• Title/Summary/Keyword: Gamma-ray spectrum

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Assessment of Nuclear Characteristics of NAA #1 Irradiation Hole in HANARO Research Reactor for Application of the $K_0$-NAA Methodology

  • Moon, Jong-Hwa;Kim, Sun-Ha;Chung, Yong-Sam;Dung, Ho-Mahn
    • Nuclear Engineering and Technology
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    • v.34 no.6
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    • pp.566-573
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    • 2002
  • Neutron activation analysis based on $textsc{k}$$_{o}$-standardization method# ($textsc{k}$o-NAA) is Com as one of the most remarkable progresses of the NAA with advantages of experimental simplicity, high accuracy, excellent flexibility with respect to irradiation and counting conditions, and suitability for computerization. This study was carried out to determine the reactor neutron spectrum parameters, i.e. $\alpha$ and f as the main factors of irradiation quality at NAA #1 irradiation hole on HANARO research reactor, to evaluate peak detection efficiency of the gamma-ray spectrometer for the use in the $textsc{k}$$_{o}$ experiments and to compare the measured concentration results with the certified values of some SRMs applying the experimentally determined to-parameters.ers.

MDA Assessment of NaI(Tl), LaBr3(Ce), and CeBr3 Detectors for Freshly Deposited Radionuclides on the Soil (지표면 침적 방사성핵종에 대한 NaI(Tl), LaBr3(Ce) 및 CeBr3 검출기의 MDA 비교 평가)

  • Lee, Jun-Ho;Kim, Bong-Gi;Lee, Dong Myung;Byun, Jong-In
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.17 no.3
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    • pp.321-328
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    • 2019
  • The detection performances of the NaI(Tl), $LaBr_3$(Ce) and $CeBr_3$ scintillation detectors, which can be used to rapidly evaluate the major artificial radionuclides deposited on the soil surface in a nuclear accident or radiological emergency, were compared. Detection performance was assessed by calculating the minimum detectable activity (MDA). The detection efficiency of each detector for artificial radionuclides was semi-empirically determined using mathematical modelling and point-like sources having certified radioactivity. The background gamma-ray energy spectrum for MDA evaluation was obtained from relatively wide and flat grassland, and the MDA values of each detector for the major artificial radionuclides that could be released in nuclear accidents were calculated. As a result, the relative MDA values of each detector regarding surface deposition distribution at normal environmental radiation level were evaluated as high in the order of the NaI(Tl), $LaBr_3$(Ce), and $CeBr_3$ detectors. These results were compared based on each detector's intrinsic and measurement environment background, detection efficiency, and energy resolution for the gamma-ray energy region of the radionuclide of interest.

Measurement of MDA of Soil Samples Using Unsuppression System and Compton Suppression of Environmental Radioactivity in Processing Technology (환경 방사능 처리기술에서의 Compton suppression 및 Unsuppression system을 이용한 토양시료의 MDA 측정)

  • Kang, Suman;Im, Inchul;Lee, Jaeseung;Jang, Eunsung;Lee, Mihyeon;Kwon, Kyungtae;Kim, Changtae
    • Journal of the Korean Society of Radiology
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    • v.8 no.6
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    • pp.293-299
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    • 2014
  • Compton suppression device is a device by using the Compton scattering reaction and suppress the Compton continuum portion of the spectrum, so can be made more clear analysis of gamma ray peak in the Compton continuum region. Measurements above background occurs or, radioactivity counts of radioactivity concentration value of $^{40}K$ nuclides $^{137}Cs$ and natural radioactivity artificial radioactivity detected from the surface soil sample, unwanted non-target analysis and interference peak who dotted line you know the calibration of the measurement energy is allowed to apply the (Compton suppression) non-suppressed spectrum inhibition spectrum and (Compton Unsuppression) the background to the measured value of the activity concentration value of the standard-ray source is detected relative to the peak of By measuring according to the different distances cause $^{137}Cs$, and comparative analysis of the Monte Carlo simulation, in order to obtain a detection capability for efficient, looking at the Compton inhibitor, as the CSF value increases with increase in the distance, more It was found that the background due to Compton continuum of the measured spectrum suppression mode Compton unrestrained mode can know that the Compton suppression many were made, using a $^{137}Cs$ is reduced.

Growth and Characterization of ZnSe Thin Film for Blue Diode (청색 Diode 개발을 위한 ZnSe 박막성장과 특성에 관한 연구)

  • 박창선;홍광준
    • Proceedings of the Korean Institute of Electrical and Electronic Material Engineers Conference
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    • 2001.07a
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    • pp.533-538
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    • 2001
  • The ZnSe sample grown by chemical bath deposition (CBD) method were annealed in Ar gas at 450$^{\circ}C$ Using extrapolation method of X-ray diffraction pattern, it was found to have zinc blend structure whose lattice parameter a$\_$o/ was 5.6687 ${\AA}$. From Hall effect, the mobility was likely to be decreased by impurity scattering at temperature range from 10 K to 150 K and by lattice scattering at temperature range from 150 K to 29 3K. The band gap given by the transmission edge changed from 2.7005 eV at 293 K to 2.8739 eV at 10 K. Comparing photocurrent peak position with transmission edge, we could find that photocurrent peaks due to excition electrons from valence band, $\Gamma$$\_$8/ and $\Gamma$$\_$7/ to conduction band $\Gamma$$\_$6/ were observed at photocurrent spectrum. From the photocurrent spectra by illumination of polarized light on the ZnSe thin film, we have found that values of spin orbit coupling splitting Δso is 0.0981 eV. From the PL spectra at 10 K, the peaks corresponding to free bound excitons and D-A pair and a broad emission band due to SA is identified. The binding energy of the free excitons are determined to be 0.0612 eV and the dissipation energy of the donor -bound exciton and acceptor-bound exciton to be 0.0172 eV, 0.0310 eV, respectively.

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Pulse pileup correction method for gamma-ray spectroscopy in high radiation fields

  • Lee, Minju;Lee, Daehee;Ko, Eunbie;Park, Kyeongjin;Kim, Junhyuk;Ko, Kilyoung;Sharma, Manish;Cho, Gyuseong
    • Nuclear Engineering and Technology
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    • v.52 no.5
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    • pp.1029-1035
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    • 2020
  • The detector suffers from pulse pileup by overlapping of the signals when it was used in high radiation fields. The pulse pileup deteriorates the energy spectrum and causes count losses due to random co-incidences, which might not resolve within the resolving time of the detection system. In this study, it is aimed to propose a new pulse pileup correction method. The proposed method is to correct the start point of the pileup pulse. The parameters are obtained from the fitted exponential curve using the peak point of the previous pulse and the start point of the pileup pulse. The amplitude at the corrected start point of the pileup pulse can be estimated by the peak time of the pileup pulse. The system is composed of a NaI (Tl) scintillation crystal, a photomultiplier tube, and an oscilloscope. A 61 μCi 137Cs check-source was placed at a distance of 3 cm, 5 cm, and 10 cm, respectively. The gamma energy spectra for the radioisotope of 137Cs were obtained to verify the proposed method. As a result, the correction of the pulse pileup through the proposed method shows a remarkable improvement of FWHM at 662 keV by 29, 39, and 7%, respectively.

The detection efficiency study of NaI(Tl) scintillation detector with the different numbers of SiPMs

  • Wang, Bao;Zhang, Xiongjie;Wang, Qingshan;Wang, Dongyang;Li, Dong;Xiahou, Mingdong;Zhou, Pengfei;Ye, Hao;Hu, Bin;Zhang, Lijiao
    • Nuclear Engineering and Technology
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    • v.54 no.7
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    • pp.2564-2571
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    • 2022
  • SiPMs are generally coupled into whole columns in gamma energy spectrum measurement, but the relationship between the distribution of whole SiPM columns and the energy resolution of the measured energy spectra is rarely reported. In this work, ∅ 3 × 3 inch NaI scintillator is placed on an 8 × 8 SiPM array, and the energy resolution of the 137Cs peak at 662 keV corresponding to the γ-ray is selected as a reference. Each SiPM is switched to explore the influence of the number of SiPM arrays, distribution position, and reflective layer on the energy resolution of SiPMs. Results show that without coupling, the energy resolution is greatly improved when the number of SiPMs ranges from 4 to 32. However, after 32 slices (the area covered by SiPMs relative to the scintillator reaches 25.9%), the improvement in energy resolution and total pulse count is not obvious. In addition, the position of SiPMs relative to the scintillator does not exert much impact on the energy resolution. Results also indicate that by adding a reflective film (ESR), the energy resolution of the tested group increases by 10.38% on average. This work can provide a reference for the design and application of miniaturized SiPM gamma spectrometers.

Development of High-Sensitivity and Entry-Level Nuclide Analysis Module (고감도 보급형 핵종 분석 모듈 개발)

  • Oh, Seung-Jin;Lee, Joo-Hyun;Lee, Seung-Ho
    • Journal of IKEEE
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    • v.26 no.3
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    • pp.515-519
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    • 2022
  • In this paper, we propose the development of a high-sensitivity entry-level nuclide analysis module. The proposed measurement sensor module consists of an electronic driving circuit for nuclide analysis resolution, prototype production with nuclide analysis function, and GUI development applied to prototypes. The electronic part driving circuit for nuclide analysis resolution is divided into nuclide analysis resolution process by the electronic part driving circuit block diagram, MCU circuit design used for radiation measurement, and PC program design for Spectrum acquisition. Prototyping with nuclide analysis function is made by adding a 128×128 pixel OLED display, three buttons for operation, a Li-ion battery, and a USB-C type port for charging the battery. The GUI development department applied to the prototype develops the screen composition such as the current time, elapsed measurement time, total count, and nuclide Spectrum. To evaluate the performance of the proposed measurement sensor module, an expert witness test was conducted. As a result of the test, it was confirmed that the calculated result by applying the resolution formula to the Spectrum (FWHM@662keV) obtained using the Cs-137 standard source in the nuclide analysis device had a resolution of 17.77%. Therefore, it was confirmed that the nuclide analysis resolution method proposed in this paper produces improved performance while being cheaper than the existing commercial nuclide analysis module.

LATEST RESULTS OF THE MAXI MISSION

  • MIHARA, TATEHIRO
    • Publications of The Korean Astronomical Society
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    • v.30 no.2
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    • pp.559-563
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    • 2015
  • Monitor of All-sky X-ray Image (MAXI) is a Japanese X-ray all-sky surveyer mounted on the International Space Station (ISS). It has been scanning the whole sky since 2009 during every 92-minute ISS rotation. X-ray transients are quickly found by the real-time nova-search program. As a result, MAXI has issued 133 Astronomer's Telegrams and 44 Gamma-ray burst Coordinated Networks so far. MAXI has discovered six new black holes (BH) in 4.5 years. Long-term behaviors of the MAXI BHs can be classified into two types by their outbursts; a fast-rise exponential-decay type and a fast-rise flat-top one. The slit camera is suitable for accumulating data over a long time. MAXI issued a 37-month catalog containing 500 sources above a ~0.6 mCrab detection limit at 4-10 keV in the region ${\mid}{b}{\mid}$ > $10^{\circ}$. The SSC instrument utilizing an X-ray CCD has detected diffuse soft X-rays extending over a large solid angle, such as the Cygnus super bubble. MAXI/SSC has also detcted a Ne emission line from the rapid soft X-ray nova MAXI J0158-744. The overall shapes of outbursts in Be X-ray binaries (BeXRB) are precisely observed with MAXI/GSC. BeXRB have two kinds of outbursts, a normal outburst and a giant one. The peak dates of the subsequent giant outbursts of A0535+26 repeated with a different period than the orbital one. The Be stellar disk is considered to either have a precession motion or a distorted shape. The long-term behaviors of low-mass X-ray binaries (LMXB) containing weakly magnetized neutron stars are investigated. Transient LMXBs (Aql X-1 and 4U 1608-52) repeated outbursts every 200-1000 days, which is understood by the limit-cycle of hydrogen ionization states in the outer accretion disk. A third state (very dim state) in Aql X-1 and 4U 1608-52 was interpreted as the propeller effect in the unified picture of LMXB. Cir X-1 is a peculiar source in the sense that its long-term behavior is not like typical LMXBs. The luminosity sometimes decreases suddenly at periastron. It might be explained by the stripping of the outer accretion disk by a clumpy stellar wind. MAXI observed 64 large flares from 22 active stars (RS CVns, dMe stars, Argol types, young stellar objects) over 4 years. The total energies are $10^{34}-10^{36}$ erg $s^{-1}$. Since MAXI can measure the spectrum (temperature and emission measure), we can estimate the size of the plasma and the magnetic fields. The size sometimes exceeds the size of the star. The magnetic field is in the range of 10-100 gauss, which is a typical value for solar flares.

Statistical Analysis of Count Rate Data for On-line Seawater Radioactivity Monitoring

  • Lee, Dong-Myung;Cong, Binh Do;Lee, Jun-Ho;Yeo, In-Young;Kim, Cheol-Su
    • Journal of Radiation Protection and Research
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    • v.44 no.2
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    • pp.64-71
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    • 2019
  • Background: It is very difficult to distinguish between a radioactive contamination source and background radiation from natural radionuclides in the marine environment by means of online monitoring system. The objective of this study was to investigate a statistical process for triggering abnormal level of count rate data measured from our on-line seawater radioactivity monitoring. Materials and Methods: Count rate data sets in time series were collected from 9 monitoring posts. All of the count rate data were measured every 15 minutes from the region of interest (ROI) for $^{137}Cs$ ($E_{\gamma}=661.6keV$) on the gamma-ray energy spectrum. The Shewhart ($3{\sigma}$), CUSUM, and Bayesian S-R control chart methods were evaluated and the comparative analysis of determination methods for count rate data was carried out in terms of the false positive incidence rate. All statistical algorithms were developed using R Programming by the authors. Results and Discussion: The $3{\sigma}$, CUSUM, and S-R analyses resulted in the average false positive incidence rate of $0.164{\pm}0.047%$, $0.064{\pm}0.0367%$, and $0.030{\pm}0.018%$, respectively. The S-R method has a lower value than that of the $3{\sigma}$ and CUSUM method, because the Bayesian S-R method use the information to evaluate a posterior distribution, even though the CUSUM control chart accumulate information from recent data points. As the result of comparison between net count rate and gross count rate measured in time series all the year at a monitoring post using the $3{\sigma}$ control charts, the two methods resulted in the false positive incidence rate of 0.142% and 0.219%, respectively. Conclusion: Bayesian S-R and CUSUM control charts are better suited for on-line seawater radioactivity monitoring with an count rate data in time series than $3{\sigma}$ control chart. However, it requires a continuous increasing trend to differentiate between a false positive and actual radioactive contamination. For the determination of count rate, the net count method is better than the gross count method because of relatively a small variation in the data points.

Radioactive Concentrations in Chemical Fertilizers

  • Gwang-Ho Kim;Jae-Hwan Cho
    • Journal of Radiation Protection and Research
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    • v.47 no.4
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    • pp.195-203
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    • 2022
  • Background: The aim of the present study was to determine radioactive concentrations in fertilizers known to contain essential nutrients. Results of this study could be used as basic data to monitor the impact of chemical fertilizers on the environment and public health. Nitrogen fertilizers, calcium fertilizers, sulfur fertilizers, phosphate acid fertilizers, and potassium chloride fertilizers were used in this study. Materials and Methods: Five chemical fertilizers were pulverized, placed in polyethylene containers, and weighed. The time to measure each specimen was set to be 3,600 seconds for a scintillator-based gamma-ray spectroscopy system. Concentration of gamma radionuclide was analyzed based on obtained spectra. At the end of the measurement, the spectrum file was stored and used to calculate radioactive concentrations using a gamma-ray spectrometer software. Results and Discussion: In the nitrogen fertilizer, 3.49 ± 5.71 Bq/kg of 137Cs, 34.43 ± 7.61 Bq/kg of 134Cs, and 569.16 ± 91.15 of 40K were detected whereas 131I was not detected. In the calcium fertilizer, 5.74 ± 4.40 Bq/kg of 137Cs (the highest concentration among all fertilizers), 22.37 ± 5.39 Bq/kg of 134Cs, and 433.67 ± 64.24 Bq/kg of 40K were detected whereas 131I was not detected. In the sulfur fertilizer, 347.31 ± 55.73 Bq/kg of 40K, 19.42 ± 4.53 Bq/kg of 134Cs, 2.21 ± 3.49 of 137Cs, and 0.04 ± 0.22 Bq/Kg of 131I were detected. In the phosphoric acid fertilizer, 70,007.34 ± 844.18 Bq/kg of 40K (the highest concentration among all fertilizers) and 46.07 ± 70.40 Bq/kg of 134Cs were detected whereas neither 137Cs nor 131I was detected. In the potassium chloride fertilizer, 12,827.92 ± 1542.19 Bq/kg of 40K was and 94.76 ± 128.79 Bq/kg of 134Cs were detected whereas neither 137Cs nor 131I was detected. The present study examined inorganic fertilizers produced by a single manufacturer. There might be different results according to the country and area from which fertilizers are imported. Further studies about inorganic fertilizers in more detail are needed to create measures to reduce 40K. Conclusion: Measures are needed to reduce radiation exposure to 40K contained in fertilizers including phosphoric acid and potassium chloride fertilizers.