• Analytical Science and Technology
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• v.18 no.4
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• pp.329-337
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• 2005

TL dating using pre-dose effect is concerned with the sensitivity increase of $110^{\circ}C$ TL peak in quartz following the pre-exposure of irradiation (pre-dose) in antiquity and heating to thermal activation temperature. Using the multiple activation (MA) method for determining an equivalent dose, the activation temperature was selected to $500^{\circ}C$ and the region of interest was selected from $85^{\circ}C$ to $105^{\circ}C$ on quartz sample from archaeological remains, roof-tile kiln. which was excavated at Chudong-Ri cultural site. It was concluded that the resultant date was determined to the age of $1725{\pm}25years$ AD (l ${\sigma}$ SD), which had more improved precision considering with e radiocarbon dates and was in good agreement with the age derived by archaeological assessment. Also it was concluded that the pre-dose dating should contribute significantly to future archaeological dating work in the range of the last 2000 years.

• Journal of Conservation Science
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• v.23
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• pp.73-80
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• 2008

This article aims to turn out the authentication of archaeological materials by using the paleodose measurement to fine sand-size quartz grains obtained by micro sampling technique. We firstly revealed the validity of micro sampling technique from the paleodoses of two bricks related to Muryong Royal Tomb of Baekje Kingdom. For the purpose of authentication test, four archaeological materials were selected, because they have been insisted that they were manufactured in Goguryeo Kingdom era. After obtaining very few quartz grains by micro sampling technique, each paleodose was evaluated by using SGR (single grain regenerative dose method). All values were very low below 0.2Gy and the reliability was found from those values by using SAR (single aliquot regenerative dose method). Considering the archaeological situation and the general paleodose, the burial time for 1,000 years generally corresponds to about 3.5Gy in Korea, it is concluded that these archaeological materials are all modern counterfeits.

• Analytical Science and Technology
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• v.12 no.6
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• pp.558-564
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• 1999

A method for measuring archaeological dose of Packjae pottery shards using thermoluminescence dosimetry(TLD) has been studied. TL measurement has been achieved using quartz crystals in the size range of 90 to $125{\mu}m$ diameter extracted from the pottery shards. The stable temperature region of the TL glow curve which is devoid of anomalous fading components was identified by the plateau test and found to exist from 265 to $300^{\circ}C$. The archaeological dose of the pottery shards was estimated to be 7.43 Gy using the dose calibration curves obtained from sequential irradiation of $^{137}Cs$ gamma source to the samples and TL measurement of natural samples.

• Journal of Conservation Science
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• v.34 no.6
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• pp.481-492
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• 2018

We conducted TL/OSL dating for the earthenware kilns in the Bongsan-ri archaeological site, Osong, which was occupied from the late nineteenth to the late twentieth century. With the SAR-TL/OSL method, paleodose was determined from the equivalent dose during the burial period($ED_{burial}$), the background dose($ED_{BG}$), the fading correction factor(f), and the overestimation correction factor(C). The annual dose rates and their provenance were evaluated from the measurement of natural radionuclides $^{238}U$, $^{232}Th$, and $^{40}K$. Because the comprehensive absolute age was provided by combining the resulting TL/OSL and radiocarbon data, we concluded that, for the absolute chronology of a modern archaeological site, TL/OSL dating and radiocarbon dating must be carried out together and summed. The construction and occupation of earthenware kilns in the Bongsan-ri site had changed from stage I (No.5, 6 kilns), to stage II (No.1, 2, 3 kilns), to stage III (No.4) in chronological order. When Bayesian statistics were applied, we found that the absolute ages of occupation for stages I, II, and III correspond to AD $1910{\pm}23$, AD $1970{\pm}10$, and AD $1987{\pm}4$. These results were in good agreement with the archaeological context or chronology.

• Journal of the Korean Magnetic Resonance Society
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• v.6 no.2
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• pp.84-88
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• 2002

Dating and dosimetry using electron spin resonance (ESR) in 20th Century developed at both Yamaguchi University and Osaka University have been reviewed with emphasis on new prospects and strategies in 21th century. Natural radiation have been generating radicals that accumulated in archaeological and geological materials. ESR detects these radicals and the ESR signal intensity is proportional to the radiation dose and therefore the age. The assessment of the total dose of natural radiation and the annual dose rate give their ESR ages. The ESR dating of stalactites and stalagmites ant Akiyoshi cave in Yamaguchi prefecture in 1975 was extended to anthropological dating using bones and tooth enamel excavated in Greek Petralona cave. Fossils of shells and corals gave the ages of marine terraces and sea-level changes. Quartz grains gave the ages of geothermal alteration and fault movements. Future ESR dating of ices at outer planets anf their satellite are also investigated as basic studies for ices od $H_2O,\;CO_2,\;SO_2$ as well as terrestrial hydrates in laboratory. Atomic bomb radiation dosimetry at Hiroshima and Nagasaki using ESR lead to the dosimetry of personnel, Chemobyl and JCO criticality accidents. Monitoring of radiation dose with sensitive materials with tissue equivalence are being developed. finally a new scanning ESR imaging apparatus (a near field microwave microscope) developed in our laboratory gave ESR images of Radicals from fossils to Si-CVD and diamond films as summarized in my book in 2002.

• Analytical Science and Technology
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• v.13 no.4
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• pp.403-411
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• 2000

This study described a method of thermoluminescence dating of pottery shards using subtraction method. TL measurement was achieved using two different types of samples prepared by quartz inclusion method and fine-grain technique. Fine grains (size range: $5-10{\mu}m$) were separated by suspending grounded pottery samples into acetone solution and sedimentation quantitatively. In quartz inclusion method quartz grains in the size range of 90 to $125{\mu}m$ diameter were obtained by extracting the quartz crystals embed in the pottery shards and etching them with 1.0 M HF solutions. The archaeological dose of both the quartz and fine grains was determined from the dose calibration curves obtained from sequential irradiation of $^{137}Cs$ gamma and $^{241}Am$ alpha source to the samples and TL measurement of natural samples, in which the alpha dose of 4.60 Gy for the Packjae pottery was obtained using subtraction method. Annual alpha dose rates ($3.05{\pm}0.11$ mGy/yr.) were determined by the analysis of U, Th contents in the pottery shards and evaluation of the values with Bell's equation. Dividing the alpha dose accumulated in the pottery shards by the annual alpha dose rate, we found age of approximately $1508{\pm}80$ years B.P. (AD. ca. 492 yr.) for the Packjae pottery. It matches well with the archeological age estimate (middle of 5th century) within 10 percent uncertainty and thereby conforms the age of the pottery sample.

• Journal of Radiation Protection and Research
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• v.36 no.2
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• pp.52-58
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• 2011

OSL dating for three hearths having the sequence of use and discard in No. 29 and 29-1 dwelling sites at Sogol cultural site was carried out. Resulting from the deconvolution of natural CW-OSL decay curve and thermal zeroing test, it was turned out that OSL signal was entirely composed of the heat- and light-sensitive fast component with high photoionization cross-section and all quartz OSL signals were thermally bleached under $300^{\circ}C$ which is the minimum temperature related to heating and cooking in Bronze age. After dose recovery test and plateau test, paleodose of each hearth sample was evaluated by using SAR method, and OSL age was determined from the ratio of paleodose to annual dose rate. For the purpose of the precision improvement of OSL age, Bayesian statistics was applied to each hearth's age and the archaeological sequence information. Finally, it could be concluded to the accurate use period of each hearth from the resultant OSL ages.

• Analytical Science and Technology
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• v.29 no.6
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• pp.269-276
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• 2016

Gosan-ri site is known as the early Neolithic cultural heritage, in which an archaic plainware, called as the Gosan-ri-type pottery, was excavated regarding as the first pottery manufactured in Korea. In this study, OSL dating was carried out to five soil layer samples collected in stratigraphic cross-section for evaluating the formation and occupation of the Gosan-ri site. Paleodose of each soil sample was calculated using the single aliquot regenerative dose (SAR) method with preheat of $220^{\circ}C$ and finally determined using maximum age model, considering its deposition process. The OSL age was determined from the ratio of paleodose to annual dose rate. From the resultant OSL ages and the related 14C dates, it was concluded that the Gosan-ri site was formed after 9,000 BC and a variety of cultural feature including the Gosan-ri-type pottery were occupied ranging from the early Neolithic to the middle of 4,000 BC. Finally, the Gosan-ri site was discarded in the middle of 4,000 BC and has been arrived at present through natural deposits.

• Analytical Science and Technology
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• v.32 no.4
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• pp.131-138
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• 2019

This paper reports results on the physical properties of a powder type of $Al_2O_3:C$ commonly used as a luminescence dosimeter using the LM-OSL technique. On the analysis with the general order kinetics model, the LM-OSL signal measured appeared to be composed of three components (fast, medium, slow) showing the largest area in the medium component. The photoionization cross sections of three components were distributed between $10^{-19}{\sim}10^{-21}cm^2$. The values of the thermal assistance energy were evaluated the largest in slow component and the smallest in fast component, which indicates the electrons trapped in defects attributed to slow component should be the most sensitive to thermal vibration among three components. In illumination to blue light, the fast component showed a rapid linear decay and completely disappeared after light exposure time of about 5 s. The medium component decayed with two exponential elements but the slow component did not observed any noticeable change until light exposure time of 40 s. In a dose response study, all components exhibited a linear behaviour up to approximately 10 Gy.

• Analytical Science and Technology
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• v.25 no.5
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• pp.324-332
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• 2012

Construction era of Pungnabtoseong earthen wall is one of the most popular controversial issues in Korean archaeological research. For the evaluation of construction era, OSL dating was carried out using seven pottery pieces collected in each construction stage. From TL/OSL characteristics, and the results of absolute zeroing test and recovery test, it was proved that the pottery samples were completely bleached. The reliable paleodose was evaluated by using the SAR method with preheat at $220^{\circ}C$, and the pottery OSL age was determined from the ratio of paleodose to annual dose rate. Considering the resultant OSL ages, archaeological context and the related 14C ages, the first construction era was determined as $294{\pm}52$ yrs AD ($1{\sigma}$ SE). Also we found that the enlargement of construction stage III was $328{\pm}30$ yrs AD ($1{\sigma}$ SE) and final construction was finished within $400{\pm}76$ yrs AD ($1{\sigma}$ SE). Therefore, it is suggested that the construction of Pungnabtoseong earthen wall was firstly started in the late $3^{rd}$ century AD and several enlargements and repairs had been carried out, before the transfer of the capital of Baekje dynasty to Woongjin (Gongju) at 475 AD.