• 제목/요약/키워드: Fluxes of air pollutants

검색결과 12건 처리시간 0.018초

항공기를 이용한 서해안에서의 SO$_2$ 및 NO$_{x}$의 측정 (Aircraft Measurement of SO$_2$, NO$_{x}$ over Yellow Sea Area)

  • 김병곤;차준석;한진석;박일수;김정수;나진균;최덕일;안준영;강창국
    • 한국대기환경학회지
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    • 제13권5호
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    • pp.361-369
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    • 1997
  • In order to investigate the abundance and transboundary fluxes of air pollutants over the Yellow Sea, airborne measurements were made aboard the SF-600 aircraft (Pan-Asia Engineering) in March, 1996. The data presented in this paper are preliminary results and airborne experiment will be carried out until 1999. The vertical profile of relevant meteorological parameters such as temperature, water vapor, wind direction and wind speed were also observed at Taean. Mixing layer height was about 1000~1100m during the flights. The SO$_2$ and NO$_{x}$ concentrations were 3~6 ppb and 5~7 ppb below 1000 m, within 1 ppb and 3~5 ppb at 1000~2000m, respectively. Backward trajectory analyses were also carried out. A mathematical method by Lelieveld et al.(1989) was used to estimate the flux of air pollutants through the planetary boundary layer of Yellow Sea area. Transboundary fluxes were calculated using the measurement results with respect to the pollutants concentration, depth of the planetary boundary layer, wind speed and wind direction. The estimated transboundary flux of SO$_2$through the western boundary of Korea was about 39~42 tons/hour.r.

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ISCLT3를 이용한 수도권 도시간 대기오염물질 유출입량 추정 (Estimation of Fluxes of Air Pollutants in Seoul Conurbation Using ISCLT3)

  • 홍민선;김순태;김영제;양소희;이동섭;장영기
    • 한국대기환경학회지
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    • 제17권2호
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    • pp.147-155
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    • 2001
  • ISCLT3 model was applied in Seoul metropolitan area to investigate the source-receptor relationships among 17 cities in the Kyonggi Province. For the purpose of the model simulation, emission rates of NO$_2$, SOx, and PM(sub)10 were prepared for grid scale with 1$\times$1 km, and receptors were located on every 2$\times$2 km grid. Meterological data for the last 10 years(88~97) were used as input data. According to our study, NO$_2$ concentration of the cities ranged from 10 to 45 ppb with the highest value appearing from Puchon city. The concentrations of SOx and PM(sub)10 concentrations fell in the range of 5~20 ppb and 20~70$\mu\textrm{g}$/㎥, respectively. It was also found out that air quality in one city can be affected greatly by the air pollutants originating from other cities.

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용담호 주변지역 가스상 대기오염물질 침적량 추정 (Estimation of Gaseous Air Pollutants Deposition Fluxes at Yong-dam Reservoir)

  • 김학민;정구회;김재분;정재호;이범진;김선태
    • 한국대기환경학회:학술대회논문집
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    • 한국대기환경학회 2003년도 추계학술대회 논문집
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    • pp.364-365
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    • 2003
  • 최근 대기기인 오염물질이 환경계에 미치는 영향에 대한 관심이 높아짐에 따라 호소수질에 직ㆍ간접적으로 영향을 주는 대기오염물질에 대한 관심이 커지고 있다. 특히 호소에 유입되는 영양염류 중 질소화합물에 대한 기여수준을 평가한 최근자료에 의하면 대규모 호소 중 89%에 상당하는 호소수내의 질소성분이 자연적으로 존재하는 양을 초과하고 있는 것으로 판단하고 있으며, 초과된 질소성분 중 최고 38%가 대기오염물질과 관련된 질소성분인 것으로 보고하고 있다. (중략)

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터널 내 대기오염물질의 공간분포 예측 (Prediction of spatial distribution of air pollutants within tunnel)

  • 박일건;홍민선;김범석;강호근
    • 한국터널지하공간학회 논문집
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    • 제14권6호
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    • pp.607-616
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    • 2012
  • 지속적인 터널 건설의 증가는 터널 내 대기질 관리에 대한 필요성을 점증시키고 있어 측정 및 모델 모사를 통한 터널 내 대기질 거동에 대한 연구를 수행하였다. 남산1호 터널 입구와 출구의 $CO_2$ 농도차는 250 ppm~400 ppm으로 출구쪽이 높았으며 환기를 안 하는 차량 내부의 농도는 외부에 비해 200 ppm~300 ppm 낮게 측정되었다. 교통량이 적을 시 터널 내 유속은 빨라지며 일정한 농도 구배를 나타내고, 교통량이 증가하면 일정치 않은 농도 구배를 나타내는 것으로 나타났다.

Estimation of Atmospheric Deposition Velocities and Fluxes from Weather and Ambient Pollutant Concentration Conditions : Part I. Application of multi-layer dry deposition model to measurements at north central Florida site

  • Park, Jong-Kil;Eric R. Allen
    • Environmental Sciences Bulletin of The Korean Environmental Sciences Society
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    • 제4권1호
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    • pp.31-42
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    • 2000
  • The dry deposition velocities and fluxes of air pollutants such as SO2(g), O3(g), HNO3(g), sub-micron particulates, NO3(s), and SO42-(s) were estimated according to local meteorological elements in the atmospheric boundary layer. The model used for these calculations was the multiple layer resistance model developed by Hicks et al.1). The meteorological data were recorded on an hourly basis from July, 1990 to June, 1991 at the Austin Cary forest site, near Gainesville FL. Weekly integrated samples of ambient dry deposition species were collected at the site using triple-fiter packs. For the study period, the annual average dry deposition velocities at this site were estimated as 0.87$\pm$0.07 cm/s for SO2(g), 0.65$\pm$0.11 cm/s for O3(g), 1.20$\pm$0.14cm/s for HNO3(g), 0.0045$\pm$0.0006 cm/s for sub-micron particulates, and 0.089$\pm$0.014 cm/s for NO3-(s) and SO42-(s). The trends observed in the daily mean deposition velocities were largely seasonal, indicated by larger deposition velocities for the summer season and smaller deposition velocities for the winter season. The monthly and weekly averaged values for the deposition velocities did not show large differences over the year yet did show a tendency of increased deposition velocities in the summer and decreased values in the winter. The annual mean concentrations of the air pollutants obtained by the triple filter pack every 7 days were 3.63$\pm$1.92 $\mu\textrm{g}$/m3 for SO42-, 2.00$\pm$1.22 $\mu\textrm{g}$/m-3 for SO2, 1.30$\pm$0.59 $\mu\textrm{g}$/m-3 for HNO3, and 0.704$\pm$0.419 $\mu\textrm{g}$/m3 for NO3-, respectively. The air pollutant with the largest deposition flux was SO2 followed by HNO3, SO42-(S), and NO3-(S) in order of their magnitude. The sulfur dioxide and NO3- deposition fluxes were higher in the winter than in the summer, and the nitric acid and sulfate deposition fluxes were high during the spring and summer.

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한국에서 분진 및 금속원소의 건식 침착속도 추정에 관한 연구 (Studies on Estimating Dry Deposition Velocities for Atmospheric Aerosol and Metal Elements in Korea)

  • 김성천;김동술
    • 한국대기환경학회지
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    • 제12권1호
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    • pp.101-112
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    • 1996
  • Dry and wet deposition is an impertant removal mechanism of the amobient aerosol in the atmospheric environment. Since the deposition flut provides adverse impacts on various encironmental media including aquatic and ecological system as well as human health, it is essential to quantitatively estimate the removal fluxes of many air pollutants. Thus, the purposes of this experimental study are to investigate seasonal deposition flux variations of the total dustfall and various inorganic elements in the local ambient air and then to finally estimate their dry deposition velocities. To perform the study, the total of 90 dustfall samples were collected from January, 1994 thru February, 1995 in 5 different cities of Korea including Seoul, Suwon, Daejon, Kwangju, and Kangrung. Each sample was analyzed by an AAS and an ICP to determine the quantities of the 11 inorganic elements, such as Zn, Cd, Cr, K, Na, Pb, Ca, Fe, Mn, Mi, and Cu. As results, deposition fluxes, soluble/insoluble fractions, and deposition velocities for each element were extensively investigated. The resulting dry deposition velocities of some elements in Suwon were estimated by ranges of 0.57 .sim. 0.87 cm/sec for Zn, 0.35 .sim. 0.45 cm/sec for Pb, 1.25 .sim. 3.52 cm/sec for Ca, 0.21 .sim. 0.48 cm/sec for Fe, 0.95 .sim. 9.31 cm/sec for Mn, and 2.08 cm/sec for Cu.

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Deposition Process of Sulfate and Elemental Carbon in Japanese and Thai Forests

  • Sase, Hiroyuki;Matsuda, Kazuhide;Visaratana, Thiti;Garivait, Hathairatana;Yamashita, Naoyuki;Kietvuttinon, Bopit;Hongthong, Bundit;Luangjame, Jesada;Khummongkol, Pojanie;Shindo, Junko;Endo, Tomomi;Sato, Keiichi;Uchiyama, Shigeki;Miyazawa, Masamitsu;Nakata, Makoto;Lenggoro, I. Wuled
    • Asian Journal of Atmospheric Environment
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    • 제6권4호
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    • pp.246-258
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    • 2012
  • Particulate matter deposited on leaf surfaces may cause erosion/abrasion of epicuticular wax and the malfunction of stomata. However, the deposition processes of particulate matter, such as elemental carbon (EC), has not been studied sufficiently in Asian forest ecosystems. Deposition processes for particulate ${SO_4}^{2-}$ and EC were studied in a Japanese cedar forest in Kajikawa, Niigata Prefecture, Japan, and in a dry evergreen forest and a dry deciduous forest in Sakaerat, Nakhon Ratchasima province, Thailand. The ${SO_4}^{2-}$ fluxes attributed to rainfall outside the forest canopy (RF), throughfall (TF), and stemflow (SF) showed distinct seasonalities at both sites, increasing from November to February at the Kajikawa site and in March/April at the Sakaerat site. Seasonal west/northwest winds in winter may transport sulfur compounds across the Sea of Japan to the Kajikawa site. At the Sakaerat site, pollutants suspended in the air or dry deposits from the dry season might have been washed away by the first precipitations of the wet season. The EC fluxes from RF and TF showed similar variations by season at the Kajikawa site, while the flux from TF was frequently lower than that from RF at the Sakaerat site. Particulate matter strongly adsorbed onto leaf surfaces is not washed away by rainfall and contributes to the EC flux. At the Kajikawa site, Japanese cedar leaf surfaces accumulated the highest levels of particulate matter and could not be neglected when calculating the total flux. When such leaf-surface particles were considered, the contribution of dry deposition to the total EC flux was estimated to be 67%, 77%, and 82% at the Kajikawa site, and at the evergreen and deciduous forests of the Sakaerat site, respectively. Leaf-surface particles must be included when evaluating the dry and total fluxes of particulate matter, in particular for water-insoluble constituents such as EC.

수체로의 대기오염물질 건식침적량 측정 (Measurement of Dry Deposition Flux of Air Pollutants to the Waterbody)

  • 김영성;진현철;김용표
    • 한국대기환경학회지
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    • 제20권3호
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    • pp.421-426
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    • 2004
  • Dry deposition fluxes of inorganic acidic species to the waterbody were measured by the dry deposition sampler (DDS). DDS was composed of three pans filled with pure water. An average concentration increase during the sampling time, after removing an abnormal value if existed, was considered as the input by deposition. Important operation parameters such as the amount of water used and sampling time were determined through a series of laboratory experiments. The deposition flux measured by DDS was compared with that by the water surface sampler developed by Yi et ai. (1997a,b).

Assessment of DMS photochemistry at Jeju Island During the Asian Oust-Storm Period of Spring 2001 : Comparison of Model Simulations with Field Observations

  • Shon, Zang-Ho;Hilton Swan;Keith N. Bower;Kim, Ki-Hyun;Lee, Gangwoong;Kim, Jiyoung
    • 한국대기환경학회:학술대회논문집
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    • 한국대기환경학회 2002년도 추계학술대회 논문집
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    • pp.343-343
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    • 2002
  • This study examines the influence of long-range transport of dust particles and air pollutants on both local/regional DMS oxidation chemistry and the distribution of sulfur compounds at Jeju Island (33.17$^{\circ}$ N. 126.10$^{\circ}$ E) during the Asian dust-storm(ADS) period in April 2001. The atmospheric concentrations of these sulfur species were measured at a ground station on Jeju Island. Korea as Part of the ACE-Asia intensive operation. Three ADS events were observed during the periods of 10-12, 13-14. and 25-26 April. respectively. The concentrations of DMS and CS$_2$ were higher during the ADS period than during the non-Asian-dust-storm (NADS) period. Conversely. a difference in SO$_2$ levels during the ADS period was not distinguishable from those during the NADS period. The diurnal variation pattern of DMS observed was largely different from that in the remote marine boundary layer. DMS loss by NO$_3$ in the atmospheric boundary layer was dominant due to significantly high NOx levels influenced by the long-range transport of pollutants from East Asia to Jeju Island The DMS maximum during the ADS period was observed in the late afternoon. The oceanic fluxes of DMS during the ADS and NADS periods were estimated to be 5.7$\pm$2.3 and 2.9 (+2.8/-1.5) mole m$^{-2}$ day$^{-1}$ . respectively. The contribution of oxidized DMS to SO$_2$ levels at Jeju Island during the study period was found to be insignificant.

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2001년 봄철 황사기간 중 서해안지역에서 관측한 대기 중 수은의 환경유동특성 연구 (Environmental Mobilization Characteristics of Total Gaseous Mercury in the Western Coast of Korea During the Yellow Sand Period, 2001)

  • 김민영;신재영;조석주;김준;이강웅;김기현
    • 한국지구과학회지
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    • 제22권6호
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    • pp.480-490
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    • 2001
  • 2001년 3월말 기간을 중심으로 강화도 하리지점에서 대기 중 수은의 토양-대기간 교환율의 측정을 시도하였다. 본 연구에서 수은의 농도구배를 측정하고 이를 미기상학적 인자와 결합하는 방식으로 수은의 플럭스값을 산축하였다. 본 연구의 결과에 따르면, 강화지역의 수은 농도는 일반적으로 도심환경에서 발견되는 수준보다는 현저하게 낮은 수준인 것을 확인할 수 있었다. 그러나 측정된 플럭스값은 200ng/m$^2$/h에 근접하여 일반적으로 청정한 환경에서 발견되는 수준을 훨씬 초과하는 것으로 나타났다. 연구기간 동안 관측된 주요 환경변수들의 분포경향을 비교해 보면, NOx와 PM등을 포함하는 대부분의 변수들은 배출시의 농도가 침적시의 농도에 비해 높게 나타났다. 반면 기상학적 요인들은 이러한 경향성이 고온 또는 저습도에서 뚜렷하게 확인되었다. 상관분석의 결과에 따르면, 배출시에 대부분의 오염인자들이 수은과 강한 양의 상관성을 보여주었지만, 침적시에는 그러한 경향이 역전되는 것으로 나타났다. 특히 흥미로운 사실은 침적시에 수은관련 변수들은 미세입자와 어느 정도 연계성을 띠는 것을 확인시켜 주었다.

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