• Title/Summary/Keyword: Inert matrix fuel

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Modelling of effective irradiation swelling for inert matrix fuels

  • Zhang, Jing;Wang, Haoyu;Wei, Hongyang;Zhang, Jingyu;Tang, Changbing;Lu, Chuan;Huang, Chunlan;Ding, Shurong;Li, Yuanming
    • Nuclear Engineering and Technology
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    • v.53 no.8
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    • pp.2616-2628
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    • 2021
  • The results of effective irradiation swelling in a wide range of burnup levels are numerically obtained for an inert matrix fuel, which are verified with DART model. The fission gas swelling of fuel particles is calculated with a mechanistic model, which depends on the external hydrostatic pressure. Additionally, irradiation and thermal creep effects are included in the inert matrix. The effects of matrix creep strains, external hydrostatic pressure and temperature on the effective irradiation swelling are investigated. The research results indicate that (1) the above effects are coupled with each other; (2) the matrix creep effects at high temperatures should be involved; and (3) ranged from 0 to 300 MPa, a remarkable dependence of external hydrostatic pressure can be found. Furthermore, an explicit multi-variable mathematic model is established for the effective irradiation swelling, as a function of particle volume fraction, temperature, external hydrostatic pressure and fuel particle fission density, which can well reproduce the finite element results. The mathematic model for the current volume fraction of fuel particles can help establish other effective performance models.

Neutronics study on small power ADS loaded with recycled inert matrix fuel for transuranic elements transmutation using Serpent code

  • Vu, Thanh Mai;Hartanto, Donny;Ha, Pham Nhu Viet
    • Nuclear Engineering and Technology
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    • v.53 no.7
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    • pp.2095-2103
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    • 2021
  • A small power ADS design using thorium oxide and diluent matrix reprocessed fuel is proposed for a high transmutation rate, small reactivity swing, and strong safety features. Two fuel matrices (CERCER and CERMET) and different recycled fuel compositions recovered from UO2 spent fuels with 45 GWd/tU and 60 GWd/tU burnup were investigated to determine the suitable fuel for the ADS. It was found that the transmutation of each isotope depends on TRU initial loading amount. After examining the cores, the results show that CERCER fueled ADS has a negative coolant void reactivity (CVR) and a smaller radiotoxicity at discharge compared to that of CERMET core. It implies that CERCER fuel has enhanced safety features and more flavor in terms of radiotoxicity management. To increase fuel utilization and core operation efficiency, a simple assembly shuffling pattern for the CERCER fueled ADS is also proposed. Eigenvalue and burnup calculations were conducted using Serpent 2 with ENDF/B-VII.0 library in both kcode and external source modes, and it indicates that the results of transmutation analyses obtained by kcode only is reliable to discuss the transmutation potential of ADS. Burnup calculation with the fixed-source mode is essential to be used for more practical results of the transmutation by ADS.

IRRADIATION TEST OF MOX FUEL IN THE HALDEN REACTOR AND THE ANALYSIS OF MEASURED DATA WITH THE FUEL PERFORMANCE CODE COSMOS

  • WIESENACK WOLFGANG;LEE BYUNG-HO;SOHN DONG-SEONG
    • Nuclear Engineering and Technology
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    • v.37 no.4
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    • pp.317-326
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    • 2005
  • The burning-out of excess plutonium from the reprocessing of spent nuclear fuel and from the dismantlement of nuclear weapons is recently emphasized due to the difficulties in securing the final repository for the spent fuel and the necessity to consume the ex-weapons plutonium. An irradiation test in the Halden reactor was launched by the OECD Halden Reactor Project (HRP) to investigate the in-pile behavior of plutonium-embedded fuel as a form of mixed oxide (MOX) and of inert matrix fuel (IMF). The first cycle of irradiation was successfully accomplished with good integrity of test fuel rods and without any undesirable fault of instrumentations. The test results revealed that the MOX fuel is more stable under irradiation environments than IMF. In addition, MOX fuel shows lower thermal resistance due to its better thermal conductivity than IMF. The on-line measured in-pile performance data of attrition milled MOX fuel are used in the analysis of the in-pile performance of the fuel with the fuel performance code, COSMOS. The COSMOS code has been developed for the analysis of MOX fuel as well as $UO_2$ fuel up to high burnup and showed good capability to analyze the in-reactor behavior of MOX fuel even with different instrumentation.

Phase analysis of simulated nuclear fuel debris synthesized using UO2, Zr, and stainless steel and leaching behavior of the fission products and matrix elements

  • Ryutaro Tonna;Takayuki Sasaki;Yuji Kodama;Taishi Kobayashi;Daisuke Akiyama;Akira Kirishima;Nobuaki Sato;Yuta Kumagai;Ryoji Kusaka;Masayuki Watanabe
    • Nuclear Engineering and Technology
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    • v.55 no.4
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    • pp.1300-1309
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    • 2023
  • Simulated debris was synthesized using UO2, Zr, and stainless steel and a heat treatment method under inert or oxidizing conditions. The primary U solid phase of the debris synthesized at 1473 K under inert conditions was UO2, whereas a (U, Zr)O2 solid solution formed at 1873 K. Under oxidizing conditions, a mixture of U3O8 and (Fe, Cr)UO4 phases formed at 1473 K, whereas a (U, Zr)O2+x solid solution formed at 1873 K. The leaching behavior of the fission products from the simulated debris was evaluated using two methods: the irradiation method, for which fission products were produced via neutron irradiation, and the doping method, for which trace amounts of non-radioactive elements were doped into the debris. The dissolution behavior of U depended on the properties of the debris and aqueous solution for immersion. Cs, Sr, and Ba leached out regardless of the primary solid phases. The leaching of high-valence Eu and Ru ions was suppressed, possibly owing to their solid-solution reaction with or incorporation into the uranium compounds of the simulated debris.

FABRICATION OF ZrO2-BASED NANOCOMPOSITES FOR TRANSURANIC ELEMENT-BURNING INERT MATRIX FUEL

  • MISTARIHI, QUSAI;UMER, MALIK A.;KIM, JOON HUI;HONG, SOON HYUNG;RYU, HO JIN
    • Nuclear Engineering and Technology
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    • v.47 no.5
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    • pp.617-623
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    • 2015
  • $ZrO_2$-based composites reinforced with 6.5 vol.% of carbon foam, carbon fiber, and graphite were fabricated using spark plasma sintering, and characterized using scanning electron microscopy and X-ray diffractometry. Their thermal properties were also investigated. The microstructures of the reinforced composites showed that carbon fiber fully reacted with $ZrO_2$, whereas carbon foam and graphite did not. The carbothermal reaction of carbon fiber had a negative effect on the thermal properties of the reinforced $ZrO_2$ composites because of the formation of zirconium oxycarbide. Meanwhile, the addition of carbon foam had a positive effect, increasing the thermal conductivity from 2.86 to $3.38Wm^{-1}K^{-1}$ at $1,100^{\circ}C$. These findings suggest that the homogenous distribution and chemical stability of reinforcement material affect the thermal properties of $ZrO_2$-based composites.