• Title/Summary/Keyword: Aerosol data

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Development and Performance Evaluation of Radial Exhaust Multi-port System for Real-time Particle Size Distribution Measurement (실시간 입자분포 측정을 위한 Radial Exhaust Multi-port System의 개발 및 성능평가)

  • Lee, Hong Ku;Lee, Yang-Woo;Jeon, Ki Soo;Ahn, Kang-Ho
    • Particle and aerosol research
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    • v.9 no.3
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    • pp.133-137
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    • 2013
  • Measuring particle size distribution is one of the primary concerns in aerosol studies. For a nano-particle size distribution measurement, many scientists use a combination of a differential mobility analyzer (DMA) and a condensation particle counter (CPC) system, which is a called scanning mobility particle sizer (SMPS). Although it has a very high particle size resolution, some issues still remain. These problems include residence time between a DMA and a CPC, discontinuity of a CPC, and disturbance due to long scanning time during the precise measurement of particles. In particular, long scanning time is not adequate for measuring particle size distribution since the particle concentration is changing during the measurement. In this study, we developed radial exhaust multi-port system (REM-system) with no scanning time and high resolution to measure real-time particle size distribution. As a result of the REM-system performed using mono-disperse particle, it is expected that this system will be suitable for measuring continuously changing aerosol. If the counting efficiency of multi-condensation particle counter (M-CPC) and data inversion matrix are completed, REM-system will be a very adequate system for unsteady aerosol, which changes for SMPS scanning time.

Nephelometer Measurement of Aerosol Scattering Coefficients at Seoul (네펠로미터로 관측한 서울의 에어러솔 산란계수 특성)

  • Shim, Sungbo;Yoon, Young Jun;Yum, Seong Soo;Cha, Joo Wan;Kim, Jong Hwan;Kim, Jhoon;Lee, Bang-Yong
    • Atmosphere
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    • v.18 no.4
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    • pp.459-474
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    • 2008
  • Aerosol scattering coefficients for three different wavelengths ($\lambda$=450,550,700 nm) are measured almost continuously by a nephelometer in Seoul for a period of 13 months (February 2007-February 2008), which includes two weeks break in August 2007 for measurements at Daegwallyeong and YoungJongdo. The mean of the daily average scattering coefficients at $\lambda$=550 nm is $194.1{\pm}144.2Mm^{-1}$ and the minimum and maximum are $14.3Mm^{-1}$ and $998.1Mm^{-1}$, respectively. The scattering coefficient shows a general increasing trend with atmospheric relative humidity (RH). When the data are classified according to weather conditions, the days with no major weather events show the smallest scattering coefficient and also the lowest RH. Surprisingly haze/fog days show the largest scattering coefficient and Asian dust days comes in second. Although the variation is large within a season, winter shows the largest and autumn shows the smallest scattering coefficient. The average ${\AA}ngstr{\ddot{o}}m$ exponent is $1.40{\pm}0.32$ for the entire Seoul measurement. As expected, Asian dust days show the smallest ${\AA}ngstr{\ddot{o}}m$ exponent and haze/fog days are the next, suggesting more efficient hygroscopic growth of aerosols for this weather condition. Aerosol scattering coefficient seems to show better correspondence with CCN concentration rather than total aerosol concentration, which may indicate that CCN active aerosols are also good scattering aerosols.

Synthesis of Multiwall Carbon Nanotube/Graphene Composite by Aerosol Process and Its Characterization for Supercapacitors (에어로졸 공정에 의한 Multiwall carbon nanotube/Graphene 복합체 제조 및 슈퍼커패시터 특성평가)

  • Jo, Eun Hee;Kim, Sun Kyung;Chang, Hankwon;Lee, Chong Min;Park, Su-Ryeon;Choi, Ji-hyuk;Jang, Hee Dong
    • Particle and aerosol research
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    • v.12 no.4
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    • pp.127-134
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    • 2016
  • A multiwall carbon nanotube (MWCNT)/graphene (GR) composite was synthesized for an enhanced supercapacitor. Aerosol spray pyrolysis (ASP) was employed to synthesize the MWCNT/GR composites using a colloidal mixture of MWCNT and graphene oxide (GO). The effect of the weight ratio of the MWCNT/GO on the particle properties including the morphology and layered structure were investigated. The morphology of MWCNT/GR composites was generally the shape of a crumpled paper ball, and the average composite size was about $5{\mu}m$. MWCNT were uniformly dispersed in GR sheets and the MWCNT not only increase the basal spacing but also bridge the defects for electron transfer between GR sheets. Thus, it was increasing electrolyte/electrode contact area and facilitating transportation of electrolyte ion and electron in the electrode. Electrochemical data demonstrate that the MWCNT/GR (weight ratio=0.1) composite possesses a specific capacitance of 192 F/g at 0.1 A/g and good rate capability (88% capacity retention at 4 A/g) using two-electrode testing system.

The variation of aerosol optical depth over the polar stations of Korea (남북극 과학기지에서의 에어로졸 광학 깊이 변동성)

  • Koo, Ja-Ho;Choi, Taejin;Cho, Yeseul;Lee, Hana;Kim, Jaemin;Ahn, Dha Hyun;Kim, Jhoon;Lee, Yun Gon
    • Particle and aerosol research
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    • v.13 no.4
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    • pp.141-150
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    • 2017
  • Using the NASA's Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis for aerosol optical depth (AOD) and satellite-observed carbon monoxide (CO) data, we examined the basic pattern of AOD variations over the three polar stations of Korea: Jangbogo and King Sejong stations in the Antarctica, and Dasan station in the Arctic area. AOD values at King Sejong and Dasan station show the maximum peaks in spring, which looks associated with the high amount of atmospheric CO emitted from the natural burning and the biomass burning. Jangbogo station shows the much less AOD compared to other two stations, and seems not strongly affected by the transport of airborne particles generated from mid-latitude regions. All three polar stations show the AOD increasing trend in general, indicating that the polar background air quality becomes polluted.

Application of MODIS Aerosol Data for Aerosol Type Classification (에어로졸 종류 구분을 위한 MODIS 에어로졸 자료의 적용)

  • Lee, Dong-Ha;Lee, Kwon-Ho;Kim, Young-Joon
    • Korean Journal of Remote Sensing
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    • v.22 no.6
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    • pp.495-505
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    • 2006
  • In order to classify aerosol type, Aerosol Optical Thickness (AOT) and Fine mode Fraction (FF), which is the optical thickness ratio of small particles$(<1{\mu}m)$ to total particles, data from MODIS (MODerate Imaging Spectraradiometer) aerosol products were analyzed over North-East Asia during one year period of 2005. A study area was in the ocean region of $20^{\circ}N\sim50^{\circ}N$ and $110^{\circ}E\simt50^{\circ}E$. Three main atmospheric aerosols such as dust, sea-salt, and pollution can be classified by using the relationship between AOT and FF. Dust aerosol has frequently observed over the study area with relatively high aerosol loading (AOT>0.3) of large particles (FF<0.65) and its contribution to total AOT in spring was up to 24.0%. Pollution aerosol, which is originated from anthropogenic sources as well as a natural process like biomass burning, has observed in the regime of high FF (>0.65) with wide AOT variation. Average pollution AOT was $0.31{\pm}0.05$ and its contribution to total AOT was 79.8% in summer. Characteristic of sea-salt aerosol was identified with low AOT (<0.3), almost below 0.1, and slightly higher FF than dust and lower FF than pollution. Seasonal analysis results show that maximum AOT $(0.33{\pm}0.11)$ with FF $(0.66{\pm}0.21)$ in spring and minimum AOT $(0.19{\pm}0.05)$, FF $(0.60{\pm}0.14)$ in fall were observed in the study area. Spatial characteristic was that AOT increasing trend is observed as closing to the eastern part of China due to transport of aerosols from China by the prevailing westerlies.

Sensitivity of Aerosol Optical Parameters on the Atmospheric Radiative Heating Rate (에어로졸 광학변수가 대기복사가열률 산정에 미치는 민감도 분석)

  • Kim, Sang-Woo;Choi, In-Jin;Yoon, Soon-Chang;Kim, Yumi
    • Atmosphere
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    • v.23 no.1
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    • pp.85-92
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    • 2013
  • We estimate atmospheric radiative heating effect of aerosols, based on AErosol RObotic NETwork (AERONET) and lidar observations and radiative transfer calculations. The column radiation model (CRM) is modified to ingest the AERONET measured variables (aerosol optical depth, single scattering albedo, and asymmetric parameter) and subsequently calculate the optical parameters at the 19 bands from the data obtained at four wavelengths. The aerosol radiative forcing at the surface and the top of the atmosphere, and atmospheric absorption on pollution (April 15, 2001) and dust (April 17~18, 2001) days are 3~4 times greater than those on clear-sky days (April 14 and 16, 2001). The atmospheric radiative heating rate (${\Delta}H$) and heating rate by aerosols (${\Delta}H_{aerosol}$) are estimated to be about $3\;K\;day^{-1}$ and $1{\sim}3\;K\;day^{-1}$ for pollution and dust aerosol layers. The sensitivity test showed that a 10% uncertainty in the single scattering albedo results in 30% uncertainties in aerosol radiative forcing at the surface and at the top of the atmosphere and 60% uncertainties in atmospheric forcing, thereby translated to about 35% uncertainties in ${\Delta}H$. This result suggests that atmospheric radiative heating is largely determined by the amount of light-absorbing aerosols.

Characteristics of Aerosol Mass Concentration and Chemical Composition of the Yellow and South Sea around the Korean Peninsula Using a Gisang 1 Research Vessel (기상1호에서 관측된 한반도 서해 및 남해상의 에어로졸 질량농도와 화학조성 특성)

  • Cha, Joo Wan;Ko, Hee-Jung;Shin, Beomchel;Lee, Hae-Jung;Kim, Jeong Eun;Ahn, Boyoung;Ryoo, Sang-Boom
    • Atmosphere
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    • v.26 no.3
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    • pp.357-372
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    • 2016
  • Northeast Asian regions have recently become the main source of anthropogenic and natural aerosols. Measurement of aerosols on the sea in these regions have been rarely conducted since the experimental campaigns such as ACE-ASIA (Asian Pacific Regional Aerosol Characterization Experiment) in 2001. Research vessel observations of aerosol mass and chemical composition were performed on the Yellow and south sea around the Korean peninsula. The ship measurements showed six representative cases such as aerosol event and non-event cases during the study periods. On non-event cases, the anthropogenic chemical and natural soil composition on the Yellow sea were greater than those on the south sea. On aerosol event cases such as haze, haze with dust, and dust, the measured mass concentrations of anthropogenic chemical and element compositions were clearly changed by the events. In particular, methanesulfonate ($MSA^-$, $CH_3SO_3^-$), a main component of natural oceanic aerosol important for sulfur circulation on Earth, was first observed by the vessel in Korea, and its concentration on the Yellow sea was three times that on the south sea during the study period. Sea salt concentration important to chemical composition on the sea is related to wind speed. Coefficients of determination ($R^2$) between wind speed and sea salt concentration were 0.68 in $PM_{10}$ and 0.82 in $PM_{2.5}$. Maximum wave height was not found to be correlated to the sea salt concentration. When sea-salt comes into contact with pollutants, the total sea-salt mass is reduced, i.e., a loss of $Cl^-$ concentration from NaCl, the main chemical composing sea salt, is estimated by reaction with $HNO_3$(gas) and $H_2SO_4$(gas). The $Cl^-$ concentration loss by $SO_4^{2-}$ and $NO_3^-$ more easily increased for $PM_{10}$ compared to $PM_{2.5}$. The results of this study will be applied to verifying a dust-haze forecasting model. In addition, continued vessel measurements of aerosol data will become important to research for climate change studies in the future.

Quantitative Source Estimation of Particulate Matters in Suwon Area Using the Target Transformation Factor Analysis Based on Size Segregation Scheme (입경 분류에 입각하여 목표변환 인자분석법을 이용한 수원지역 분진 오염원의 정량적 기여도 추정)

  • 김동술;이태정
    • Journal of Korean Society for Atmospheric Environment
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    • v.9 no.1
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    • pp.44-50
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    • 1993
  • The suspended particulate matters had been collected by a cascade impactor having 9 size fragnated stages for 2 years (Dec. 1989 to Nov. 1991) in Kyung Hee University-Suwon Campus. The particulate matters were then collected on each stage by membrane filters. The weight concentration on each stage was estimated by a microbalance and further chemical element concentrations were determined by an XRF system. The study focused on developing of a receptor model using the TTFA (target transformation factor analysis) to apportion aerosol mass with the 30 ambient data sets. Each data set consists of the 8 size-ranged subdata sets characterized by 13 element variables. Even though a couple of sources could not be identified, three to five sources were extracted from each aerosol size-range, and then 9 statistical source profiles were generated. Finally, source contribution of particulate matters on each size-range could be estimated in Suwon area.

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Influence of atmospheric aerosol on satellite ocean color data in the East/Japan Sea (동해에서 대기에어로졸이 해색위성자료에 미치는 영향)

  • Yamada, Keiko;Kim, Sang-Woo
    • Proceedings of KOSOMES biannual meeting
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    • 2009.06a
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    • pp.53-54
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    • 2009
  • The influence of atmospheric aerosol on satellite ocean color data were evaluated using SeaWiFS monthly standard mapped image products. The atmospheric optical thickness (AOT) was increased in spring and summer, and it showed the strong positive correlation with remote sensing reflectance, normalized waterleaving radiance /solar irradiance, at 555 nm (Rrs555) which is a component of the satellite chlorophyll estimation. Such the high AOT and high Rrs555 pixels showed overestimation of satellite chlorophyll in spring, especially in the area which showed large phytoplankton absorption which 1s expressed by low remote sensing reflectance at 443, 490 and 510 nm (Rrs 443, Rrs490 and Rrs510).

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Numerical Simulation of Impactor Collection Efficiency according to Altitude (대기 고도에 따른 입자 포집용 관성 임팩터의 설계 및 포집효율 예측)

  • Kim, Gyuho;Yook, Se-Jin;Ahn, Kang-Ho
    • Particle and aerosol research
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    • v.8 no.1
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    • pp.1-8
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    • 2012
  • In this study, the collection efficiency of inertial impactors was numerically simulated by employing the statistical Lagrangian particle tracking(SLPT) model. The SLPT model was proven to be correct in predicting the impactor collection efficiency, when the numerically obtained collection efficiencies were compared with the experimental data of Marple et al.(1987) at normal pressure level and the experimental data of $Marjam{\ddot{a}}ki$ et al.(2000) at low pressure level. Based on the validation results, balloon-borne impactors with the cut-off sizes of $1{\mu}m$, $2.5{\mu}m$, and $10{\mu}m$ were designed. Then, the sampling flowrates of the inertial impactors, required to keep the cut-off sizes constant at different pressures and temperatures, were estimated according to the altitude.