• Journal of the Optical Society of Korea
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• v.15 no.1
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• pp.90-95
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• 2011

12-year LIDAR observations of tropospheric aerosol vertical distribution using a Mie scattering LIDAR in Hefei ($31.9^{\circ}N$, $117.2^{\circ}E$) from 1998 to 2009 are presented and analyzed in this paper. Characters of temporal variation and vertical distribution of tropospheric aerosol over Hefei are summarized from the LIDAR measurements. The impacts of natural source and human activities on the aerosol vertical distribution over Hefei could be seen clearly. Dust particles from the north in spring could affect the aerosol distributions below about 12 km over Hefei, and aerosol scale height in April reaches $2.29{\pm}0.68\;km$. Both LIDAR measurements and surface visibility imply that aerosols in the lower troposphere have been increasing since about 2005.

• New & Renewable Energy
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• v.20 no.1
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• pp.79-87
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• 2024

This study introduces a method for estimating Aerosol Optical Depth (AOD) using Broadband Aerosol Optical Depth (BAOD) derived from direct normal irradiance and meteorological factors observed between 2016 and 2017. Through correlation analyses between BAOD and atmospheric components such as Rayleigh scattering, water vapor, and tropospheric nitrogen dioxide, significant relationships were identified, enabling accurate AOD estimation. The methodology demonstrated high correlation coefficients and low Root Mean Square Errors (RMSE) compared to actual AOD₅₀₀ measurements, indicating that the attenuation effects of water vapor and the direct impact of tropospheric nitrogen dioxide concentration are crucial for precise aerosol optical depth estimation. The application of BAOD for estimating AOD₅₀₀ across various time scales-hourly, daily, and monthly-showed the approach's robustness in understanding aerosol distributions and their optical properties, with a high coefficient of determination (0.96) for monthly average AOD₅₀₀ estimates. This study simplifies the aerosol monitoring process and enhances the accuracy and reliability of AOD estimations, offering valuable insights into aerosol research and its implications for climate modeling and air quality assessment. The findings underscore the viability of using BAOD as a surrogate for direct AOD₅₀₀ measurements, presenting a promising avenue for more accessible and accurate aerosol monitoring practices, crucial for improving our understanding of aerosol dynamics and their environmental impacts.

• Mass Spectrometry Letters
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• v.8 no.1
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• pp.1-7
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• 2017

Studies performed on heterogeneous reactions of hydroxyl radicals (OH) in aerosol materials of tropospheric interest are presented, focusing on the chemical ionization mass spectrometric approach. Kinetic investigations of these reactions reduced deviation in the estimation of OH concentration in the troposphere by atmospheric modeling from field measurements. Recently, OH uptake was investigated under wet conditions to acquire kinetic information under more realistic conditions representative of the troposphere. The information on the mechanism and kinetics of OH uptake by tropospheric aerosol materials will contribute to the updating of atmospheric models, allowing a better understanding of the troposphere.

• Proceedings of the Korea Air Pollution Research Association Conference
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• 2008.10a
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• pp.159-163
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• 2008

• Proceedings of the Korea Air Pollution Research Association Conference
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• 2003.05b
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• pp.123-124
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• 2003

Fishman and Larson (1987) derived tropical tropospheric column ozone by subtracting stratospheric column ozone measured by the Stratospheric Aerosol and Gas Experiment (SAGE) from total column ozone obtained by the Total Ozone Mapping Spectrometer (TOMS). Later, the Convective Cloud Differential (CCD) method (Ziemke et al., 1998) indicated stratospheric ozone is invariant with longitude and concluded the zonal variation of total ozone determines the zonal variation of tropospheric ozone. (omitted)

• Proceedings of the KSRS Conference
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• 2003.11a
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• pp.1243-1245
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• 2003

Mean radiative forcing efficiencies (${\Delta}$F/${\Delta}{\tau}_{0.5}$) over East Asia range from -65 to -95 W m$^{-2}$ at the surface while -20 to -40 W m$^{-2}$ at TOA under clear-sky conditions. These aerosol direct radiative forcings over East Asia are similar to other experimental results for different regions, i.e., the Indian Ocean Experiment (INDOEX) and the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX), from which radiative forcing efficiencies of -75 Wm$^{-2}$ and -70 Wm$^{-2}$ for the Indian Ocean and the East Coast of the United States are reported. Nevertheless, the differences in aerosol parameters and relatively large STD values with regard to spatiotemporal variations suggest that the impact of aerosol on ARF over East Asia is more significant than previously recognized for other regions and should be continuously observed to determine the relation between increasing aerosols and associated radiative forcings in the region.

• Proceedings of the Korea Air Pollution Research Association Conference
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• 2003.05b
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• pp.205-206
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• 2003

대기중의 에어로졸은 지구-대기 시스템에 직접효과(direct effect)와 간접효과(inderect effec)로 불리우는 복사효과를 나타내어 지구복사수지에 영향을 미치는 인자이다. 또한 대기중에서 비교적 짧은 체류시간과 공간적인 변화성으로 인하여 제역적인 효과가 매우 크게 일어남에도 불구하고 그 효과가 정확히 알려져 있지 않다 (IPCC, 200l). 따라서 지역적인 규모의 에어로졸의 복사특성 관측이 중요한 요소가 되었다. 이러한 연구의 일환으로 수행된 일련의 프로젝트들은 TARFOX(Tropospheric Aerosol Radiative Forcing Obserational Experiment; Russel et al., 1999). (중략)

• Journal of Korean Society for Atmospheric Environment
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• v.17 no.5
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• pp.385-393
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• 2001

We have developed a Differential Absortion LIDAR (DIAL) method for the measurement of lower tropospheric ozone concentration. We used two laser beams from quadrupled Nd:YAG (266 nm) for the resonance wavelength and dye lasers (299.5 nm) for non -resonance wavelength. Aerosol extinction coefficients in the lower troposphere was computed by both Klett and Slope methods. To correct the SIN (Signal -Induced Noise) effect caused by photo detector, we subtracted a new-fitted baseline on the background part of a LIDAR signal, after the subtraction of the DC level. This is because SIN can be treated as an exponentially decaying tail. Using theme results, ozone profiles were obtained approximately 2km at daytime and 3km at nighttime. We compared the results derided by the Slope method with those measured by UV spectrometer. The computed results are in mostly good agreement with experimental results. In the measurement of the vertical layer, we observed the variation of the ozone profiles around the top mixed layer.

• Journal of Korean Society for Atmospheric Environment
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• v.15 no.6
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• pp.739-746
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• 1999

The spectral aerosol optical thickness of vertical air columns were measured by a ground-based multi-channel sunphotometer at the BAPMoN station(36$^{\circ}$31'N, 126$^{\circ}$19'E) in Anmyon Island, Korea, from 1 March 1998 to 31 May 1998. We used the data of three yellow sand and two clear sky days in order to analyze the temporal variations in aerosol optical thickness at the station. The basic aerosol optical thickness generally represented smaller than 0.3 in a clear sky and the range 0.5 to 1.1 in yellow sand. Especially the aerosol optical thickness represented larger than 0.9 in a heavy yellow sand. It was found that the aerosol optical thickness of yellow sand was highly increased in comparison with the case of a clear sky andparticles larger than 0.5$mu extrm{m}$ were also increased in the spectral distribution of aerosol volume during yellow sand. Consequently the spectral variations in tropospheric aerosol caused by yellow sand were determined by the number concentration of particles larger than 0.5${\mu}{\textrm}{m}$ and the magnitude of yellow sand.

• Journal of Korean Society for Atmospheric Environment
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• v.15 no.6
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• pp.713-725
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• 1999

Air pollutants($SO_2$, NOx, $O_3$ and aerosol number) were measured using an aircraft to investigate the characteristical features of long-range transport of sulfur compounds over the Yellow Sea for the periods of 26~27 April and 7~10 November in 1998. The mean $SO_2$ concentrations of April 26th~27th and November 7th~10th flight were 0.6~1.8 ppb and 0.5~8.3 ppb, respectively, and the sulfur transport was largely limited to the atmospheric boundary layer. Especially, $SO_2$ increased up to 8.3 ppb altogether with the increase of particle number concentraton especially on November 8, 1998. In addition, $O_3$ was remarkably decreased against the increase of $SO_2$and particle number concentrations. This enhanced $SO_2$ concentration occurred in the low level westerlies in association with the anticyclonic flow over Southern China and the cyclonic circulation over Manchuria. Aerosol analyses at Taean site also showed that sulfate concentration increased 2~3 times higher than those of another sampling days, which could suggest possible interactions between aerosol particels and tropospheric ozone. A rigorous evaluation will be possible after the more intensive measurements and quantitative analyses with detailed chemistry model including the postulated heterogeneous mechanism.