• Title/Summary/Keyword: Radioactive soil

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Investigation on Natural Radioactivity of Environmental Samples Near the Bauxite Processing Facility (보오크사이트 사용업체 주변 환경시료의 자연방사능 조사)

  • Moon, Dong-Hyeok;Koh, Sang-Mo;Chang, Byung-Uck;Kim, Tong-Kwon;Kim, Yong-Ug
    • Journal of the Mineralogical Society of Korea
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    • v.23 no.4
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    • pp.347-356
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    • 2010
  • Bauxite is a main raw material for the production of alumina and aluminum hydroxide in the processing plant of KC company. It is a NORM (Naturally Occurring Radioactive Materials), and its waste, red mud, is a TENORM (Technologically Enhanced Naturally Occurring Radioactive Materials). The purpose of the geochemical and mineralogical investigations of the bedrock and soils in and around the plant, a large NORM source, was to provide basic data for measuring the radiation dose and protecting from radioactive hazards. Soils were mixtures of minerals derived from the country rock (quartz, feldspar, mica, kaolin, gibbsite, and sepiolite) and bauxite (hematite, boehmite, and calcite) of open-air storage. Average U and Th contents of the soil samples were 4.7 ppm and 23 ppm, respectively, indicating somewhat Th anomaly. The average concentrations of radionuclides are $^{40}K$ 100~1,433 Bq/kg, $^{226}Ra$ anomaly in the red mud open-air storage. Soil external hazard indices range from 0.10 to 1.66 with an average of 0.63. Although most of the indices are below 1.0 that is a regulation value, those of 4 samples of total 41 soil samples exceed 1.0, requiring further detailed investigation.

Determine the hazards of radioactive elements and radon gas manufacturing processes in an Egyptian fertilizer factory

  • Soad Saad Fares
    • Nuclear Engineering and Technology
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    • v.56 no.5
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    • pp.1781-1795
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    • 2024
  • This study investigated the levels of radioactivity in soil surrounding a phosphate fertilizer factory in Egypt, aiming to assess potential risks to the population exposed to radiation. Concentrations of 238U, 226Ra, 232Th, and 40K were measured in soil samples collected from two subsites: one near the factory (subsite 1) and another further away (subsite 2). Two different systems were used for measuring radioactivity, a high-purity gamma ray spectroscopy system with an HPGe detector for gamma-emitting isotopes and a CR-39 solid nuclear track detector for alpha-emitting radon gas. Subsite 1, located close to the factory, displayed significantly elevated levels of 226Ra compared to global background levels (514 and 456 Bq/kg vs. 35 Bq/kg). Additionally, the concentrations of 238U (241.06 Bq/kg vs. global average 35 Bq/kg), 232Th (16.15 Bq/kg vs. global average 30 Bq/kg), and 40K (146.36 Bq/kg vs. global average 400 Bq/kg) were all above global averages. Furthermore, a high concentration of radon gas (337.06 μSv/y) was measured at subsite 1. The strong positive correlation observed between 226Ra and 238U (0.96256) provides further evidence of potentially elevated radioactivity levels near the factory. In contrast, subsite 2, situated farther from the factory, exhibited natural radioactive background levels within international limits. Quantitative analysis revealed that gamma ray absorbed doses for 226Ra and 232Th exceeded global averages in some samples. Specifically, 226Ra doses ranged from 7.8 to 46.26 ppm (exceeding the 20 ppm global average in some cases), and 232Th doses ranged from 1.98 to 9.14 ppm (exceeding the 10 ppm global average in some cases). The concentration of 40K, however, remained within the global range (0.07%-0.69 %). The observed imbalances in the ratios of Th/U (0.17-0.24 Bq/kg and 0.73-0.24 ppm) and U/Ra (0.81-0.73 Bq/kg and 0.73-0.17 ppm), both of which are significantly lower than their respective global averages of 4 and 2.4, point towards the presence of fertilizer-derived contamination. This conclusion is further supported by the high phosphate concentrations detected in the samples. Overall, this study suggests that radioactive contamination near the phosphate fertilizer factory significantly exceeds global background levels and international limits in some cases. This raises concerns about potential risks posed to surrounding agricultural land and crops.

Radioactivity Analysis of Soils Stored in KAERI for Regulatory Clearance (연구소 내 저장 중인 토양의 규제해제를 위한 방사능 분석)

  • Hong D.S.;Kim T.K.;Kang I.S.;Cho H.S.;Shon J.S.
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2005.06a
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    • pp.161-166
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    • 2005
  • In KAERI, about 3,100 drums containing soil have been stored. The soils were generated from the decommissioning process of Seoul office in 1988. Those soils occupy about $27\%$ of the capacity of the radioactive waste storage facility and make it difficult to maintain the storage facility. The major radioactive nuclides contained in the soils were expected to be Co-60 and Cs-137. As 16 years have passed, the radioactivity of those nuclides have decayed a lot. In this study, as a basis of regulatory clearance, radionuclides and radioactivity concentration of soils were analyzed. As a result, there are only Co-60 and Cs-137 in soils as ${\gamma}-emitters$. The total concentration of ${\gamma}-emitters$ in soil is analyzed as about $0.01\;{\sim}\;0.12$ Bq/g. As the soils are expected to be regulatory cleared in 2009, those concentrations will decay to be less than 0.1 Bq/g. This concentration can be meet the regulatory criteria suggested by IAEA. The regulatory clearance will be proceeded based on not only the assessment results of environmental influence but also related regulations.

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Numerical Simulation of Groundwater Flow in Feterogenetic Rockmass of Unsaturated Condition (암반의 불균질성을 고려한 불포화대 지하수 유동 평가)

  • Ha, Jaechul;Lee, Jeong Hwan;Cheong, Jae-yeol;Jung, Haeryong
    • The Journal of Engineering Geology
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    • v.26 no.1
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    • pp.87-99
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    • 2016
  • We present the results of two-dimensional numerical simulations predicting the flow of groundwater in a fractured unsaturated zone. We applied the k-field distribution of permeability derived from discrete fracture network (DFN) modeling as the hydraulic properties of a model domain. To model an unsaturated zone, we set the depth from the ground surface to the underground aquifer. The rate of water infiltration into the unsaturated zone was divided into two parts, an artificial structure surface and unsaturated soil zone. The movement of groundwater through the unsaturated zone was simulated with particular emphasis on contaminant transport. It was clearly observed that the contaminants dissolved in groundwater transported vertically from the ground surface to the saturated zone.

Predictive Contamination of Animal Products Due th the Inhalation of Air and the Ingestion of Soil of Cattle in an Accidental Release of Radioactive Materials - Focusing on Contaminative Influence for Milk (원자력 사고시 가축의 공기 흡입과 토양 섭취에 의한 축산물의 오염 - 우유에 대한 오염 영향을 중심으로)

  • Hwang, Won-Tae;Kim, Eun-Han;Suh, Kyung-Suk;Jeong, Hyo-Joon;Han, Moon-Hee;Lee, Chang-Woo
    • Journal of Radiation Protection and Research
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    • v.28 no.4
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    • pp.299-309
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    • 2003
  • In an accidental release of radioactive materials to the environment the contaminative influence of animal products due to the inhalation of air and the ingestion of soil of livestock, both of which are dealt with as minor contaminative pathways in most radioecological models but may not be neglected, was investigated with the improvement of the Korean dynamic food chain model DYNACON Although mathematical models for both contaminative pathways have been established for considering all animal products and incorporated into the model, investigation was limited to milk. As a result, it was found that both pathways are influential in the contamination of milk in the case of an accidental release during the non-grazing period of dairy cows. In the case of an accidental release during the non-grazing period, the inhalation of air was more influential than the ingestion of soil in the early days following an accidental release. While, it was the opposite with the lapse of time. If precipitation is encountered during an accidental release, contaminative influence due to the ingestion of soil was greater compared with the cases of no precipitation, in general, because of a stealer deposition of radionuclides onto the ground. Precipitation during an accidental release was a less influential factor in $^{131}I$ (elemental iodine) contamination compared with the $^{137}Cs\;and\;^{90}Sr$ contaminations. In the case of an accidental release during the grazing period of dairy cows, the contaminative influence due to the inhalation of air was negligible.

Transport Parameters of 99Tc, 137Cs, 90Sr, and 239+240Pu for Soils in Korea

  • Keum, D.K.;Kim, B.H.;Jun, I.;Lim, K.M.;Choi, Y.H.
    • Journal of Nuclear Fuel Cycle and Waste Technology
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    • v.1 no.1
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    • pp.49-55
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    • 2013
  • To characterize quantitatively the transport of $^{99}Tc$ and the global fallout ($^{137}Cs$, $^{90}Sr$, and $^{239+240}Pu$) for soils in Korea, the transport parameters of a convective-dispersion model, apparent migration velocity, and apparent dispersion coefficient were estimated from the vertical depth profiles of the radionuclides in soils. The vertical profiles of $^{99}Tc$ were measured from a pot experiment for paddy soil that had been sampled from a rice-field around the Gyeongju radioactive waste repository in Korea, and the vertical depth distributions of the global fallout $^{137}Cs$, $^{90}Sr$, and $^{239+240}Pu$ were measured from the soil samples that were taken from local areas in Korea. The front edge of the $^{99}Tc$ profiles reached a depth of about 12 cm in 138 days, indicating a faster movement than the fallout radionuclides. A weak adsorption of $^{99}Tc$ on the soil particles by the formation of Tc(VII) and a high water infiltration velocity seemed to have controlled the migration of $^{99}Tc$. The apparent migration velocity and dispersion coefficient of $^{99}Tc$ for the disturbed paddy soil were 2.88 cm/y and 6.3 $cm^2/y$, respectively. The majority of the global fallout $^{137}Cs$, $^{90}Sr$, and $^{239+240}Pu$ were found in the top 20 cm of the soils even after a transport of about 30 years. The transport parameters for the global fallout radionuclides were 0.01-0.1cm/y ($^{137}Cs$), 0.09-0.13cm/y ($^{90}Sr$), and 0.09-0.18cm/y ($^{239+240}Pu$) for the apparent migration velocity: 0.21-1.09 $cm^2/y$ ($^{137}Cs$), 0.12-0.7$cm^2/y$ ($^{90}Sr$), and 0.09-0.36$cm^2/y$ ($^{239+240}Pu$) for the apparent dispersion coefficient.

Development of volume reduction method of cesium contaminated soil with magnetic separation

  • Yukumatsu, Kazuki;Nomura, Naoki;Mishima, Fumihito;Akiyama, Yoko;Nishijima, Shigehiro
    • Progress in Superconductivity and Cryogenics
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    • v.18 no.1
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    • pp.10-13
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    • 2016
  • In this study, we developed a new volume reduction technique for cesium contaminated soil by magnetic separation. Cs in soil is mainly adsorbed on clay which is the smallest particle constituent in the soil, especially on paramagnetic 2:1 type clay minerals which strongly adsorb and fix Cs. Thus selective separation of 2:1 type clay with a superconducting magnet could enable to reduce the volume of Cs contaminated soil. The 2:1 type clay particles exist in various particle sizes in the soil, which leads that magnetic force and Cs adsorption quantity depend on their particle size. Accordingly, we examined magnetic separation conditions for efficient separation of 2:1 type clay considering their particle size distribution. First, the separation rate of 2:1 type clay for each particle size was calculated by particle trajectory simulation, because magnetic separation rate largely depends on the objective size. According to the calculation, 73 and 89 % of 2:1 type clay could be separated at 2 and 7 T, respectively. Moreover we calculated dose reduction rate on the basis of the result of particle trajectory simulation. It was indicated that 17 and 51 % of dose reduction would be possible at 2 and 7 T, respectively. The difference of dose reduction rate at 2 T and 7 T was found to be separated a fine particle. It was shown that magnetic separation considering particle size distribution would contribute to the volume reduction of contaminated soil.

Preliminary Study on Rapid Measurement of Gross Alpha/Beta and 90Sr Activities in Surface Soil by Mobile ZnS(Ag)/PTV Array and Handheld PVT Rod with Gated Energy Channels

  • Lee, Chanki;Kim, Hee Reyoung
    • Journal of Radiation Protection and Research
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    • v.46 no.4
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    • pp.194-203
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    • 2021
  • Background: Surface soil radiation monitoring around nuclear facilities is important to classify and characterize the contaminated areas. A scanning and direct measurement technique can survey the sites rapidly before starting sampling analysis. Materials and Methods: Regarding this, we test and suggest a measurement technique for gross alpha/beta and 90Sr activities in surface soil based on a mobile ZnS(Ag)/PVT (polyvinyltoluene) array and a handheld PVT rod, respectively. To detect 90Sr selectively in soil mixed with naturally occurring radioactive materials, chosen energy channel counts from the multichannel analyzers were used instead of whole channel counts. Soil samples contaminated with exempt liquid 90Sr with 1 Bq·g-1, 3 Bq·g-1, and 10 Bq·g-1 were prepared and hardened by flocculation. Results and Discussion: The mobile ZnS(Ag)/PVT array could discriminate gross alpha, gross beta, and gamma radiation by the different pulse-shaped signal features of each sensor material. If the array is deployed on a vehicle, the scan minimum detectable concentration (MDC) range will be about 0.11-0.17 Bq·g-1 at 18 km·h-1 speed, highly sensitive to actual sites. The handheld PVT rod with 12 mm (Φ) × 20 mm (H) size can directly measure 90Sr selectively if channels on which energies are from 1,470 and 2,279 keV are gated, minimizing crossdetection of other radionuclides. These methods were verified by measuring soil samples fabricated with homogeneous 90Sr concentrations, showing static MDC of 2.16 Bq·g-1 at a measurement time of 300 seconds. Conclusion: Based on the results, comprehensive procedures using these detectors are suggested to optimize soil sites survey.

Correlation Analysis of Radon Levels using Cluster Algorithm

  • Oh, Myeong Hwan;Jung, Yong Gyu;Kang, Min Soo;Lee, John
    • International journal of advanced smart convergence
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    • v.4 no.1
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    • pp.93-98
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    • 2015
  • Recently, Radon has been gotten attention for problems of Nuclear Generating Station and a variety of nuclear. It is naturally arises that is accumulated in the interior through the soil with radioactive materials. People exposed to indoor a Radon increase the high risks of lung cancer. The data are consisted of regional Country, The Location, Average Radon pCi/L, Geo Mean and Geo S.D etc. The research is experimented using E-M algorithm. The research result appears to make a division of soil distance, regional and cluster. It requires in effort to minimize exposure to people who live in areas with high radon levels. A country must apprise to people about Radon risk and needs to work out measures plan.