• Title/Summary/Keyword: Radiation Transport

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Dry storage of spent nuclear fuel and high active waste in Germany-Current situation and technical aspects on inventories integrity for a prolonged storage time

  • Spykman, Gerold
    • Nuclear Engineering and Technology
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    • v.50 no.2
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    • pp.313-317
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    • 2018
  • Licenses for the storage of spent nuclear fuel (SNF) and vitrified highly active waste in casks under dry conditions are limited to 40 years and have to be renewed for prolonged storage periods. If such a license renewal has to be expected since as in accordance with the new site selection procedure a final repository for spent fuel in Germany will not be available before the year 2050. For transport and possible unloading and loading in new casks for final storage, the integrity and the maintenance of the geometry of the cask's inventory is essential because the SNF rod cladding and the cladding of the vitrified highly active waste are stipulated as a barrier in the storage concept. For SNF, the cladding integrity is ensured currently by limiting the hoop stress and hoop strain as well as the maximum temperature to certain values for a 40-year storage period. For a prolonged storage period, other cladding degradation mechanisms such as inner and outer oxide layer formation, hydrogen pick up, irradiation damages in cladding material crystal structure, helium production from alpha decay, and long-term fission gas release may become leading effects driving degradation mechanisms that have to be discussed.

Monte Carlo approach for calculation of mass energy absorption coefficients of some amino acids

  • Bozkurt, Ahmet;Sengul, Aycan
    • Nuclear Engineering and Technology
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    • v.53 no.9
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    • pp.3044-3050
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    • 2021
  • This study offers a Monte Carlo alternative for computing mass energy absorption coefficients of any material through calculation of photon energy deposited per mass of the sample and the energy flux obtained inside a sample volume. This approach is applied in this study to evaluate mass energy absorption coefficients of some amino acids found in human body at twenty-eight different photon energies between 10 keV and 20 MeV. The simulations involved a pencil beam source modeled to emit a parallel beam of mono-energetic photons toward a 1 mean free path thick sample of rectangular parallelepiped geometry. All the components in the problem geometry were surrounded by a 100 cm vacuum sphere to avoid any interactions in materials other than the absorber itself. The results computed using the Monte Carlo radiation transport packages MCNP6.2 and GAMOS5.1 were checked against the theoretical values available from the tables of XMUDAT database. These comparisons indicate very good agreement and support the conclusion that Monte Carlo technique utilized in this fashion may be used as a computational tool for determining the mass energy absorption coefficients of any material whose data are not available in the literature.

Experimental validation of a nuclear forensics methodology for source reactor-type discrimination of chemically separated plutonium

  • Osborn, Jeremy M.;Glennon, Kevin J.;Kitcher, Evans D.;Burns, Jonathan D.;Folden, Charles M. III;Chirayath, Sunil S.
    • Nuclear Engineering and Technology
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    • v.51 no.2
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    • pp.384-393
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    • 2019
  • An experimental validation of a nuclear forensics methodology for the source reactor-type discrimination of separated weapons-useable plutonium is presented. The methodology uses measured values of intra-element isotope ratios of plutonium and fission product contaminants. MCNP radiation transport codes were used for various reactor core modeling and fuel burnup simulations. A reactor-dependent library of intra-element isotope ratio values as a function of burnup and time since irradiation was created from the simulation results. The experimental validation of the methodology was achieved by performing two low-burnup experimental irradiations, resulting in distinct fuel samples containing sub-milligram quantities of weapons-useable plutonium. The irradiated samples were subjected to gamma and mass spectrometry to measure several intra-element isotope ratios. For each reactor in the library, a maximum likelihood calculation was utilized to compare the measured and simulated intra-element isotope ratio values, producing a likelihood value which is proportional to the probability of observing the measured ratio values, given a particular reactor in the library. The measured intra-element isotope ratio values of both irradiated samples and its comparison with the simulation predictions using maximum likelihood analyses are presented. The analyses validate the nuclear forensics methodology developed.

Water quality big data analysis of the river basin with artificial intelligence ADV monitoring

  • Chen, ZY;Meng, Yahui;Wang, Ruei-yuan;Chen, Timothy
    • Membrane and Water Treatment
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    • v.13 no.5
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    • pp.219-225
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    • 2022
  • 5th Assessment Report of the Intergovernmental Panel on Climate Change Weather (AR5) predicts that recent severe hydrological events will affect the quality of water and increase water pollution. To analyze changes in water quality due to future climate change, input data (precipitation, average temperature, relative humidity, average wind speed, and solar radiation) were compiled into a representative concentration curve (RC), defined using 8.5. AR5 and future use are calculated based on land use. Semi-distributed emission model Calculate emissions for each target period. Meteorological factors affecting water quality (precipitation, temperature, and flow) were input into a multiple linear regression (MLR) model and an artificial neural network (ANN) to analyze the data. Extensive experimental studies of flow properties have been carried out. In addition, an Acoustic Doppler Velocity (ADV) device was used to monitor the flow of a large open channel connection in a wastewater treatment plant in Ho Chi Minh City. Observations were made along different streams at different locations and at different depths. Analysis of measurement data shows average speed profile, aspect ratio, vertical position Measure, and ratio the vertical to bottom distance for maximum speed and water depth. This result indicates that the transport effect of the compound was considered when preparing the hazard analysis.

Measurement of low energy beta radiation from Ni-63 by using peeled-off Gafchromic EBT3 film

  • Ji, Wanook;Kim, Jong-Bum;Kim, Jin-Joo
    • Nuclear Engineering and Technology
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    • v.54 no.10
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    • pp.3811-3815
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    • 2022
  • Ni-63 is pure beta source which emits low energy beta particles. The Ni-63 sources were fabricated to develop the beta-voltaic battery which converts decay energy into electrical energy for power generation. Activity distribution of the source was important factor of power producibility of the beta-voltaic battery. Liquid scintillation counter widely used for measurement of low energy beta emitters was not suitable to measure activity distribution. In this study, we used the peeled-off Gafchromic™ EBT3 film to measure the activity distribution of the Ni-63 source. Absorbed dose was increased proportionally to the source activity and exposure duration. The low energy beta particles could transport the energy into the active layer without the polyester protective layer. Also, Activity distribution was measured by using the peeled-off EBT3 film. Two-dimensional dosimetric distribution was suitable to measure the activity distribution. To use the peeled-off EBT3 film is user-friendly and cost-effective method for quality assurance of the Ni-63 sources for the beta-voltaic battery.

Evaluation of Effects of Impurities in Nuclear Fuel and Assembly Hardware on Radiation Source Term and Shielding

  • Taekyung Lee;Dongjin Lee;Kwangsoon Choi;Hyeongjoon Yun
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.2
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    • pp.193-204
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    • 2023
  • To ensure radiological safety margin in the transport and storage of spent nuclear fuel, it is crucial to perform source term and shielding analyses in advance from the perspective of conservation. When performing source term analysis on UO2 fuel, which is mostly used in commercial nuclear power plants, uranium and oxygen are basically considered to be the initial materials of the new fuel. However, the presence of impurities in the fuel and structural materials of the fuel assembly may influence the source term and shielding analyses. The impurities could be radioactive materials or the stable materials that are activated by irradiation during reactor power operation. As measuring the impurity concentration levels in the fuel and structural materials can be challenging, publicly available information on impurity concentration levels is used as a reference in this evaluation. To assess the effect of impurities, the results of the source term and shielding analyses were compared depending on whether the assumed impurity concentration is considered. For the shielding analysis, generic cask design data developed by KEPCO-E&C was utilized.

Evaluation of neutron attenuation properties using helium-4 scintillation detector for dry cask inspection

  • Jihun Moon;Jisu Kim;Heejun Chung;Sung-Woo Kwak;Kyung Taek Lim
    • Nuclear Engineering and Technology
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    • v.55 no.9
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    • pp.3506-3513
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    • 2023
  • In this paper, we demonstrate the neutron attenuation of dry cask shielding materials using the S670e helium-4 detector manufactured by Arktis Radiation Ltd. In particular, two materials expected to be applied to the TN-32 dry cask manufactured by ORANO Korea and KORAD-21 by the Korea Radioactive Waste Agency (KORAD) were utilized. The measured neutron attenuation was compared with our Monte Carlo N-Particle Transport simulation results, and the difference is given as the root mean square (RMS). For the fast neutron case, a rapid decline in neutron counts was observed as a function of increasing material thickness, exhibiting an exponential relationship. The discrepancy between the experimentally acquired data and simulation results for the fast neutron was maintained within a 2.3% RMS. In contrast, the observed thermal neutron count demonstrated an initial rise, attained a maximum value, and exhibited an exponential decline as a function of increasing thickness. In particular, the discrepancy between the measured and simulated peak locations for thermal neutrons displayed an RMS deviation of approximately 17.3-22.4%. Finally, the results suggest that a minimum thickness of 5 cm for Li-6 is necessary to achieve a sufficiently significant cross-section, effectively capturing incoming thermal neutrons within the dry cask.

A PRELIMINARY STUDY OF EFFECT OF THE GREEN FEATURE - WING WALLS ON NATURAL VENTILATION IN BUILDINGS

  • Cheuk Ming Mak;Jian Lei Niu;Kai Fat Chan
    • International conference on construction engineering and project management
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    • 2005.10a
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    • pp.814-819
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    • 2005
  • There is growing consciousness of the environmental performance of buildings in Hong Kong. The Buildings Department, the Lands Department and the Planning Department of the Hong Kong Government issued the first of a series of joint practice notes [1] to promote the construction of green and innovative buildings. Green features are architectural features used to mitigate migration of noise and various air-borne pollutants and to moderate the transport of heat, air and transmission of daylight from outside to indoor environment in an advantageous way. This joint practice note sets out the incentives to encourage the industry in Hong Kong to incorporate the use of green features in building development. The use of green features in building design not only improves the environmental quality, but also reduces the consumption of non-renewable energy used in active control of indoor environment. Larger window openings in the walls of a building may provide better natural ventilation. However, it also increases the penetration of direct solar radiation into indoor environment. The use of wing wall, one of the green features, is an alternative to create effective natural ventilation. This paper therefore presents a preliminary numerical study of its ventilation performance using Computational Fluid Dynamics (CFD). The numerical results will be compared with the results of the wind tunnel experiments of Givoni.

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Criticality analysis of pyrochemical reprocessing apparatuses for mixed uranium-plutonium nitride spent nuclear fuel using the MCU-FR and MCNP program codes

  • P.A. Kizub ;A.I. Blokhin ;P.A. Blokhin ;E.F. Mitenkova;N.A. Mosunova ;V.A. Kovrov ;A.V. Shishkin ;Yu.P. Zaikov ;O.R. Rakhmanova
    • Nuclear Engineering and Technology
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    • v.55 no.3
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    • pp.1097-1104
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    • 2023
  • A preliminary criticality analysis for novel pyrochemical apparatuses for the reprocessing of mixed uranium-plutonium nitride spent nuclear fuel from the BREST-OD-300 reactor was performed. High-temperature processing apparatuses, "metallization" electrolyzer, refinery remelting apparatus, refining electrolyzer, and "soft" chlorination apparatus are considered in this work. Computational models of apparatuses for two neutron radiation transport codes (MCU-FR and MCNP) were developed and calculations for criticality were completed using the Monte Carlo method. The criticality analysis was performed for different loads of fissile material into the apparatuses including overloading conditions. Various emergency situations were considered, in particular, those associated with water ingress into the chamber of the refinery remelting apparatus. It was revealed that for all the considered computational models nuclear safety rules are satisfied.

The Study of Dose Change by Field Effect on Atomic Number of Shielding Materals in 6 MeV Electron Beam (6 MeV 전자선의 차폐물질 원자번호와 조사야 크기에 따른 선량변화 연구)

  • Lee, Seung Hoon;Kwak, Keun Tak;Park, Ju Kyeong;Gim, Yang Soo;Cha, Seok Yong
    • The Journal of Korean Society for Radiation Therapy
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    • v.25 no.2
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    • pp.145-151
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    • 2013
  • Purpose: In this study, we analyzed how the dose change by field size effects on atomic number of shielding materials while using 6 MeV election beam. Materials and Methods: The parallel plate chamber is mounted in $25{\times}25cm^2$ the phantom such that the entrance window of the detector is flush with the phantom surface. phantom was covered laterally with aluminum, copper and lead which thickness have 5% of allowable transmission and then the doses were measured in field size $6{\times}6$, $10{\times}10$ and $20{\times}20cm^2$ respectively. 100 cGy was irradiated using 6 MeV electron beam and SSD (Source Surface Distance) was 100 cm with $10{\times}10cm^2$ field size. To calculate the photon flux, electron flux and Energy deposition produced after pass materals respectively, MCNPX code was used. Results: The results according to the various shielding materials which have 5% of allowable transmission are as in the following. Thickness change rate with field size of $6{\times}6cm^2$ and $20{\times}20cm^2$ that compared to the field size of $10{\times}10cm^2$ found to be +0.06% and -0.06% with aluminum, +0.13% and -0.1% with copper, -1.53% and +1.92% with lead respectively. Compare to the field size $10{\times}10cm^2$, energy deposition for $6{\times}6cm^2$ and $20{\times}20cm^2$ had -4.3% and +4.85% respectively without shielding material. With aluminum it had -0.87% and +6.93% respectively and with lead it had -4.16% and +5.57% respectively. When it comes to photon flux with $6{\times}6cm^2$ and $20{\times}20cm^2$ of field sizes the chance -8.95% and +15.92% without shielding material respectively, with aluminum the number -15.56% and +16.06% respectively and with copper the chance -12.27% and +15.53% respectively, with lead the number +12.36% and -19.81% respectively. In case of electron flux in the same condition, the number -3.92% and +4.55% respectively without shielding material respectively, with aluminum the number +0.59% and +6.87% respectively, with copper the number -1.59% and +3.86% respectively, with lead the chance -5.15% and +4.00% respectively. Conclusion: In this study, we found that the required thickness of the shielding materials got thinner with low atomic number substance as the irradiation field is increasing. On the other hand, with high atomic number substance the required thickness had increased. In addition, bremsstrahlung radiation have an influence on low atomic number materials and high atomic number materials are effected by scattered electrons.

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