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Electrical Conductivity of the Solid Solutions X $ZrO_2+ (1-X) Yb_2O_3; 0.01{\leq}X{\leq}0.09$

  • Published : 1992.06.20

Abstract

$ZrO_2-dopedYb_2O_3solid$ solutions containing 1, 3, 5, 7 and 9 mol% $ZrO_2were$ synthesized from spectroscopically pure $Yb_2O_3$ and $ZrO_2$ powders and found to be rare earth C-type structure by XRD technique. Electrical conductivities were measured as a function of temperatures from 700 to $1050^{\circ}C$ and oxygen partial pressures from 1${\times}$$10^-5$ to 2${\times}$ $10^-1$atm. The electrical conductivities depend simply on temperature and the activation energies are determined to be 1.56-1.68 $_eV$. The oxygen partial pressure dependence of the electrical conductivity shows that the conductivity increases with increasing oxygen partial pressure, indicating p-type semiconductor. The $PO_2$ dependence of the system is nearly power of 1/4. It is suggested from the linearity of the temperature dependence of electrical conductivity and only one value of 1/n that the solid solutions of the system have single conduction mechanism. From these results, it is concluded that the main defects of the system are negatively doubly charged oxygen interstitial in low. $ZrO_2doping$ level and negatively triply charged cation vacancy in high doping level and the electrical conduction is due to the electronic hole formed by the defect structure.

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References

  1. Rev. Int. Hautes Temper. Refract. v.3 M. Foex;J. P. Traverse
  2. Nonstoichiometric Oxides v.21 O. T. Sorensen
  3. J. Kor. Chem. Soc. v.29 no.6 J. H. Cho;K. H. Chang;K. H. Kim;Y. B. Kim;J. S. Choi
  4. Bull. Kor. Chem. Soc. v.11 no.4 S. H. Park;Y. Y. Kim;K. H. Kim
  5. J. Kor. Chem. Soc. v.18 no.1 Y. H. Kang;J. S. Choi;K. H. Yoon
  6. Physica Status Solid(a) v.71 C. R. Dutta;K. Barua
  7. Z. Phys chem. v.43 V. B. Tare;H. Schmalzried
  8. J. Solid St. Chem. v.2 G. V. Subba Rao;S. Ramdas;P. N. Mehrotra;C. N. Rao
  9. J. Phys. Chem. Solids v.43 no.10 J. L .Carpentier;A. Lebrun;F. Perdu;P. Tellier
  10. Proc. IRE. v.42 L. B. Valdes
  11. Proc. Phys. Soc. London v.57 J. B. Nelson;D. P. Riley
  12. Nonsoichiometry, Diffusion and Electrical Conductivity in Binary Metal Oxides P. Kofstad
  13. Z. Elecktrochem. v.63 W. Noddack;H. Walch
  14. J. Solid State Chem. v.2 G. V. Subba Rao;S. Ramdas;P. N. Mehrotra;C. N. Rao
  15. Compt. Rend. Ser. C. v.280 Y. Wilbert;N. Dherbomez;H. Breuil