noon whereas it was low in the afternoon. This study demonstrates that UV scanning spectrometer observations of the oxygen dimer can serve as a potential method for determination of atmospheric aerosol vertical distributions and optical properties.

Optical Properties of Asian Dust with LIDAR System (LIDAR 시스템을 이용한 황사의 광학적 특성 연구)

  • 최성철;차형기;김덕현;김영상
    • Proceedings of the Korea Air Pollution Research Association Conference
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    • 2002.04a
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    • pp.213-214
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    • 2002
  • 황사는 몽골이나 중국 북부의 황토지대에서 강한 바람에 의하여 고공으로 올라간 많은 미세한 모래먼지가 대기 중에 넓게 퍼져 하늘 전체를 덮고 떠다니다가 상층의 편서풍에 의해서 운반되어 서서히 하강하는 현상 또는 하강하는 모래먼지로 알려져 있다 최근 몇몇 연구가들에 의해 황사기간 중 대류권 내에서 편광소멸도를 측정하고 있다(Sakai 2000, Kobayashi 1985). 이들은 황사기간 중 편광소멸도는 0.2이상으로 높게 나타난다고 하였다. (중략)

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Aerosol Direct Radiative Forcing by Three Dimensional Observations from Passive- and Active- Satellite Sensors (수동형-능동형 위성센서 관측자료를 이용한 대기 에어러솔의 3차원 분포 및 복사강제 효과 산정)

  • Lee, Kwon-Ho
    • Journal of Korean Society for Atmospheric Environment
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    • v.28 no.2
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    • pp.159-171
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    • 2012
  • Aerosol direct radiative forcing (ADRF) retrieval method was developed by combining data from passive and active satellite sensors. Aerosol optical thickness (AOT) retrieved form the Moderate Resolution Imaging Spectroradiometer (MODIS) as a passive visible sensor and aerosol vertical profile from to the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) as an active laser sensor were investigated an application possibility. Especially, space-born Light Detection and Ranging (Lidar) observation provides a specific knowledge of the optical properties of atmospheric aerosols with spatial, temporal, vertical, and spectral resolutions. On the basis of extensive radiative transfer modeling, it is demonstrated that the use of the aerosol vertical profiles is sensitive to the estimation of ADRF. Throughout the investigation of relationship between aerosol height and ADRF, mean change rates of ADRF per increasing of 1 km aerosol height are smaller at surface than top-of-atmosphere (TOA). As a case study, satellite data for the Asian dust day of March 31, 2007 were used to estimate ADRF. Resulting ADRF values were compared with those retrieved independently from MODIS only data. The absolute difference values are 1.27% at surface level and 4.73% at top of atmosphere (TOA).