• Title/Summary/Keyword: Low-enriched uranium

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MEASUREMENT OF $^{235}U$ ENRICHMENT USING THE SEMI-PEAK-RATIO TECHNIQUE WITH CdZnTe GAMMA-RAY DETECTOR

  • Ha, J.H.;Ko, W.I.;Lee, S.Y.;Song, D.Y.;Kim, H.D.;Yang, M.S.
    • Journal of Radiation Protection and Research
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    • v.26 no.3
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    • pp.275-279
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    • 2001
  • In uranium enrichment plants and nuclear fuel fabrication facilities, exact measurement of fissile isotope enrichment of uranium is required for material accounting in international safeguards inspection as well as process quality control. The purpose of this study was to develop a simple measurement system which can portably be used at nuclear fuel fabrication plants especially dealing with low enriched uranium. For this purpose, a small size CZT (CdZnTe) detector was used, and the detector performance in low uranium gamma/X -rays energy range was investigated by use of various enriched uranium oxide samples. New enrichment measurement technique and analysis method for low enriched uranium oxide, so-called, 'semi-peak ratio technique' was developed. The newly developed method was considered as an alternative technique for the low enrichment and would be useful to account nuclear material in safeguarding activity at nuclear fuel fabrication facility.

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A method for purifying reprocessed uranium from even isotopes under conditions of multiple recycle

  • Smirnov, A.Yu.;Palkin, V.A.;Chistov, A.V.;Sulaberidze, G.A.
    • Nuclear Engineering and Technology
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    • v.54 no.10
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    • pp.3650-3659
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    • 2022
  • We proposed a modification of a double cascade scheme to enrich reprocessed uranium. Such a cascade scheme represents a combination of one cascade with "broadening" of the flow and an ordinary three-flow cascade. A calculation and optimization method has been developed for the proposed scheme according to various efficiency criteria. It is shown that the proposed scheme makes it possible to obtain low-enriched uranium of commercial quality using reprocessed uranium of different initial compositions. For example, the enrichment of reprocessed uranium, which had gone through five consequent recycles, was considered. The proposed scheme allowed to enrich it with simultaneous fulfillment of restrictions on isotopes 232U, 234U, and 236U. Such results indicate the scheme's applicability under conditions of multiple recycling of uranium in reactor fuel. Computational experiments have shown that in the proposed modification, a noticeable saving of natural uranium in the cycle (~18%) can be achieved, provided that the additional consumption of separative work does not exceed 10%, compared with the case of enrichment of natural uranium to obtain LEU of equivalent quality.

Radioactive Waste Issues Related to Production of Fission-based 99Mo by using Low Enriched Uranium (LEU) (저농축 우라늄을 사용하는 핵분열 몰리브덴-99 생산에 관련된 방사성 폐기물 연구)

  • Hassan, Muhmood ul;Ryu, Ho Jin
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.13 no.2
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    • pp.155-161
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    • 2015
  • Technetium-99m (99mTc) is an important, short-lived decay product of molybdenum-99 (99Mo), and it is considered the backbone of the modern nuclear diagnostic procedures. Since fission of 235U is the main source of production of 99Mo, either highly-enriched uranium (HEU) targets or low-enriched uranium (LEU) targets are irradiated in the research reactors. The use of LEU targets is being promoted by the international community to avoid the proliferation issues linked with the use of HEU. In order to define the waste management strategy at the planning stage of establishment of an LEU based 99Mo production facility, the impact of the use of LEU targets on the radioactive waste stream of the 99Mo production facility was analyzed. Because the volume of uranium waste is estimated to increase six times, the use of high uranium density targets and the utilization of hot isostatic pressing were recommended to reduce the increased waste volume from the use of LEU based targets.

Development of Industrial-Scale Fission 99Mo Production Process Using Low Enriched Uranium Target

  • Lee, Seung-Kon;Beyer, Gerd J.;Lee, Jun Sig
    • Nuclear Engineering and Technology
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    • v.48 no.3
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    • pp.613-623
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    • 2016
  • Molybdenum-99 ($^{99}Mo$) is the most important isotope because its daughter isotope, technetium-99m ($^{99m}Tc$), has been the most widely used medical radioisotope for more than 50 years, accounting for > 80% of total nuclear diagnostics worldwide. In this review, radiochemical routes for the production of $^{99}Mo$, and the aspects for selecting a suitable process strategy are discussed from the historical viewpoint of $^{99}Mo$ technology developments. Most of the industrial-scale $^{99}Mo$ processes have been based on the fission of $^{235}U$. Recently, important issues have been raised for the conversion of fission $^{99}Mo$ targets from highly enriched uranium to low enriched uranium (LEU). The development of new LEU targets with higher density was requested to compensate for the loss of $^{99}Mo$ yield, caused by a significant reduction of $^{235}U$ enrichment, from the conversion. As the dramatic increment of intermediate level liquid waste is also expected from the conversion, an effective strategy to reduce the waste generation from the fission $^{99}Mo$ production is required. The mitigation of radioxenon emission from medical radioisotope production facilities is discussed in relation with the monitoring of nuclear explosions and comprehensive nuclear test ban. Lastly, the $^{99}Mo$ production process paired with the Korea Atomic Energy Research Institute's own LEU target is proposed as one of the most suitable processes for the LEU target.

The characteristics of nuclear powered submarine and the use of enriched uranium (원자력 추진 잠수함의 특성과 농축우라늄 사용)

  • Jang, Jun-Seop
    • Strategy21
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    • s.41
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    • pp.261-293
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    • 2017
  • Nuclear power is a way of attaining an enormous amount of energy with relatively small amount of resources and after it has been introduced to the submarine since 1954, there are approximately 150 of nuclear powered submarine currently on a mission around the world. This is due to the maneuverability, mountability and covertness of nuclear submarines. However, there are other tasks, not only the high level of nuclear technology that are needed to be dealt with in order to construct nuclear powered submarine. The biggest task of all is to secure the enriched uranium. Accordingly, this research is about the way of enriching and securing the nuclear fuel that are used in the nuclear submarine with the characteristics, merits and demerits of the nuclear submarine. Due to the fact that the pressurized water reactor in South Korea is the reactor that was originally built for the development of nuclear powered submarine, many parts is designed to be suitable for the submarine propulsion. However, in order to apply this to submarine it is needed to consider additional requests such as the position of reactor, accident-coping system, radioactive covering, reactor output adjustment and ship's pitch and roll in order to apply this to submarine. Nuclear submarines have much higher speed based on the powerful propulsion in comparison with diesel-electric submarine and also have bigger loading area. Besides, there is no need to snorkel and they also have advantages in covertness with the multi-noise proof system. The nuclear technology in South Korea has seen the dramatic development since 1962 and in 1998 reached to the level that we have succeeded in the localization of nuclear plant and exported the world-class one-piece small-sized reactor (SMART) to UAE. To operate these reactors, we import the whole quantity of low-enriched uranium and having our own uranium enrich facility is not probable because of the budget and international regulations. With the ROK/US nuclear agreement revised on 2015 November, the enrichment of uranium that are available without special permission has changed up to 20%. According to the assumption that we use the 20% enrichment of Uranium on U.S. virginia class submarine, it is necessary to change the fuel after 11 years and it will cause additional cost of 1 billion dollars. But the replace period by the uranium's enrichment rate is not fixed so that it is possible to change according to the design of reactor. Therefore, I would like to make a suggestion on two types of design concepts of nuclear submarine that can be operated for 30 years without nuclear fuel change by using the 20% enriched uranium from ONNp.First of all, it is possible by increasing the size of reactor by 3 times and it results in the 1,000t increase of the weight. And secondly, it is by designing the one piece reactor to insert devices such as steam turbine, condenser into the inside of nuclear core like the Rubis class submarines of France.

DEVELOPMENT OF HIGH-DENSITY U/AL DISPERSION PLATES FOR MO-99 PRODUCTION USING ATOMIZED URANIUM POWDER

  • Ryu, Ho Jin;Kim, Chang Kyu;Sim, Moonsoo;Park, Jong Man;Lee, Jong Hyun
    • Nuclear Engineering and Technology
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    • v.45 no.7
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    • pp.979-986
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    • 2013
  • Uranium metal particle dispersion plates have been proposed as targets for Molybdenum-99 (Mo-99) production to improve the radioisotope production efficiency of conventional low enriched uranium targets. In this study, uranium powder was produced by centrifugal atomization, and miniature target plates containing uranium particles in an aluminum matrix with uranium densities up to 9 $g-U/cm^3$ were fabricated. Additional heat treatment was applied to convert the uranium particles into UAlx compounds by a chemical reaction of the uranium particles and aluminum matrix. Thus, these target plates can be treated with the same alkaline dissolution process that is used for conventional $UAl_x$ dispersion targets, while increasing the uranium density in the target plates.

Restoration of the isotopic composition of reprocessed uranium hexafluoride using cascade with additional product

  • Palkin, Valerii;Maslyukov, Eugenii
    • Nuclear Engineering and Technology
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    • v.52 no.12
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    • pp.2867-2873
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    • 2020
  • In reprocessed uranium, derived from an impoverished fuel of light-water moderated reactors, there are isotopes of 232, 234, 236U, which make its recycling remarkably difficult. A method of concentration of 235U target isotope in cascade's additional product was proposed to recover the isotopic composition of reprocessed uranium. A general calculation procedure is presented and a parameters' optimization of multi-flow cascades with additional products. For the first time a numeric model of a cascade that uses the cuts of partial flows of stages with relatively high separation factors was applied in this procedure. A novel computing experiment is carried out on separation of reprocessed uranium hexafluoride with providing a high concentration of 235U in cascade's additional product with subsequent dilution. The parameters of cascades' stages are determined so as to allow reducing the 232, 234, 236U isotope content up to the acceptable. It was demonstrated that the dilution of selected products by the natural waste makes it possible to receive a low enriched uranium hexafluoride that meets the ASTM C996-15 specification for commercial grade.

Study concerning the Scope of Merchandise under the U.S. Antidumping Law through Case (사례를 통한 미반덤핑법상 상품의 범위에 관한 연구)

  • Ha, Choong-Lyong;Han, Na-Hee
    • International Commerce and Information Review
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    • v.11 no.3
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    • pp.265-286
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    • 2009
  • Dumping describes the practice of international price discrimination whereby a producer or exporter sells merchandise in an export market at less than fair value. The U.S. antidumping statutory framework is embodied in the Tariff Act of 1930. The Act states that "dumping" refers to the sale or likely sale of goods at less than fair value. 19 U.S.C. $\S$ 1677(34). The Commerce Department and the Commission are jointly responsible for administering the antidumping law. Commerce determines whether foreign merchandise is being sold in the United States at less than fair value, and the Commission determines whether a domestic industry producing a product like the imported merchandise has been materially injured or threatened with material injury by reason of imports of that product. Recently, in U.S. v. Eurodif, the Supreme Court held the question whether the Commerce can reasonably determin that foreign merchandise has been sold within the meaning of the antidumping law in U.S.. Should 19 U.S.C. Section 1673, which calls for "antidumping" duties on foreign goods, but not services, that sell at less than fair value in the U.S., apply to imported low enriched uranium? Yes. In a unanimous opinion written by Justice David H. Souter, the Supreme Court held that the Commerce Department's view of imported low enriched uranium, as the sale of goods rather than services, was permissible. It reasoned that, since 19 U.S.C. Section 1673 did not specify whether it applied to the production of low enriched uranium, it was left to the reasonable interpretation of the Commerce Department to determine. Accordingly, the Court found the Commerce Department interpreted the statute reasonably.

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IRRADIATION PERFORMANCE OF U-Mo MONOLITHIC FUEL

  • Meyer, M.K.;Gan, J.;Jue, J.F.;Keiser, D.D.;Perez, E.;Robinson, A.;Wachs, D.M.;Woolstenhulme, N.;Hofman, G.L.;Kim, Y.S.
    • Nuclear Engineering and Technology
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    • v.46 no.2
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    • pp.169-182
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    • 2014
  • High-performance research reactors require fuel that operates at high specific power to high fission density, but at relatively low temperatures. Research reactor fuels are designed for efficient heat rejection, and are composed of assemblies of thin-plates clad in aluminum alloy. The development of low-enriched fuels to replace high-enriched fuels for these reactors requires a substantially increased uranium density in the fuel to offset the decrease in enrichment. Very few fuel phases have been identified that have the required combination of very-high uranium density and stable fuel behavior at high burnup. U-Mo alloys represent the best known tradeoff in these properties. Testing of aluminum matrix U-Mo aluminum matrix dispersion fuel revealed a pattern of breakaway swelling behavior at intermediate burnup, related to the formation of a molybdenum stabilized high aluminum intermetallic phase that forms during irradiation. In the case of monolithic fuel, this issue was addressed by eliminating, as much as possible, the interfacial area between U-Mo and aluminum. Based on scoping irradiation test data, a fuel plate system composed of solid U-10Mo fuel meat, a zirconium diffusion barrier, and Al6061 cladding was selected for development. Developmental testing of this fuel system indicates that it meets core criteria for fuel qualification, including stable and predictable swelling behavior, mechanical integrity to high burnup, and geometric stability. In addition, the fuel exhibits robust behavior during power-cooling mismatch events under irradiation at high power.