• Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
• /
• v.19 no.1
• /
• pp.9-27
• /
• 2021

As an example of research activities in decontamination for decommissioning, new data are presented on the options for corrosion layer dissolution during the decommissioning decontamination, or persulfate regeneration for decontamination solutions re-use. For the management of spent decontamination solutions, new method based on solvent extraction of radionuclides into ionic liquid followed by electrodeposition of the radionuclides has been developed. Fields of applications of composite inorganic-organic absorbers or solid extractants with polyacrylonitrile (PAN) binding matrix for the treatment of liquid radioactive waste are reviewed; a method for americium separation from the boric acid containing NPP evaporator concentrates based on the TODGA-PAN material is discussed in more detail. Performance of a model of radionuclide transport, developed and implemented within the GoldSim programming environment, for the safety studies of the LLW/ILW repository is demonstrated on the specific case of the Richard repository (Czech Republic). Continuation and even broadening of these activities are expected in connection with the approaching end of the lifespan of the first blocks of the Czech NPPs.

• Nuclear Engineering and Technology
• /
• v.54 no.10
• /
• pp.3766-3777
• /
• 2022

It is essential to ensure the safety of spent nuclear fuel (SNF) transport cask in drop situation that is included in transport accident scenarios. The safety of the drop situation is affected by the impact absorption performance of impact limiters. Therefore, when designing an impact limiter, the uncertainty in the material properties that affect the impact absorption performance must be considered. In this study, the material properties of the wood inside the impact limiter were selected as the variables for a parametric study. The sensitivity analysis of the drop response of the SNF transport cask with impact limiter was performed. The minimum wood strength required to prevent a direct collision between the cask and floor was derived from the analysis results. In addition, the plastic strain response was analyzed and strain-based evaluation was performed. Based on this result, the critical values of wood properties that change the impact dynamic characteristics were investigated. Finally, the optimal material properties of wood were obtained to secure the structural safety of the SNF transport cask. The results of this study can contribute to the development of SNF transport cask, thereby ensuring safety in transport accident conditions.

• Nuclear Engineering and Technology
• /
• v.52 no.12
• /
• pp.2717-2724
• /
• 2020

Silicon, especially silicon in the form of SiO₂, is a major component of rocks. Final spent fuel storages, which are being designed, are located in suitable rock formations in the Earth's crust. Reduction of the uncertainty of silicon neutron scattering and capture is needed; improved silicon evaluations have been recently produced by the ORNL/IAEA collaboration within the INDEN project. This paper deals with the nuclear data validation of that evaluation performed at the LR-0 reactor by means of critical experiments and measurement of reaction rates. Large amounts of silicon were used both as pure crystalline silicon and SiO₂ sand. The critical moderator level was measured for various core configurations. Reaction rates were determined in the largest core configuration. Simulations of the experimental setup were performed using the MCNP6.2 code. The obtained results show the improvement in silicon cross-sections in the INDEN evaluations compared to existing evaluations in major libraries. The new Thermal Scattering Law for SiO₂ published in ENDF/B-VIII.0 additionally reduces the discrepancy between calculation and experiments. However, an unphysical peak is visible in the neutron spectrum in SiO₂ obtained by calculation with the new Thermal Scattering Law.

• Nuclear Engineering and Technology
• /
• v.54 no.5
• /
• pp.1579-1587
• /
• 2022

The effects of hydride amount (20-850 wppm), orientation (circumferential and radial), and temperature (room temperature, 100 ℃, 200 ℃) on the axial mechanical properties of Zircaloy-4 cladding were comprehensively examined. The fraction of radial hydride fraction in the cladding was quantified using PROPHET, an in-house radial hydride fraction analysis code. Uniaxial tensile tests (UTTs) were conducted at various temperatures to obtain the axial mechanical properties. Hydride orientation has a limited effect on the axial mechanical behavior of hydrided Zircaloy-4 cladding. Ultimate tensile stress (UTS) and associated uniform elongation demonstrated limited sensitivity to hydride content under UTT. Statistical uncertainty of UTS was found small, supporting the deterministic approach for the load-failure analysis of hydrided Zircaloy-4 cladding. These properties notably decrease with increasing temperature in the tested range. The dependence of yield strength on hydrogen content differed from temperature to temperature. The ductility-related parameters, such as total elongation, strain energy density (SED), and offset strain decrease with increasing hydride contents. The abrupt loss of ductility in UTT was found at ~700 wppm. Demonstrating a strong correlation between total elongation and offset strain, SED can be used as a comprehensive measure of ductility of hydrided zirconium alloy.

• Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
• /
• v.21 no.1
• /
• pp.1-8
• /
• 2023

The major concern in the deep geological disposal of spent nuclear fuels include sulfide-induced corrosion and stress corrosion cracking of copper canisters. Sulfur diffusion into copper canisters may induce copper embrittlement by causing Cu₂S particle formation along grain boundaries; these sulfide particles can act as crack initiation sites and eventually cause embrittlement. To prevent the formation of Cu₂S along grain boundaries and sulfur-induced copper embrittlement, copper alloys are designed in this study. Alloying elements that can act as chemical anchors to suppress sulfur diffusion and the formation of Cu₂S along grain boundaries are investigated based on the understanding of the microscopic mechanism of sulfur diffusion and Cu₂S precipitation along grain boundaries. Copper alloy ingots are experimentally manufactured to validate the alloying elements. Microstructural analysis using scanning electron microscopy with energy dispersive spectroscopy demonstrates that Cu₂S particles are not formed at grain boundaries but randomly distributed within grains in all the vacuum arc-melted Cu alloys (Cu-Si, Cu-Ag, and Cu-Zr). Further studies will be conducted to evaluate the mechanical and corrosion properties of the developed Cu alloys.

• Nuclear Engineering and Technology
• /
• v.55 no.3
• /
• pp.1009-1014
• /
• 2023

Muon tomography is a useful method for monitoring special nuclear materials (SNMs) such as spent nuclear fuel inside dry cask storage. Multiple Coulomb scattering of muons can be used to provide information about the 3-dimensional structure and atomic number(Z) of the inner materials. Tomography using muons is less affected by the shielding material and less harmful to health than other measurement methods. We developed a muon detector for muon tomography, which consists of a plastic scintillator, 64 long wavelength-shifting (WLS) fibers attached to the top of the plastic scintillator, and silicon photomultipliers (SiPMs) connected to both ends of each WLS fiber. The muon detector can acquire X and Y positions simultaneously using a position determination algorithm. The design parameters of the muon detector were optimized using DETECT2000 and Geant4 simulations, and a muon detector prototype was built based on the results. Spatial resolution measurement was performed using simulations and experiments to evaluate the feasibility of the muon detector. The experimental results were in good agreement with the simulation results. The muon detector has been confirmed for use in a muon tomography system.

• Journal of Radiation Protection and Research
• /
• v.47 no.4
• /
• pp.226-236
• /
• 2022

Background: An effective communication strategy for reducing conflicts in South Korea has been designed through the analysis of public perception and communication variables on nuclear power under the conditions of rapidly changing nuclear power policies. Materials and Methods: This study conducted both qualitative research through group discussions based on social psychology and quantitative research through surveys. Results and Discussion: Nuclear power plant (NPP) area residents in favor of nuclear power indicated higher levels of communication, safety perception, and contribution than those against it. NPP area residents trusted the civilian expert groups (18.3%) and local government (17.3%) the most, while metropolitan city residents trusted the Nuclear Safety and Security Commission and the Korea Institute of Nuclear Safety (20.7%) the most. In determining nuclear power policy, both the NPP area residents (18.1%) and metropolitan city residents (17.1%) prioritized safety, health, and the environment. While metropolitan city residents thought that energy security and economic growth (16.4%) were important, NPP area residents thought the current issue of spent fuel rods (14.1%) to be important. Conclusion: It is necessary for the nuclear power industry to have and actively implement communication and conflict resolution strategies based on the patterns obtained in the study results.

• Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
• /
• v.21 no.3
• /
• pp.411-417
• /
• 2023

During the operation of a nuclear power plant (NPP), the generation of radioactive waste, including dry active waste (DAW), concentrates, spent resin, and filters, mandates the implementation of appropriate disposal methods to adhere to Korea's waste acceptance criteria (WAC). In this context, this study investigates the potential use of polymer concrete (PC) as a high-integrity container (HIC) material for solidifying and packaging these waste materials. PC is a versatile composite material comprising binding polymers, aggregates, and additives, known for its exceptional strength and chemical stability. A comprehensive analysis of PC's long-term integrity was conducted in this study. First, its compressive strength, which is crucial for ensuring the structural stability of HICs over extended periods, was evaluated. Subsequently, the resilience of PC was tested under various stress conditions, including biological, radiological, thermal, and chemical stressors. The findings of this study indicate that PC exhibits remarkable long-term properties, demonstrating exceptional stability even when subjected to diverse stressors. The results therefore underscore the potential viability of PC as a reliable material for constructing high-integrity containers, thus contributing to the safe and sustainable management of radioactive waste in NPPs.

• Nuclear Engineering and Technology
• /
• v.56 no.5
• /
• pp.1913-1924
• /
• 2024

This paper presents the design and operation of an autonomous robot for pyroprocess automation, which requires unique approaches beyond those used in industrial applications to achieve the desired performance. Maintaining an extremely dry atmosphere is crucial to handle various materials, including chloride, and an autonomous system ensures this dry environment. The drying room dehumidifier was carefully selected and designed to generate dry air, and different types of dry air conditioning performance were evaluated, including assessing worker accessibility inside the mock-up to determine the system's feasibility. Containers used for process materials were modified to fit the gripper system of the gantry robot for automation. The loading and unloading of process materials in each equipment were automatically performed to connect the process equipment with the robotic system. The gantry robot primarily operated through macro motion to approach waypoints containing process materials, eliminating the need for precise approach motion. The robot's tapered jaw design allowed it to grasp the target object even with imperfect positioning. Robot motions were programmed using a robot simulator for initial positioning and motion planning, and real accuracy was tested in a mock-up facility using the OPC platform.

• Corrosion Science and Technology
• /
• v.23 no.4
• /
• pp.266-277
• /
• 2024

Due to its good corrosion and heat resistance with excellent mechanical properties, 304L stainless steel is commonly used in the fabrication of spent nuclear fuel dry storage canisters. However, welds are sensitive to stress corrosion cracking (SCC) due to residual stress generation. Although SCC resistance can be improved by stress relieving the weld and changing the chloride environment, it is difficult to change corrosion environment for certain applications. Stress control in the weld can improve SCC resistance. Ultrasonic shot peening (USP) needs further research as compressive residual stresses and microstructure changes due to plastic deformation may play a role in improving SCC resistance. In this study, 304L stainless steel was welded to generate residual stresses and exposed to a chloride environment after USP treatment to improve SCC properties. Effects of USP on SCC resistance and crack growth of specimens with compressive residual stresses generated more than 1 mm from the surface were studied. In addition, correlations of compressive residual stress, grain size, intergranular corrosion properties, and pitting potential with crack propagation rate were determined and the improvement of SCC properties by USP was analyzed.