• 제목/요약/키워드: Actinides

검색결과 76건 처리시간 0.029초

Conceptual Study of Fusion-Fission Hybrid Reactor for Transmutation of a Nuclear Waste

  • Hong, B.G.
    • 한국진공학회:학술대회논문집
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    • 한국진공학회 2013년도 제44회 동계 정기학술대회 초록집
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    • pp.670-670
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    • 2013
  • The concept of a fusion-driven transmutation reactor based on LAR (Low Aspect Ratio) tokamak as a neutron source is studied based on ITER physics and technology. The radial build of transmutation reactor components are self-consistently determined by coupling the systems analysis with radiation transport analysis and an optimal configuration of a transmutation reactor for aspect ratio, A in the range of 1.5 to 2.0 is found. The performance of a transmutation reactor is investigated and shows that a transmutation reactor with a neutron source producing fusion power less than 150 MW can destroy the transuranic actinides contained in the spent fuels produced from more than two 1 GWe PWRs with production of the fission power being greater than 2 GW.

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Preliminary Corrosion Model in Isothermal Pb and LBE Flow Loops

  • Lee, Sung Ho;Cho, Choon Ho;Song, Tae Yung
    • Corrosion Science and Technology
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    • 제5권6호
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    • pp.201-205
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    • 2006
  • HYPER(Hybrid Power Extraction Reactor) is the accelerator driven subcritical transmutation system developed by KAERI(Korea Atomic Research Institute). HYPER is designed to transmute long-lived transuranic actinides and fission products such as Tc-99 and I-129. Liquid lead-bismuth eutectic (LBE). Has been a primary candidate for coolant and spallation neutron target due to its appropriate thermal-physical and chemical properties, However, it is very corrosive to the common steels used in nuclear installations at high temperature. This corrosion problem is one of the main factors considered to set the upper limits of temperature and velocity of HYPER system. In this study, a parametric study for a corrosion model was performed. And a preliminary corrosion model was also developed to predict the corrosion rate in isothermal Pb and LBE flow loops.

A negative reactivity feedback driven by induced buoyancy after a temperature transient in lead-cooled fast reactors

  • Arias, Francisco J.
    • Nuclear Engineering and Technology
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    • 제50권1호
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    • pp.80-87
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    • 2018
  • Consideration is given to the possibility to use changes in buoyancy as a negative reactivity feedback mechanism during temperature transients in heavy liquid metal fast reactors. It is shown that by the proper use of heavy pellets in the fuel elements, fuel rods could be endowed with a passive self-ejection mechanism and then with a negative feedback. A first estimate of the feasibility of the mechanism is calculated by using a simplified geometry and model. If in addition, a neutron poison pellet is introduced at the bottom of the fuel, then when the fuel element is displaced upward by buoyancy force, the reactivity will be reduced not only by disassembly of the core but also by introducing the neutron poison from the bottom. The use of induced buoyancy opens up the possibility of introducing greater amounts of actinides into the core, as well as providing a palliative solution to the problem of positive coolant temperature reactivity coefficients that could be featured by the heavy liquid metal fast reactors.

Fission Product Inventory Calculation by a CASMO/ORIGEN Coupling Program

  • Kim, Do-Heon;Kim, Jong-Kyung;Park, Hangbok;Roh, Gyu-hong;Inha Jung
    • 한국원자력학회:학술대회논문집
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    • 한국원자력학회 1997년도 추계학술발표회논문집(1)
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    • pp.70-75
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    • 1997
  • A CASMO/ORIGEN coupling utility program was developed to predict the composition of all the fission products in spent PWR fuels. The coupling program reads the CASMO output file, modifies the ORIGEN cross section library and reconstructs the ORIGEN input file at each depletion step. In ORIGEN, the burnup equation is solved for actinides and fission products based on the fission reaction rates and depletion flux of CASMO. A sample calculation has been performed using a 14$\times$14 PWR fuel assembly and the results are given in this paper.

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Reprocessing of spent nuclear fuel in carbonate media: Problems, achievements, and prospects

  • Stepanov, Sergei I.;Boyarintsev, Alexander V.
    • Nuclear Engineering and Technology
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    • 제54권7호
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    • pp.2339-2358
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    • 2022
  • The review discusses various alternative approaches for spent nuclear fuel (SNF) reprocessing in aqueous carbonate media. The main stages, schemes, and methods of the most well-known and well-described processes for reprocessing SNF and some high-level radioactive waste using carbonate systems developed by research groups in Japan, the United States of America, the Republic of Korea, and the Russian Federation described and compared. The main advantages of such methods are outlined compared to the SNF reprocessing in nitric acid media. The levels of development and proximity of the designed processes to the industrial implementation are shown. The main principle achievements, prospects, and routes for the refinement of such methods for the technology of SNF reprocessing and handling of high-level radioactive waste formulated.

A surrogate model for the helium production rate in fast reactor MOX fuels

  • D. Pizzocri;M.G. Katsampiris;L. Luzzi;A. Magni;G. Zullo
    • Nuclear Engineering and Technology
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    • 제55권8호
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    • pp.3071-3079
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    • 2023
  • Helium production in the nuclear fuel matrix during irradiation plays a critical role in the design and performance of Gen-IV reactor fuel, as it represents a life-limiting factor for the operation of fuel pins. In this work, a surrogate model for the helium production rate in fast reactor MOX fuels is developed, targeting its inclusion in engineering tools such as fuel performance codes. This surrogate model is based on synthetic datasets obtained via the SCIANTIX burnup module. Such datasets are generated using Latin hypercube sampling to cover the range of input parameters (e.g., fuel initial composition, fission rate density, and irradiation time) and exploiting the low computation requirement of the burnup module itself. The surrogate model is verified against the SCIANTIX burnup module results for helium production with satisfactory performance.

Separation and purification of elements from alkaline and carbonate nuclear waste solutions

  • Alexander V. Boyarintsev ;Sergei I. Stepanov ;Galina V. Kostikova ;Valeriy I. Zhilov;Alfiya M. Safiulina ;Aslan Yu Tsivadze
    • Nuclear Engineering and Technology
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    • 제55권2호
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    • pp.391-407
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    • 2023
  • This article provides a survey of wet (aqueous) methods for recovery, separation, and purification of uranium from fission products in carbonate solutions during the reprocessing of spent nuclear fuel and methods for removal of radionuclides from alkaline radioactive waste. The main methods such as selective direct precipitation, ion exchange, and solvent extraction are considered. These methods were compared and evaluated for reprocessing of spent nuclear fuel in carbonate media according to novel alternative non-acidic methods and for treatment processes of alkaline radioactive waste.

DUPIC핵연료주기에 의한 사용 후 경수로핵연료의 방사선적 특성변화 분석 (Study on Decay Characteristics Change of Spent Fuel Materials by DUPIC Fuel Cycle)

  • 최종원;고원일;이재설;박현수
    • Journal of Radiation Protection and Research
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    • 제21권1호
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    • pp.27-39
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    • 1996
  • DUPIC핵연료주기로 인해 변화되는 경수로 사용 후 핵연료 물질의 핵종별 농도, 방사능, 붕괴열, 위해지수 및 방사선원항등을 시간의 함수로 그 변화특성을 분석하고, 각 인자별로 크게 영향을 미치는 주요핵종의 거동을 물질농도 측면에서 추적 분석평가하였다. 방사성물질 농도에 있어서 연소도 19,000 MWD/MTU의 사용 후 DUPIC핵연료에 존재하는 악티나이드 양은 연소도 35,000 MWD/MTU의 경수로 사용후 핵연료에 비해 약 2% 감소한 반면 핵분열생성물의 양은 약 20% 증가된 것으로 나타났다. 그리고 사용 후 DUPIC핵연료의 방사능 및 붕괴열은 일반적인 사용후핵연료 특성과는 달리, 방사성물질 농도 변화와 비례하지 않는 것으로 나타났다. 사용후 DUPIC핵연료가 갖는 감마 스펙트럼을 경수로핵연료의 경우와 비교해 볼 때, 전체적인 특징은 사용후 DUPIC핵연료의 경우가 $0.01{\sim}0.575MeV$의 낮은 에너지 범위에서는 경수로핵연료 보다 약 $40{\sim}50%$ 낮은 감마선 세기를 보여주고 있으나, 3.5 MeV이상의 높은 에너지 범위에서는 사용후 DUPIC핵연료의 감마선 세기가 휭씬 크게 나타났다. 중성자 선원항은 모두 악티나이드 물질의$({\alpha},\;n)$ 반응 및 자발핵분열에 의해 결정되고 있고, 특히 Cm-244의 자발 핵분열에 의한 중성자선원이 지배적인 것으로 나타났다. 이런 이유 때문에 Cm-244의 농도가 약 3.3배 큰 사용후 DUPIC핵연료의 중성자 선원이 경수로핵연료보다 4배 이상 크게 나타났다.

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Assessment of three European fuel performance codes against the SUPERFACT-1 fast reactor irradiation experiment

  • Luzzi, L.;Barani, T.;Boer, B.;Cognini, L.;Nevo, A. Del;Lainet, M.;Lemehov, S.;Magni, A.;Marelle, V.;Michel, B.;Pizzocri, D.;Schubert, A.;Uffelen, P. Van;Bertolus, M.
    • Nuclear Engineering and Technology
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    • 제53권10호
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    • pp.3367-3378
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    • 2021
  • The design phase and safety assessment of Generation IV liquid metal-cooled fast reactors calls for the improvement of fuel pin performance codes, in particular the enhancement of their predictive capabilities towards uranium-plutonium mixed oxide fuels and stainless-steel cladding under irradiation in fast reactor environments. To this end, the current capabilities of fuel performance codes must be critically assessed against experimental data from available irradiation experiments. This work is devoted to the assessment of three European fuel performance codes, namely GERMINAL, MACROS and TRANSURANUS, against the irradiation of two fuel pins selected from the SUPERFACT-1 experimental campaign. The pins are characterized by a low enrichment (~ 2 wt.%) of minor actinides (neptunium and americium) in the fuel, and by plutonium content and cladding material in line with design choices envisaged for liquid metal-cooled Generation IV reactor fuels. The predictions of the codes are compared to several experimental measurements, allowing the identification of the current code capabilities in predicting fuel restructuring, cladding deformation, redistribution of actinides and volatile fission products. The integral assessment against experimental data is complemented by a code-to-code benchmark focused on the evolution of quantities of engineering interest over time. The benchmark analysis points out the differences in the code predictions of fuel central temperature, fuel-cladding gap width, cladding outer radius, pin internal pressure and fission gas release and suggests potential modelling development paths towards an improved description of the fuel pin behaviour in fast reactor irradiation conditions.

Electrolytic Deposition of Metal Ions Using A Liquid Cadmium Cathode

  • Shim, Joon-Bo;Ahn, Byung-Gil;Kwon, Sang-Woon;Kim, Eung-Ho;Yoo, Jae-Hyung
    • 한국방사성폐기물학회:학술대회논문집
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    • 한국방사성폐기물학회 2004년도 학술논문집
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    • pp.337-337
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    • 2004
  • As one of researches for the P & T purposes, a basic experiment on the recovery of actinide elements from the mixture with rare earth elements by means of electrorefining using a liquid cadmium cathode in the LiCl-KC1 eutectic melt was carried out. In order to examine the behaviors of electrodeposition of metal ions on a liquid electrode, recovery experiments of rare earth metals resulting from forming electrodeposits were performed by a galvanostatic electrolysis method at various current densities. A cyclic voltammetric technique was applied to determine reduction-oxidation potential of each metal element in the melt and to detect the changes of the multi component melt composition for on-line monitoring. Also, a collaboration study with RIAR was completed to test the preliminary feasibility on a recovery of actinide elements from the mixture with rare earth elements using a liquid cadmium cathode and actinide metals. Experimental results showed that the ratio of actinides to rare earths, 9: 0.5∼1 led to the rare earth content of about 5∼10 wt% in the deposit.

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