• Title/Summary/Keyword: atmospheric fine dust

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Characterization of Wintertime Atmospheric Aerosols in Seoul Using PIXE and Supplementary Analyzers

  • Ma, Chang-Jin;Mikio Kasahara;Hwang, Kyung-Chul;Yeo, Hyun-Gu;Park, Kum-Chan
    • Journal of Korean Society for Atmospheric Environment
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    • v.16 no.E
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    • pp.19-27
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    • 2000
  • Particle Induced X-ray Emission (PIXE) and Elemental Analysis Syztem (EAS) were applied to the investiga-tion of the Characteristics and sources of wintertime atmospheric aerosols in Seoul. Atmospheric aerosols were collected by both fine and coarse fractions using a two-stage filter pack sampler from Kon-Kuk university during the winter season of 1999. PIXE was applied to the analysis of the middle and heavy elements with atomic numbers greater than 14(Si) and EAS was applied to the measurement of the light elements such as H, C and N. The fact that 64.2% of mass of fine particles in Seoul consists of the light elements (N, C , and H) suggests that the measurement of light elements is extremely important. The average mass concentration is Seoul was 38.6$\mu\textrm{g}$m(sup)-3. Elements such as Ca, Fe, Mg, and Ti appeared to have very low Fine/Coarse ratios(0.1∼0.4), whereas che-mical components related to anthropogenic sources such as Br, V, Pb, and Zn were observed to accumulate in the fine fraction. In the Asian Dust Storm(ADS) event, the concentation of soil components increased dramatically. Reconstruction of the fine mass concentrations estimated by a newly revised simple model was fairly in good agreement with the measured ones. Source identification was attempted using the enrichment factor and Pearsons coefficient of correlation. The typical elements derived from each source could be classified by this method.

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A Study of Heavy Metal Pollutants in the Respirable Dust in Seoul Area (호흡성분진중의 중금속 오염도에 관한 조사연구)

  • Lim, Young-Wook;Chung, Young
    • Journal of Korean Society for Atmospheric Environment
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    • v.5 no.1
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    • pp.68-78
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    • 1989
  • The heavy metal of suspended particulates with human health has long been studied in environmental interest concerned. This study was intended to identify harmful heavy metals of the ambient air borne dusts which were related with the respirable sizes in the aerodynamics. Two sampling sites were selected comparatively; one was in the Shinchon area, which is the commercial district with heavy traffic and the other site was in the Bulgwang area which is residential area. The supended particulates were sampled by high volume air sample with 6 cascade impactor stages. The heavy metals in terms of As, Cd, Cr, Cu, Fe, Hg, Mn, Ni, Pb, Se, V and Zn were determined by stomic absorption spectrometry or inductively coupled plasma emission spectrometry. The samples weretaken bimothly for seven consecutive days from May 1987 to March 1988. The annual average concentration of the respirable suspended dust of which diameter is less than 10$\mum$ was 152.59 $\mug/m^3$ of the Shinchon air samples; the respirable dust was equivalent to approximately 85% of the total suspended particulates. The annual average concentration of the respirable suspended dust of the Bulgwang air samples was 112.56 $\mug/m^3$; that was approximately 86% of the total suspended particulates. The concentration of heavy metals was investigated in relation to the particle size. The concentration of Cr, Fe, Mn and V were tended to be much more in the coarse particles than in the fine particles. Cd and Pb in the fine particles were more than in the coarse particles. In the partial correlation coefficients; in the Shinchon area, high correlations among Fe, Se and Mn were determined; it is assumed that those sources would be originated from coal, gasolineand diesel. In Bulgwang area, would be high correlation among Fe, Se, Hg and Mn considered to be originated from coal, Bunker-C and heavy oil as well. From the above results, the hazardous heavy merals in air should be measured and controlled in originally their sources.

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Introducing SPARTAN Instrument System for PM Analysis (PM 관측을 위한 스파르탄 시스템)

  • Sujin Eom;Sang Seo Park;Jhoon Kim;Seoyoung Lee;Yeseul Cho;Seungjae Lee;Ehsan Parsa Javid
    • Atmosphere
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    • v.33 no.3
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    • pp.319-330
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    • 2023
  • As the need for PM type observation increases, Surface Particulate Matter Network (SPARTAN), PM samplers analyzes aerosol samples for PM mass concentration and chemical composition, were recently installed at two sites: Yonsei University at Seoul and Ulsan Institute of Science and Technology (UNIST) at Ulsan. These SPARTAN filter samplers and nephelometers provide the PM2.5 mass concentration and chemical speciation data with aerosol type information. We introduced the overall information and installation of SPARTAN at the field site in this study. After installation and observation, both Seoul and Ulsan sites showed a similar time series pattern with the daily PM2.5 mass concentration of SPARTAN and the data of Airkorea. In particular, in the case of high concentrations of fine particles, daily average value of PM2.5 was relatively well-matched. During the Yonsei University observation period, high concentrations were displayed in the order of sulfate, black carbon (BC), ammonium, and calcium ions on most measurement days. The case in which the concentration of nitrate ions showed significant value was confirmed as the period during which the fine dust alert was issued. From the data analysis, SPARTAN data can be analyzed in conjunction with the existing urban monitoring network, and it is expected to have a synergetic effect in the research field. Additionally, the possibility of being analyzed with optical data such as AERONET is presented. In addition, the method of installing and operating SPARTAN has been described in detail, which is expected to help set the stage for the observation system in the future.

Chemical Composition Characteristics of Size-fractionated Particles during Heavy Asian Dust Event in Spring, 2010 (2010년 봄철 고농도 황사의 입경별 화학조성 특성)

  • Lee, Dong-Eun;Kim, Won-Hyung;Ko, Hee-Jung;Oh, Yong-Soo;Kang, Chang-Hee
    • Journal of Korean Society for Atmospheric Environment
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    • v.29 no.3
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    • pp.325-337
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    • 2013
  • The size-fractionated aerosol samples have been collected at Gosan Site of Jeju Island during the spring season of 2010, in order to examine the chemical composition characteristics of the Asian Dust and Non-Asian Dust particles. The concentrations of ${HCO_3}^-$, Al, and nss-$Ca^{2+}$ in $PM_{10}$ had tremendously increased during the heavy Asian Dust (March 20, 2010). The concentration ratios of Asian Dust to Non-Asian Dust for the soil species (nss-$Ca^{2+}$, ${HCO_3}^-$, Al, Fe, Ti, Mn) were 12.2~30.7, meanwhile those for the anthropogenic species (nss-${SO_4}^{2-}$, ${NH_4}^+$, ${NO_3}^-$, $K^+$, Zn, Pb, and Cu) were 2.9~7.8. During the heavy Asian Dust event, the concentration increase of ${NO_3}^-$ in $PM_{2.5}$ were much more apparent than those of nss-${SO_4}^{2-}$ and ${NH_4}^+$, and the soil species (nss-$Ca^{2+}$ and ${HCO_3}^-$) showed much higher concentration increase. The neutralization factor of $NH_3$ was higher than that of $CaCO_3$. However, the neutralization factor of $CaCO_3$ in $PM_{10}$ was exceptionally high during the heavy Asian Dust, showing the evidence of heavy migration of soil particles. From the study for size fractionated particles, it was found that nss-${SO_4}^{2-}$ and ${NH_4}^+$ were mostly distributed in fine particle mode, on the other hand, ${NO_3}^-$ existed evenly in both fine and coarse particle modes, and the soil species (nss-$Ca^{2+}$, Al, Fe, etc.) were mainly in the latter mode. During the heavy Asian Dust, in particular, the concentrations of ${NH_4}^+$, nss-${SO_4}^{2-}$, $K^+$, Zn, and Pb had increased in coarse particle mode as well.

Concentration Characteristics of Atmospheric PM2.5, PM10 and TSP during the Asian Dust Storm in Iksan Area (익산지역에서 황사발생시 PM2.5, PM10 TSP의 농도 특성)

  • Kang, Gong-Unn;Kim, Nam-Song;Kim, Kyung-Suk;Kim, Mi-Kyung;Lee, Hyun-Ju
    • Journal of Environmental Health Sciences
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    • v.33 no.5
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    • pp.408-421
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    • 2007
  • The concentration characteristics of atmospheric particle matters (PM) including $PM_{2.5},\;PM_{10}$, and TSP were evaluated through the measurement data of PM_{2.5}$ (fine particulate), PM_{10-2.5}$ (coarse particulate), and PM_{over-10}$ collected using a MCI (multi-nozzle cascade impactor) sampler of a three-stage filter pack in spring of 2006 in Iksan area. During the sampling period of 10-15 March and 24 days from 8 April to 2 May, 32 samples for PM of each size fractions were collected, and then measured for PM mass concentrations and water-soluble inorganic ion species. Average concentrations of $PM_{2.5},\;PM_{10}$, TSP were $57.9{\pm}44.1mg/m^3$, $96.6{\pm}89.1mg/m^3$, and $114.8{\pm}99.7mg/m^3$, respectively. Water-soluble inorganic ion fractions to PM mass were found to be 36.5%, 18.0%, and 11.1% for $PM_{2.5}$, $PM_{10-2.5}$ and $PM_{over-10}$, respectively. By showing the high concentrations of PM samples during Asian dust events, those three fractions of PM were distinguished between the samples of Asian dust event and the samples of no event. However, the increase of PM concentrations observed during Asian dust events showed a different pattern for some Asian dust events. The differences of those three fractions in the size distribution may depend on differences on place of occurrence of Asian dust storm and course of transport from China continent to Iksan area in Korea. However, the extent of PM mass contribution during Asian dust events was generally dominated by the coarse particles rather than the fine fraction of PM. The variations of water-soluble inorganic ion species concentration in those three PM fractions between the samples of Asian dust event and the samples of no event were also discussed in this study.

A Study on Filtration Performance Test with Electrostatically Enhanced Fabric Filter (정전형여과집진방식에서 여과특성에 관한 연구)

  • 천중국;박출재;최금찬
    • Journal of Korean Society for Atmospheric Environment
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    • v.11 no.4
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    • pp.361-367
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    • 1995
  • This study has been carried out to investigate the filteration performance of Electrostatically Stimulated Fabric Filter(ESFF) at high temperature condition. The electric field was maintained parallel to the fabric surface. The benefits of ESFF are lower residual pressure drop, improvement of fine particle removal efficiency and increasing reduced rate of pressure drop during a filteration cycle, stable operation at higher filtering velocities. According to the variance of filtering velocities and dust loadings, the results are summarized as follows; By imposing an electric field on the filter, the reduced rate of pressure drop was 7.sim.18% at room temperature, and when filtering velocity was 1.8m/min and dust loading was 1g/m$^{3}$, the value of reduced rate of pressure drop was shown the highest. Under the electric field around the filter, the reduced rate of pressure drop was 10.sim.35% at high temperature, and when filtering velocity was 1.8m/min and dust loading was 1g/m$^{3}$, the value of reduced rate of pressure drop was shown the highest. Most of all, at high temperature, the value of reduced rate of pressure drop was resulted to 25%. Also the collecting efficiency was shown clearly improved. By the SEM photo analysis, the number of penetrated particles at the Conventional Fabric Filter was approximately two times that of Electrostatically Stimulated Fabric Filter.

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Concentration Variations of Persistent Organic Pollutants in Gosan, Jeju during the Polluted Period in November 2001 and the Yellow Sand Period in Spring 2002 (2001년 11월 오염시기와 2002년 봄 황사시기 제주도 고산에서의 잔류성 유기오염물질 농도 변화)

  • 김영성;김진영;김연제;문길주;문광주;한진석;김상우;윤순창;권성안
    • Journal of Korean Society for Atmospheric Environment
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    • v.19 no.5
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    • pp.469-490
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    • 2003
  • Atmospheric concentrations of persistent organic pollutants (POPs) were measured at Gosan, Jeju in November 2001 and spring 2002, each time for two weeks. Primary target pollutants were organochlorine pesticides, coplanar polychlorinated biphenyls (co- PCBs), and dioxin/furans listed in the Stockholm Convention adopted in May 2001. Polycyclic aromatic hydrocarbons (PAHs) were also measured in order to understand the overall characteristics of the POPs distribution as well as PM$_{2.5}$, a potent carrier of POPs. In the latter part of the measurement period of November 2001, almost every pollutant of combustion origin including dioxin/furans went high probably due to influence of emissions in the nearby area. The characteristics of atmospheric environment at Gosan in this period were rather close to urban areas far from those of a background area. A severe dust storm swept for three days at the end of the measurement period of spring 2002. However, changes in pollutant concentrations were relatively small except PM$_{10}$. Nevertheless, increases in particulate PAHs and OCDD (octachlorinated dibenzo-p-dioxins), mostly present in fine particles, were observed. Trends in organochlorine pesticide variations were mixed although possible volatilization of DDT residues from soil was inferred from the measurements of spring 2002.2.2.

Exploiting GOCI-II UV Channel to Observe Absorbing Aerosols (GOCI-II 자외선 채널을 활용한 흡수성 에어로졸 관측)

  • Lee, Seoyoung;Kim, Jhoon;Ahn, Jae-Hyun;Lim, Hyunkwang;Cho, Yeseul
    • Korean Journal of Remote Sensing
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    • v.37 no.6_1
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    • pp.1697-1707
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    • 2021
  • On 19 February 2020, the 2nd Geostationary Ocean Color Imager (GOCI-II), a maritime sensor of GEO-KOMPSAT-2B, was launched. The GOCI-II instrument expands the scope of aerosol retrieval research with its improved performance compared to the former instrument (GOCI). In particular, the newly included UV band at 380 nm plays a significant role in improving the sensitivity of GOCI-II observations to the absorbing aerosols. In this study, we calculated the aerosol index and detected absorbing aerosols from January to June 2021 using GOCI-II 380 and 412 nm channels. Compared to the TROPOMI aerosol index, the GOCI-II aerosol index showed a positive bias, but the dust pixels still could be clearly distinguished from the cloud and clear pixels. The high GOCI-II aerosol index coincided with ground-based observations indicating dust aerosols were detected. We found that 70.5% of dust and 80% of moderately-absorbing fine aerosols detected from the ground had GOCI-II aerosol indices larger than the 75th percentile through the whole study period.

Characteristics of Water Soluble Ions in Fine Particles during the Winter and Spring in Daegu (대구지역 겨울철과 봄철 미세먼지의 수용성 이온성분 특성)

  • Park, Ji-Yeon;Lim, Ho-Jin
    • Journal of Korean Society for Atmospheric Environment
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    • v.22 no.5
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    • pp.627-641
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    • 2006
  • Atmospheric $PM_{2.5}$ and $PM_{10}$ were measured to investigate their levels and water-soluble ions(${SO_4}^{2-},\;{NO_3}^-,\;{NO_2}^-,\;Cl^-,\;{NH_4}^+,\;Na^+,\;Ca^{2+},\;Mg^{2+},\;and\;K^+$) in Daegu between February 17 and April 18, 2006. Four Asian dust episodes during the period were examined for the influence of Asian dust on the particulate properties. Daily $PM_{2.5}\;and\;PM_{2.5-10}$ concentrations ranged between $10.83{\sim}136.76{\mu}g/m^3$ with a mean of $38.43{\mu}g/m^3$ and $16.13{\sim}409.13{\mu}g/m^3$ with a mean of $79.98{\mu}g/m^3$, respectively. For all measured ions the mean fractions of $PM_{2.5}\;and\;PM_{2.5-10}$ were 51.8% and 28.9% being lowered to 30.7% and 9.4%, respectively, during the dust episodes. Secondary ions (i.e., non-sea salt ${SO_4}^{2-},\;{NO_3}^-,\;and\;{NH_4}^+$) contributed 44.3% and 14.8% to $PM_{2.5}\;and\;PM_{2.5-10}$, respectively, with a decreased contribution during the episodes. The average equivalent ratio of ${NH_4}^+$ to the sum of ${SO_4}^{2-}\;and\;{NO_3}^-$ was 0.99 and 0.89 for $PM_{2.5}\;and\;PM_{2.5-10}$, respectively, indicating high source strength of $NH_3$ and its dominance in the neutralization of the acidic ions. Correlations and charge balance between ions suggest that neutralization of the acidic ions results in substantial depletions of carbonate both in $PM_{2.5}\;and\;PM_{2.5-10}$ and chloride only in $PM_{2.5}$.

Evaluation of Environmental Benefit and Cost for Management of Air Quality - [Based on Fine Dust Pollution on Donghae Harbor] (공기질 관리에 관한 환경 비용편익 연구[동해항만 주변 미세먼지오염을 기준])

  • Kim, Eun-Joo;Lee, Choon-Gil;Kim, Ji-Hyun;Park, Young-Koo
    • Journal of the Korean Applied Science and Technology
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    • v.29 no.4
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    • pp.561-569
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    • 2012
  • Study attempts to evaluate the environmental cost and benefit for management of particulate matters of Donghae harbor in Gangwondo. The level of fine dust suspended in the vicinity of the harbor was quite high, exceeding the national standard ($100{\mu}g/m^3$) depending on the places. The test field harbor deals with lots of limestone and coal, so that fine particulates could be generated while loading it and unloading. It was estimated that the direct handling of cargos might produce 12 tons of PM10(Particulate Matters of $10{\mu}m$) a year. In addition, heavy vehicles for transportation of various cargos including raw materials emit huge amount of diesel soots and cause to redispersion of road dust. The local government spends more than 2 billion won every year, and it contributes to reduce the atmospheric dust. According to the prediction of cost to benefit, it will present the effectiveness in 720 % maximum and at least 240 %.