• Title/Summary/Keyword: aerosols

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Size-segregated mass and ion concentrations of atmospheric aerosols in Cheonan City between 2006 and 2007 (2006~2007년 천안시 대기 에어로졸의 입경별 농도 및 이온성분 특성)

  • Lee, Hyung-Bae;Oh, Se-Won
    • Journal of the Korea Academia-Industrial cooperation Society
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    • v.9 no.5
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    • pp.1349-1353
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    • 2008
  • Size-segregated mass and ion concentrations of atmospheric aerosols in Cheonan City were measured using a high volume air sampler equipped with a 5-stage cascade impactor and a ion chromatography between March 2006 and April 2007. The mean values of 24-hr average concentrations of TSP, PM10, PM2.5, and PM1 were 61.7, 55.2, 43.7, $33.2{\mu}g/m^3$, respectively. Mass size distributions of atmospheric aerosols were bimodal distributions with a saddle point in $1.5\;{\sim}\;3.0{\mu}m$ range in diameter separating coarse and fine particle modes. Fine particles, PM2.5 were 70.8% of the total mass of aerosols. Major ion components in aerosols were ${NH_{4}}^+$, $Na^+$, $K^+$, $Ca^{2+}$, $Mg^{2+}$ for cations, and ${SO_{4}}^{2-}$, ${NO_{3}}^-$, $Cl^-$ for anions. ion components occupied 37.4% of coarse particles and 46.2% of fine particles in mass.

Variation of Concentration of Air Pollutants with Air Mass Back-Trajectory Analysis in Gyeongju (기단 역궤적분석에 의한 경주시 대기오염물질의 농도 변화)

  • Kim, Kyung-Won;Bang, So-Yung;Jung, Jong-Hyun
    • Journal of Korean Society for Atmospheric Environment
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    • v.24 no.2
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    • pp.162-175
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    • 2008
  • Gyeongju, which was the central city of the ancient civilization at Silla Kingdom, has various kinds of stone cultural properties. It is significantly important to preserve historical sources of Korea. However, recent air quality data measured in Gyeongju did not show good air quality level. In order to investigate variation of the concentration of the air pollutants with meteorological condition, an air quality monitoring and an aerosol sampling were conducted during the intensive monitoring period in Gyeongju. Impacts of the meteorological factors on the air pollutants were also analyzed based on the air mass pathway categories using HYSPLIT model and the local wind patterns using MM5 model. The prevailing air mass pathways were classified into four categories as following; category I affected by easterly marine aerosols, category II affected by northwesterly continental aerosols, category III affected by southwesterly continental aerosols, and category IV affected by northerly continental aerosols. The concentrations of the air quality standards were relatively lower during the fall intensive monitoring period. At that time, the easterly marine air mass pattern was dominated. The seasonal average mass concentration of $PM_{10,Opt}$, which optically measured at the monitoring site, was the highest value of $77.6{\pm}28.3\;{\mu}g\;m^{-3}$ during the spring intensive monitoring period but the lowest value of $20.1{\pm}5.3\;{\mu}g\;m^{-3}$ during the fall intensive monitoring period. The concentrations of $SO_2$ and CO were relatively higher when the air mass came from the northwestern continent or the northern continent. The concentrations of ${SO_4}^{2-}$ and ${NO_3}^-$ increased under the northwesterly continental condition. It was estimated that the acidic aerosols were dominated in the atmosphere of Gyeongju when the air mass came from the continental regions.

Monitoring of Climate Change of Northeast Asia and Background Atmosphere in Korea

  • Oh, Sung-Nam;Chung, Hyo-Sang;Choi, Jae-Cheon;Bang, So-Young;Hyun, Myung-Suk
    • Proceedings of the Korean Environmental Sciences Society Conference
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    • 2003.11a
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    • pp.232-235
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    • 2003
  • In general, the parameters of climate change include aerosol chemical compounds, aerosol optical depth, greenhouse gases(carbon dioxide, CFCs, methane, nitrous oxide, tropospheric ozone), ozone distribution, precipitation acidity and chemical compounds, persistent organic pollutants and heavy metals, radioactivity, solar radiation including ultra-violet and standard meteorological parameters. Over the last ten years, the monitoring activities of Korea regarding to the climate change have been progressed within the WMO GAW and ACE-Asia IOP programs centered at the observation sites of Anmyeon and Jeju Gosan islands respectively. The Greenhouse gases were pointed out that standard air quality monitoring techniques are required to enhance data comparability and that data presentation formats need to be harmonized and easily understood. Especially, the impact of atmospheric aerosols on climate depends on their optical properties, which, in turn, are a function of aerosol size distribution and the spectral reflective indices. Aerosol optical depth and single scattering albedo in the visible are used as the two basic parameters in the atmospheric temperature variation studies. The former parameter is an indicator of the attenuation power of aerosols, while the latter represents the relative strength of scattering and absorption by aerosols. For aerosols with weak absorption, surface temperature decreases as the optical depth increases because of the domination of backscattering. For aerosols with strong absorption, however, warming could occur as the optical depth increases. The objective of the study is to characterize the means, variability, and trends of Greenhouse gases and aerosol properties on a regional basis using data from its baseline observatories in Korea peninsula. A further goal is to understand the factors that control radiative forcing of the greenhouse and aerosol.

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3-D Perspectives of Atmospheric Aerosol Optical Properties over Northeast Asia Using LIDAR on-board the CALIPSO satellite (CALIPSO위성 탑재 라이다를 이용한 동북아시아 지역의 대기 에어러솔 3차원 광학특성 분포)

  • Lee, Kwon-Ho
    • Korean Journal of Remote Sensing
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    • v.30 no.5
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    • pp.559-570
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    • 2014
  • Backscatter signal observed from the space-borne Light Detection And Ranging (LIDAR) system is providing unique 3-dimensional spatial distribution as well as temporal variations for atmospheric aerosols. In this study, the continuous observations for aerosol profiles were analyzed during a years of 2012 by using a Cloud-Aerosol LIDAR with Orthogonal Polarization (CALIOP), carried on the Cloud-Aerosol LIDAR and Infrared Pathfinder Satellite Observation (CALIPSO) satellite. The statistical analysis on the particulate extinction coefficient and depolarization ratio for each altitude was conducted according to time and space in order to estimate the variation of optical properties of aerosols over Northeast Asia ($E110^{\circ}-140^{\circ}$, $N20^{\circ}$ $-50^{\circ}$). The most frequent altitudes of aerosols are clearly identified and seasonal mean aerosol profiles vary with season. Since relatively high particle depolarization ratios (>0.5) are found during all seasons, it is considered that the non-spherical aerosols mixed with pollution are mainly exists over study area. This study forms initial regional 3-dimensional aerosol information, which will be extended and improved over time for estimation of aerosol climatology and event cases.

A Review of Clouds and Aerosols (구름과 에어로졸 고찰)

  • Yum, Seong Soo;Kim, Byung Gon;Kim, Sang Woo;Chang, Lim Seok;Kim, Seong Bum
    • Journal of Climate Change Research
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    • v.2 no.4
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    • pp.253-267
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    • 2011
  • This study summarizes some important results from the studies on clouds and aerosols, and their effects on climate in the northeast Asia that were made mainly by Korean scientists and some other scientists from around the world. Clouds and aerosols are recognized as one of the most important factors that contributes to uncertainties in climate predictions and therefore become the subject of active research in the western developed countries in recent years. However, the researches on clouds and aerosols are very weakly done in Korea except ground based measurements of aerosol physical, chemical and optical properties. These measurements indicate that aerosol loadings in the northeast Asia are generally much higher than other parts of the world. On the other hand, researches on clouds are few in Korea. Satellite and ground remote sensing, numerical modeling and aircraft in-situ measurements of clouds are highly needed for better assessment of the role of clouds on climate in the northeast Asia.

Improvement and validation of aerosol models for natural deposition mechanism in reactor containment

  • Jishen Li ;Bin Zhang ;Pengcheng Gao ;Fan Miao ;Jianqiang Shan
    • Nuclear Engineering and Technology
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    • v.55 no.7
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    • pp.2628-2641
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    • 2023
  • Nuclear safety is the lifeline for the development and application of nuclear energy. In severe accidents of pressurized water reactor (PWR), aerosols, as the main carrier of fission products, are suspended in the containment vessel, posing a potential threat of radioactive contamination caused by leakage into the environment. The gas-phase aerosols suspended in the containment will settle onto the wall or sump water through the natural deposition mechanism, thereby reducing atmospheric radioactivity. Aiming at the low accuracy of the aerosol model in the ISAA code, this paper improves the natural deposition model of aerosol in the containment. The aerosol dynamic shape factor was introduced to correct the natural deposition rate of non-spherical aerosols. Moreover, the gravity, Brownian diffusion, thermophoresis and diffusiophoresis deposition models were improved. In addition, ABCOVE, AHMED and LACE experiments were selected to validate and evaluate the improved ISAA code. According to the calculation results, the improved model can more accurately simulate the peak aerosol mass and respond to the influence of the containment pressure and temperature on the natural deposition rate of aerosols. At the same time, it can significantly improve the calculation accuracy of the residual mass of aerosols in the containment. The performance of improved ISAA can meet the requirements for analyzing the natural deposition behavior of aerosol in containment of advanced PWRs in severe accident. In the future, further optimization will be made to address the problems found in the current aerosol model.

Thermal Distribution of Size-resolved Carbonaceous Aerosols and Water Soluble Organic Carbon in Emissions from Biomass Burning

  • Bae, Min-Suk;Park, Seung-Shik
    • Asian Journal of Atmospheric Environment
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    • v.7 no.2
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    • pp.95-104
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    • 2013
  • The study of carbonaceous aerosols in the atmosphere is critical to understand the role of aerosols in human health and climate. Using standardized thermal optical transmittance methods, organic carbon (OC), elemental carbon (EC), and water soluble organic carbon (WSOC) were determined using a combustion sampling system for four types of agricultural crop residues (rice straw, red pepper stems, soybean stems, and green perilla stems) and eight types of forest trees (pine stems, pine needles, ginkgo stems, ginkgo leaves, maple stems, maple leaves, cherry stems, and cherry leaves). The aerosol particles between 0.056 and $5.6{\mu}m$ in size were analyzed using a Micro-Orifice Uniform Deposit Impactor (MOUDI). In the current study, the Carbonaceous Thermal Distribution (CTD) by carbon analyzer was discussed in order to understand the carbon fractions from the twelve types of biomass burning. Also, the concentration of OC, EC, WSOC, and water insoluble organic carbon (WIOC) detected in the emissions were described.

Development of algorithm for determination of cloud and aerosol in Mie scattering Laser Radar System (Mie 산란 레이저 레이다 시스템을 위한 에어로졸과 구름의 판별 알고리즘 개발)

  • Kim, Sheen-Ja;Lee, Young-Woo;Park, Chan-Bong
    • Proceedings of the Korean Institute of Information and Commucation Sciences Conference
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    • 2012.05a
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    • pp.568-570
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    • 2012
  • The algorithm to distinguish cloud from aerosols in the measurements of Laser Radar is developed. This method use the difference of slope between return signals of cloud and aerosols. The parameters achieved from the algorithm are altitude of cloud top, cloud base, and boundary layer.

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Experimental Studies on Wet Scavenging of Atmospheric Aerosols by Rain Drops

  • Park Jeong-Ho;Suh Jeong-Min;Choi Kum-Chan
    • Journal of Korean Society for Atmospheric Environment
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    • v.21 no.E3
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    • pp.87-94
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    • 2005
  • Wet scavenging by rain drops is a most important removal process of air pollutants. In order to study the scavenging mechanisms of aerosol particles, the characteristics of chemical components in the rain water were examined as a function of the amount of rainfall. Rain water were collected continuously and separated into the soluble and insoluble components. The elemental concentrations in both components were determined by a PIXE analysis. The physical and chemical characteristics of atmospheric aerosols during the rainfall events were measured simultaneously. The elemental concentrations in rain water decreased substantially just after rain started and then gradually declined in subsequential rain fall exceeding 1.0 mm. The large particles were scavenged more easily than the fine particles. Fe, Ti and Si in rain water were in high insoluble state. Contrarily, almost whole of S was dissolved in rain water.

Morphology of Sub-Microscale Atmospheric Aerosols composed of Two Liquid Phases According to the Loading Ratio of Organics/Water

  • Yoo, Kee-Youn
    • Korean Chemical Engineering Research
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    • v.55 no.1
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    • pp.130-134
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    • 2017
  • Organic aerosols dispersed in the atmosphere likely undergo phase separation. Such internally mixed particles are often described as comprising an organic phase and an aqueous phase separately. We studied the morphology of two liquid separated aerosols in the sub-microscale by using a simple thermodynamic model with Russian doll geometry. The morphology of particles can be easily predicted from the simple criteria on the surface tension and two algebraic equations (the volume constraint and Young equation). This result may give the potential explanation about the complex morphology of the organic airborne particles.