• Title/Summary/Keyword: gamma-radiation

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Study on the Illite Modification for Removal of Radioactive Cesium in Water Environment near Nuclear Facilities (원자력 시설 인근 수계에서 방사성 세슘 제거를 위한 일라이트 개질 연구)

  • Hwang, Jeonghwan;Choung, Sungwook;Shin, Woosik;Han, Weon Shik
    • Economic and Environmental Geology
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    • v.51 no.2
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    • pp.113-120
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    • 2018
  • Radioactive cesium($^{137}Cs$) can be released into the environment through severe nuclear accidents such as the Chernobyl and Fukushima, The $^{137}Cs$ is one of major monitoring radionuclides due to its chemical toxicity, ${\gamma}$ radiation and long half-life($t_{1/2}=30.2yrs$). It has been known well that illite adsorb selectively and strongly the cesium due to frayed edge sites. The quantity of the FES in the illite could be controlled by weathering processes. Therefore, this study was modified illite samples through artificial weathering in the laboratory to increase sorption efficiency for cesium. Abundant interlayer cations(i.e., K, Ca) were eluted within 1 day, while Si and Al were gradually released from the crystal structure. In addition, broad peaks of XRD indicated the occurrence of chemical weathering. The cesium sorption distribution coefficients increased up to approximately 2 times after the weathering. These results suggested that sorption capacity of illite could be enhanced for cesium through artificial weathering under low temperature.

A Study on the Assessment of Source-term for PWR Primary System Using MonteCarlo Code (MonteCarlo 코드를 이용한 PWR 일차 계통 선원항 평가에 관한 연구)

  • Song, Jong Soon;Lee, Sang Heon;Shin, Seung Su
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.16 no.3
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    • pp.331-337
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    • 2018
  • The decommissioning of nuclear power plants is generally executed in five steps, including preparation, decontamination, cutting/demolition, waste disposal and environmental restoration. So, for efficient decommissioning of nuclear power plants, worker safety, effects compared to cost, minimization of waste, possibility of reuse, etc., shall be considered. Worker safety and measurement technology shall be secured to exert optimal efficiency of nuclear power plant decommissioning work, for which accurate measurement technology for systems and devices is necessary. Typical In-Situ methods for decommissioning of nuclear plants are CZT, Gamma Camera and ISOCS. This study used ISOCS, which can be applied during the decommissioning of a nuclear power plant site without collecting representative samples, to take measurements of the S/G Water Chamber. To validate the measurement values, Microshield and the GEANT4 code was used as the actual method were used for modeling, respectively. The comparison showed a difference of $1.0{\times}10^1Bq$, which indicates that it will be possible to reduce errors due to the influence of radiation in the natural environment and the precision of modeling. Based on the research results of this paper, accuracy and reliability of measurement values will be analyzed and the applicability of the direct measurement method during the decommissioning of NPPs will be assessed.

Gamma Knife Radiosurgery for Metastatic Brain Tumors with Exophytic Hemorrhage

  • Park, Eun Suk;Lee, Eun Jung;Yun, Jung-Ho;Cho, Young Hyun;Kim, Jeong Hoon;Kwon, Do Hoon
    • Journal of Korean Neurosurgical Society
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    • v.61 no.5
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    • pp.592-599
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    • 2018
  • Objective : Metastatic brain tumors (MBTs) often present with intracerebral hemorrhage. Although Gamma Knife surgery (GKS) is a valid treatment option for hemorrhagic MBTs, its efficacy is unclear. To achieve oncologic control and reduce radiation toxicity, we used a radiosurgical targeting technique that confines the tumor core within the hematoma when performing GKS in patients with such tumors. We reviewed our experience in this endeavor, focusing on local tumor control and treatment-associated morbidities. Methods : From 2007 to 2014, 13 patients with hemorrhagic MBTs were treated via GKS using our targeting technique. The median marginal dose prescribed was 23 Gy (range, 20-25). GKS was performed approximately 2 weeks after tumor bleeding to allow the patient's condition to stabilize. Results : The primary sites of the MBTs included the liver (n=7), lung (n=2), kidney (n=1), and stomach (n=1); in two cases, the primary tumor was a melanoma. The mean tumor volume was $4.00cm^3$ (range, 0.74-11.0). The mean overall survival duration after GKS was 12.5 months (range, 3-29), and three patients are still alive at the time of the review. The local tumor control rate was 92% (tumor disappearance 23%, tumor regression 46%, and stable disease 23%). There was one (8%) instance of local recurrence, which occurred 11 months after GKS in the solid portion of the tumor. No GKS-related complications were observed. Conclusion : Our experience shows that GKS performed in conjunction with our targeting technique safely and effectively treats hemorrhagic MBTs. The success of this technique may reflect the presence of scattered metastatic tumor cells in the hematoma that do not proliferate owing to the inadequate microenvironment of the hematoma. We suggest that GKS can be a useful treatment option for patients with hemorrhagic MBTs that are not amenable to surgery.

New Boron Compound, Silicon Boride Ceramics for Capturing Thermal Neutrons (Possibility of the material application for nuclear power generation)

  • Matsushita, Jun-ichi
    • Proceedings of the Materials Research Society of Korea Conference
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    • 2011.05a
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    • pp.15-15
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    • 2011
  • As you know, boron compounds, borax ($Na_2B_4O_5(OH)_4{\cdot}8H_2O$) etc. were known thousands of years ago. As for natural boron, it has two naturally occurring and stable isotopes, boron 11 ($^{11}B$) and boron 10 ($^{10}B$). The neutron absorption $^{10}B$ is included about 19~20% with 80~81% $^{11}B$. Boron is similar to carbon in its capability to form stable covalently bonded molecular networks. The mass difference results in a wide range of ${\beta}$ values between the $^{11}B$ and $^{10}B$. The $^{10}B$ isotope, stable with 5 neutrons is excellent at capturing thermal neutrons. For example, it is possible to decrease a thermal neutron required for the nuclear reaction of uranium 235 ($^{235}U$). If $^{10}B$ absorbs a neutron ($^1n$), it will change to $^7Li+^1{\alpha}$ (${\alpha}$ ray, like $^4He$) with prompt ${\gamma}$ ray from $^{11}B$ $^{11}B$ (equation 1). $$^{10}B+^1n\;{\rightarrow}\;^{11}B\;{\rightarrow}\; prompt \;{\gamma}\;ray (478 keV), \;^7Li+4{\alpha}\;(4He)\;\;\;\;{\cdots}\; (1)$$ If about 1% boron is added to stainless steel, it is known that a neutron shielding effect will be 3 times the boron free steel. Enriched boron or $^{10}B$ is used in both radiation shielding and in boron neutron capture therapy. Then, $^{10}B$ is used for reactivity control and in emergency shutdown systems in nuclear reactors. Furthermore, boron carbide, $B_4C$, is used as the charge of a nuclear fission reaction control rod material and neutron cover material for nuclear reactors. The $B_4C$ powder of natural B composition is used as a charge of a control material of a boiling water reactor (BWR) which occupies commercial power reactors in nuclear power generation. The $B_4C$ sintered body which adjusted $^{10}B$ concentration is used as a charge of a control material of the fast breeder reactor (FBR) currently developed aiming at establishment of a nuclear fuel cycle. In this study for new boron compound, silicon boride ceramics for capturing thermal neutrons, preparation and characterization of both silicon tetraboride ($SiB_4$) and silicon hexaboride ($SiB_6$) and ceramics produced by sintering were investigated in order to determine the suitability of this material for nuclear power generation. The relative density increased with increasing sintering temperature. With a sintering temperature of 1,923 K, a sintered body having a relative density of more than 99% was obtained. The Vickers hardness increased with increasing sintering temperature. The best result was a Vickers hardness of 28 GPa for the $SiB_6$ sintered at 1,923K for 1 h. The high temperature Vickers hardness of the $SiB_6$ sintered body changed from 28 to 12 GPa in the temperature range of room temperature to 1,273 K. The thermal conductivity of the SiB6 sintered body changed from 9.1 to 2.4 W/mK in the range of room temperature to 1,273 K.

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Search of Characteristic for Dose Distribution Presented by Multi­isocentric Stereotactic Radiosurgical Plan Using Linear Accelerator (선형 가속기를 이용한 정위적 방사선 수술시 병소내 선량분포의 특성조사)

  • 최경식;오승종;이형구;최보영;전흥재;서태석
    • Progress in Medical Physics
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    • v.14 no.4
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    • pp.225-233
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    • 2003
  • The goal of a radiation treatment plan is to deliver a homogeneous dose to a target with minimal irradiation of the adjacent normal tissues. Dose uniformity is especially important for stereotactic radiosurgery using a linear accelerator. The dose uniformity and high dose delivery of a single spherical dose distribution exceed 70%. This also results with a similar stereotactic radiosurgical plan using a Gamma Knife. The dose distribution produced in a stereotactic radiosurgical plan using a Gamma Knife and Linear accelerator is spherical, and the application of the sphere packing arrangement in a real radiosurgical plan requires much time and skill. In this study, we found a characteristic of dose distribution with transformation of beam parameters that must be considered in a radiosurgical plan for effective radiosurgery. First, we assumed a cylinder type tumor model and a cube type tumor model. Secondly, the results of the tumor models were compared and analyzed with dose profiles and DVH_(Dose Volume Histogram) representative dose distribution. We found the optimal composition of beam parameters_(i.e. collimator size, number of isocenter, gap of isocenters etc.), which allowed the tumor models to be involved in the isodose curve at a high level. In conclusion, the characteristics found in this study are helpful for improving the effectiveness and speed of a radiosurgical plan for stereotactic radiosurgery.

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The Characteristics for BNCT facility in Hanaro Reactor

  • Soheigh Suh;Lee, Dong-Han;Ji, Young-Hoon;Lee, Dong-Hoon;Yoo, Seong-Yul;Rhee, Chang-Hun;Rhee, Soo-Yong;Jun, Byung-Jin
    • Proceedings of the Korean Society of Medical Physics Conference
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    • 2002.09a
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    • pp.161-163
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    • 2002
  • The BNCT(Boron Neutron Capture Therapy) facility has been developed in Hanaro(High-flux Advanced Neutron Application Reactor), a research reactor of Korea Atomic Energy Research Institute. A typical tangenial beam port is utilized with this BNCT facility. Thermal neutrons can be penetrated within the limits of the possible maximum instead of being filtered fast neutrons and gamma rays as much as possible using the silicon and bismuth single crystals. In addition to, the liquid nitrogen (LN$_2$) is used to cool down the silicon and bismuth single crystals for the increase of the penetrated thermal neutron flux. Neutron beams for BNCT are shielded using the water shutter. The water shutter was designed and manufactured not to interfere with any other subsystem of Hanaro when the BNCT facility is operated. Also, it is replaced with conventional beam port plug in order to cut off helium gas leakage in the beam port. A circular collimator, composed of $\^$6/Li$_2$CO$_3$ and polyethylene compounds, is installed at the irradiation position. The measured neutron flux with 24 MW reactor power using the Au-198 activation analysis method is 8.3${\times}$10$\^$8/ n/cm$^2$ s at the collimator, exit point of neutron beams. Flatness of neutron beams is proven to ${\pm}$ 6.8% at 97 mm collimator. According to the result of acceptance tests of the water shutter, the filling time of water is about 190 seconds and drainage time of it is about 270 seconds. The radiation leakages in the irradiation room are analyzed to near the background level for neutron and 12 mSv/hr in the maximum for gamma by using BF$_3$ proportional counter and GM counter respectively. Therefore, it is verified that the neutron beams from BNCT facility in Hanaro will be enough to utilize for the purpose of clinical and pre-clinical experiment.

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Crystal Structure of Probenecid, $C_{13}H_{19}NO_4S$ (Probenecid, $C_{13}H_{19}NO_4S$의 結晶構造)

  • Kim, Eui-Sung;Shin, Hyun-So
    • Journal of the Korean Chemical Society
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    • v.35 no.6
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    • pp.603-606
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    • 1991
  • The crystal structure of Probenecid has been determined from 2574 independent reflections collected on an automatic ENRAF-NONIUS CAD-4 diffractometer using graphite-monochromated $Mo-K{\alpa}$ radiation. The crystal is triclinic, space group P$\bar{1}$ with unit cell dimensions a = 7.535(2)${\AA}$, b = 18.473 (5)${\AA}$, c = 5.317(9)${\AA}$, ${\alpha} = 92.00(5)^{\circ}$, ${\beta} = 99.02(5)^{\circ}$, ${\gamma} = 94.89(2)^{\circ}$, V = 727.4(2)${\AA}^3$, Z = 2, $D_m$ = 1.310, $D_x$ = $1.302 gcm^{-3}$, ${\mu}$ = $1.88 cm^{-1}$, F(000) = 304, and T = 298 K. Final R = 0.0676 and $R_w$ = O.0630 for 1209 reflections > 5${\sigma}(F_o)$. In the spacial arrangement about N(13), the sum of bond angles about nitrogen is 350.9° and the nitrogen lies only 0.268(6)${\AA}$ out of S(1)-C(14)-C(17) plane. The S(1)-C(4) distance is 1.792(6)${\AA}$ and the C(4)-S(1)-N(13) angle is $106.5(3)^{\circ}$. The overall conformation of the molecule is folded with respect to sulfur.

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Study on the Mating Ability and Competitiveness of the Radiation Irradiated Males of Rice Stem Borer (Chile suppressalis Walker) (방사선 조사 이화명나방의 교미능력 및 경쟁력에 관한 연구)

  • Hyun Jai Sun;Ryu Joon;Chung Kyu Hoi;Kwon Shin Han
    • Korean journal of applied entomology
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    • v.11 no.1
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    • pp.25-30
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    • 1972
  • Five to seven day old pupae were irradiated with gamma rays, the mating ability, and competability of the irradiated males were examined. The results obtained are summarized as follows: 1. There is no difference in percentage of males that mated, nor in the maximum number of matings of the males, when individual matings were made, and fresh females were provided every day for his life time. 2. The average days for the first mating of the emerged were 1.5 days for the control, and 2.4 days for the males irradiated with 25 and 30 Krad. The average days between first and second mating were 3.0 days for the irradiated males, and 1.3 days for the control. 3. The average matings of a male were 1.2 and 2.5 times when 5 and 10 females were provided to a normal male respectively. No significant different in average numbers of mated female per male were observed between the normal and irradiated males. 4. To test the mating competitiveness of the irradiated and normal males (1:0, 1:1, 2:1, 1:2, 5:1, 1:5, 0:1) were confined together with five virgin females. The greatest reduction in hatching percentage was found with 5 : 1 : 1 (30 Krad) where $26.6\%$ was hatched.5, The results showed that the irradiated males were not fully competitive with normal males, but if the reduced number of eggs produced by the female mated with irradiated male is considered, it might be used sterile male techniques in rice stem borer control.

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Evaluation of Residual Radioactivity and Dose Rate of a Target Assembly in an IBA Cyclotron (IBA 사이클로트론 표적집합체에서의 잔류 방사화 분석 및 선량률 평가)

  • Hwang, Seon Yong;Kim, Youngju;Lee, Seung Wook
    • Journal of radiological science and technology
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    • v.39 no.4
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    • pp.643-649
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    • 2016
  • When a cyclotron produces $^{18}F^-$, accelerated protons interact with metal parts of the cyclotron machine and induces radioactivity. Especially, the target window and chamber of the target assembly are the main parts where long-lived radionuclides are generated as they are incident by direct beams. It is of great importance to identify radionuclides induced in the target assembly for the safe operation and maintenance of a cyclotron facility. In this study, we analyzed major radionuclides generated in the target assembly by an operation of the Cyclotron 18/9 machine and measured dose rates after the operation to establish the radiation safety guideline for operators and maintenance personnel of the machine. Gamma spectroscopy with HPGe was performed on samples from the target chamber and Havar foil target window to identify the radionuclides generated during the operation for production of $^{18}F^-$- isotope and their specific activity. Also, the dose rates from the target were measured as a function of time after an operation. These data will help improve radiological safety of operating the cyclotron facilities.

The distribution of 137Cs activities in sediment samples of South-Han River basin (남한강수계 하천 퇴적물 시료 중 137Cs 분포)

  • Kim, Jiyu;Kang, Tae-Woo;Hong, Jung-Ki;An, Mijeong;Chang, Chaewon;Kim, Kyunghyun;Han, Young-Un;Kang, Taegu
    • Analytical Science and Technology
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    • v.29 no.6
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    • pp.293-299
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    • 2016
  • $^{137}Cs$ was investigated in river bottom sediments located in South-Han River basin and it was compared with international case studies to estimate the concentration level of $^{137}Cs$ in river sediment of Korea. The obtained values of $^{137}Cs$ which was analyzed by gamma-ray spectrometry were in the range of <$MDA{\sim}3.80{\pm}0.14Bq/kg{\cdot}dry$ and similar to the $^{137}Cs$ activities in soil of Korea. According to international case studies, $^{137}Cs$ activities were between 3.7 to $15,396Bq/kg{\cdot}dry$, when pollutants such as nuclear power plant accidents and radiation leaks were present near the rivers. The $^{137}Cs$ activities showed a variety of distribution depending on the country, when pollution occurs and survey time. Also, $^{137}Cs$ activities of river sediments without pollution sources were mostly less than $10Bq/kg{\cdot}dry$ in other countries. It was comparable with the obtained $^{137}Cs$ activities in this study. The obtained values provide useful information on the background concentration of $^{137}Cs$ in river sediment and will be able to use a basis for determining contamination of $^{137}Cs$ in the river.