• 제목/요약/키워드: Gamma-ray spectroscopy

검색결과 133건 처리시간 0.032초

Gamma-ray Full Spectrum Analysis for Environmental Radioactivity by HPGe Detector

  • Jeong, Meeyoung;Lee, Kyeong Beom;Kim, Kyeong Ja;Lee, Min-Kie;Han, Ju-Bong
    • Journal of Astronomy and Space Sciences
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    • 제31권4호
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    • pp.317-323
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    • 2014
  • Odyssey, one of the NASA's Mars exploration program and SELENE (Kaguya), a Japanese lunar orbiting spacecraft have a payload of Gamma-Ray Spectrometer (GRS) for analyzing radioactive chemical elements of the atmosphere and the surface. In these days, gamma-ray spectroscopy with a High-Purity Germanium (HPGe) detector has been widely used for the activity measurements of natural radionuclides contained in the soil of the Earth. The energy spectra obtained by the HPGe detectors have been generally analyzed by means of the Window Analysis (WA) method. In this method, activity concentrations are determined by using the net counts of energy window around individual peaks. Meanwhile, an alternative method, the so-called Full Spectrum Analysis (FSA) method uses count numbers not only from full-absorption peaks but from the contributions of Compton scattering due to gamma-rays. Consequently, while it takes a substantial time to obtain a statistically significant result in the WA method, the FSA method requires a much shorter time to reach the same level of the statistical significance. This study shows the validation results of FSA method. We have compared the concentration of radioactivity of $^{40}K$, $^{232}Th$ and $^{238}U$ in the soil measured by the WA method and the FSA method, respectively. The gamma-ray spectrum of reference materials (RGU and RGTh, KCl) and soil samples were measured by the 120% HPGe detector with cosmic muon veto detector. According to the comparison result of activity concentrations between the FSA and the WA, we could conclude that FSA method is validated against the WA method. This study implies that the FSA method can be used in a harsh measurement environment, such as the gamma-ray measurement in the Moon, in which the level of statistical significance is usually required in a much shorter data acquisition time than the WA method.

Positional correction of a 3D position-sensitive virtual Frisch-grid CZT detector for gamma spectroscopy and imaging based on a theoretical assumption

  • Younghak Kim ;Kichang Shin ;Aleksey Bolotnikov;Wonho Lee
    • Nuclear Engineering and Technology
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    • 제55권5호
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    • pp.1718-1733
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    • 2023
  • The virtual Frisch-grid method for room-temperature radiation detectors has been widely used because of its simplicity and high performance. Recently, side electrodes were separately attached to each surface of the detectors instead of covering the entire detector surface with a single electrode. The side-electrode structure enables the measurement of the three-dimensional (3D) gamma-ray interaction in the detector. The positional information of the interaction can then be utilized to precisely calibrate the response of the detector for gamma-ray spectroscopy and imaging. In this study, we developed a 3D position-sensitive 5 × 5 × 12 mm3 cadmium-zinc-telluride (CZT) detector and applied a flattening method to correct detector responses. Collimated gamma-rays incident on the surface of the detector were scanned to evaluate the positional accuracy of the detection system. Positional distributions of the radiation interactions with the detector were imaged for quantitative and qualitative evaluation. The energy spectra of various radioisotopes were measured and improved by the detector response calibration according to the calculated positional information. The energy spectra ranged from 59.5 keV (emitted by 241Am) to 1332 keV (emitted by 60Co). The best energy resolution was 1.06% at 662 keV when the CZT detector was voxelized to 20 × 20 × 10.

방사선 처리에 의한 선충 방제 효과 (Experimental Study on Physical Control of Nematodes Using The Ionizing Radiation)

  • 이재광;유대현;이면주
    • 한국환경과학회지
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    • 제14권12호
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    • pp.1113-1117
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    • 2005
  • Gamma-ray treatment was used to exterminate nematodes, which were harmful to agriculture When gamma-ray at the dose range of $5\~75$ kGy was irradaidated, nematodes were reduced by $40\~50\%$ When irradiated over 30 kGy, almost nematodes were non-mobile and fluorochromatic reactions showed that $60\;\~80\%$ of nematodes with non-mobility died after irradiation. The results of electron spin resonance spectroscopy suggested that radicals generated by radiolysis could damage to nematodes.

Green synthesis of Lead-Nickel-Copper nanocomposite for radiation shielding

  • B.M. Chandrika;Holaly Chandrashekara Shastry Manjunatha;R. Munirathnam;K.N. Sridhar;L. Seenappa;S. Manjunatha;A.J. Clement Lourduraj
    • Nuclear Engineering and Technology
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    • 제55권12호
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    • pp.4671-4677
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    • 2023
  • For the first time Pb, Ni, and Cu nanocomposites were synthesized by versatile solution combustion synthesis using Aloevera extract as a reducing agent, to study the potential applications in X-ray/gamma, neutron, and Bremsstrahlung shielding. The synthesized Lead-Nickel-Copper (LNC) nanocomposites were characterized by PXRD, SEM, UV-VIS, and FTIR for the confirmation of successful synthesis. PXRD analysis confirmed the formation of multiphase LNC NCs and the Scherrer equation and the W-H plot gave the average crystal sizes of 19 nm and 17 nm. Surface morphology using SEM and EDX confirmed the presence of LNC NCs. Strong absorption peaks were analyzed by UV visible spectroscopy and the direct energy gap is found to be 3.083 eV. Functional groups present in the LNC NCs were analyzed by FTIR spectroscopy. X-ray/gamma radiation shielding properties were measured using NaI(Tl) detector coupled with MCA. It is found to be very close to Pb. Neutron shielding parameters were compared with traditional shielding materials and found LNC NCs are better than lead and concrete. Secondary radiation shielding known as Bremsstrahlung shielding characteristics also studied and found that LNC NCs are best in secondary radiation shielding. Hence LNC NCs find shielding applications in ionizing radiation such as X-ray/gamma and neutron radiation.

KOMAC 양성자 선형가속기를 이용한 천연 텅스텐 핵반응에 대한 감마선 스펙트럼 측정에 대한 연구 (A Study on Measurement of Gamma-ray Spectrum for the Natural Tungsten nuclear reaction by using KOMAC proton Linear Accelerator)

  • 이삼열
    • 한국방사선학회논문지
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    • 제12권2호
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    • pp.133-138
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    • 2018
  • 양성자가속기연구센터(KOMAC)의 100-MeV 양성자 선형가속기에서 생성된 고에너지 양성자를 사용하여 천연 텅스텐과 핵반응을 일으켰다. 핵반응을 통해 생성된 다양한 핵종으로 부터의 감마선은 HPGe 검출기 감마선 분광시스템을 사용하여 측정하였다. 감마선 표준선원은 에너지 교정 및 검출기의 효율 측정에 사용되었다. 측정된 스펙트럼에서 관찰된 감마선을 분석한 결과 방사성 핵종은 $^{167}Re$, $^{178}Re$, $^{179}Re$, $^{180}Re$, $^{181}Re$, $^{182}Re$, $^{184}Re$, $^{172}Ta$, $^{174}Ta$, $^{178}Ta$, $^{182}Ta$, $^{184}Ta$, $^{175}W$, $^{176}W$, $^{177}W$$^{179}W$ 으로 총 16 종류의 핵종이 생성되었다. 이 연구의 결과는 미래의 핵융합, 천체 물리학 및 핵의학 응용 분야에 적용될 것으로 생각된다.

즉발감마선 측정을 위한 HPGe 검출기의 전계수 또는 동시계수모드에서의 광대역 계측효율 보정 (Efficiency Calibration of HPGe Detector in Normal ana Coincidence Mode for the Determination of Prompt Gamma-ray)

  • 송병철;박용준;지광용
    • 방사성폐기물학회지
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    • 제2권2호
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    • pp.97-104
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    • 2004
  • NIPS 시스템은 중성자 핵반응 결과 방출되는 즉발 감마선을 정량적으로 측정하는 장치이며 고체 및 액체 폐기물 중 존재하는 다양한 원소를 비파괴적으로 분석할 수 있는 장점이 있다. 본 연구에서는 NIPS 시스템에 이용된 고순도반도체 검출기의 계측효율을 $^{l33}$Ba 및 $^{152}$Eu 방사성 동위원소 선원과 $^{35}$ Cl(n, ${\gamma}$)$^{36}$ Cl 핵반응 시 발생되는 즉발감마선을 이용하여 80 keV에서 8 MeV까지 넓은 영역에 대하여 구하였다. $^{35}$ Cl(n, ${\gamma}$)$^{36}$ Cl 핵반응을 이용한 고에너지 감마선의 계측효율은 즉발감마선의 방사능 값을 정확히 알 수 없기 때문에 저 에너지 영역에서 정확히 알고 있는 검출기 효율곡선에 규격화시켜 전 에너지 영역에서의 효율보정곡선을 구하였다. 또한 KCl 표준용액에 $^{252}$ Cf 중성자 선원을 조사시켜 표준용액으로부터 방출되는 즉발 감마선을 고순도반도체 검출기로 측정하고 광대역 계측효율 곡선을 이용하여 수용액 시료에서의 평균 열중성자 속을 예측하였다. NIPS 측정시스템은 주변 재료 물질의 핵반응으로 방출되는 감마선 background를 줄이기 위해 두 개의 고순도반도체 검출기를 이용한 동시계수 장치가 고안되었으며, 동시계수 모드에서의 계측효율도 함께 고려되었으며, 표준선원을 이용하여 전 계수 또는 동시계수모드에서의 background에 대한 측정감도를 비교하였다.다.

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Background reduction by Cu/Pb shielding and efficiency study of NaI(TI) detector

  • Ramadhan, Revink A.;Abdullah, Khairi MS.
    • Nuclear Engineering and Technology
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    • 제50권3호
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    • pp.462-469
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    • 2018
  • The background spectrum of a $3^{{\prime}{\prime}}{\times}3^{{\prime}{\prime}}$ NaI(Tl) well-type scintillation SILENA detector was measured without shielding, in 6 cm thick lead shielding, and with 2 mm thick electrolytic copper covering the detector inside the lead shielding. The relative remaining background of the lead shield lined with copper was found to be ideal for low-level environmental radioactive spectroscopy. The background total count rate in the (20-2160 KeV) was reduced 28.7 times by the lead and 29 times by the Cu + Pb shielding. The effective reduction of background (1.04) by the copper mainly appeared in the energy range from X-ray up to 500 KeV, while for the total energy range the ratio is 1.01 relative to the lead only. In addition, a strong relation between the full-energy peak absolute efficiency and the detector well height was found using gamma-ray isotropic radiation point sources placed inside the detector well. The full-energy peak efficiency at a midpoint of the well (at 2.5 cm) is three times greater than that on the detector surface. The energy calibrations and the resolution of any single energy line are independent of the locations of the gamma source inside or outside of the well.

Uranium Enrichment Determination Using a New Analysis Code for the U XKα Region: HyperGam-U

  • Kim, Junhyuck;Choi, Hee-Dong;Park, Jongho
    • Nuclear Engineering and Technology
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    • 제48권3호
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    • pp.778-784
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    • 2016
  • HyperGam-U was recently developed to determine uranium enrichment based on ${\gamma}$- and X-ray spectroscopy analysis. The $XK_{\alpha}$ region of the uranium spectrum contains 13 peaks for $^{235}U$ and $^{238}U$ and is used mainly for analysis. To describe the X-ray peaks, a Lorentzian broadened shape function was used, and methods were developed to reduce the number of fitting parameters for decomposing the strongly overlapping peaks using channel-energy, energy-width, and energy-efficiency calibration functions. For validation, eight certified reference material uranium samples covering uranium enrichments from 1% to 99% were measured using a high-resolution planar high-purity germanium detector and analyzed using the HyperGam-U code. When corrections for the attenuation and true coincidence summing were performed for the detection geometry in this experiment, the goodness of fit was improved by a few percent. The enrichment bias in this study did not exceed 2% compared with the certified values for all measured samples.

양성자 에너지 변화에 따른 핵반응 생성핵종 분석 (Analysis of Proton Nuclear Reaction-Generated Nuclides for Different Proton Energy)

  • 이삼열
    • 한국방사선학회논문지
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    • 제13권5호
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    • pp.819-824
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    • 2019
  • 본 연구에서 서로 다른 양성자 에너지를 사용하여 핵반응에 의해 생성된 감마선의 차이를 통해 고에너지 양성자 Pb(p, nx) 핵반응에서 생성된 동위원소를 식별하는 방법을 제안했다. 한국원자력연구원의 100-M eV 양성자 선형 가속기에서 생성된 고 에너지 양성자를 이용하여 실험을 수행 하였다. 양성자 핵반응을 통해 생성된 다양한 핵종에 의해 생성된 감마선은 HPGe 검출기로 구성된 감마선 분광법 시스템을 사용하여 측정되었습니다. 감마선 표준선원은 감마선 검출기의 정확한 에너지교정 및 효율측정을 위해 사용되었습니다. 제안한 방법을 위하여 동일한 천연 납 시료에 서로 다른 100 및 60 MeV 양성자 에너지빔을 사용하였다. 이 방법은 동일한 시료에서 발생되는 감마선들을 서로 비교함으로써 생성된 핵종들을 확인하는데 매우 효과적임을 알 수 있었다. 이 연구의 결과는 향후 다른 양성자 핵반응 결과를 얻는데도 매우 효과적으로 적용될 것이라 생각된다.