• Title/Summary/Keyword: Atmospheric aerosol

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Physical Characteristics of Atmospheric Aerosols in Seoul : Scattering of Visible Light (서울 대기 Aerosol의 물리적 특성 : 가시광선의 산란)

  • 김필수
    • Journal of Korean Society for Atmospheric Environment
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    • v.4 no.2
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    • pp.28-37
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    • 1988
  • Light scattering coefficient of visible light by atmospheric aerosol over the size range 0.01-10$\mu$m is determined from scattering efficiency and aerosol size distribution. Aerosol number distribution as a function of particle diameter dN/dlog D decreases rapidly as increasing particle size. Distribution of scattering coefficient d$\sigma_s/dlog$ D is mostly accumulated in diameter 0.1-2.0 $\mu$m showing its maximum in the vicinity of 0.6$\mu$m. This means that the visible light in the atmosphere is mainly scattered by these particles. Diurnal variation of scattering coefficient $\sigma_s$ appears its maximum in the morning, while minimum in the afternoon which agrees with the aerosol number distribution in the size range 0.1-2.0 $\mu$m.

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Numerical Computation of the Mass Transfer between Gaseous and Particulate Materials Considering the Hysteresis Phenomena of Atmospheric Aerosol (에어로솔의 이력현상을 고려한 대기 중 기체상/입자상 간의 물질전달 수치모사)

  • Kim, Du-Eil;Yoo, Kee-Youn
    • Journal of Korean Society for Atmospheric Environment
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    • v.26 no.2
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    • pp.202-218
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    • 2010
  • It is well known that the atmospheric inorganic aerosol has the hysteresis phenomena depending on the history of relative humidity. However, the current computational researches have assumed that the physical/chemical state of atmospheric aerosol is only determined by a branch of hysteresis, efflorescence or deliquescence. In this work, we applied the MATLAB-based UHAEROm thermodynamics module to simulate the dynamic interaction between gaseous species $NH_3$ and $HNO_3$, and the two mono-disperse particulate populations in the course of efflorescence and deliquescence, respectively. We conducted the 10 case studies considering the particulate phase with the atmospherically prevailing chemical composition and found that the final states of the particles are determined through the qualitatively five different trajectories by the dynamic interaction between gaseous and two different kinds of particulates. As a result, we show that the coexistence of meta-stable and stable particles drives the different physical/chemical destination comparing with the ones generated from the solitary efflorescence or deliquescence branch.

An Iterative Algorithm to Estimate LIDAR Ratio for Thin Cirrus Cloud over Aerosol Layer

  • Wang, Zhenzhu;Liu, Dong;Xie, Chenbo;Zhou, Jun
    • Journal of the Optical Society of Korea
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    • v.15 no.3
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    • pp.209-215
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    • 2011
  • A new iterative algorithm is developed to estimate LIDAR ratio for a thin cirrus cloud over an aerosol layer. First, the thin cirrus cloud is screened out and replaced by a modeled LIDAR signal and the extinction coefficients of the aerosol layer are derived using the Fernald backward method. These aerosol coefficients are referred as the "actual values". Second, the original LIDAR signal which includes the thin cirrus cloud is also inverted by the Fernald backward method down to the aerosol layer but using different LIDAR ratio for the thin cirrus cloud. Depending on the different assumptions about the LIDAR ratio of the thin cirrus cloud, different sets of aerosol extinction can be derived. The "actual values" which are found in the first step can be used to constrain this iterative progress and the correct LIDAR ratio of the thin cirrus cloud can be found. The detailed description of this method and retrieval examples are given in the paper. The cases compared with other methods are presented and the statistical result is also shown and agrees well with other studies.

Aerosol Direct Radiative Forcing by Three Dimensional Observations from Passive- and Active- Satellite Sensors (수동형-능동형 위성센서 관측자료를 이용한 대기 에어러솔의 3차원 분포 및 복사강제 효과 산정)

  • Lee, Kwon-Ho
    • Journal of Korean Society for Atmospheric Environment
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    • v.28 no.2
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    • pp.159-171
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    • 2012
  • Aerosol direct radiative forcing (ADRF) retrieval method was developed by combining data from passive and active satellite sensors. Aerosol optical thickness (AOT) retrieved form the Moderate Resolution Imaging Spectroradiometer (MODIS) as a passive visible sensor and aerosol vertical profile from to the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) as an active laser sensor were investigated an application possibility. Especially, space-born Light Detection and Ranging (Lidar) observation provides a specific knowledge of the optical properties of atmospheric aerosols with spatial, temporal, vertical, and spectral resolutions. On the basis of extensive radiative transfer modeling, it is demonstrated that the use of the aerosol vertical profiles is sensitive to the estimation of ADRF. Throughout the investigation of relationship between aerosol height and ADRF, mean change rates of ADRF per increasing of 1 km aerosol height are smaller at surface than top-of-atmosphere (TOA). As a case study, satellite data for the Asian dust day of March 31, 2007 were used to estimate ADRF. Resulting ADRF values were compared with those retrieved independently from MODIS only data. The absolute difference values are 1.27% at surface level and 4.73% at top of atmosphere (TOA).

Major factors determining the size distributions of atmospheric water-soluble aerosol particles at an urban site during winter (겨울철 도시지역 대기 수용성 에어로졸 입자의 크기 분포를 결정하는 주요 인자)

  • Park, Seungshik
    • Particle and aerosol research
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    • v.17 no.3
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    • pp.43-54
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    • 2021
  • Size distributions of atmospheric particulate matter (PM) and its water-soluble organic and inorganic components were measured between January and February 2021 at an urban site in Gwangju in order to identify the major factors that determine their size distributions. Their size distributions during the study period were mainly divided into two groups. In the first group, PM, NO3-, SO42-, NH4+ and water-soluble organic carbon (WSOC) exhibited bi-modal size distributions with a dominant condensation mode at a particle size of 0.32 ㎛. This group was dominated by local production of secondary water-soluble components under atmospheric stagnation and low relative humidity (RH) conditions, rather than long-range transportation of aerosol particles from China. On the other hand, in the second group, they showed tri-modal size distributions with a very pronounced droplet mode at a diameter of 1.0 ㎛. These size distributions were attributable to the local generation and accumulation of secondary aerosol particles under atmospheric conditions such as atmospheric stagnation and high RH, and an increase in the influx of atmospheric aerosol particles by long-distance transportation abroad. Contributions of droplet mode NO3-, SO42-, NH4+ and WSOC to fine particles in the second group were significantly higher than those in the first group period. However, their condensation mode contributions were about two-fold higher in the first group than in the second group. The significant difference in the size distribution of the accumulation mode of the WSOC and secondary ionic components between the two groups was due to the influx of aerosol particles with a long residence time by long-distance transport from China and local weather conditions (e.g., RH).

An Analysis of Aerosol Optical Properties around Korea using AERONET (지상원격관측(AERONET)을 통한 한반도 주변 에어로솔 광학특성 분석)

  • Kim, Byung-Gon;Kim, You-Joon;Eun, Seung-Hee
    • Journal of Korean Society for Atmospheric Environment
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    • v.24 no.6
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    • pp.629-640
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    • 2008
  • This study investigates long-term trends and characteristics of aerosol optical depth ($\tau_a$) and Angstrom exponent (${\AA}$) around Korea in order to understand aerosol effects on the regional climate change. The analysis period is mainly from 1999 to 2006, and the analysis sites are Anmyun and Gosan, the background monitoring sites in Korea, and two other sites of Xianghe in China and Shirahama in Japan. The annual variations of $\tau_a$ at Anmyun and Gosan have slightly systematic increasing and decreasing trends, respectively. $\tau_a$ at Anmyun shows more substantial variation, probably because of it's being closer and vulnerable to anthropogenic influence from China and/or domestic sources than Gosan. Both values at Gosan and Anmyun are approximately 1.5 times greater than those at Shirahama. The monthly variation of $\tau_a$ exhibits the highest values at late Spring and the lowest at late-Summer, which are thought to be associated with the accumulation of fine aerosol formed through the photochemical reaction before the Jangma period and the scavenging effect after the Jangma period, respectively. Meanwhile, the episode-average $\tau_a$ for the Yellow dust period increases 2 times greater than that for the non-Yellow dust period. A significant decrease in ${\AA}$ for the Yellow dust period is attributable to an increase in the loading of especially the coarse particles. Also we found no weekly periodicity of $\tau_a$'s, but distinct weekly cycle of $PM_{10}$ concentrations, such as an increase on weekdays and a decrease on weekends at Anmyun and Gosan. We expect these findings would help to initiate a study on aerosol-cloud interactions through the combination of surface aerosol and satellite remote sensing (MODIS, Calipso and CloudSat) in East Asia.

Visibility Estimated from the Multi-wavelength Sunphotometer during the Winter 2011 Intensive Observation Period at Seoul, Korea (2011년 겨울철 서울시 대기 집중 관측 기간 동안 다파장 복사계로 분석된 에어러솔 연직분포와 시정 거리)

  • Lee, Kwon-Ho;Kim, Kyung-Won;Kim, Gwanchul;Jung, Kweon;Lee, Soon-Hee
    • Journal of Korean Society for Atmospheric Environment
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    • v.29 no.5
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    • pp.682-691
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    • 2013
  • The aerosol extinction vertical profile and surface visibility have been derived from the Microtops-II sunphotometer observation during the winter 2011 intensive observation period (IOP) at Seoul, Korea. Using models of degradation of aerosol optical thickness (AOT) and aerosol scale height, we have performed extinction-visibility modulation to determine the height dependent aerosol extinction and visibility. It is shown that the aerosol loading is relatively low during IOP (mean $AOT_{550}=0.22{\pm}0.08$, ${\AA}$ngstr$\ddot{o}$m exponent=$1.14{\pm}0.26$). Modeled extinction by use of Microtops II sunphotometer data shows good agreement with measurements by the Multi-wavelenth Polarization Lidar (MPoLAR), and the derived surface visibility are consistent with data from the transmissometer. These results emphasize the use of a vertically resolved extinction from AOT to predict visibility conditions at ground level.

An Algorithm to Determine Aerosol Extinction Below Cirrus Cloud from Mie-LIDAR Signals

  • Wang, Zhenzhu;Wu, Decheng;Liu, Dong;Zhou, Jun
    • Journal of the Optical Society of Korea
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    • v.14 no.4
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    • pp.444-450
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    • 2010
  • The traditional approach to inverting aerosol extinction makes use of the assumption of a constant LIDAR ratio in the entire Mie-LIDAR signal profile using the Fernald method. For the large uncertainty in the cloud optical depth caused by the assumed constant LIDAR ratio, an not negligible error of the retrieved aerosol extinction below the cloud will be caused in the backward integration of the Fernald method. A new algorithm to determine aerosol extinction below a cirrus cloud from Mie-LIDAR signals, based on a new cloud boundary detection method and a Mie-LIDAR signal modification method, combined with the backward integration of the Fernald method is developed. The result shows that the cloud boundary detection method is reliable, and the aerosol extinction below the cirrus cloud found by inverting from the modified signal is more efficacious than the one from the measured signal including the cloud-layer. The error due to modification is less than 10% taken in our present example.

Comparison of particle size distribution and particle number concentration measured by APS 3321 and Dust Monitor 1.108 (APS 3321과 Dust Monitor 1.108을 이용한 입자 크기분포 및 수농도 측정결과 비교)

  • Lim, Kyoung-Soo;Park, Hyun-Seol
    • Particle and aerosol research
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    • v.5 no.2
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    • pp.63-70
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    • 2009
  • The size distribution and number concentration of atmospheric aerosol were measured and compared using APS 3321 and Dust Monitor 1.108. The particle size distribution and number concentration measured by two devices were also compared at a particle generation system of standard PSL and fly ash. The number concentration of atmospheric aerosol measured by APS was higher than that by Dust Monitor in particle size range of less than $3.0{\mu}m$, but there was good accordance between them in particle size range of over $3.0{\mu}m$. In the particle generation system of PSL and fly ash, different measurement results were shown because the particle concentration was higher than that of atmospheric aerosol. The number concentration measured by Dust Monitor was higher than that by APS in most particle size ranges. However, the peak concentration of PSL particles measured by Dust Monitor was lower than that by APS. The difference of the collection efficiency in a scrubber by APS and Dust Monitor measurement was less than 10%, but in the particle size of $1.5{\mu}m$, it was over 20%.

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