• Title/Summary/Keyword: Nuclear material

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Novel homogeneous burnable poisons in pressurized water reactor ceramic fuel

  • Dodd, Brandon;Britt, Taylor;Lloyd, Cody;Shah, Manit;Goddard, Braden
    • Nuclear Engineering and Technology
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    • v.52 no.12
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    • pp.2874-2879
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    • 2020
  • Due to excess reactivity, fresh nuclear fuel often contains burnable poisons. This research looks at six different burnable poisons and their impacts on reactivity, material attractiveness, and waste management. An MCNP simulation of a PWR fuel pin was performed with a fuel burnup of 60 GWd/MTHM to determine when each burnable poison fuel type would decrease below a k of 1. For determining the plutonium material attractiveness in each burnable poison fuel type, the plutonium isotopic content of the used fuel was evaluated using Bathke's Figure of Merit formula. For the waste management analysis, the thermal output of each burnable poison fuel type was determined through ORIGEN decay simulations at 100 and 300 years after being discharged from the core. The performance of all six burnable poisons varied over the three criteria considered and no single burnable poison performed best in all three considerations.

Towards inferring reactor operations from high-level waste

  • Benjamin Jung;Antonio Figueroa;Malte Gottsche
    • Nuclear Engineering and Technology
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    • v.56 no.7
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    • pp.2704-2710
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    • 2024
  • Nuclear archaeology research provides scientific methods to reconstruct the operating histories of fissile material production facilities to account for past fissile material production. While it has typically focused on analyzing material in permanent reactor structures, spent fuel or high-level waste also hold information about the reactor operation. In this computational study, we explore a Bayesian inference framework for reconstructing the operational history from measurements of isotope ratios from a sample of nuclear waste. We investigate two different inference models. The first model discriminates between three potential reactors of origin (Magnox, PWR, and PHWR) while simultaneously reconstructing the fuel burnup, time since irradiation, initial enrichment, and average power density. The second model reconstructs the fuel burnup and time since irradiation of two batches of waste in a mixed sample. Each of the models is applied to a set of simulated test data, and the performance is evaluated by comparing the highest posterior density regions to the corresponding parameter values of the test dataset. Both models perform well on the simulated test cases, which highlights the potential of the Bayesian inference framework and opens up avenues for further investigation.

Determination of dosimetric dependence for effective atomic number of LDR brachytherapy seed capsule by Monte Carlo simulation

  • Berkay Camgoz;Dilara Tarim
    • Nuclear Engineering and Technology
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    • v.55 no.8
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    • pp.2734-2741
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    • 2023
  • Brachytherapy is a special case of radiotherapy. It should be arranged according to some principles in medical radiation applications and radiation physics. The primary principle is to use as low as reasonably achievable dose in all ionizing radiation applications for diagnostic and therapeutic treatments. Dosimetric distributions are dependent on radioactive source properties and radiation-matter interactions in an absorber medium such as phantom or tissue. In this consideration, the geometrical structure and material of the seed capsule, which surrounds a radioactive material, are directly responsible for isodose profiles and dosimetric functions. In this study, the radiometric properties of capsule material were investigated on dose distribution in a water phantom by changing its nuclear properties using the EGSnrc Monte Carlo (MC) simulation code. Effective atomic numbers of hypothetic mixtures were calculated by using different elements with several fractions for capsule material. Model 6711 brachytherapy seed was modeled by EGSnrc/Dosrcnrc Code and dosimetric functions were calculated. As a result, dosimetric parameters of hypothetic sources have been acquired in large-scale atomic number. Dosimetric deviations between the data of hypothetic seeds and the original one were analyzed. Unit dose (Gy/Particle) distributions belonging to different types of material in seed capsule have remarkably differed from the original capsule's data. Capsule type is major variable to manage the expected dose profile and isodose distribution around a seed. This study shows us systematically varied scale of material type (cross section or effective atomic number dependent) offers selective material usage in production of seed capsules for the expected isodose profile of a specific source.

Nuclide composition non-uniformity in used nuclear fuel for considerations in pyroprocessing safeguards

  • Woo, Seung Min;Chirayath, Sunil S.;Fratoni, Massimiliano
    • Nuclear Engineering and Technology
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    • v.50 no.7
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    • pp.1120-1130
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    • 2018
  • An analysis of a pyroprocessing safeguards methodology employing the Pu-to-$^{244}Cm$ ratio is presented. The analysis includes characterization of representative used nuclear fuel assemblies with respect to computed nuclide composition. The nuclide composition data computationally generated is appropriately reformatted to correspond with the material conditions after each step in the head-end stage of pyroprocessing. Uncertainty in the Pu-to-$^{244}Cm$ ratio is evaluated using the Geary-Hinkley transformation method. This is because the Pu-to-$^{244}Cm$ ratio is a Cauchy distribution since it is the ratio of two normally distributed random variables. The calculated uncertainty of the Pu-to-$^{244}Cm$ ratio is propagated through the mass flow stream in the pyroprocessing steps. Finally, the probability of Type-I error for the plutonium Material Unaccounted For (MUF) is evaluated by the hypothesis testing method as a function of the sizes of powder particles and granules, which are dominant parameters to determine the sample size. The results show the probability of Type-I error is occasionally greater than 5%. However, increasing granule sample sizes could surmount the weakness of material accounting because of the non-uniformity of nuclide composition.

INVESTIGATION ON MATERIAL DEGRADATION OF ALLOY 617 IN HIGH TEMPERATURE IMPURE HELIUM COOLANT

  • Kim, Dong-Jin;Lee, Gyeong-Geun;Jeong, Su-Jin;Kim, Woo-Gon;Park, Ji-Yeon
    • Nuclear Engineering and Technology
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    • v.43 no.5
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    • pp.429-436
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    • 2011
  • The corrosion of materials exposed to high temperature helium in a very high temperature reactor is caused by interaction with the impurities in the helium. This interaction then induces high temperature mechanical deterioration. By considering the effect of the impurity concentration on material corrosion, a long-term coolant chemistry guideline can be determined for the range of impurity concentration at which the material is stable for a long time. In this work, surface reactions were investigated by analyzing the thermodynamics and the experimental results for Alloy 617 exposed to controlled impure helium at $950^{\circ}C$. Moreover, the surfaces were examined for the Alloy 617 crept in air and in uncontrolled helium, which was explained by possible surface reactions.

Nuclear Material Containment/Surveillance System for Nuclear Facility (핵물질 취급 시설의 격납/감시 시스템)

  • Song, D.Y.;Lee, S.Y.;Kim, H.D.
    • Proceedings of the KIEE Conference
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    • 2005.10b
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    • pp.490-492
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    • 2005
  • Unattended continuous containment/surveillance systems for safeguards of nuclear facility result in large amounts of image and radiation data, which require much time and effort to inspect. Therefore, it is necessary to develop system that automatically pinpoints and diagnoses the anomalies from data. In this regards, this paper presents the nuclear material containment/surveillance system that integrates visual image and radiation data.

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Preliminary PINC(Program for the Inspection of Nickel Alloy Components) RRT(Round Robin Test) - Pressurizer Dissimilar Metal Weld -

  • Kim, Kyung-Cho;Kang, Sung-Sik;Shin, Ho-Sang;Chung, Ku-Kab;Song, Myung-Ho;Chung, Hae-Dong
    • Journal of the Korean Society for Nondestructive Testing
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    • v.29 no.3
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    • pp.248-255
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    • 2009
  • After several damages by PWSCC were found in the world, USNRC and PNNL(Pacific Northwest National Laboratory) started the research on PWSCC under the project name of PINC. The aim of the project was 1) to fabricate representative NDE mock-ups with flaws to simulate PWSCCs, 2) to identify and quantitatively assess NDE methods for accurately detecting, sizing and characterizing PWSCCs, 3) to document the range of locations and morphologies of PWSCCs and 4) to incorporate results with other results of ongoing PWSCC research programs, as appropriate. Korea nuclear industries have also been participating in the project. Thermally and mechanically cracked-four mockups were prepared and phased array and manual ultrasonic testing(UT) techniques were applied. The results and lessons learned from the preliminary RRT are summarized as follows: 1) Korea RRT teams performed the RRT successfully. 2) Crack detection probability of the participating organizations was an average 87%, 80% and 80% respectively. 3) RMS error of the crack sizing showed comparatively good results. 4) The lessons learned may be helpful to perform the PINC RRT and PSI /ISI in Korea in the future.