• Title/Summary/Keyword: Fission track

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Determination of Uranium Concentration in Solid- and Liquid-state Geological Materials by Fission Track Registration Technique and its Applicability (피션트랙 검출기법에 의한 고체 및 액체상태 지질물질의 우라늄 정량과 그 적용성)

  • Shin, Seong-Cheon
    • The Journal of the Petrological Society of Korea
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    • v.24 no.2
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    • pp.77-90
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    • 2015
  • The fission track registration techniques for accurate determinations of uranium in solid- and liquid-state geological materials were recommended and their applicability were examined. The determination of uranium can be achieved by optical counting of neutron-induced fission tracks of $^{235}U$ registered on solid-state track detectors under high magnification. In a dry registration method using powdered pellets of rocks (e.g., granite and coal) showing good uranium-affinity, it was not easy to decide an overall mean concentration over the total sample owing to track-clusters caused by frequent presence of uranium-bearing minerals. Separate scanning for homogeneous and track-clustered parts may be an alternative choice. Assuring the homogeneity over the whole sample, high reproducibilities were confirmed both from duplicate detections using mica and Lexan polycarbonate detectors and from multiple measurements at different thermal neutron fluences. The wet registration method using sealed quartz tubes is recommended to overcome the common heterogeneity in uranium concentrations of $10^1ppm$ and more. Adopting the wet registration, the uranium homogeneity was recovered below the $10^0ppm$ level and the lower detection limit was proved to reach without difficulty the $10^2ppb$ (i.e. $ng\;g^{-1}$) level.

Elemental analysis by neutron induced nuclear reaction - Nuclear track method for the analysis of fissile materials

  • Ha, Yeong-Keong;Pyo, Hyung Yeol;Park, Yong Joon;Jee, Kwang Yong;Kim, Won Ho
    • Analytical Science and Technology
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    • v.18 no.4
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    • pp.263-270
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    • 2005
  • Nuclear track is an useful tool for elemental analysis of radionuclides, such as uranium, plutonium and thorium, etc., and for elements undergoing nuclear reactions with thermal neutrons such as lithium and boron. This method has various application fields such as detecting fissionable radionuelides, measuring the fission rate in nuclear technology, analyzing cosmic radiation from meteorite, calculating the age of minerals as well as their history, etc. Track registration method has been applied to the microscopic analysis of boron and fissionable element such as uranium in KAERI. This report reviews the theoretical background of the nuclear track formation, practical procedures to obtain etched tracks and a perspective of the future.

Determination of the Spontaneous Fission Rate of $^{238}U$ Using Solid State Track Recorder (고체비적검출기(固體飛跡檢出器)를 이용(利用)한 $^{238}U$의 자발핵분열율(自發核分裂率) 결정(決定))

  • Ro, Seung-Gy;Yook, Chong-Chul;Koh, Byung-Ryung
    • Journal of Radiation Protection and Research
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    • v.10 no.2
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    • pp.144-147
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    • 1985
  • The spontaneous fission rate of $^{238}U$ has been determined using a solid state track recorder that was a pre-etched mica. Counting the tracks revealed in mica made it possible to calculate the spontaneous fission rate. The mica remained in close contact with a $^{238}UO_2$ foil for about five years. The resulting fission rate was $5.21{\pm}0.33$ fissions/g-sec.

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Thermal and uplift histories of Mesozoic granites in Southeast Korea: new fission track evidences

  • Shin, Seong-Cheon;Susumu Nishimura
    • The Journal of the Petrological Society of Korea
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    • v.2 no.2
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    • pp.104-121
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    • 1993
  • Fission track (FT) thermochronological analyses on Mesozoic granites provide new information about cooling and uplift histories in Southeast Korea. Twenty-nine new FT sphene, zircon and apatite ages and seven track length measurements are presented for eleven granite samples. Measured mineral ages against assumed closure temperatures yield cooling rates for each sample. Relatively rapid (7-$15^{\circ}C$/Ma) and simple cooling patterns from the middle Cretaceouss (ca. 90-100 Ma) granites are caused mainly by a high thermal contrast between the intruding magma and country rocks at shallow crustal levels (ca. 1-2.5 km-depths). On the contrary, a slow overall cooling (1-$4^{\circ}C$/Ma) of the Triassic to Jurassic granites (ca. 250-200 Ma), emplaced at deep depths (>>9 km), may mainly depend upon very slow denudation of the overlying crust. The uplift history of the Triassic Yeongdeog Pluton in the Yeongyang Subbasin, west of the Yangsan Fault, is characterized by a relatively rapid uplift (~0.4 mm/a) before the total unroofing of the pluton in the earliest Cretaceous (~140 Ma) followed by a subsidence (~0.2mm/a) during the Hayang Group sedimentation. Stability of original FT zircon ages (156 Ma) and complete erasure of apatite ages suggest a range of 3 to 5.5 km for the basin subsidence. Since 120 Ma up to present, the Yeongyang Subbasin has been slowly uplifted (~0.04 mm/a). The FT age patterns of Jurassic granites both from the northeastern wing of the Ryeongnam Massif and from the northern edge of the Pohang-Kampo Block indicate that the two geologic units have been slowly uplifted with a same mean rate (~0.04 mm/a) since early Cretaceous. Estimates of Cenozoic total uplifts since 100 Ma are different: Ryeongnam Massif (~6 km)=Pohang-Kampo Block (~6 km)>Yeongyang Subbasin(~4 km).

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Determination of the number of 235U target nuclei in the irregular target using a fission time projection chamber

  • Jiajun Zhang;Jun Xiao;Junjie Sun;Mingzhi Zhang;Taiping Peng;Pu Zheng
    • Nuclear Engineering and Technology
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    • v.56 no.2
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    • pp.444-450
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    • 2024
  • Based on multiple measurements of ionization loss, the Time Projection Chamber (TPC) combines strong tracking ability with particle identification ability in a large momentum range, which is an important advantage of TPC detection technology over traditional ionization measurement technology. According to these two characteristics of TPC, applying it to the measurement of fission cross-section can greatly improve the measurement accuracy. During the measurement of the fission cross-section, the number of target nuclei is required to be accurately measured. So this paper introduces a method for measuring the number of 235U target nuclei using a fission TPC system. The measurement result agrees with the reference value, and relative error is around 1 %.

Study on the Enhancement of Reproducibility for Track Technology Using a Multi-dot Plate (다중시료 점적판을 이용한 트랙기입법의 재현성 증대 연구)

  • Park, Y.J.;Pyo, H.Y.;Song, B.C.;Jee, K.Y.
    • Analytical Science and Technology
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    • v.17 no.5
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    • pp.434-437
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    • 2004
  • Alpha track technology can provide useful isotopic information of boron in the primary coolant water. In the quantitative analysis using the alpha track analysis, the shape or area of sample on the solid track detector becomes very important, especially for the analysis of liquid samples. In this research, a multi-dot plate has been developed for this purpose. The multi-dot plate provides fixed standard shape of the sample solution that stays inside of the printed circle, and consequently increases the reproducibility of the boron analysis.