• Title/Summary/Keyword: Gaseous radioactive waste

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Selection of a carrying agent for obtaining radioactive methyliodide vapors under dynamic conditions

  • Obruchikov, Alexander V.;Merkushkin, Aleksei O.;Magomedbekov, Eldar P.;Anurova, Olga M.;Vanina, Elena A.
    • Nuclear Engineering and Technology
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    • v.53 no.8
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    • pp.2761-2766
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    • 2021
  • A method for preparing "reagent" for radioactive methyliodide vapors production using an isotopic exchange reaction has been developed. Based on the obtained data of the isotopic exchange efficiency and hydraulic resistance, white fused alumina (700-840 ㎛) was selected as the carrying agent material for "reagent" production. The radioiodine isotopic exchange dependences on such parameters as temperature, gas flow velocity, and the methyliodide concentration in it were determined. Optimal conditions have been selected to achieve 85% of the isotopic exchange rate in 1 h of the experiment. The obtained data allowed to develop an approach to the test of iodine filters for nuclear power plants and to determine their efficiency.

A method for properties evaluation of activated charcoal sorbents in iodine capture under dynamic conditions

  • Magomedbekov, Eldar P.;Obruchikov, Alexander V.
    • Nuclear Engineering and Technology
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    • v.51 no.2
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    • pp.641-645
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    • 2019
  • Experimental equipment for studying the sorption properties of iodine sorbents using radioactive methyliodide has been developed. The sorption capacity index ${\alpha}$ is proposed as a criterion parameter for assessing the quality of impregnated activated charcoals. It was found that this parameter does not depend on the dynamic conditions during the sorbent test. It was shown that values of the sorption capacity index allow to recommend iodine sorbents for industrial gas cleaning processes.

A Study on Annual Release Objectives and Annual Release Limits of Gaseous Effluents During Decommissioning of Nuclear Power Plants (원전 해체 시 기체상 유출물의 연간 방출관리치 및 방출한도치에 관한 연구)

  • Lee, Seung-Hee;Hwang, Won-Tae;Kim, Chang-Lak
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.17 no.3
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    • pp.299-311
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    • 2019
  • Decommissioning is a critical issue in Korea. Although compared with the operation of nuclear power plants the release of radioactive materials during decommissioning is not expected to be significant, residents should always be protected from radiation exposure. To manage this effectively, Annual Release Objectives (ARO) and Annual Release Limits (ARL) were derived from dose standards in the NSSC Notice and dose limit for the public. Based on meteorological data for the three years from 2008 to 2010 in the Shin Kori nuclear power plant site, atmospheric dispersion and ground deposition factors of gaseous effluent were evaluated using the XOQDOQ computer code. The exposure dose was evaluated using the ENDOS-G computer code. Because of differences in radiological sensitivity according to age groups, the results of Annual Release Objectives (ARO) and Annual Release Limits (ARL) showed significant differences depending on the radionuclides. The evaluation methodology of this study will provide meaningful information for radioactive effluent management for decommissioning of nuclear power plants.

Practical Radiation Safety Control: (II) Application of Numerical Guidance for the Discharges of Radioactive Gaseous and Liquid Effluents (방사선안전관리 실무: (II) 배기중 및 배수중 배출관리기준의 적용)

  • Kim, Hyun Kee
    • Journal of Radiation Protection and Research
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    • v.39 no.1
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    • pp.61-64
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    • 2014
  • Radioactive materials are in use and have many applications from the generation of electricity to the purposes of research, industry and medicine such as diagnosis and therapy. In the course of their use some of radioactive substances may be discharged into the environment from facilities using the unsealed radioactive materials, which are main artificial sources occurring the public exposure. Discharges are in the form of gases, particles or liquids. This paper provides procedures to estimate the level of the public exposure based on the conservative assumptions and simple calculations in the facility using unsealed liquid sources. They consist of two processes; (1) to calculate maximum concentration of gaseous effluents discharged through the exhaust pipe and average concentration of liquid effluents discharged through the drain of the storage tank, (2) to compare each of them to numerical guidances for the discharges of radioactive gaseous and liquid effluents mentioned in the related notification. For this purpose followings are assumed properly; daily usage, form and dispersion rate of radionuclides, daily amount of radioactive liquid waste and exhaust and drainage equipment. The procedures are readily applicable to evaluate environmental effects by planned effluent discharges from facilities using the unsealed radioactive materials. In addition they may be utilized to obtain practical requirements for radiation safety control necessary for the reductions of the public exposure.

Removal of radioactive methyliodide from the gas stream with a composite sorbent based on polyurethane foam

  • Obruchikov, Alexander V.;Magomedbekov, Eldar P.;Merkushkin, Aleksei O.
    • Nuclear Engineering and Technology
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    • v.52 no.5
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    • pp.1093-1097
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    • 2020
  • A composite iodine sorbent was obtained in the form of porous polymer matrix with activated carbon particles impregnated with triethylenediamine deposited on its surface. A comparative assessment of the radioactive methyliodide capturing efficiency by the composite sorbent and a sample of industrial charcoal sorbent was conducted. It was shown that under the selected testing conditions, the hydraulic resistance of the composite sorbent is lower, and the sorption capacity is higher than that of the industrial charcoal sorbent. A method for comparing the effectiveness of iodine sorbents, based on the calculation of the ratio of the sorption capacity index to the minimum capacity index, needed for the required purification degree was proposed.

Improvement of Evaluation Method for Anticipated Radio-Iodine Release Considering Design Characteristics of KSNP's Auxiliary Building (KSNP의 보조건물 설계특성을 반영한 옥소방사능 예상배출량 평가방법의 개선)

  • 이관희;정재학;박원재
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.463-469
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    • 2003
  • PWR-GALE Code is a computerized mathematical model for calculating the releases of radioactive material in gaseous and liquid effluents from PWRs. In PWR-GALE Code, Auxiliary building iodine removal efficiency, one of the code input data, did not reflect adequately the new design of KSNP which has two auxiliary buildings(PAB and SAB). In this study, we developed a revised method how to correct iodine removal efficiency in KSNP. And newly proposed methodology through case study using Ul-Jin 5, 6 design data was verified.

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Adsorption of Ruthenium on the alkaline Earth Metal Compounds (알카리토금속 화합물에 의한 루테늄의 흡착)

  • 류경옥;문세기;이근범
    • Journal of the Korean Ceramic Society
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    • v.19 no.2
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    • pp.145-151
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    • 1982
  • Many materials such as silica gel, metallic oxide, activated alumina and alkaline earth metal carbonates were employed as filter media for gaseous oxides of ruthenium volatilized during high level radioactive waste processing. The adsorption efficiency of ruthenium on these materials was evaluated. For the purpose of observing behavior of ruthenium oxides, thermogravimetric analysis of ruthenium oxide in a stream of oxygen was carried out. The rate of volatilization was proportional to the square root of oxygen partial pressure, and increased exponentially with temperature. At $650^{\circ}C$, gaseous ruthenium oxides showed a strongly marked effect of deposition. Of all the materials available, calcium oxide proved to be the best that could be used to adsorb ruthenium.

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Periodic Safety Review of Wolsong Unit 1 - Environmental Impact as gaseous and liquid effluents (월성 1호기 주기적안전성평가 - 기체 및 액체 방사성폐기물에 의한 환경영향)

  • 김성민;이은미;김미자;이갑복;정양근;엄희문
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.455-462
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    • 2003
  • According to Korean nuclear code requires Periodic Safety Review(PSR) every 10 years should be perform for operating reactor, and selects the eleven PSR safety factors. Among them the review objective of the environmental impact is to determine whether the operator has an adequate programme for surveillance of the environmental impact of the nuclear power plant based on current safety standards. In this paper, the environmental impact in PSR of Wolsong Unit 1 was reflected current safety standards as of the evaluation date. As a result, all items generally satisfied the standards, and the staff also verified that the population dose due to the operation of Wolsong Unit 1 was controlled safely as of the evaluation date.

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Tritium and 14C in the Environment and Nuclear Facilities: Sources and Analytical Methods

  • Hou, Xiaolin
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.16 no.1
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    • pp.11-39
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    • 2018
  • Tritium and $^{14}C$ are two most important radionuclides released from nuclear facilities to the environment, and $^{14}C$ contributes dominant radiation dose to the population around nuclear power plants. This paper presents an overview of the production, pathway, species and levels of tritium and $^{14}C$ in nuclear facilities, mainly nuclear power plants. The methods for sampling and collection of different species of tritium and $^{14}C$ in the discharge gas from the stack in the nuclear facilities, atmosphere of the nuclear facilities and environment are presented, and the features of different methods are reviewed. The on-line monitoring methods of gaseous tritium and $^{14}C$ in air and laboratory measurement methods for sensitive determination of tritium and $^{14}C$ in collected samples, water and environmental solid samples are also discussed in detailed. Meanwhile, the challenges in the determination and speciation analysis of tritium and $^{14}C$ are also highlighted.

중수로 환형기체 계통의 방사능 inventory 평가

  • Kim, Jin-Tae;Kang, Deok-Won;Son, Uk
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.90-95
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    • 2003
  • Chemical management of annulus gas system is carried out for the purpose of ensuring the safety and reliability of the system via securing the integrity of the system, detecting the D$_2$O in-leakage of coolant and/or moderator, and reducing the radiation dose. Since the quality of CO_2$ gas, which is used as a filling gas for annulus gas system at CANDU plants, has a propound effect on the integrity of the system material and the radiation dose, CO_2$ gas of high quality is needed. If the quality of CO_2$ gas does not meet the specification, it may give rise to undesirable effect not only on the annulus gas system, but also on the environment due to the production of radioactive nuclei. Therefore, it is very important to check the impurities of CO_2$ gas. Based on this background, the inventories of C-14 and Ar-41 in CO_2$ gas that is supplied as annulus gas were estimated using the data on concentrations of the impurities of $CO_2$ such as C, N_2$ and Ar. The results of this study is expect to give useful information on optimization of CO_2$ impurities maintenance and management of gaseous radioactive wastes produced at CANDU plants.

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