• Title/Summary/Keyword: Atmospheric aerosols

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Columnar Aerosol Properties at Yongin According to Transport Paths of Back Trajectories (역궤적 이동경로별 용인지역의 컬럼에어로졸 특성)

  • Park, Jisoo;Choi, Yongjoo;Ghim, Young Sung
    • Journal of Korean Society for Atmospheric Environment
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    • v.33 no.2
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    • pp.97-107
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    • 2017
  • Columnar aerosol properties retrieved from solar radiation were investigated at the Yongin (YGN) SKYNET site over seven years from October 2008 to October 2015. Hourly averages were calculated when the data were available, and back trajectories were calculated to examine the effects of regional transport. Data recovery rate was low at 6.6%, primarily because solar radiation was measured only under daytime clear-sky conditions. Mean values of the fine-mode volume fraction (FMVF) as well as its seasonal variation were similar to those of $PM_{2.5}/PM_{10}$ although the coarse-mode fraction of column aerosols tended to be slightly larger. The values of single scattering albedo (SSA) and FMVF were lower in spring due to the effects of mineral dust, and higher in summer due to secondarily-formed inorganic ions. Back trajectories were grouped into five clusters according to the directions of transport paths. Aerosol loading was highest for Cluster 2 from the northwest, but SSA and FMVF were not particularly high or low because aerosols were composed of various materials with different properties. Aerosol loading was lowest for Cluster 5 from the Pacific Ocean passing through the south end of Japan, whose SSA and FMVF were highest as secondarily-formed inorganic ions were mixed.

A Study on the PM2.5 Source Characteristics Affecting the Seoul Area Using a Chemical Mass Balance Receptor Model (수용모델을 이용한 서울지역 미세입자 (PM2.5)에 영향을 미치는 배출원 특성에 관한 연구)

  • Lee Hak Sung;Kang Choong-Min;Kang Byung-Wook;Lee Sang-Kwun
    • Journal of Korean Society for Atmospheric Environment
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    • v.21 no.3
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    • pp.329-341
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    • 2005
  • The purpose of this study is to study the $PM_{2.5}$ source characteristics affecting the Seoul area using a chemical mass balance (CMB) receptor model. This study was also to evaluate the $PM_{2.5}$ source profiles, which were directly measured and developed. Asian Dust Storm usually occurred in the spring, and very high $PM_{2.5}$ concentrations were observed in the fall among the sampling periods. So the ambient data collected in the spring and fall were evaluated. The CMB model results as well as the $PM_{2.5}$ source profiles were validated using the diagnostic categories, such as: source contribution estimate, t-statistic, R-square, Chi-square, and percent of total mass explained. In the spring months, the magnitude of $PM_{2.5}$ mass contributors was in the following order: Chinese aerosol $(31.7\%)>$ secondary aerosols ($22.3\%$: ammonium sulfate $13.4\%$ and ammonium nitrate $8.9\%)>$ vehicles ($16.1\%$: gasoline vehicle $1.4\%$ and diesel vehicles $14.7\%)>$biomass burning $(15.5\%)>$ geological material $(10.5\%)$. In the fall months, the general trend of the $PM_{2.5}$ mass contributors was the following: biomass burning $(31.1\%)>$ vehicles ($26.9\%$: gasoline vehicle $5.1\%$ and diesel vehicles $21.8\%)>$ secondary aerosols ($23.0\%$: ammonium sulfate $9.1\%$ and ammonium nitrate $13.9\%)>$ Chinese aerosol $(10.7\%)$. The results show that the $PM_{2.5}$ mass in the Seoul area was mainly affected by the Chinese area.

Composition and pollution characteristics of TSP, PM2.5 atmospheric aerosols at Gosan site, Jeju Island (제주도 고산지역 TSP, PM2.5 대기에어로졸의 조성 및 오염 특성)

  • Lee, Soon-Bong;Kang, Chang-Hee;Jung, Duk-Sang;Ko, Hee-Jung;Kim, Haeng-Bum;Oh, Yong-Soo;Kang, Hae-Lim
    • Analytical Science and Technology
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    • v.23 no.4
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    • pp.371-382
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    • 2010
  • TSP and PM2.5 atmospheric aerosols have been collected at Gosan site of Jeju Island, and their compositions were analyzed to understand the pollution characteristics. The composition ratios of nss (non-sea salt)-$SO_4^{2-}$ and $NH_4^+$ were higher in Gosan site than those in other Korean background and urban sites. However the composition ratio of $NO_3^-$ was conversely lower in Gosan site. From the study of aerosol components according to particle sizes, the anthropogenic nss-$SO_4^{2-}$, $NO_3^-$ and $NH_4^+$ components were mostly existed in the fine particles. But the nss-$Ca^{2+}$, $Na^+$, $Cl^-$ and $Mg^{2+}$ originated from soil and marine sources were distributed relatively in the coarse particles. In the seasonal comparison, the concentrations of nss-$Ca^{2+}$, Al, Fe, Ca and $NO_3^-$ increased in spring season, and nss-$SO_4^{2-}$ showed higher concentration in summer and spring seasons. Based on the factor analysis, the atmospheric aerosols in Gosan site have been found to be influenced largely by anthropogenic sources, and next by marine and soil sources. The backward trajectory analyses showed that the concentrations of nss-$SO_4^{2-}$, $NO_3^-$, Pb and nss-$Ca^{2+}$ increased when the air mass moved from Chinese continent to Jeju area. On the other hand, their concentrations decreased when the air mass moved in from the North Pacific Ocean.

Measurement and Control of Hazardous PAHs Reaction Products (위해성 이차 PAHs 성분 측정 및 관리 방안)

  • Lee, Ji Yi;Hong, Ji Hyung;Jung, Chang Hoon;Kim, Yong Pyo
    • Particle and aerosol research
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    • v.9 no.2
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    • pp.111-125
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    • 2013
  • Among the hazardous air pollutions(HAPs), characteristics of secondary organic aerosols are not well understood. In this study, the current state for the measurement and analysis of representative secondary PAHs such as oxy-PAHs and nitro-PAHs are presented with the discussion of their toxicity. Also, further research directions for the secondary PAHs are suggested. It was found that the chemical reaction mechanisms and products of PAHs in the air are poorly identified and their toxicities are not well studied. Moreover ambient concentrations of those secondary PAHs are not well documented. Sampling methodologies of those secondary PAHs are similar with PAHs but the analytical protocols for those secondary PAHs are more complicated than PAHs. Future management directions are suggested along with future research directions.

Carbonaceous Aerosols Generated from Wood Charcoal Production Plants in the South Korea Context

  • Magnone, Edoardo;Park, Seong-Kyu;Park, Jung Hoon
    • Journal of the Korean Wood Science and Technology
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    • v.47 no.3
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    • pp.277-289
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    • 2019
  • Herein, a case study discussing the effect of carbonaceous aerosol pollution, which is emitted during the charcoal kiln manufacturing processes or carbonization processes, on the atmospheric environment is presented . In South Korea, in situ analysis of different charcoal production plants specialized in the production of charcoal sauna indicate that the emitted organic carbon (OC) and elemental carbon (EC) aerosols are significantly influenced by the nature of the biomass and technological processes, i.e., treatment or emissions abatement systems for the exhaust effluent gases. In detail, total carbon (TC), which is calculated as the sum of OC and EC emission factors, varied widely from a charcoal production site to another ranging from 21.8 to 35.8 gTC/kg-oak, where the mean value for the considered production sites was approximately 28 gTC/kg-oak (N = 7 and sum = 196.4). Results indicate that the emission factors from a modern charcoal production process in South Korea are quantitatively lower in comparison with the traditional kiln. This study aims to propose advanced wood processes for the production of charcoal from the viewpoint of environmental protection policy and green engineering.

Source-Receptor Relationships of Transboundary Air Pollutants in East Asia Region Simulated by On-Line Transport Model

  • Jang, Eun-Suk;Itsushi Uno
    • Environmental Sciences Bulletin of The Korean Environmental Sciences Society
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    • v.4 no.2
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    • pp.111-116
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    • 2000
  • Transboundary air pollution has recently become an area of increasing scientific interest and political concern as countries are receiving air pollutants from their neighbors. In order to gain a better understanding of the long-range transport processes of air pollutants and the source-receptor relationships among neighboring countries, an atmospheric transport model coupled with a RAMS(Regional Atmospheric Modeling System) model was applied to the East Asia region during the entire month of January 1993. The scalar transport option of the RAMS model was used to calculate special atmospheric constituents such as trace gases or aerosols. The sulfate production in clouds and rainwater and its removal processes by dry and wet deposition were considered. The sulfate budget from source regions to receptor regions was estimated by analysing the source-receptor relationships. When a specific receptor site revealed a sulfate value higher than the sulfate concentration based on its own source origin, this was taken to indicate long-range transport from another source region. The contribution ratio from various source region was calculated. The contribution ratio of dry and wet deposition was higher on the main continent of the East region. Furthermore, the high deposition amounts were identified on the west coast of Korea and the East China Sea.

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The Detection of Yellow Sand Dust Using the Infrared Hybrid Algorithm

  • Kim, Jae-Hwan;Ha, Jong-Sung;Lee, Hyun-Jin
    • Proceedings of the KSRS Conference
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    • 2005.10a
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    • pp.370-373
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    • 2005
  • We have developed Hybrid algorithm for yellow sand detection. Hybrid algorithm is composed of three methods using infrared bands. The first method used the differential absorption in brightness temperature difference between $11\mu m\;and\;12\mu m$ (BID _1), through which help distinguish the yellow sand from various meteorological clouds. The second method uses the brightness temperature difference between $3.7\mu m\;and\;11\mu m$ (BID_2). The technique would be most sensitive to dust loading during the day when the BID _2 is enhanced by reflection of $3.7\mu m$ solar radiation. The third one is a newly developed algorithm from our research, the so-called surface temperature variation method (STY). We have applied the three methods to MODIS for derivation of the yellow sand dust and in conjunction with the Principle Component Analysis (PCA), a form of eigenvector statistical analysis. PCI shows better results for yellow sand detection in comparison with the results from individual method. The comparison between PCI and MODIS aerosols optical depth (AOD) shows remarkable good correlations during daytime and relatively good correlations over the land.

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On the Contrast of Aerosol Size Distribution and Cloud Condensation Nuclei Concentrations between the East and the West of the Korean Peninsula (대관령과 영종도에서 측정한 에어러솔 크기분포 및 CCN 수농도에 관한 연구)

  • Kim, Jong Hwan;Park, Min-Su;Shim, Sungbo;Yum, Seong Soo
    • Atmosphere
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    • v.22 no.1
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    • pp.87-96
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    • 2012
  • Aerosol number concentration ($N_{CN}$), size distribution and cloud condensation nuclei (CCN) concentration ($N_{CCN}$) were measured during 16-21 August 2008 at Daegwallyeong (DG) located in the eastern rural region of the Korean Peninsula. In the very next week (22-29 August 2008) the same aerosol properties were measured at Yeongjong Island (YJ) in the Yellow Sea. $N_{CN}$ for all 3 size cuts (above 3, 6 and 10 nm) was significantly higher at DG than YJ, but $N_{CCN}$ was significantly lower at the former and resulted in the $N_{CCN}/N_{CN}$ ratio more than twice higher at YJ ($0.94{\pm}0.09$ vs. $0.35{\pm}0.15$ at 0.53% supersaturation). The geometric mean diameter at DG, $53{\pm}15nm$, was much smaller than that at YJ, $91{\pm}6nm$, due to the particle formation events that were likely to have occurred continuously at DG. For given mean diameter, aerosols were more likely to act as CCN at YG compared to those at DG.

Development of Ozone Generator with using DC Voltage for Swinery (돈사 적용용 DC전압을 이용한 오존발생장치 개발에 관한 연구)

  • 문승일;채재우;이대엽;장기현;정태균
    • Journal of Korean Society for Atmospheric Environment
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    • v.19 no.1
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    • pp.77-84
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    • 2003
  • HS, Ammonia, CH$_4$, VOCs, Microorganism, Bacteria etc produced from swineries or henhouses are known to prevent the growth of livestock. Moreover, they give an unpleasant feeling to the workers. In this study, a methodology to remove odors and toxic gases by oxidation of ozone was thus accomplished. However, most ozone generators which use the atmospheric surrounding air have problems of contamination of electrode for discharge. Therefore in this work, a wire-cylinder type plasma reactor with DC voltage has been used both in a laboratory scale test and in the real swinery to solve the existing problems. About 6 cm of electrode gap could decrease the attachment of dusts, humid aerosols and other polymers, which are contained in the air. This compact designed device could produce ozone to oxidize and remove the air pollutants. But the amount of ozone was not large enough to be harmful to human Health. Also, the concentration of ozone was able to be varied by the input voltage. which makes it available for the proposed system to be installed in various kinds of pig houses. With this device, at maximum 43 mg/㎥ (20 ppm) of ozone could be produced at 40 ㎸ input voltage (consumed energy was 0.1 Wh/㎥). A program was also made in this work to calculate the optimum parameters for design of a plasma reactor in wide range of conditions.

Trace Elements Characterization of PM10 in Seoul Area (서울지역의 PM10 중 미량원소의 특성 평가)

  • 신은상;최민규;영선우;정용삼
    • Journal of Korean Society for Atmospheric Environment
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    • v.18 no.5
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    • pp.363-372
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    • 2002
  • PM$_{10}$ aerosols were collected using low volume air sampler every month intervals from September 1992 to August 1991 in Seoul. These samples were analyzed for 20 trace elements (Al, As, Ba, Br, Ca, Cl, Co, Cr, Fe, K, Mn, Na, Ni, Pb, Sc, Se, Si, Ti, V and Zn) by INAA (instrumental neutron activation analysis), XRF (x-ray fuorescence spectrometer), and ICP (inductively coupled plasma). PM$_{10}$ mass concentrations higher than 70 $\mu$g/m$^3$ were 32% of 60 samples and had significantly higher concentrations in spring and winter than in summer and fall (p-value<0.001). The elements of As, Br, Cl, Ni, Pb, Se, V, and Zn are enriched by factors of 20 to 2,000 relative to their natural abundance in crustal soil. To further identify common sources of pollution-related trace elements, factor analysis was applied to the trace elements concentration data. Major sources that contribute to the atmospheric loading of these elements were found to include fossil fuel combustion, automobile and waste incineration (33.2%), metal processing industry (18.2%), and soil(29.8%).8%).