• Title/Summary/Keyword: neutron shielding

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Optimization of target, moderator, and collimator in the accelerator-based boron neutron capture therapy system: A Monte Carlo study

  • Cheon, Bo-Wi;Yoo, Dohyeon;Park, Hyojun;Lee, Hyun Cheol;Shin, Wook-Geun;Choi, Hyun Joon;Hong, Bong Hwan;Chung, Heejun;Min, Chul Hee
    • Nuclear Engineering and Technology
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    • v.53 no.6
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    • pp.1970-1978
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    • 2021
  • The aim of this study was to optimize the target, moderator, and collimator (TMC) in a neutron beam generator for the accelerator-based BNCT (A-BNCT) system. The optimization employed the Monte Carlo Neutron and Photon (MCNP) simulation. The optimal geometry for the target was decided as the one with the highest neutron flux among nominates, which were called as angled, rib, and tube in this study. The moderator was optimized in terms of consisting material to produce appropriate neutron energy distribution for the treatment. The optimization of the collimator, which wrapped around the target, was carried out by deciding the material to effectively prevent the leakage radiations. As results, characteristic of the neutron beam from the optimized TMC was compared to the recommendation by the International Atomic Energy Agent (IAEA). The tube type target showed the highest neutron flux among nominates. The optimal material for the moderator and collimator were combination of Fluental (Al203+AlF3) with 60Ni filter and lead, respectively. The optimized TMC satisfied the IAEA recommendations such as the minimum production rate of epithermal neutrons from thermal neutrons: that was 2.5 times higher. The results can be used as source terms for shielding designs of treatment rooms.

New Boron Compound, Silicon Boride Ceramics for Capturing Thermal Neutrons (Possibility of the material application for nuclear power generation)

  • Matsushita, Jun-ichi
    • Proceedings of the Materials Research Society of Korea Conference
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    • 2011.05a
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    • pp.15-15
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    • 2011
  • As you know, boron compounds, borax ($Na_2B_4O_5(OH)_4{\cdot}8H_2O$) etc. were known thousands of years ago. As for natural boron, it has two naturally occurring and stable isotopes, boron 11 ($^{11}B$) and boron 10 ($^{10}B$). The neutron absorption $^{10}B$ is included about 19~20% with 80~81% $^{11}B$. Boron is similar to carbon in its capability to form stable covalently bonded molecular networks. The mass difference results in a wide range of ${\beta}$ values between the $^{11}B$ and $^{10}B$. The $^{10}B$ isotope, stable with 5 neutrons is excellent at capturing thermal neutrons. For example, it is possible to decrease a thermal neutron required for the nuclear reaction of uranium 235 ($^{235}U$). If $^{10}B$ absorbs a neutron ($^1n$), it will change to $^7Li+^1{\alpha}$ (${\alpha}$ ray, like $^4He$) with prompt ${\gamma}$ ray from $^{11}B$ $^{11}B$ (equation 1). $$^{10}B+^1n\;{\rightarrow}\;^{11}B\;{\rightarrow}\; prompt \;{\gamma}\;ray (478 keV), \;^7Li+4{\alpha}\;(4He)\;\;\;\;{\cdots}\; (1)$$ If about 1% boron is added to stainless steel, it is known that a neutron shielding effect will be 3 times the boron free steel. Enriched boron or $^{10}B$ is used in both radiation shielding and in boron neutron capture therapy. Then, $^{10}B$ is used for reactivity control and in emergency shutdown systems in nuclear reactors. Furthermore, boron carbide, $B_4C$, is used as the charge of a nuclear fission reaction control rod material and neutron cover material for nuclear reactors. The $B_4C$ powder of natural B composition is used as a charge of a control material of a boiling water reactor (BWR) which occupies commercial power reactors in nuclear power generation. The $B_4C$ sintered body which adjusted $^{10}B$ concentration is used as a charge of a control material of the fast breeder reactor (FBR) currently developed aiming at establishment of a nuclear fuel cycle. In this study for new boron compound, silicon boride ceramics for capturing thermal neutrons, preparation and characterization of both silicon tetraboride ($SiB_4$) and silicon hexaboride ($SiB_6$) and ceramics produced by sintering were investigated in order to determine the suitability of this material for nuclear power generation. The relative density increased with increasing sintering temperature. With a sintering temperature of 1,923 K, a sintered body having a relative density of more than 99% was obtained. The Vickers hardness increased with increasing sintering temperature. The best result was a Vickers hardness of 28 GPa for the $SiB_6$ sintered at 1,923K for 1 h. The high temperature Vickers hardness of the $SiB_6$ sintered body changed from 28 to 12 GPa in the temperature range of room temperature to 1,273 K. The thermal conductivity of the SiB6 sintered body changed from 9.1 to 2.4 W/mK in the range of room temperature to 1,273 K.

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Study on the design and experimental verification of multilayer radiation shield against mixed neutrons and γ-rays

  • Hu, Guang;Hu, Huasi;Yang, Quanzhan;Yu, Bo;Sun, Weiqiang
    • Nuclear Engineering and Technology
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    • v.52 no.1
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    • pp.178-184
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    • 2020
  • The traditional methods for radiation shield design always only focus on either the structure or the components of the shields rather than both of them at the same time, which largely affects the shielding performance of the facilities, so in this paper, a novel method for designing the structure and components of shields simultaneously is put forward to enhance the shielding ability. The method is developed by using the genetic algorithm (GA) and the MCNP software. In the research, six types of shielding materials with different combinations of elements such as polyethylene (PE), lead (Pb) and Boron compounds are applied to the radiation shield design, and the performance of each material is analyzed and compared. Then two typical materials are selected based on the experiment result of the six samples, which are later verified by the Compact Accelerator Neutron Source (CANS) facility. By using this method, the optimal result can be reached rapidly, and since the design progress is semi-automatic for most procedures are completed by computer, the method saves time and improves accuracy.

Synthesis, physical, optical and radiation shielding properties of Barium-Bismuth Oxide Borate-A novel nanomaterial

  • B.M. Chandrika;Holaly Chandrashekara Shastry Manjunatha;K.N. Sridhar;M.R. Ambika;L. Seenappa;S. Manjunatha;R. Munirathnam;A.J. Clement Lourduraj
    • Nuclear Engineering and Technology
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    • v.55 no.5
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    • pp.1783-1790
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    • 2023
  • Barium Bismuth Oxide Borate (BBOB) has been synthesized for the first time using solution combustion technique. SEM analysis reveal flower shape of the nanoparticles. The formation of the nanoparticles has been confirmed through XRD & FTIR studies which gives the physical and chemical structure of the novel material. The UV light absorption is observed in the range 200-300 nm. The present study highlights the radiation shielding ability of BBOB for different radiations like X/Gamma rays, Bremsstrauhlung and neutrons. The gamma shielding efficiency is comparable to that of lead in lower energy range and lesser than lead in the higher energy range. The bremsstrauhlung exposure constant is comparably larger for BBOB NPs than that of concrete and steel however it is lesser than that of lead. The beauty of BBOB nanoparticles lies in, high absorption of radiations and low emission of secondary radiations when compared to lead. In addition, the neutron shielding parameters like scattering length, absorption and scattering cross sections of BBOB are found to be much better than lead, steel and concrete. Thus, BBOB nanoparticles are highly efficient in absorbing X/Gamma rays, neutrons and bremsstrauhlung radiations.

Effectiveness of the neutron-shield nanocomposites for a dual-purpose cask of Bushehr's Water-Water Energetic Reactor (VVER) 1000 nuclear-power-plant spent fuels

  • Rezaeian, Mahdi;Kamali, Jamshid;Ahmadi, Seyed Javad;Kiani, Mohammad Amin
    • Nuclear Engineering and Technology
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    • v.49 no.7
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    • pp.1563-1570
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    • 2017
  • In order to perform dry interim storage and transportation of the spent-fuel assemblies of the Bushehr Nuclear Power Plant, dual-purpose casks can be utilized. The effectiveness of different neutron-shield materials for the dual-purpose cask was analyzed through a set of calculations carried out using the Monte Carlo N-Particle (MCNP) code. The dose rate for the dual-purpose cask utilizing the recently developed materials of $epoxy/clay/B_4C$ and $epoxy/clay/B_4C/carbon$ fiber was less than the allowable radiation level of 2 mSv/h at any point and 0.1 mSv/h at 2 m from the external surface of the cask. By utilization of $epoxy/clay/B_4C$ instead of an ethylene glycol/water mixture, the dose rates on the side surface of the cask due to neutron sources and consequent secondary gamma rays will be reduced by 17.5% and 10%, respectively. The overall dose rate in this case will be reduced by 11%.

Simulation, design optimization, and experimental validation of a silver SPND for neutron flux mapping in the Tehran MTR

  • Saghafi, Mahdi;Ayyoubzadeh, Seyed Mohsen;Terman, Mohammad Sadegh
    • Nuclear Engineering and Technology
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    • v.52 no.12
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    • pp.2852-2859
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    • 2020
  • This paper deals with the simulation-based design optimization and experimental validation of the characteristics of an in-core silver Self-Powered Neutron Detector (SPND). Optimized dimensions of the SPND are determined by combining Monte Carlo simulations and analytical methods. As a first step, the Monte Carlo transport code MCNPX is used to follow the trajectory and fate of the neutrons emitted from an external source. This simulation is able to seamlessly integrate various phenomena, including neutron slowing-down and shielding effects. Then, the expected number of beta particles and their energy spectrum following a neutron capture reaction in the silver emitter are fetched from the TENDEL database using the JANIS software interface and integrated with the data from the first step to yield the origin and spectrum of the source electrons. Eventually, the MCNPX transport code is used for the Monte Carlo calculation of the ballistic current of beta particles in the various regions of the SPND. Then, the output current and the maximum insulator thickness to avoid breakdown are determined. The optimum design of the SPND is then manufactured and experimental tests are conducted. The calculated design parameters of this detector have been found in good agreement with the obtained experimental results.

Verification of multilevel octree grid algorithm of SN transport calculation with the Balakovo-3 VVER-1000 neutron dosimetry benchmark

  • Cong Liu;Bin Zhang;Junxia Wei;Shuang Tan
    • Nuclear Engineering and Technology
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    • v.55 no.2
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    • pp.756-768
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    • 2023
  • Neutron transport calculations are extremely challenging due to the high computational cost of large and complex problems. A multilevel octree grid algorithm (MLTG) of discrete ordinates method was developed to improve the modeling accuracy and simulation efficiency on 3-D Cartesian grids. The Balakovo-3 VVER-1000 neutron dosimetry benchmark is calculated to verify and validate this numerical technique. A simplified S2 synthetic acceleration is used in the MLTG calculation method to improve the convergence of the source iterations. For the triangularly arranged fuel pins, we adopt a source projection algorithm to generate pin-by-pin source distributions of hexagonal assemblies. MLTG provides accurate geometric modeling and flexible fixed source description at a lower cost than traditional Cartesian grids. The total number of meshes is reduced to 1.9 million from the initial 9.5 million for the Balakovo-3 model. The numerical comparisons show that the MLTG results are in satisfactory agreement with the conventional SN method and experimental data, within the root-mean-square errors of about 4% and 10%, respectively. Compared to uniform fine meshing, approximately 70% of the computational cost can be saved using the MLTG algorithm for the Balakovo-3 computational model.

Comparison of Physics Model for 600 MeV Protons and 290 MeV·n-1 Oxygen Ions on Carbon in MCNPX

  • Lee, Arim;Kim, Donghyun;Jung, Nam-Suk;Oh, Joo-Hee;Oranj, Leila Mokhtari;Lee, Hee-Seock
    • Journal of Radiation Protection and Research
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    • v.41 no.2
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    • pp.123-131
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    • 2016
  • Background: With the increase in the number of particle accelerator facilities under either operation or construction, the accurate calculation using Monte Carlo codes become more important in the shielding design and radiation safety evaluation of accelerator facilities. Materials and Methods: The calculations with different physics models were applied in both of cases: using only physics model and using the mix and match method of MCNPX code. The issued conditions were the interactions of 600 MeV proton and $290MeV{\cdot}n^{-1}$ oxygen with a carbon target. Both of cross-section libraries, JENDL High Energy File 2007 (JENDL/HE-2007) and LA150, were tested in this calculation. In the case of oxygen ion interactions, the calculation results using LAQGSM physics model and JENDL/HE-2007 library were compared with D. Satoh's experimental data. Other Monte Carlo calculations using PHITS and FLUKA codes were also carried out for further benchmarking study. Results and Discussion: It was clearly found that the physics models, especially intra-nuclear cascade model, gave a great effect to determine proton-induced secondary neutron spectrum in MCNPX code. The variety of physics models related to heavy ion interactions did not make big difference on the secondary particle productions. Conclusion: The variations of secondary neutron spectra and particle transports depending on various physics models in MCNPX code were studied and the result of this study can be used for the shielding design and radiation safety evaluation.

A study on the calculation of the shielding wall thickness in Medical Linear Accelerator (의료용 선형가속기 차폐벽의 두께 산정에 관한 연구)

  • Lee, Dong-Yeon;Park, Eun-Tae;Kim, Jung-Hoon
    • Journal of radiological science and technology
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    • v.40 no.2
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    • pp.281-287
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    • 2017
  • The purpose of this study is to calculate the thickness of shielding for concrete which is mainly used for radiation shielding and study of the walls constructed to shield medical linear accelerator. The optimal shielding thickness was calculated using MCNPX(Ver.2.5.0) for 10 MV of photon beam energy generated by linear accelerator. As a result, the TVL for photon shielding was formed at 50~100 cm for pure concrete and concrete with Boron+polyethylene at 80~100 cm. The neutron shielding was calculated 100~140 cm for pure concrete and concrete with Boron+polyethylene at 90~100 cm. Based on this study, the concrete is considered to be most efficient method of using steel plates and adding Boron+polyethylene th the concrete.

Development of Neutron Induced Prompt γ-ray Spectroscopy System Using 252Cf (252Cf 선원을 이용한 즉발감마선 계측시스템 구성)

  • Park, Yong-Joon;Song, Byung-Chul;Jee, Kwang-Yong
    • Analytical Science and Technology
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    • v.16 no.1
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    • pp.12-24
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    • 2003
  • For the design and set-up of neutron induced prompt ${\gamma}$-ray spectroscopy system using $^{252}Cf$ neutron source, the effects of shielding and moderator materials have been examined. The $^{252}Cf$ source being used for TLD badge calibration in Korea Atomic Energy Research Institute was utilized for this preliminary experiment. The ${\gamma}$-ray background and prompt ${\gamma}$-ray spectrum of the sample containing Cl were measured using HPGe (GMX 60% relative efficiency) located at the inside of the system connected to notebook PC at the outside of the system (about 20 meter distance). The background activities of neutron and ${\gamma}$-rays were measured with neutron survey meter as well as ${\gamma}$-ray survey meters, respectively and the system was designed to minimize the activities. Prompt ${\gamma}$-ray spectrum was measured using ${\gamma}$-${\gamma}$ coincident system for reduce the background and the continuum spectrum. The optimum system was designed and set up using the experimental data obtained.