• 제목/요약/키워드: Neutron capture

검색결과 118건 처리시간 0.03초

보론 중성자 포획 암치료 기술 - 현황과 전망 (BNCT, Boron Neutron Capture Therapy)

  • 조남진;박정환
    • 원자력산업
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    • 제16권8호통권162호
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    • pp.53-64
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    • 1996
  • 미국의 경우 질병으로 인한 사망자의 절반 정도가 암으로 인한 사망이다. 정산 세포 속에 위치한 암세포만을 선택적으로 손상시키기에는 미흡한 기존의 암치료 방법에 비해, 열중성자와 표적핵을 사용하여 방사선에 민감한 암조직 세포만을 효과적으로 죽일 수 있는 방사선 치료 방법 중의 하나인 BNCT 기술이 새롭게 주목을 끌고 있다. BNCT 기술의 현황과 전망을 알아본다.

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Conceptual design of hybrid target for molybdenum-99 production based on heavywater

  • Ali Torkamani ;Ali Taghibi Khotbehsara ;Faezeh Rahmani ;Alexander Khelvas ;Alexander Bugaev ;Farshad Ghasemi
    • Nuclear Engineering and Technology
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    • 제55권5호
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    • pp.1863-1870
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    • 2023
  • Molybdenum-99 (99Mo) is used for preparing Technetium-99 m (99mTc), which is the most widely used isotope in nuclear medicine. In this work, a study for 99Mo production based on a high-power electron accelerator has been performed as an alternative approach to produce 99mTc. In this study, Monte Carlo MCNPX2.6 code has been used to examine a novel idea of simultaneous hybrid production of 99Mo via both photoneutron and neutron capture reactions using an electron accelerator in heavy water tank. It is expected that this conceptual design including an arrangement of metallic plates of 100Mo and 98Mo produces total activity of 97.5 Ci at the end of 20-h continuous e-beam irradiation (30 MeV, 10 mA).

Simulation, design optimization, and experimental validation of a silver SPND for neutron flux mapping in the Tehran MTR

  • Saghafi, Mahdi;Ayyoubzadeh, Seyed Mohsen;Terman, Mohammad Sadegh
    • Nuclear Engineering and Technology
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    • 제52권12호
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    • pp.2852-2859
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    • 2020
  • This paper deals with the simulation-based design optimization and experimental validation of the characteristics of an in-core silver Self-Powered Neutron Detector (SPND). Optimized dimensions of the SPND are determined by combining Monte Carlo simulations and analytical methods. As a first step, the Monte Carlo transport code MCNPX is used to follow the trajectory and fate of the neutrons emitted from an external source. This simulation is able to seamlessly integrate various phenomena, including neutron slowing-down and shielding effects. Then, the expected number of beta particles and their energy spectrum following a neutron capture reaction in the silver emitter are fetched from the TENDEL database using the JANIS software interface and integrated with the data from the first step to yield the origin and spectrum of the source electrons. Eventually, the MCNPX transport code is used for the Monte Carlo calculation of the ballistic current of beta particles in the various regions of the SPND. Then, the output current and the maximum insulator thickness to avoid breakdown are determined. The optimum design of the SPND is then manufactured and experimental tests are conducted. The calculated design parameters of this detector have been found in good agreement with the obtained experimental results.

Fabrication of a superheated emulsion based on Freon-12 and LiCl suitable for thermal neutrons detection

  • Sara Sadat Madani Kouchak;Dariush Rezaei Ochbelagh;Peiman Rezaeian;Majid Abdouss
    • Nuclear Engineering and Technology
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    • 제56권4호
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    • pp.1425-1430
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    • 2024
  • This study develops superheated emulsion detectors that are both sensitive to fast neutrons, and thermal neutrons owing to the exergonic 63Li(n, α)31H capture reaction caused by the 6Li-containing compound dispersed throughout the gel-like medium. The experimental research was conducted on two SEDs. One detector was an ordinary Freon-12 detector and the other was a Freon-12 detector containing 3.4 % (by weight) LiCl. In order to investigate the sensitivity of lithium-containing SEDs to thermal neutrons, two types of SEDs were simultaneously exposed to various flux levels of thermal neutrons from 241Am-Be neutron source inside a cylindrical tank filled with water. A Boron-lined proportional counter was used to estimate the thermal neutron flux and the relevant MCNP code was developed for flux and dose calculations in the prepared set-up around 241Am-Be source. The results demonstrate that there is a proportional relationship between the variations of SED response and the change in thermal neutron flux and dose. Also, the sensitivity of SED was estimated.

Enhancing the performance of a long-life modified CANDLE fast reactor by using an enriched 208Pb as coolant

  • Widiawati, Nina;Su'ud, Zaki;Irwanto, Dwi;Permana, Sidik;Takaki, Naoyuki;Sekimoto, Hiroshi
    • Nuclear Engineering and Technology
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    • 제53권2호
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    • pp.423-429
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    • 2021
  • The investigation of the utilization of enriched 208Pb as a coolant to enhance the performance of a long-life fast reactor with a Modified CANDLE (Constant Axial shape of Neutron flux, nuclide densities, and power shape During Life of Energy production) burnup scheme has performed. The analyzes were performed on a reactor with thermal power of 800 MegaWatt Thermal (MWTh) with a refueling process every 15 years. Uranium Nitride (enriched 15N), 208Pb, and High-Cr martensitic steel HT-9 were employed as fuel, coolant, and cladding materials, respectively. One of the Pb-nat isotopes, 208Pb, has the smallest neutron capture cross-section (0.23 mb) among other liquid metal coolants. Furthermore, the neutron-producing cross-section (n, 2n) of 208Pb is larger than sodium (Na). On the other hand, the inelastic scattering energy threshold of 208Pb is the highest among Na, natPb, and Bi. The small inelastic scattering cross-section of 208Pb can harden the neutron energy spectrum. Therefore, 208Pb is a better neutron multiplier than any other liquid metal coolant. The excess neutrons cause more production than consumption of 239Pu. Hence, it can reduce the initial fuel loading of the reactor. The selective photoreaction process was developing to obtain enriched 208Pb. The neutronic was calculated using SRAC and JENDL 4.0 as a nuclear data library. We obtained that the modified CANDLE reactor with enriched 208Pb as coolant and reflector has the highest k-eff among all reactors. Meanwhile, the natPb cooled reactor has the lowest k-eff. Thus, the utilization of the enriched 208Pb as the coolant can reduce reactor initial fuel loading. Moreover, the enriched 208Pb-cooled reactor has the smallest power peaking factor among all reactors. Therefore, the enriched 208Pb can enhance the performance of a long-life Modified CANDLE fast reactor.

Evaluation of Neutron Cross Sections of Dy Isotopes in the Resonance Region

  • Oh, Soo-Youl;Gil, Choong-Sup;Jonghwa Chang
    • Nuclear Engineering and Technology
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    • 제33권1호
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    • pp.46-61
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    • 2001
  • The neutron cross sections of $^{160}$ Dy, $^{161}$ Dy, $^{162}$ Dy, $^{l63}$Dy, and $^{164}$ Dy have been evaluated in the resonance region of which upper energy is set to several tens of keV. The cross sections are formulated with resonance parameters in the energy region under consideration. In the resolved resonance region, the positive-energy resonance parameters were adopted from the BNL compilation published in 1984 with slight, if any, modifications. A bound level resonance for each isotope except $^{162}$ Dy was invoked to reproduce the reference 2200 m/s cross sections and the bound coherent scattering length. Subsequently, the statistical behavior of the resolved resonance parameters was analyzed, and thus obtained s-wave average parameters were adopted in the unresolved resonance region. In addition, recent measurements of the capture cross sections in the unresolved region were taken into account in adjusting the average resonance parameters for high orbital angular momentum resonances. The present evaluation resulted in large improvements in the cross sections over the ENDF/B-Vl release 6.6.

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Design and neutronic analysis of the intermediate heat exchanger of a fast-spectrum molten salt reactor

  • Terbish, Jamiyansuren;van Rooijen, W.F.G.
    • Nuclear Engineering and Technology
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    • 제53권7호
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    • pp.2126-2132
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    • 2021
  • Various research groups and private interprises are pursuing the design of a Molten Salt Reactor (MSR) as one of the Generation-IV concepts. In the current work a fast neutron MSR using chloride fuel is analyzed, specially analyzing the power production and neutron flux level in the Intermediate Heat Exchanger (IHX). The neutronic analysis in this work is based on a chloride-fuel MSR with 600 MW thermal power. The core power density was set to 100 MW m-3 with a core H/D [[EQUATION]] 1.0 amd four Intermediate Heat Exchanger (IHX). This leads to a power of 150 MW per IHX; this power is also comparable to the IHX proposed in the SAMOFAR framework. In this work, a preliminary design of a 150 MW helical-coil IHX for a chloride-fueled MSR is prepared and the fission rate, capture rate, and inelastic scatter rate are evaluated.

붕소 중성자 포획 치료에서 치료 영역 영상화를 위한 예비 연구 (Preliminary Study for Imaging of Therapy Region from Boron Neutron Capture Therapy)

  • 정주영;윤도군;한성민;장홍석;서태석
    • 한국의학물리학회지:의학물리
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    • 제25권3호
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    • pp.151-156
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    • 2014
  • 본 연구의 목적은 붕소 중성자 포획 치료 시 집적된 붕소 영역에서 중성자 선속의 변화와 그에 따른 방출된 즉발 감마선의 검출 시뮬레이션을 통하여 치료 영역에 대한 영상화의 가능성을 확인하고자 함이다. 전산 모사를 통하여 (1) 붕소 유무에 따른 중성자의 영향, (2) 내부와 외부에서의 즉발 감마선량 검출, (3) 즉발 감마선에 대한 에너지 스펙트럼 검출을 수행하였다. 모든 전산 모사는 Monte Carlo n-particle extended (MCNPX, Ver.2.6.0, Los Alamos National Laboratory, Los Alamos, NM, USA)를 이용하여 가상의 물 팬텀과 열중성자(thermal neutron) 소스, 붕소 영역을 지정하였다. 열중성자의 에너지는 1 eV 이하의 에너지였으며 선속은 2,000,000 n/sec.로 설정하였다. 이 때, 발생된 즉발 감마선의 검출은 물 팬텀과 수직 방향으로 위치시키고 납으로 둘러싸인 lutetium-yttrium oxyorthosilicate (Lu0,6Y1,4Si0,5:Ce; LYSO) 섬광체 검출기를 이용하였다. 붕소가 존재하는 영역인 5 cm 깊이에서의 28 분할로서 대략 0.18 cm의 bin을 도출하여 붕소 영역의 얕은 깊이에서부터 급격하게 저하되는 것을 확인하였다. 또한 붕소 영역이 시작되는 지점인 9 cm 깊이에서 감마선의 피크 레벨을 확인하였다. 그리고 478 keV 지점에서 정확한 즉발 감마선 피크가 관찰되는 것을 확인하였다. 478 keV의 즉발 감마선 피크는 41 keV의 반치폭으로 에너지 분해능 값은 8.5%로 측정되었다. 결론적으로 붕소 중성자 포획 치료 시 발생되는 즉발 감마선의 계측으로 치료가 행해지는 부위를 감마 카메라 또는 단일 광자 방출 단층 촬영 기기에서 영상화할 수 있는 가능성을 확인하였다.