• Title/Summary/Keyword: Deep geological disposal of high-level radioactive waste

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A Review of the Influence of Sulfate and Sulfide on the Deep Geological Disposal of High-level Radioactive Waste (고준위방사성폐기물 심층처분에 미치는 황산염과 황화물의 영향에 대한 고찰)

  • Jin-Seok Kim;Seung Yeop Lee;Sang-Ho Lee;Jang-Soon Kwon
    • Economic and Environmental Geology
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    • v.56 no.4
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    • pp.421-433
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    • 2023
  • The final disposal of spent nuclear fuel(SNF) from nuclear power plants takes place in a deep geological repository. The metal canister encasing the SNF is made of cast iron and copper, and is engineered to effectively isolate radioactive isotopes for a long period of time. The SNF is further shielded by a multi-barrier disposal system comprising both engineering and natural barriers. The deep disposal environment gradually changes to an anaerobic reducing environment. In this environment, sulfide is one of the most probable substances to induce corrosion of copper canister. Stress-corrosion cracking(SCC) triggered by sulfide can carry substantial implications for the integrity of the copper canister, potentially posing a significant threat to the long-term safety of the deep disposal repository. Sulfate can exist in various forms within the deep disposal environment or be introduced from the geosphere. Sulfate has the potential to be transformed into sulfide by sulfate-reducing bacteria(SRB), and this converted sulfide can contribute to the corrosion of the copper canister. Bentonite, which is considered as a potential material for buffering and backfilling, contains oxidized sulfate minerals such as gypsum(CaSO4). If there is sufficient space for microorganisms to thrive in the deep disposal environment and if electron donors such as organic carbon are adequately supplied, sulfate can be converted to sulfide through microbial activity. However, the majority of the sulfides generated in the deep disposal system or introduced from the geosphere will be intercepted by the buffer, with only a small amount reaching the metal canister. Pyrite, one of the potential sulfide minerals present in the deep disposal environment, can generate sulfates during the dissolution process, thereby contributing to the corrosion of the copper canister. However, the quantity of oxidation byproducts from pyrite is anticipated to be minimal due to its extremely low solubility. Moreover, the migration of these oxidized byproducts to the metal canister will be restricted by the low hydraulic conductivity of saturated bentonite. We have comprehensively analyzed and summarized key research cases related to the presence of sulfates, reduction processes, and the formation and behavior characteristics of sulfides and pyrite in the deep disposal environment. Our objective was to gain an understanding of the impact of sulfates and sulfides on the long-term safety of high-level radioactive waste disposal repository.

An Improved Concept of Deep Geological Disposal System Considering Arising Characteristics of Spent Fuels From Domestic Nuclear Power Plants (국내 원자력발전소에서의 사용후핵연료 발생 특성을 고려한 심층 처분시스템 개선)

  • Lee, Jongyoul;Kim, Inyoung;Choi, Heuijoo;Cho, Dongkeun
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.17 no.4
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    • pp.405-418
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    • 2019
  • Based on spent fuels characteristics from domestic nuclear power plants and a disposal scenario from the current basic plan for high-level radioactive waste management, an improved disposal system has been proposed that enhances disposal efficiency and economic effectiveness compared to the existing disposal system. For this purpose, two disposal canisters concepts were derived from the length of the spent fuel generated from the nuclear power plants. In the disposal scenario, the acceptable amount of decay heat for each disposal container was determined, taking into account the discharge and disposal times of spent fuels in accordance with the current basic plan. Based on the determined decay heat of the two types of disposal canisters and the associated disposal system, thermal stability analyses were performed to confirm their suitability to the proposed disposal system design requirement and disposal efficiency assessment. The results of this study confirm 20% reduction in the disposal area and 20% increase in disposal density for the proposed disposal system compared to the existing system. These results can be used to establish a spent fuel management policy and to design a viable commercial disposal system.

Evaluation of Mazars damage model of KURT granite under simulated coupled environment of geological disposal (처분 복합환경을 고려한 KURT 화강암의 Mazars 손상모델 평가)

  • Kim, Jin-Seop;Hong, Chang-Ho;Kim, Geon-Young
    • Journal of Korean Tunnelling and Underground Space Association
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    • v.22 no.4
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    • pp.419-434
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    • 2020
  • In this study, the damage parameters of Mazars model for KURT (KAERI Underground Research Tunnel) granite are measured form uniaxial compressive and Brazilian tests under the simulated coupled condition of a deep geological disposal. The tests are conducted in three different temperatures (15℃, 45℃, and 75℃) and dry/saturated conditions. Major model parameters such as maximum effective tensile strain (𝜖d0), At, Bt, Ac, and Bc differ from the typical reference values of concrete specimens. This is likely due to the difference in elastic modulus between rock and concrete. It is found that the saturation of specimens causes an increase in value of Bt and Bc while, the rise in temperature increases 𝜖d0 and Bt and decreases Bc. The damage model obtained from this study will be used as the primary input parameters in the development of coupled Thermo-Hydro-Mechanical Damage numerical model in KAERI.

Analyses of the Double-Layered Repository Concepts for Spent Nuclear Fuels (사용후핵연료 심지층 처분장 복층개념 분석)

  • Lee, Jongyoul;Kim, Hyeona;Lee, Minsoo;Choi, Heui-Joo;Kim, Kyungsu
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.15 no.2
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    • pp.151-159
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    • 2017
  • A deep geological disposal at a depth of 500 m in stable host rock is considered to be the safest method with current technologies for disposal of spent fuels classified as high-level radioactive waste. The most important requirement is that the temperature of the bentonite buffer, which is a component of the engineered barrier, should not exceed $100^{\circ}C$. In Korea, the amount of spent fuel generated by nuclear power generation, which accounts for about 30% of the total electricity, is continuously increasing and accumulating. Accordingly, the area required to dispose of it is also increasing. In this study, various duplex disposal concepts were derived for the purpose of improving the disposal efficiency by reducing the disposal area. Based on these concepts, thermal analyses were carried out to confirm whether the critical disposal system requirements were met, and the thermal stability of the disposal system was evaluated by analyzing the results. The results showed that upward 75 m or downward 75 m apart from the reference disposal system location of 500 m depth would qualify for the double layered disposal concept. The results of this study can be applied to the establishment of spent fuel management policy and the design of practical commercial disposal system. Detailed analyses with data of a real disposal site are necessary.

Heat Transfer Modeling by the Contact Condition and the Hole Distance for A-KRS Vertical Disposal (A-KRS 수직 처분공 접촉 조건 및 처분공 간의 거리에 따른 열전달 해석)

  • Kim, Dae-Young;Kim, Seung-Hyun
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.17 no.3
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    • pp.313-319
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    • 2019
  • The A-KRS (Advanced Korean Reference Disposal System) is the disposal concept for pyroprocessed waste, which has been developed by the Korea Atomic Energy Research Institute. In this disposal concept, the amount of high-level radioactive waste is minimized using pyrochemical process, called pyroprocessing. The produced pyroprocessed waste is then solidified in the form of monazite ceramic. The final product of ceramic wastes will be disposed of in a deep geological repository. By the way, the decay heat is generated due to the radioactive decay of fission products and raises the temperature of buffer materials in the near field of radioactive waste repository. However, the buffer temperature must be kept below $100^{\circ}C$ according to the safety regulation. Usually, the temperature can be controlled by variation of the canister interdistance. However, KAERI has modelled thermal analysis under the boundary condition, where the waste canisters are in direct contact with each other. Therefore, a reliable temperature analysis in the disposal system may fail because of unknown thermal resistence values caused by the spatial gap between waste canisters. In the present work, we have performed thermal analyses considering the gap between heating elements and canisters at the beginning of canister loading into the radioactive waste repository. All thermal analyses were performed using the COMSOL software package.

Case Study of Deep Geological Disposal Facility Design for High-level Radioactive Waste (스웨덴 고준위방사성폐기물 심층처분시설의 설계 사례 분석)

  • Juhyi Yim;Jae Hoon Jung;Seokwon Jeon;Ki-Il Song;Young Jin Shin
    • Tunnel and Underground Space
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    • v.33 no.5
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    • pp.312-338
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    • 2023
  • The underground disposal facility for spent nuclear fuel demands a specialized design, distinct from conventional practices, to ensure long-term thermal, mechanical, and hydraulic integrity, preventing the release of radioactive isotopes from high-temperature spent nuclear fuel. SKB has established design criteria for such facilities and executed practical design implementations for Forsmark. Moreover, in response to subsurface uncertainty, SKB has proposed an empirical approach involving monitoring and adaptive design modifications, alongside stepwise development. SKB has further introduced a unique support system, categorizing ground types and behaviors and aligning them with corresponding support types to confirm safety through comparative analyses against existing systems. POSIVA has pursued a comparable approach, developing a support system for Onkalo while accounting for distinct geological characteristics compared to Forsmark. This demonstrates the potential for domestic implementation of spent nuclear fuel disposal facility designs and the establishment of a support system adapted to national attributes.

Analysis of the Disposal Tunnel and Disposal Pit Spacing for the Spent Fuel Repository Layout (사용후핵연료 지하 처분장 배치를 위한 처분공 및 처분터널 간격 분석)

  • Lee, Jong-Youl;Lee, Yang;Choi, Heui-Joo;Choi, Jong-Won
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.4 no.4
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    • pp.393-400
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    • 2006
  • In design of a deep geological repository for the high level wastes, it is very important that the temperature of the bentonite block should not be over $100^{\circ}C$ to maintain the integrity of the bentonite buffer block from the decay heat. In this study, for the layout of the repository to meet the requirement, the analysis of the disposal tunnel and disposal pit spacing was carried out. To do this, based on the reference repository concept, several cases of cooling times and disposal tunnel and disposal pit spacing were compared. The thermal stabilities of the disposal systems were analyzed in terms of the cooling time and spacing. The results showed that it was more desirable to determine the layout of the repository in terms of disposal pit spacing than the disposal tunnel spacing. The results of these analyses can be used in the deep geological repository design. The detailed analyses with the exact site characteristics data will reduce the uncertainty of the results.

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Rock Mechanics Site Characterization for HLW Disposal Facilities (고준위방사성폐기물 처분시설 부지에 대한 암반역학 부지특성화)

  • Um, Jeong-Gi;Hyun, Seung Gyu
    • Economic and Environmental Geology
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    • v.55 no.1
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    • pp.1-17
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    • 2022
  • The mechanical and thermal properties of the rock masses can affect the performance associated with both the isolating and retarding capacities of radioactive materials within the deep geological disposal system for High-Level Radioactive Waste (HLW). In this study, the essential parameters for the site descriptive model (SDM) related to the rock mechanics and thermal properties of the HLW disposal facilities site were reviewed, and the technical background was explored through the cases of the preceding site descriptive models developed by SKB (Swedish Nuclear and Fuel Management Company), Sweden and Posiva, Finland. SKB and Posiva studied parameters essential for the investigation and evaluation of mechanical and thermal properties, and derived a rock mechanics site descriptive model for safety evaluation and construction of the HLW disposal facilities. The rock mechanics SDM includes the results obtained from investigation and evaluation of the strength and deformability of intact rocks, fractures, and fractured rock masses, as well as the geometry of large-scaled deformation zones, the small-scaled fracture network system, thermal properties of rocks, and the in situ stress distribution of the disposal site. In addition, the site descriptive model should provide the sensitivity analysis results for the input parameters, and present the results obtained from evaluation of uncertainty.

Status of Researches of Excavation Damaged Zone in Foreign Underground Research Laboratories Constructed for Developing High-level Radioactive Waste Disposal Techniques (고준위방사성폐기물 처분 기술개발을 위해 건설된 해외 지하연구시설에서의 암반손상대 연구 현황)

  • Park, Seunghun;Kwon, Sangki
    • Explosives and Blasting
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    • v.35 no.3
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    • pp.31-54
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    • 2017
  • In the countries operating nuclear reactors, the development of high-level radioactive waste(HLW) disposal technique is considered as an urgent and important issue for sustainable utilization of nuclear energy. In Korea, in which a low and intermediate radioactive waste repository is already operating, the construction of an underground research laboratory for in situ validation studies became a matter of interest with increasing concerns on the management of HLW. In order to construct and to operate an underground HLW repository safely in deep underground, the stability of rock mass should be guaranteed. As an important factor on rock stability, excavation damaged zone (EDZ) has been studied in many underground research laboratories in foreign countries. For accurate evaluation of the characteristics and effects of EDZ under disposal condition, it is required to use reliable investigation method based on the analysis of previous studies in similar conditions. In this study, status of foreign underground research laboratories in other countries, approaches for investigation the characteristics, size, and effect of EDZ, and major findings from the researches were surveyed and reported. This will help the accomplishment of domestic researches for developing HLW management techniques in underground research laboratory.

Site Selection Methods for High-Level Radioactive Waste Disposal Facilities: An International Comparison (고준위방사성폐기물 처분시설 부지선정 방식 해외사례 분석)

  • HyeRim Kim;MinJeong Kim;SunJu Park;WoonSang Yoon;JungHoon Park;JeongHwan Lee
    • The Journal of Engineering Geology
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    • v.33 no.2
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    • pp.335-353
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    • 2023
  • Site selection processes for high-level radioactive waste disposal facilities in different countries differ in terms of local geology and degree of public engagement. There seem to be three alternative processes for site selection: (1) selection with community consent after government choice; (2) selection with continuous community engagement after exclusion of unsuitable areas based on existing survey data; or (3) site selection where communities have expressed a willingness to participate. The Yucca Mountain site in Nevada, USA, was selected as the final disposal site by process (1) through six stages, but its development was suspended owing to opposition from the local governor and environmental groups. In Sweden, Switzerland, and Germany, process (2) is used and sites are selected through three stages. Sweden and Switzerland have completed site selection, and Germany is currently engaged in the process. The UK adopted process (3) with six stages, although the process has been suspended owing to poor community participation. In Korea, temporary storage facilities for spent nuclear fuel will reach saturation from 2030, so site selection must be promoted through various laws and systems, with continuous communication with local communities based on transparent and scientifically undertaken procedures.