• 한국대기환경학회지
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• 제22권5호
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• pp.535-553
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• 2006

2003년 12월 '수도권 대기환경 개선에 관한 특별법'이 국회를 통과하면서, 서울을 포함한 수도권 대기에서 미세먼지 농도를 저감하는 것을 주요 목표로 하는 '수도권 대기환경관리 기본계획'이 수립되었다. 효과적인 미세먼지 저감 대책을 수립하기 위해서는 정확한 추이와 현황, 그리고 주요 기여원을 알아야만 한다. 이 연구에서는 2006년 9월까지 국내외 학술지와 학술대회 등에서 발표된 연구 결과를 종합적으로 검토, 분석하여 서울 대기의 미세먼지에 대해 (1)변화 추이를 파악하고, (2)농도에 영향을 미치는 주요 변수는 무엇인지를 찾고자 하였다. 아황산가스, 미세먼지 등의 대기환경기준물질 농도와 체감 대기오염의 지표인 시정의 지난 20여 년간의 변화를 검토한 결과 서울의 대기환경은 1990년 이후 개선되고 있음을 알았다. 그러나 서울의 미세먼지 관련 대기환경은 아직 우리나라 다른 대도시나 외국의 대도시에 비해 미세먼지 질량 농도나, 시정, 먼지의 화학조성 등 여러 면에서 나쁘다. 서울 대기의 미세먼지 농도에 영향을 미치는 주요 인자는 자체에서의 배출, 반응에 의한 생성, 외부로부터의 유입 세 가지이다. 현재의 측정 자료는 서울 대기의 미세먼지의 화학조성의 추이를 이해하기에 충분하지 않아, 외부로부터의 장거리이동과 반응에 의한 생성을 구분하기 힘들다. 그럼에도 불구하고, 측정 자료와 모사 결과를 종합하면 서울의 경우에는 배출과 외부로부터의 유입만큼이나 반응에 의한 생성의 영향이 큰 것으로 나타났다. 이는 서울의 미세먼지 농도를 줄이기 위해서는 직접 배출을 줄이는 것도 중요하지만, 광화학반응에 의한 생성과 외부에서의 유입을 줄이는 것도 중요함을 의미한다. 보다 효과적인 미세먼지 저감대책을 수립하기 위해서는 시공간적으로 대표성 있는 미세먼지 성분 분석 결과가 필요함을 다시 한 번 확인하였다.

• 대기
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• 제28권2호
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• pp.175-185
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• 2018

Characteristics of precipitation response to enhanced aerosols have been investigated during the severe haze events observed in Korea for 2011 to 2016. All 6-years haze events are classified into long-range transported haze (LH: 31%), urban haze (UH: 28%), and yellow sand (YS: 18%) in order. Long-range transported one is mainly discussed in this study. Interestingly, both LH (68%) and YS (87%) appear to be more frequently accompanied with precipitation than UH (48%). We also found out the different timing of precipitation for LH and YS, respectively. The variations of precipitation frequency for the LH event tend to coincide with aerosol variations specifically in terms of temporal covariation, which is in contrast with YS. Increased aerosol loadings following precipitation for the YS event seems to be primarily controlled by large scale synoptic forcing. Meanwhile, aerosols for the LH event may be closely associated with precipitation longevity through changes in cloud microphysics such that enhanced aerosols can increase smaller cloud droplets and further extend light precipitation at weaker rate. Notably, precipitation persisted longer than operational weather forecast not considering detailed aerosol-cloud interactions, but the timescale was limited within a day. This result demonstrates active interactions between aerosols and meteorology such as probable modifications of cloud microphysics and precipitation, synoptic-induced dust transport, and precipitation-scavenging in Korea. Understanding of aerosol potential effect on precipitation will contribute to improving the performance of numerical weather model especially in terms of precipitation timing and location.

• Nuclear Engineering and Technology
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• 제54권6호
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• pp.2077-2083
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• 2022

In the unlikely event of core disruptive accident in sodium cooled fast reactors, the reactor containment building would be bottled up with sodium and fission product aerosols. The behavior of these aerosols is crucial to estimate the in-containment source term as a part of nuclear reactor safety analysis. In this work, the evolution of sodium aerosol characteristics (mass concentration and size) is simulated using HAARM-S code. The code is based on the method of moments to solve the integro-differential equation. The code is updated to FORTRAN-77 and run in Microsoft FORTRAN PowerStation 4.0 (on Desktop). The sodium aerosol characteristics simulated by HAARM-S code are compared with the measured values at Aerosol Test Facility. The maximum deviation between measured and simulated mass concentrations is 30% at initial period (up to 60 min) and around 50% in the later period. In addition, the influence of humidity on aerosol size growth for two different aerosol mass concentrations is studied. The measured and simulated growth factors of aerosol size (ratio of saturated size to initial size) are found to be matched at reasonable extent. Since sodium is highly reactive with atmospheric constituents, the aerosol growth factor depends on the hygroscopic growth, chemical transformation and density variations besides coagulation. Further, there is a scope for the improvement of the code to estimate the aerosol dynamics in confined environment.

• Nuclear Engineering and Technology
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• 제56권1호
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• pp.132-140
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• 2024

In the event of a severe accident in Sodium Cooled Fast Reactors (SFR), the sodium combustion aerosols along with fission product aerosols would migrate to the environment through leak paths of the Reactor Containment Building (RCB) concrete wall under positive pressure. Understanding the characteristics of sodium aerosol transport through concrete leak paths is important as it governs the environmental source term. In this context, experiments are conducted to study the influence of various parameters like pressure, initial mass concentration, leak path diameter, humidity etc., on the transport and deposition of sodium aerosols in straight leak paths of concrete. The leak paths in concrete specimens are prepared by casting and the diameter of the leak path is measured using thermography technique. Aerosol transport experiments are conducted to measure the transported and plugged aerosol mass in the leak paths and corresponding plugging times. The values of differential pressure, aerosol concentration and relative humidity taken for the study are in the ranges 10-15 kPa, 0.65-3.04 g/m³ and 30-90% respectively. These observations are numerically simulated using 1-Dimensional transport equation. The simulated values are compared with the experimental results and reasonable agreement among them is observed. From the safety assessment view of reactor, the approach presented here is conservative as it is with straight leak paths.

• 대한기계학회논문집B
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• 제28권3호
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• pp.349-358
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• 2004

A low pressure impactor is an impaction device to separate airborne particles into aerodynamic size classes at low pressure condition. We designed a two-stage low-pressure impactor to classify submicron sized environmental aerosols. Performance evaluation was carried out for stages 1 and 2 by using an electrical method. Monodisperse liquid dioctyl sebacate (DOS) particles were generated using evaporation-condensation process followed by electrostatic classification using a DMA (differential mobility analyzer). The test particles were in the range of 0.08∼0.8$\mu\textrm{m}$. For the evaluation of the impactor we used two electrometers; one was connected to the impaction plate of the impactor and the other was to the Faraday cage used as a backup filter. The effect of polydispersity of test aerosols on the performance was investigated. The results showed that the experimental 50-% cutoff diameters at each impactor's operation pressure were 0.53 and 0.187$\mu\textrm{m}$ for stages 1 and stage 2, respectively. The effects of operation pressure on the cutoff diameter and the steepness of collection efficiency curves were also investigated.

• 한국대기환경학회지
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• 제19권1호
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• pp.67-76
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• 2003

Recently consideration of health and interest on bio aerosols have been growing steadily. In this study, inertial impactor, which can be used to collect airborne particles and bio aerosols, was newly devised for real-time observation on the particles collected on impaction plate. and named Visual Impactor. Flow field and particle trajectory in the space between nozzle and impaction plate was analyzed numerically, and the collection effciencies were calculated. Calibration and performance evaluation of the Visual Impactor was conducted with polydisperse aerosols generated from 0.1％ sodium chloride solution. Cut-off diameter from numerical simulation was in good agreement with that from experimental results. Because of particle bounce and particle deposition on nozzle tip due to short jet-to-plate distance, the collection efficiencies from numerical and experimental analyses were different slightly. Visual Impactor was used to collect airborne particles, and the features of collected particles could be seen in real-time. Airborne particles in different weather conditions (fine, cloudy, and rainy) were sampled and compared one another The features of collected airborne particles were dependent strongly upon relative humidity. In addition, with hours elapsing, shapes and colors of collected particles were changed by evaporation and surface tension, etc.

• 한국대기환경학회지
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• 제1권1호
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• pp.71-82
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• 1985

The effect on the particulate matters in the atmosphere was investigated in Seoul area from March, 1984 to Aprill, 1985. Aerosols were collected by filters on nine stages Andrsen Air Sampler, and size distribution and total concentration of the aerosols, Fe and Pb were measured. In spring with Yellow Sand the concentration of particles in aerosols was 185.55$\mug/m^3$ and CP/TA was 65.9%. But in spring without Yellow Sand those of particles was 135.45$\mug/m^3$ and CP/TA was 58.6%. Accordingly the concentration of coarse particles with Yellow Sand was higher than without them in Spring. Above results indicate that in Seoul Area the main source of air pollution originated from natural burdens, especially from soil. The concentration of Pb was similarly valued through both seasons in Seoul area but fine particles valued above coarse particles. On the other hand, in urban area, the natural and anthropogenic sources have influenced on the concentration of Pb. With referred to particle size distribution for Fe, the concentration of coarse particles was 0.168$\etag/m^3$ (CP/TA: 74.3%) in Spring with Yellow Sand, 0.096$\mug/m^3$ (CP/TA: 71.6%) without Yellow Sand and 0.083$\mug/m^3$ (CP/TA: 67.4%) in winter, respectively. Compared with fine particles, all of them were higher. It indicated that the origin of coarse particles in urban air was not related to anthropogenic source. The concentration of Fe was influenced by Yellow Sand and contributed to air pollution.

• 한국대기환경학회지
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• 제16권5호
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• pp.445-451
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• 2000

To estimate dry deposition flux of 12 elements in aerosols, aerosol particles were sampled by a low-pressure impactor(LPI) and a dust jar. The concentrations of 12 elements in aerosol particle and dry deposition were analyzed by a PIXE analysis using as a 2.0 MeV-proton beam. The mean dry deposition velocities of 12 elements were estimated by ranges of 0.74∼2.62 cm/sec. The results showed that the highest value was 3.26 cm/sec for Ca and the lowest value 0.74 cm/sec for Fe. The dry deposition flux for elements was calculated as a function of particle size by 1-step method and 12-step method. In this work, dry deposition velocities were computed with the two existing models; the coarse-particle fraction(4∼30 mm diameter) using the dry deposition velocity model of the Noll and Fang(1998) and the fine-particle fraction (0.05∼4mm diameter) using the Shemel and Hodgson(1980) model. The ratios of the mean calculated/measured fluxes were 3.59 for 1-step method and 0.60 for 12-step method respectively.

• 한국대기환경학회지
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• 제29권6호
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• pp.722-733
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• 2013

Ground-based measurements were conducted from August 25 to September 8 of 2011 for understanding characteristics of carbonaceous aerosols measured at Gosan. Chemical components and their sources were discussed by analysis of organic compounds with identification of primary and secondary products in particulate matter. Thus, organic carbon (OC) and elemental carbon (EC) based on the carbonaceous thermal distribution (CTD), which provides detailed carbon signature characteristics relative to analytical temperature, was used to improve the carbon fractionation of the analytical method. In addition, organic compounds by gas chromatography technique with the backward trajectories were discussed for characteristics of carbonaceous aerosols. Different air-masses were classified related to the OC thermal signatures and the organic molecular markers such as aromatic acids and PAHs. We concluded that the aging process was influenced by the long-range transport from East Sea area.

• Journal of Microbiology and Biotechnology
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• 제17권10호
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• pp.1622-1628
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• 2007

We characterized the efficacy of an electrostatic precipitator (ESP) air-cleaner in reducing the concentration of Serratia marcescens in an enclosed space. We used an experimental room ($4.5{\times}3{\times}2.9\;m$) in which electrostatic air-cleaners were located. Two air-cleaners enhanced the equivalent ventilation rates in the chamber by about 3.3 air changes per hour (ACH) over the 2 ACH provided by the mechanical ventilation system. Natural die-off of the organisms provided an additional equivalent of 3 ACH, so that the total ventilation rate with the ESP air-ccleaners was 8.3 ACH. We also examined whether the ESP air-cleaners altered the deposition of Serratia marcescens aerosols on the experimental room surfaces. We did not find any significant differences in the number of colony forming units recovered from surfaces with and without the air-cleaners. We installed UV lights inside the ESPs and determined if UV light, in addition to electrical fields, increased the efficacy of the ESPs. The presence of UV light inside the ESP reduced S. marcescens aerosols by approximately 2 ACH. Finally, a box model indicates that the efficiency of the air-cleaner increases for both biological and nonbiological particles at ventilation rates of 0.2-1, which are typical for residential settings.