• Title/Summary/Keyword: Disposal canister

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A Review of the Influence of Sulfate and Sulfide on the Deep Geological Disposal of High-level Radioactive Waste (고준위방사성폐기물 심층처분에 미치는 황산염과 황화물의 영향에 대한 고찰)

  • Jin-Seok Kim;Seung Yeop Lee;Sang-Ho Lee;Jang-Soon Kwon
    • Economic and Environmental Geology
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    • v.56 no.4
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    • pp.421-433
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    • 2023
  • The final disposal of spent nuclear fuel(SNF) from nuclear power plants takes place in a deep geological repository. The metal canister encasing the SNF is made of cast iron and copper, and is engineered to effectively isolate radioactive isotopes for a long period of time. The SNF is further shielded by a multi-barrier disposal system comprising both engineering and natural barriers. The deep disposal environment gradually changes to an anaerobic reducing environment. In this environment, sulfide is one of the most probable substances to induce corrosion of copper canister. Stress-corrosion cracking(SCC) triggered by sulfide can carry substantial implications for the integrity of the copper canister, potentially posing a significant threat to the long-term safety of the deep disposal repository. Sulfate can exist in various forms within the deep disposal environment or be introduced from the geosphere. Sulfate has the potential to be transformed into sulfide by sulfate-reducing bacteria(SRB), and this converted sulfide can contribute to the corrosion of the copper canister. Bentonite, which is considered as a potential material for buffering and backfilling, contains oxidized sulfate minerals such as gypsum(CaSO4). If there is sufficient space for microorganisms to thrive in the deep disposal environment and if electron donors such as organic carbon are adequately supplied, sulfate can be converted to sulfide through microbial activity. However, the majority of the sulfides generated in the deep disposal system or introduced from the geosphere will be intercepted by the buffer, with only a small amount reaching the metal canister. Pyrite, one of the potential sulfide minerals present in the deep disposal environment, can generate sulfates during the dissolution process, thereby contributing to the corrosion of the copper canister. However, the quantity of oxidation byproducts from pyrite is anticipated to be minimal due to its extremely low solubility. Moreover, the migration of these oxidized byproducts to the metal canister will be restricted by the low hydraulic conductivity of saturated bentonite. We have comprehensively analyzed and summarized key research cases related to the presence of sulfates, reduction processes, and the formation and behavior characteristics of sulfides and pyrite in the deep disposal environment. Our objective was to gain an understanding of the impact of sulfates and sulfides on the long-term safety of high-level radioactive waste disposal repository.

AN ANALYSIS OF THE THERMAL AND MECHANICAL BEHAVIOR OF ENGINEERED BARRIERS IN A HIGH-LEVEL RADIOACTIVE WASTE REPOSITORY

  • Kwon, S.;Cho, W.J.;Lee, J.O.
    • Nuclear Engineering and Technology
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    • v.45 no.1
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    • pp.41-52
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    • 2013
  • Adequate design of engineered barriers, including canister, buffer and backfill, is important for the safe disposal of high-level radioactive waste. Three-dimensional computer simulations were carried out under different condition to examine the thermal and mechanical behavior of engineered barriers and rock mass. The research looked at five areas of importance, the effect of the swelling pressure, water content of buffer, density of compacted bentonite, emplacement type and the selection of failure criteria. The results highlighted the need to consider tensile stress in the outer shell of a canister due to thermal expansion of the canister and the swelling pressure from the buffer for a more reliable design of an underground repository system. In addition, an adequate failure criterion should be used for the buffer and backfill.

Impact Force Applied on the Spent Nuclear Fuel Disposal Canister that Accidentally Drops and Collides onto the Ground (사고로 지면에 추락낙하 충돌하는 고준위폐기물 처분용기에 발생하는 충격력)

  • Kwon, Young Joo
    • Transactions of the Korean Society of Mechanical Engineers A
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    • v.40 no.5
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    • pp.469-481
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    • 2016
  • In this paper, a mathematical methodology was theoretically studied to obtain the impact force caused by the collision between rigid bodies. This theoretical methodology was applied to compute the impact force applied on the spent nuclear fuel disposal canister that accidentally drops and collides onto the ground. From this study, the impact force required to ensure a structurally safe canister design was theoretically formulated. The main content of the theoretical study concerns the rigid body kinematics and equation of motion during collision between two rigid bodies. On the basis of this study, a general impact theory to compute the impact force caused by the collision between two bodies was developed. This general impact theory was applied to theoretically formulate the approximate mathematical solution of the impact force that affects the spent nuclear fuel disposal canister that accidentally falls to the ground. Simultaneously, a numerical analysis was performed using the computer code to compute the numerical solution of the impact force, and the numerical result was compared with the approximate mathematical solution.

A Study on the Temperature Distribution Change of the Spent Nuclear Fuel Disposal Canister and its Surrounding Structures due to the Spent Fuel Heat according to the Deposition Time Elapse (고준위폐기물 열에 의한 처분용기 및 처분용기 주위 구조물의 시간경과에 따른 온도분포 변화)

  • Choi, Jong-Won;Kwon, Young-Joo
    • Journal of the Computational Structural Engineering Institute of Korea
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    • v.20 no.2
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    • pp.157-164
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    • 2007
  • The prediction of the temperature distribution change of the spent nuclear fuel disposal canister and its surrounding structures (bentonite buffer, granitic rock etc.) due to the spent fuel heat is very important for the design of the 500m deep granitic repository for the spent nuclear fuel disposal canister (about 10,000 years long) deposition. In this study, the temperature distribution change of the composite structure which comprises the canister, the bentonite buffer, the deposition tunnel due to the spent fuel heat is computed using the numerical analysis method. Specially, the temperature distribution change of the composite structure is analysed as the deposition time elapses up to m years. The analysis result shows that the temperature of each part of the repository increases slowly in different way but the latest part temperature increases slowly up to 150 years and thereafter decreases slowly.

Rigid Body Dynamic Analysis on the Spent Nuclear Fuel Disposal Canister under Accidental Drop and Impact to the Ground: Numerical analysis (사고로 지면으로 추락낙하 충돌하는 고준위폐기물 처분용기에 대한 기구동역학 해석: 수치해석)

  • Kwon, Young-Joo
    • Journal of the Computational Structural Engineering Institute of Korea
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    • v.26 no.5
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    • pp.373-384
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    • 2013
  • This paper is the second paper among two papers which constitute the paper about the rigid body dynamic analysis on the spent nuclear fuel disposal canister under accidental drop and impact to the ground. This paper performed the numerical study on the rigid body dynamic analysis. Through this study the impulsive force which is occurring in the spent nuclear fuel disposal canister under accidental drop and impact to the ground and required for the structural safety design of the canister is computed numerically. The main content of this numerical study is about the technical method how to compute the impulsive forces occurring in the canister under accidental drop and impact to the ground by using the commercial rigid body dynamic analysis computer codes. On the basis of this study the impulsive force which is occurring in the canister in the case of collision with the ground is numerically computed. This numerically computed impulsive force is increasing as the canister weight is increasing, and the canister falls plumb down and collides with the ground in three types according to the analysis results.

Creep Analysis for the Pressurized Water Reactor Spent Nuclear Fuel Disposal Canister (가압경수로 고준위페기물 처분용기에 대한 크립해석)

  • Ha Joon-Yong;Choi Jong-Won;Kwon Young-Joo
    • Journal of the Computational Structural Engineering Institute of Korea
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    • v.17 no.4
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    • pp.413-421
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    • 2004
  • In this paper, a structural analysis for the pressurized water reactor(PWR) spent nuclear fuel disposal canister which is deposited under the 500m deep underground is carried out to predict the creep deformation of the canister while the underground water and swelling bentonite pressure are applied on the canister. Usually the creep deformation may be caused due to the Pressure and the high heat applied to the canister even though additional external loads are not applied to the canister. These creep deformations depend on the time. In this paper, oかy the underground water and bentonite swelling Pressure are considered for the creep deformation analysis of the canister, because the heat distribution inside canister due the spent fuel is not simple and depends on time. A proper creep function is adopted for the creep analysis. The creep analysis is carried out during $10^8$ seconds. The creep analysis results show that the creep strains are very small and these strains occur usually in the lid and bottom of the canister not in the cast iron insert. A much smaller strain is found in the cast iron insert. Hence, the creep deformation doesn't affect the structural safety of the canister, and also the creep stress which shows the stress relaxation phenomenon doesn't affect the structural safety of the canister.

Development of an Earthquake-Resistant Model for a High-Level Waste Disposal Canister (고준위 폐기물 처분용기 내진 해석 모델 개발)

  • Choi, Young-Chul;Yoon, Chan-Hoon;Kim, Hyun-Ah;Choi, Heui-Joo
    • Tunnel and Underground Space
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    • v.24 no.4
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    • pp.316-324
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    • 2014
  • In the underground 500 m depth, the high level radioactive waste disposal system is made by boring the tunnel in the base rock and putting the high level waste disposal canister that is the surrounding form with the buffer material. According to the many statistics, it is the tendency that the earthquake increases in the Korean peninsula every year. In case that the earthquake is generated, the disposal canister in the rock mass can be broken due to the shearing force in the underground. Furthermore, a major environmental problems can be caused by the radioactive harmful substances. In this study, the earthquake-proof type buffer material was developed with the protection method safely on the earthquake. The main parameter having an effect on the earthquake-resistant performance was analyzed and the earthquake-proof type buffer material was designed. The shear analysis model was developed and the performance of the earthquake-proof type buffer material was evaluated by using ABAQUS.

Concept of the Encapsulation Process and Equipment for the Spent Fuel Disposal (심지층 처분을 위한 사용후핵연료 포장공정 장비개념 설정)

  • Lee J.Y.;Choi H.J.;Cho D.K.;Kim S.K.;Choi J.W.;Hahn P.S.
    • Proceedings of the Korean Society of Precision Engineering Conference
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    • 2005.10a
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    • pp.470-473
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    • 2005
  • Spent nuclear fuels are regarded as a high level radioactive waste and they will be disposed in a deep geological repository. To maintain the safety of the repository for hundreds of thousands of years, the spent fuels are encapsulated in a disposal canister and the canister containing spent fuels should have the structural integrity and the corrosion resistance below the several hundreds meters from the ground surface. In this study, the concept of the spent fuel encapsulation process and the process equipment fur deep geological disposal were established. To do this, the design requirements, such as the functions and the spent fuel accumulations, were reviewed. Also, the design principles and the bases were established. Based on the requirements and the bases, the encapsulation process and the equipment from spent fuel receiving process to transferring canister into the underground repository including hot cell processes was established. The established concept of the spent fuel encapsulation process and the process equipment will be improved continuously with the future studies. And this concept can be effectively used in implementing the reference repository system of our own case.

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A modularized numerical framework for the process-based total system performance assessment of geological disposal systems

  • Kim, Jung-Woo;Jang, Hong;Lee, Dong Hyuk;Cho, Hyun Ho;Lee, Jaewon;Kim, Minjeong;Ju, Heejae
    • Nuclear Engineering and Technology
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    • v.54 no.8
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    • pp.2828-2839
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    • 2022
  • This study developed a safety assessment tool for geological disposal systems called APro, a systemically integrated modeling system based on modularizing and coupling the processes which need to be considered in a geological disposal system. Thermal, hydraulic, chemical, canister failure, radionuclide release and transport processes were considered in the current version of APro. Each of the unit processes in APro consists of a single Default Module, and several Alternative Modules which can increase the flexibility of the model. As an initial stage of developing the modularization concept and modeling interface, the Default Modules of each unit process were described, with one Alternative Module of chemical process. The computation part of APro is mainly a MATLAB workspace controlling COMSOL and PHREEQC, which are coupled by an operator splitting scheme. The APro model domain is a stylized geological disposal system employing the Swedish disposal concept (KBS-3 type), but the repository layout can be freely adjusted. In order to show the applicability of APro to the total system performance assessment of geological disposal system, some sample simulations were conducted. From the results, it was confirmed that coupling of the thermal and hydraulic processes and coupling of the canister failure and the radionuclide release processes were well reflected in APro. In addition, the technical connectivity between COMSOL and PHREEQC was also confirmed.

Thermal Conductivity Evaluation of Compacted Bentonite Buffers Considering Temperature Variations (압축 벤토나이트 완충재의 온도에 따른 열전도도 평가)

  • Yoon, Seok;Park, Seunghun;Kim, Min-Seop;Kim, Geon-Young;Lee, Seung-Rae
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.18 no.1
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    • pp.43-49
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    • 2020
  • An engineered barrier system (EBS) for the geological disposal of high-level radioactive waste (HLW) consists of a disposal canister packed with spent fuel, buffer material, backfill material, and gap-filling material. The buffer material fills the space between the canister and the near-field rock, thus serving to restrain the release of radionuclides and protect the canister from groundwater penetration. Furthermore, as significant amounts of heat energy are released from the canister to the surrounding rock, the thermal conductivity of the buffer plays an important role in maintaining the safety of the entire disposal system. Therefore, given the high levels of heat released from disposal canisters, this study measured the thermal conductivities of compacted bentonite buffers from Gyeongju under temperature variations ranging 25 to 80~90℃. There was a 5~20% increase in thermal conductivity as the temperature increased, and the temperature effect increased as the degree of saturation increased.