• Title/Summary/Keyword: $UO_2$ fuel

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Measurement of Terminal Velocity for Scatter Prevention of Powder in the Voloxidizer for Oxidation of UO$_{2}$ Pellet (UO$_{2}$ 펠릿 산화로의 분말 비산 방지를 위한 최종속도 측정)

  • Kim Young-Hwan;Yoon Ji-Sup;Jung Jae-Hoo;Jin Jae-Hyun;Hong Dong-Hee
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.3 no.2
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    • pp.77-84
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    • 2005
  • A voloxidizer for a hot cell demonstration, that handles spent fuels of a high radiation level in a limited space should be small and spent fuel powders should not be dispersed out of the equipment involved. In this study a density rate equation as well as the Stokes'equation has been proposed in order to obtain the theoretical terminal velocity of powders. The terminal velocity of U$_{3}$O$_{8}$ has been predicted by using the terminal velocity of SiO$_{2}$, and then determination has been the optimum air flow rate which is able to prevent powders from scattering. An equation which has shown a relationship between theoretical terminal velocities of U$_{3}$O$_{8}$ and SiO$_{2}$ has been derived with the help of the Stokes'equation, and then an experimental verification made for the theoretical Stokes' equation of SiO$_{2}$ by means of an experimental device made of acryl. The theoretical terminal velocity based on the proposed density rate equation has been verified by detecting U$_{3}$O$_{8}$ powders in a filter installed in the mock-up voloxidizer. As the results, the optimum air flow rates seem to be 20 LPM by the Stokes'equation while they are 14.5 L/min by the density rate equation. At the experiments with the mock-up voloxidizer, a trace amount of U$_{3}$O$_{8}$ seems to be detectable at the air flow rate of 14.5 L/min by the density rate equation, but U$_{3}$O$_{8}$ powders of 7$\mu$m diameter seem detectable at the air flow rate of 20 L/min by the Stokes'equation. It is revealed that 14.5 L/min is the optimum air flowe rate which is capable of preventing U$_{3}$O$_{8}$ powders from scattering in the UO$_{2}$ voloxidizer and the proposed density rate equation is proper to calculate the terminal velocity of U$_{3}$O$_{8}$ powders.

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Analysis of the CREOLE experiment on the reactivity temperature coefficient of the UO2 light water moderated lattices using Monte Carlo transport calculations and ENDF/B-VII.1 nuclear data library

  • El Ouahdani, S.;Erradi, L.;Boukhal, H.;Chakir, E.;El Bardouni, T.;Boulaich, Y.;Ahmed, A.
    • Nuclear Engineering and Technology
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    • v.52 no.6
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    • pp.1120-1130
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    • 2020
  • The CREOLE experiment performed In the EOLE critical facility located In the Nuclear Center of CADARACHE - CEA have allowed us to get interesting and complete experimental information on the temperature effects in the light water reactor lattices. To analyze these experiments with accuracy an elaborate calculation scheme using the Monte Carlo method implemented in the MCNP6.1 code and the ENDF/B-VII.1 cross section library has been developed. We have used the ENDF/B-VII.1 data provided with the MCNP6.1.1 version in ACE format and the Makxsf utility to handle the data in the specific temperatures not available in the MCNP6.1.1 original library. The main purpose of this analysis is the qualification of the ENDF/B-VII.1 nuclear data for the prediction of the Reactivity Temperature Coefficient while ensuring the ability of the MCNP6.1 system to model such a complex experiment as CREOLE. We have analyzed the case of UO2 lattice with 1166 ppm of boron in ordinary water moderator in specified temperatures. A detailed comparison of the calculated effective multiplication factors with the reference ones [1] in room temperature presented in this work shows a good agreement demonstrating the validation of our 3D calculation model. The discrepancies between calculations and the differential measurements of the Reactivity Temperature Coefficient for the analyzed configuration are relatively small: the maximum discrepancy doesn't exceed 1,1 pcm/℃. In addition to the analysis of direct differential measurements of the reactivity temperature coefficient performed in the poisoned UO2 lattice configuration, we have also analyzed integral measurements in UO2 clean lattice configuration using equivalency of the integral temperature reactivity worth with the driver core fuel reactivity worth and soluble boron reactivity worth. In this case both of the ENDF/B-VII.1 and JENDL.4 libraries were used in our analysis and the obtained results are very similar.

A preliminary study of pilot-scale electrolytic reduction of UO2 using a graphite anode

  • Kim, Sung-Wook;Heo, Dong Hyun;Lee, Sang Kwon;Jeon, Min Ku;Park, Wooshin;Hur, Jin-Mok;Hong, Sun-Seok;Oh, Seung-Chul;Choi, Eun-Young
    • Nuclear Engineering and Technology
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    • v.49 no.7
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    • pp.1451-1456
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    • 2017
  • Finding technical issues associated with equipment scale-up is an important subject for the investigation of pyroprocessing. In this respect, electrolytic reduction of 1 kg $UO_2$, a unit process of pyroprocessing, was conducted using graphite as an anode material to figure out the scale-up issues of the C anode-based system at pilot scale. The graphite anode can transfer a current that is 6-7 times higher than that of a conventional Pt anode with the same reactor, showing the superiority of the graphite anode. $UO_2$ pellets were turned into metallic U during the reaction. However, several problems were discovered after the experiments, such as reaction instability by reduced effective anode area (induced by the existence of $Cl_2$ around anode and anode consumption), relatively low metal conversion rate, and corrosion of the reactor. These issues should be overcome for the scale-up of the electrolytic reducer using the C anode.

MULTI-SCALE MODELS AND SIMULATIONS OF NUCLEAR FUELS

  • Stan, Marius
    • Nuclear Engineering and Technology
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    • v.41 no.1
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    • pp.39-52
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    • 2009
  • Theory-based models and high performance simulations are briefly reviewed starting with atomistic methods, such as Electronic Structure calculations, Molecular Dynamics, and Monte Carlo, continuing with meso-scale methods, such as Dislocation Dynamics and Phase Field, and ending with continuum methods that include Finite Element and Finite Volume. Special attention is paid to relating thermo-mechanical and chemical properties of the fuel to reactor parameters. By inserting atomistic models of point defects into continuum thermo-chemical calculations, a model of oxygen diffusivity in $UO_{2+x}$ is developed and used to predict point defect concentrations, oxygen diffusivity, and fuel stoichiometry at various temperatures and oxygen pressures. The simulations of coupled heat transfer and species diffusion demonstrate that including the dependence of thermal conductivity and density on composition can lead to changes in the calculated centerline temperature and thermal expansion displacements that exceed 5%. A review of advanced nuclear fuel performance codes reveals that the many codes are too dedicated to specific fuel forms and make excessive use of empirical correlations in describing properties of materials. The paper ends with a review of international collaborations and a list of lessons learned that includes the importance of education in creating a large pool of experts to cover all necessary theoretical, experimental, and computational tasks.

Performance evaluation of Accident Tolerant Fuel under station blackout accident in PWR nuclear power plant by improved ISAA code

  • Zhang, Bin;Gao, Pengcheng;Xu, Tao;Gui, Miao;Shan, Jianqiang
    • Nuclear Engineering and Technology
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    • v.54 no.7
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    • pp.2475-2490
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    • 2022
  • The Accident Tolerant Fuel (ATF) is a new concept of fuel, which can not only withstand the consequences of the accident for a longer time, but also maintain or improve the performance under operating conditions. ISAA is a self-developed severe accident analysis code, which uses modular structures to simulate the development processes of severe accidents in nuclear plants. The basic version of ISAA is developed based on UO2-Zr fuel. To study the potential safety gain of ATF cladding, an improved version of ISAA, referred to as ISAA-ATF, is introduced to analyze the station blackout accident of PWR using ATF cladding. The results show that ATF cladding enable the core to maintain a longer time compared to zirconium alloy cladding, thereby enhancing the accident mitigation capability. Meanwhile, the generation of hydrogen is significantly reduced and delayed, which proves that ATF can improve the safety characteristics of the nuclear reactor.

Development and verification of PWR core transient coupling calculation software

  • Li, Zhigang;An, Ping;Zhao, Wenbo;Liu, Wei;He, Tao;Lu, Wei;Li, Qing
    • Nuclear Engineering and Technology
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    • v.53 no.11
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    • pp.3653-3664
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    • 2021
  • In PWR three-dimensional transient coupling calculation software CORCA-K, the nodal Green's function method and diagonal implicit Runge Kutta method are used to solve the spatiotemporal neutron dynamic diffusion equation, and the single-phase closed channel model and one-dimensional cylindrical heat conduction transient model are used to calculate the coolant temperature and fuel temperature. The LMW, NEACRP and PWR MOX/UO2 benchmarks and FangJiaShan (FJS) nuclear power plant (NPP) transient control rod move cases are used to verify the CORCA-K. The effects of burnup, fuel effective temperature and ejection rate on the control rod ejection process of PWR are analyzed. The conclusions are as follows: (1) core relative power and fuel Doppler temperature are in good agreement with the results of benchmark and ADPRES, and the deviation between with the reference results is within 3.0% in LMW and NEACRP benchmarks; 2) the variation trend of FJS NPP core transient parameters is consistent with the results of SMART and ADPRES. And the core relative power is in better agreement with the SMART when weighting coefficient is 0.7. Compared with SMART, the maximum deviation is -5.08% in the rod ejection condition and while -5.09% in the control rod complex movement condition.

Study on the effect of long-term high temperature irradiation on TRISO fuel

  • Shaimerdenov, Asset;Gizatulin, Shamil;Dyussambayev, Daulet;Askerbekov, Saulet;Ueta, Shohei;Aihara, Jun;Shibata, Taiju;Sakaba, Nariaki
    • Nuclear Engineering and Technology
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    • v.54 no.8
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    • pp.2792-2800
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    • 2022
  • In the core of the WWR-K reactor, a long-term irradiation of tristructural isotopic (TRISO)-coated fuel particles (CFPs) with a UO2 kernel was carried out under high-temperature gas-cooled reactor (HTGR)-like operating conditions. The temperature of this TRISO fuel during irradiation varied in the range of 950-1100 ℃. A fission per initial metal atom (FIMA) of uranium burnup of 9.9% was reached. The release of gaseous fission products was measured in-pile. The release-to-birth ratio (R/B) for the fission product isotopes was calculated. Aspects of fuel safety while achieving deep fuel burnup are important and relevant, including maintaining the integrity of the fuel coatings. The main mechanisms of fuel failure are kernel migration, silicon carbide corrosion by palladium, and gas pressure increase inside the CFP. The formation of gaseous fission products and carbon monoxide leads to an increase in the internal pressure in the CFP, which is a dominant failure mechanism of the coatings under this level of burnup. Irradiated fuel compacts were subjected to electric dissociation to isolate the CFPs from the fuel compacts. In addition, nondestructive methods, such as X-ray radiography and gamma spectrometry, were used. The predicted R/B ratio was evaluated using the fission gas release model developed in the high-temperature test reactor (HTTR) project. In the model, both the through-coatings of failed CFPs and as-fabricated uranium contamination were assumed to be sources of the fission gas. The obtained R/B ratio for gaseous fission products allows the finalization and validation of the model for the release of fission products from the CFPs and fuel compacts. The success of the integrity of TRISO fuel irradiated at approximately 9.9% FIMA was demonstrated. A low fuel failure fraction and R/B ratios indicated good performance and reliability of the studied TRISO fuel.

Sintering and Characterization of SiC-matrix Composite Including TRISO Particles (TRISO 입자를 포함하는 SiC 복합소결체의 소결 및 특성 평가)

  • Lee, Hyeon-Geun;Kim, Daejong;Park, Ji Yeon;Kim, Weon-Ju
    • Journal of the Korean Ceramic Society
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    • v.51 no.5
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    • pp.418-423
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    • 2014
  • Fully ceramic micro encapsulated (FCM) nuclear fuel is a concept recently proposed for enhancing the stability of nuclear fuel. FCM nuclear fuel consists of tristructural-isotropic (TRISO) fuel particles within a SiC matrix. Each TRISO fuel particle is composed of a $UO_2$ kernel and a PyC/SiC/PyC tri-layer which protects the kernel. The SiC ceramic matrix is created by sintering. In this FCM fuel concept, fission products are protected twice, by the TRISO coating layer and by the SiC ceramic. The SiC ceramic has proven attractive for fuel applications owing to its low neutron-absorption cross-section, excellent irradiation resistivity, and high thermal conductivity. In this study, a SiC-matrix composite containing TRISO particles was sintered by hot pressing with $Al_2O_3-Y_2O_3$ additive system. Various sintering conditions were investigated to obtain a relative density greater than 95%. The internal distribution of TRISO particles within the SiC-matrix composite was observed using an x-ray radiograph. The fracture of the TRISO particles was investigated by means of analysis of the cross-section of the SiC-matrix composite.

Analysis of Fission Products on Irradiated Fuels using EPMA (EPMA를 이용한 사용후핵연료의 연소도 측정에 관한 연구)

  • JUNG Yang-Hong;YOO Byung-Ok;OH Wan-Ho;LEE Hong-Gy;CHOO Yong-Sun;HONG Kwon-Pyo
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2005.06a
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    • pp.335-343
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    • 2005
  • The Methodology of burnup calculation with EPMA test set up in this study. The spent fuel from PWR nuclear power plant was used as specimen. This $UO_2$ fuel with $3.2\%$ of enrichment had been irradiated up to 35,000 MWd/MTU(reference data). The burnup is very important factor for nuclear fuel to estimate all fuel behaviors in reactor. To measure amounts of fission products and actinides for the burnup calcualation, chemical analysis (destructive method) has been used but it mattes long experimental time and second radio-wastes. In this study, EPMA test was available to measure amount of fission products. Neodymium is able to be detected and quantified. It can be compared with the results from chemical analysis and ORIGEN-2 code calculation. Concentration of Nd from EPMA test showed good agreement with result of ORIGEN-2 code in the same burnup.

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Design of Spent Fuel Rod Slitting Device of an Actual Proof (실증용 사용후핵연료봉 Slitting 장치 설계)

  • Jung J. H.;Yoon J. S.;Hong D. H.;Kim Y. H.;Jin J. H.
    • Proceedings of the Korean Society for Technology of Plasticity Conference
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    • 2004.05a
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    • pp.109-113
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    • 2004
  • Slitting device is equipment to separate spent fuel of 250 mm rod cut pellets and hull in order to supply required $UO_2$ pellets through the dry pulverizing/mixing device. For development of its device, We have analyzed slitting programs so that the existing device is modified an appropriate scale in the advanced spent fuel conditioning process. The results of the analysis, we added the automatic separation function of pellets and hull, After slitting. Also, we have concentrated on reducing the operation time so that the support and the body of a slitting blade could have been established in the single structure to be easily maintained. It is based on a design and manufacture of a testing device and we have performed an efficiency evaluation. We have analyzed the results of efficiency tests of the slitting device and get the specification of the slitting device. we complete the basic design of the slitting device by using of these data. Therefore, We apply to a basic data when manufacturing a slitting device.

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