• 한국입자에어로졸학회지
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• 제6권4호
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• pp.151-164
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• 2010

Inorganic ions and water are major components of ambient fine particles. Water content in fine particles is mainly determined by ambient meteorological conditions and the concentrations of hygroscopic species such as inorganic ions. Thus, to reduce fine particle mass concentration, it is important to accurately estimate the relationship between water content and the concentration of ions in fine particles. Water content in fine particles in Seoul are estimated by using a gas/particle equilibrium model to understand the characteristics of fine particle mass concentration. In addition, sensitivity of fine particle mass concentration to the changes of particulate ionic species (sulfate, nitrate, and ammonium) is estimated. It was found that water content in Seoul is mostly determined by the concentrations of the hygroscopic ionic species, especially, sulfate and ammonium, and ambient relative humidity.

• 대기
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• 제22권3호
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• pp.367-379
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• 2012

Measurements of $PM_{10}$ mass concentration, aerosol light scattering and absorption coefficients as well as aerosol size distribution were made to characterize the aerosol physical and optical properties at the two Korean WMO/GAW regional stations, Anmyeondo and Gosan. Episodic cases of the severe Asian dust events occurred in spring of 2009-2010 were studied. Results in this study show that the aerosol size distributions and optical properties at both stations are closely associated with the dust source regions and the transport routes. According to the comparison of the $PM_{10}$ mass concentration at both stations, the aerosol concentrations at Anmyeondo are not always higher than those at Gosan although the distance from the dust source region to Anmyeondo is closer than that of Gosan. The result shows that the aerosol concentrations depend on the transport routes of the dust-containing airmass. The range of mass scattering efficiencies at Anmyeon and Gosan was 0.50~1.45 and $0.62{\sim}1.51m^2g^{-1}$, respectively. The mass scattering efficiencies are comparable to those of the previous studies by Clarke et al. (2004) and Lee (2009). It is noted that anthropogenic fine particles scatter more effectively the sunlight than coarse dust particles. Finally, we found that the aerosol size distribution and optical properties at Anmyeondo and Gosan show somewhat different properties although the samples for the same dust_episodic events are compared.

• 한국환경과학회지
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• 제22권3호
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• pp.347-358
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• 2013

The aerosol number concentration have measured with an aerodynamic particle sizer spectrometer(APS) at Gosan in Jeju Island, which is known as background area in Korea, from March 2010 to February 2011. The obtained results of asian dust events and non-asian dust period have been compared. The results show that the entire averaged aerosol number concentration from APS measurement during asian dust events and non-asian dust period are about 341 particles/$cm^3$ and 240 particles/$cm^3$, respectively. During asian dust events, the number concentration in small size ranges(${\leq}0.4{\mu}m$) are similar to non-asian dust period, however, those in large size ranges(${\geq}0.7{\mu}m$) are very higher than non-asian dust period. The contributions of the size resolved number concentration(23 channel in $0.25{\sim}10.0{\mu}m$) to total number concentration in that range are dramatically decreased with increased particle size. The contributions of smaller size ranges(${\leq}0.4{\mu}m$) during asian dust events are very low compared with non-asian dust period, on the other hand, those of larger size ranges(${\geq}0.4{\mu}m$) are higher than non-asian dust period. The number concentration in each size range are strongly correlated with the concentration in adjacent size range. And the total aerosol number concentration are depended on the number concentration in range of smaller than $0.58{\mu}m$ during non-asian dust period and asian dust events. On the other hand, $PM_{10}$ mass concentration has mainly affected with the number concentration in range of smaller than $1.0{\mu}m$ during non-asian dust period, however, during asian dust events, the mass concentration has mainly affected with the number concentration in range of $0.65{\sim}3.0{\mu}m$.

• 대기
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• 제25권1호
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• pp.169-177
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• 2015

Vertical distribution of particle mass concentrations was estimated from 8-year elastic-backscatter lidar and sky radiometer data, and from ground-level PM10 concentrations measured in Seoul. Lidar ratio and mass extinction efficiency were determined from aerosol optical depth (AOD) and ground-level PM10 concentrations, which were used as constraints to estimate particle mass concentration. The mean lidar ratio (with standard deviation) and mass extinction efficiency for the entire 8-year study period were $60.44{\pm}23.17$ sr and $3.69{\pm}3.00m^2g^{-1}$, respectively. The lidar ratio did not vary significantly with the ${\AA}ngstr{\ddot{o}}m$ exponent (less than ${\pm}10%$); however, the mass extinction efficiency decreases to $1.82{\pm}1.67m^2g^{-1}$ (51% less than the mean value) when the ${\AA}ngstr{\ddot{o}}m$ exponent is less than 0.5. This result implies that the particle mass concentration from lidar measurements can be underestimated for dust events. Seasonal variation of the particle mass concentration estimated from lidar measurements for the boundary layer, was quite different from ground-level PM10 measurements. This can be attributable to an inhomogeneous vertical distribution of aerosol in the boundary layer.

• 대기
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• 제26권3호
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• pp.357-372
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• 2016

Northeast Asian regions have recently become the main source of anthropogenic and natural aerosols. Measurement of aerosols on the sea in these regions have been rarely conducted since the experimental campaigns such as ACE-ASIA (Asian Pacific Regional Aerosol Characterization Experiment) in 2001. Research vessel observations of aerosol mass and chemical composition were performed on the Yellow and south sea around the Korean peninsula. The ship measurements showed six representative cases such as aerosol event and non-event cases during the study periods. On non-event cases, the anthropogenic chemical and natural soil composition on the Yellow sea were greater than those on the south sea. On aerosol event cases such as haze, haze with dust, and dust, the measured mass concentrations of anthropogenic chemical and element compositions were clearly changed by the events. In particular, methanesulfonate ($MSA^-$, $CH_3SO_3^-$), a main component of natural oceanic aerosol important for sulfur circulation on Earth, was first observed by the vessel in Korea, and its concentration on the Yellow sea was three times that on the south sea during the study period. Sea salt concentration important to chemical composition on the sea is related to wind speed. Coefficients of determination ($R^2$) between wind speed and sea salt concentration were 0.68 in $PM_{10}$ and 0.82 in $PM_{2.5}$. Maximum wave height was not found to be correlated to the sea salt concentration. When sea-salt comes into contact with pollutants, the total sea-salt mass is reduced, i.e., a loss of $Cl^-$ concentration from NaCl, the main chemical composing sea salt, is estimated by reaction with $HNO_3$(gas) and $H_2SO_4$(gas). The $Cl^-$ concentration loss by $SO_4^{2-}$ and $NO_3^-$ more easily increased for $PM_{10}$ compared to $PM_{2.5}$. The results of this study will be applied to verifying a dust-haze forecasting model. In addition, continued vessel measurements of aerosol data will become important to research for climate change studies in the future.

• 대기
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• 제18권2호
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• pp.97-109
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• 2008

The aerosol characteristics in terms of 4 different cases (Asian dust, fog, clear sky and cloud) which had happened at Anmyeon Island in April 2006 were studied using various measurements such as the Micro Pulse Lidar (MPL), sunphotometer, $\beta$-ray $PM_{10}$ Analyzer, anemoscope and anemometer. In addition, synoptic charts, back trajectory analyses and satellite images were also used to help characterize the aerosol events. The aerosol optical properties were featured by the Aerosol Optical Depth (AOD) and ${\AA}ngstr\ddot{o}m$ exponent which were estimated by the sunphotometer. When Anmyeon Island was dominated by the Asian dust, the AOD was sharply increased as seven times as a yearly average of it (0.35). As compared with a yearly average of the ${\AA}ngstr\ddot{o}m$ exponent of 0.97, the ${\AA}ngstr\ddot{o}m$ exponent of a dust day was significantly low (0.099). In addition, $PM_{10}$ mass concentration showed an extremely high record. The maximum concentration reached $1790.5{\mu}gm^{-3}$ on 8 April 2006. The maximum mass concentration was shown with delay when the wind speed of $0ms^{-1}$ was observed. It was also found that a satellite image of the MODIS-RGB had a good agreement with the results of those measurements. It was shown that the MPL was able to describe effectively the vertical distribution of aerosol for all the cases. In particular, the MPL evidently captured the aerosol layer before the cloud observation. The aerosol layer was similarly described by the AOD. On a clear sky day, the AOD had not only a very low value (0.054) but also a feature of homogeneity.

• Asian Journal of Atmospheric Environment
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• 제3권1호
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• pp.1-8
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• 2009

Enhancement of aerosol optical thickness (AOT) and surface aerosol mass concentration in Korea for an active forest fire episode in Northeast Asia were estimated by Community Multi-scale Air Quality (CMAQ) model. MODIS/TERRA remote detects of fires in Northeast Asia for May 2003 gave a constraint for estimation of wildfire emissions with an NDVI distribution for recent five years. The simulated wildfire plumes and enhancement of AOT were evaluated and well resolved by comparing multiple satellite observations such as MODIS, TOMS, and others. Scatter plots of observed daily mean aerosol extinction coefficient versus $PM_{10}$ concentration in ground level in Korea showed distinctively different trends based on the ambient relative humidity.

• 대기
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• 제21권3호
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• pp.301-309
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• 2011

In this study, we compared light-absorption properties of aerosols observed in East and South Asia from black carbon (BC) mass concentration, aerosol scattering (${\sigma}_s$) and absorption (${\sigma}_a$) coefficients measurements at four sites: Korea Climate Observatory-Gosan (KCO-G), Korea Climate Observatory-Anmyeon (KCO-A), Maldives Climate Observatory-Hanimaadhoo (MCO-H) and Nepal Climate Observatory-Pyramid (NCO-P). No significant seasonal variations of BC mass concentration, ${\sigma}_s$ and ${\sigma}_a$, despite of wet removal of aerosols by precipitation in summer, were observed in East Asia, whereas dramatic changes of light-absorbing aerosol properties were observed in South Asia between dry and wet monsoon periods. Although BC mass concentration in East Asia is generally higher than that observed in South Asia, BC mass concentration at MCO-H during winter dry monsoon is similar to that of East Asia. The observed solar absorption efficiency (${\alpha}$) at 550 nm, where ${\alpha}={\sigma}_a/({\sigma}_s+{\sigma}_a)$, at KCO-G and KCO-A is higher than that in MCO-H due to large portions of BC emission from fossil fuel combustion. Interestingly, ${\alpha}$ at NCO-P is 0.14, which is two times great than that in MCO-H and is about 40% higher than that in East Asia, though BC mass concentration at NCO-P is the lowest among four sites. Consistently, the highest elemental carbon to sulphate ratio is found at NCO-P.

• 한국입자에어로졸학회지
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• 제14권2호
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• pp.35-40
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• 2018

Vertical particle size distribution, total particle concentration, wind velocity, temperature and humidity measurement was performed with a drone. The drone was equipped with a wind sensor, house-made optical particle count(Hy-OPC), condensation particle counter(Hy-CPC), GPS, Temperature, Relative Humidity, Pressure and communication system. Base on the wind velocity and the particle size vertical distribution measurement with drone, the particle mass flux was calculated. The vertical particle distribution showed that the particle number concentration was very strongly correlated with the relative humidity.

• 한국분무공학회지
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• 제3권3호
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• pp.14-22
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• 1998

The growth by steam condensation of an hygroscopic aerosol is investigated using the condensation rate model which has been derived from the mass and heat transfer equations. The present model accounts for both the solute and Kelvin effects. When the hygroscopicity is considered, condensation can occur on hygroscopic seed particles even under subsaturated steam conditions. This study focuses on the effect of hygroscopicity on the evolution of the particle size distribution and decay of the total aerosol concentration. It is found that hygroscopicity causes the particle size distribution to rapidly move upward even in a very short time, resulting in substantially higher decay of the total aerosol concentration than the case without considering hygroscopicity.