• Title/Summary/Keyword: Environmental radionuclide

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Uranium Levels in Groundwater of CGS (Community Groundwater System) of Korea (국내 마을상수도 지하수의 우라늄 함량)

  • Cho, Byong-Wook;Kim, Moon-Su;Kim, Dong-Su;Hwang, Jae-Hong
    • Economic and Environmental Geology
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    • v.51 no.6
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    • pp.543-551
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    • 2018
  • The uranium concentrations were determined in groundwater collected from 3,820 community groundwater system (CGS) located in remote rural areas where access to the nationwide water work is not easy. The frequency distribution of uranium concentrations shows a lognormal distribution which is common in most radionuclide surveys. The measured maximum uranium concentration was $1,757.0{\mu}g/L$ with an average of $6.46{\mu}g/L$ and a median of $0.76{\mu}g/L$. When grouping the uranium concentration results of CGS into 10 geological units, the median uranium concentration was high ($0.99-2.05{\mu}g/L$) in three granite areas, and low in sedimentary rocks areas and porous volcanic rocks areas ($0.04-0.50{\mu}g/L$). Of the 3,820 samples, 3.8% are above the guideline value of $30{\mu}g/L$ (WHO, 2011). On the other hand, the exceeding rates of JGRA and PGRA CGS are 8.5% and 7.5%, respectively. Therefore, attention should be paid for the development of new CGS along with the management of the existing CGS in JGRA and PGRA areas.

Status of a national monitoring program for environmental radioactivity and investigation of artificial radionuclide concentrations (134Cs, 137Cs, 131I) in rivers and lakes (방사성물질 측정망 현황 및 하천·호소 내 인공방사성물질 (134Cs, 137Cs, 131I) 조사)

  • Kim, Jiyu;Jung, Hyun-ji;An, Mijeong;Hong, Jung-Ki;Kang, Taegu;Kang, Tae-Woo;Cho, Yoon-Hae;Han, Yeong-Un;Seol, Bitna;Kim, Wansuk;Kim, Kyunghyun
    • Analytical Science and Technology
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    • v.28 no.6
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    • pp.377-384
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    • 2015
  • A survey of the artificial radionuclides in rivers and lakes was conducted to investigate their levels in surface water. Water samples were collected at 60 points and analyzed by gamma-ray spectrometry with a measurement time of 10,000 seconds for 134Cs, 137Cs, and 131I. The obained values were lower than MDA for all points, except one point for 131I that was 0.533±0.058 Bq/L. 131I is known as a radioactive material that occurs frequently in sewage treatment plants. Because it is often used for medical treatments and subject to spreading into the environment due to the excretion from the patients. For the point where 131I was detected, we conducted additional investigation on the upstream river point and the effluent points of nearby sewage treatment plant to find the source of 131I. 131I was not detected at the upstream points of one of the upstream sewage treatment plants but found at the downstream points with the level being 0.257±0.034 to 0.799±0.051 Bq/L, proving the sewage treatment plant was the 131Isource.

Geostatistical Interpretation of Cs-137 and K-40 Result of the Lithosphere in the Vicinity of Youngkwang Nuclear Power Plant (지구통계학적 방법에 의한 영광원전주변 토층내 Cs-137 및 K-40 측정 결과의 해석)

  • 김경웅;이재석;문승현;박철승;고일원;고은정;조병옥;정철영;전수열
    • Economic and Environmental Geology
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    • v.35 no.6
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    • pp.545-552
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    • 2002
  • In order to investigate the influence of nuclear power plant operation on its nearby environment, soil, stream and marine sediment samples were collected in the vicinity of the Youngkwang Nuclear Power Plant in Korea, and analyzed for artificial and natural radionuclide radioactivity. From the analytical result, Cs-137 was detected in most soil samples. but it may have been derived fiom past nuclear weapon tests because Cs-134 having short half-live was not detected. The radioactivities of Cs-137 in the sediment samples were also detected which are within the normal range in the sediments based upon the published literature between 1997 and 1999. For the quality control of radioactivity analysis of environmental samples, sets of marine sediments in the Gamami area were analyzed using two HPGe Gamma-ray Spectroscopes (30% and 45%) according to the geostatistical sampling strategy, and Cs-137 and K-40 results were interpreted by analysis of variance (ANOVA). In the two-way ANOVA, variances derived from the geochemical variation were significant, but errors from sampling and analytical procedures are negligible. In conclusion. all the radioanalytical procedures of this study including sampling are validated to be acceptable.

Review of Thermodynamic Sorption Model for Radionuclides on Bentonite Clay (벤토나이트와 방사성 핵종의 열역학적 수착 모델 연구)

  • Jeonghwan Hwang;Jung-Woo Kim;Weon Shik Han;Won Woo Yoon;Jiyong Lee;Seonggyu Choi
    • Economic and Environmental Geology
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    • v.56 no.5
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    • pp.515-532
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    • 2023
  • Bentonite, predominantly consists of expandable clay minerals, is considered to be the suitable buffering material in high-level radioactive waste disposal repository due to its large swelling property and low permeability. Additionally, the bentonite has large cation exchange capacity and specific surface area, and thus, it effectively retards the transport of leaked radionuclides to surrounding environments. This study aims to review the thermodynamic sorption models for four radionuclides (U, Am, Se, and Eu) and eight bentonites. Then, the thermodynamic sorption models and optimized sorption parameters were precisely analyzed by considering the experimental conditions in previous study. Here, the optimized sorption parameters showed that thermodynamic sorption models were related to experimental conditions such as types and concentrations of radionuclides, ionic strength, major competing cation, temperature, solid-to-liquid ratio, carbonate species, and mineralogical properties of bentonite. These results implied that the thermodynamic sorption models suggested by the optimization at specific experimental conditions had large uncertainty for application to various environmental conditions.

Review of Unplanned Release at Foreign Nuclear Power Plants and Radiological Monitoring at Korean Power Plants (해외원전 비계획적 방출 및 한국의 환경감시 현황 분석)

  • Park, Soo-Chan;Ham, Baknoon;Kwon, Jang-Soon;Cho, Dong-Keun;Jeong, Jihye;Kwon, Man Jae
    • Journal of Soil and Groundwater Environment
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    • v.23 no.4
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    • pp.1-15
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    • 2018
  • Despite of safety issues related to radiological hazards, 31 countries around the world are operating more than 450 nuclear power plants (NPPs). To operate NPPs safely, safety regulations from radiation protection organizations were developed and adopted in many countries. However, many cases of radionuclide releases at foreign NPPs have been reported. Almost all commercial NPPs routinely release radioactive materials to the surrounding environments as liquid and gas phases under control. These releases are called 'planned releases' which are planned, regularly monitored, and well documented. Meanwhile, the releases focused in this review, called 'unplanned releases', are neither planned nor monitored by regulatory and/or protection organizations. NPPs are generally composed of various structures, systems and components (SSCs) for safety. Among them, the SSCs near reactors are closely related to safety of NPPs, and typically fabricated to comply with stringent requirements. However, some non-safety related SSCs such as underground pipes may be constructed only according to commercial standards, causing the leakage of radioactive fluids usually containing tritium ($^3H$). This paper discusses SSCs of NPPs and introduces several cases of unplanned releases at foreign NPPs. The current regulation on the environmental radiological surveillance and assessment around the NPPs in South Korea are also examined.

Safety Assessment on Disposal of HLW from P&T Cycle (핵변환 잔류 고준위 방사성 폐기물 처분 성능 평가)

  • 이연명;황용수;강철형
    • Tunnel and Underground Space
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    • v.11 no.2
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    • pp.132-145
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    • 2001
  • The purpose and need of the study is to quantify the advantage or disadvantage of the environmental friendliness of the partitioning of nuclear fuel cycle. To this end, a preliminary study on the quantitative effect of the partition on the permanent disposal of spent PWR and CANDU fuel (HLW) was carried out. Before any analysis, the so-called reference radionuclide release scenario from a potential repository embedded into a crystalline rock was developed. Firstly, the feature, event and processes (FEPs) which lead to the release of nuclides from waste disposed of in a repository and the transport to and through the biosphere were identified. Based on the selected FEPs, the ‘Well Scenario’which might be the worst case scenario was set up. For the given scenario, annual individual doses to a local resident exposed to radioactive hazard were estimated and compared to that from direct disposal. Even though partitioning and transmutation could be an ideal solution to reduce the inventory which eventually decreases the release time as well as the peaks in the annual dose and also minimize the repository area through the proper handling of nuclides, it should overcome major disadvantages such as echnical issues on the partitioning and transmutation system, cost, and public acceptance, and environment friendly issues. In this regard, some relevant issues are also discussed to show the direction for further studies.

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Dependence Evaluation of the Self-Absorption Correction Factor for p-type High Purity Germanium Detector Characteristics (p-type HPGe 검출기 특성에 따른 밀도 보정인자 의존도 평가)

  • Jang, Mee;Ji, Young-Yong;Kim, Chang-Jong;Lee, Wanno;Kang, Mun Ja
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.13 no.4
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    • pp.295-300
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    • 2015
  • The precise determination of the activity for each radionuclide in environmental samples requires the self-absorption correction factor. In this research, we derived the self-absorption correction factor for three p-type high purity germanium detectors using the Monte Carlo code MCNPX. These detectors have different characteristics such as crystal diameter, height and size of the core. We compared the calculated full-energy peak efficiency with the experimental value using a standard sample with $1g/m^3$ density and verified the modeling. We simulated the dependency of the full-energy peak efficiency on the 0.3, 0.6, 0.9, 1.0, 1.2 and $1.5g/m^3$ samples and obtained the corresponding self-absorption correction factor. The self-absorption correction factors calculated for the three detectors differ by less than 1% over most of the energy range and sample densities considered. This indicates that the self-absorption correction factors are independent of the crystal characteristics of HPGe detector.

Analysis of radioactivity levels and hazard assessment of black sand samples from Rashid area, Egypt

  • Abdel-Rahman, Mohamed A.E.;El-Mongy, Sayed A.
    • Nuclear Engineering and Technology
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    • v.49 no.8
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    • pp.1752-1757
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    • 2017
  • The aim of this study is to evaluate the radioactivity levels and radiological impacts of representative black sand samples collected from different locations in the Rashid area, Egypt. These samples were prepared and then analyzed using the high-resolution gamma ray spectroscopy technique with a high-purity germanium detector. The activity concentration ($A_c$), minimum detectable activity, absorbed gamma dose rate, external hazard index ($H_{ex}$), annual effective dose rate equivalent, radium equivalent, as well as external and internal hazard index ($H_{ex}$ and $H_{in}$, respectively) were estimated based on the measured radionuclide concentration of the $^{238}U$($^{226}Ra$) and $^{232}Th$ decay chains and $^{40}K$. The activity concentrations of the $^{238}U$, $^{232}Th$ decay series and $^{40}K$ of these samples varied from $45.11{\pm}3.1Bq/kg$ to $252.38{\pm}34.3Bq/kg$, from $64.65{\pm}6.1Bq/kg$ to $579.84{\pm}53.1Bq/kg$, and from $403.36{\pm}20.8Bq/kg$ to $527.47{\pm}23.1Bq/kg$, respectively. The activity concentration of $^{232}Th$ in Sample 1 has the highest value compared to the other samples; this value is also higher than the worldwide mean range as reported by UNSCEAR 2000. The total absorbed gamma dose rate and the annual effective dose for these samples were found to vary from 81.19 nGy/h to 497.81 nGy/h and from $99.86{\mu}Sv/y$ to $612.31{\mu}Sv/y$, which are higher than the world average values of 59 nGy/h and $70{\mu}Sv/y$, respectively. The $H_{ex}$ values were also calculated to be 3.02, 0.47, 0.63, 0.87, 0.87, 0.51 and 0.91. It was found that the calculated value of $H_{ex}$ for Sample 1 is significantly higher than the international acceptable limit of <1. The results are tabulated, depicted, and discussed within national and international frameworks, levels, and approaches.

Calculation of Effective Half-life of Gamma Emission Radionuclide using Bio-kinetic Model (생체역동학 모델을 이용한 감마선 방출 핵종의 유효반감기 계산)

  • Lee, Sang-Kyung;Jeong, Kyu-Hwan;Lee, Ji-Yon;Kim, Bong-Gi;Kim, Jung-Min
    • Journal of Radiation Industry
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    • v.12 no.4
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    • pp.277-285
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    • 2018
  • Patients administered radioisotope for medical purposes are regulated by each country to quarantine them until their body's radioactivity contents decrease below release criteria. To predict the quarantine period and provide it to medical staffs and patients, it is necessary to approach the assessment of the exposure dose of persons due to patients in a realistic manner. For this purpose, a whole-body effective half-life should be applied to the dose assessment equation instead of the physical half-life. In this study, we constructed a bio-kinetic model for each nuclear species based on the ICRP publication to obtain a whole-body effective half-life of 10 unsealed gamma-ray emitting nuclei from the notification of Nuclear Safety and Security Commission, and calculated the effective half-life mathematically by simulating the distribution of the radioisotope administered in the whole body as well as each organ scale. The whole-body effective half-life of $^{198}Au$, $^{67}Ga$, $^{123}I$, $^{111}In$, $^{186}Re$, $^{99m}Tc$, and $^{201}TI$ were 1,93, 2.57, 0.295, 2.805, 1.561, 0.245, and 2.397 days respectively. However, it was found to be undesirable to offer a single value of the effective half-life of $^{125}I$, $^{131}I$, and $^{169}Yb$ because the changes in the effective half-life show no linearity. A bio-kinetic model created for the internal exposure assessment has been shown to be possible to calculate the effective half-life of radioisotopes administered in the patient's body, but subsequent studies of radiolabeled compounds are required as well.

Sorption and Migration Studies of Fission Products for Ground Waste Disposal

  • Lee, Sang-Hoon;Chun, Kwan-Sik;Yoon, Young-Ku
    • Nuclear Engineering and Technology
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    • v.10 no.3
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    • pp.153-163
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    • 1978
  • The problems of solid waste disposal into the ground in connection with environmental aspects in the vicinity of a site would be very significant, though ground disposal for solid waste is safe and economical method. Studies of the waste-movement and migration of radionuclides (Sr-90 and Cs-137) for the disposal into the ground were performed under laboratory and field conditions. Affinity of the soils for radionuclide solution was higher than that in the acid solution. The sorption of radionuclides by the soils showed a time-dependent reation. The migration rates of radiostrontium and radiocesium were a range of 3.73$\times$10$^{-3}$ to 10.9$\times$10$^{-3}$ cm/day. The nuclides in the soil migrate much more slowly than the water, probably due to its high exchange capacity. The observed distribution of tritium was compared with that calculated by a mathematical model based on diffusivity. This study suggests that the tritiated water can be used to trace the movement of ground water.

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