• Title/Summary/Keyword: nuclear physics

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Radiation stability and radiolysis mechanism of hydroxyurea in HNO3 solution: Alpha, beta, and gamma irradiations

  • Yilin Qin;Wei Liao;Tu Lan;Fengzhen Li;Feize Li;Jijun Yang;Jiali Liao;Yuanyou Yang;Ning Liu
    • Nuclear Engineering and Technology
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    • 제54권12호
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    • pp.4660-4670
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    • 2022
  • Hydroxyurea (HU) is a novel salt-free reductant used potentially for the separation of U/Pu in the advanced PUREX process. In this work, the radiation stability of HU were systematically investigated in solution by examining the effects of the type of rays (α, β, and γ irradiations), the absorbed dose (10-50 kGy), and the HNO3 concentration (0-3 mol L-1). The influence degree on HU radiolysis rates followed the order of the absorbed dose > the ray type > the HNO3 concentration, but the latter two had moderate effects on HU radiolysis products where NH4+ and NO2- were found to be the most abundant ones, suggesting that the differences of α, β, and γ rays should be considered in the study of irradiation effects. The radiolysis mechanism was explored using density functional theory (DFT) calculations, and it proposed the dominant radiolysis paths of HU, indicating that the radiolysis of HU was mainly a free radical reaction among ·H, eaq-, H2O, intermediates, and the radiolytic free radical fragments of HU. The results reported here provide valuable insights into the mechanistic understanding of HU radiolysis under α, β, and γ irradiations and reliable data support for the application of HU in the reprocessing of spent fuel.

The development of EASI-based multi-path analysis code for nuclear security system with variability extension

  • Andiwijayakusuma, Dinan;Setiadipura, Topan;Purqon, Acep;Su'ud, Zaki
    • Nuclear Engineering and Technology
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    • 제54권10호
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    • pp.3604-3613
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    • 2022
  • The Physical Protection System (PPS) plays an important role and must effectively deal with various adversary attacks in nuclear security. In specific single adversary path scenarios, we can calculate the PPS effectiveness by EASI (Estimated Adversary Sequence Interruption) through Probability of Interruption (PI) calculation. EASI uses a single value of the probability of detection (PD) and the probability of alarm communications (PC) in the PPS. In this study, we develop a multi-path analysis code based on EASI to evaluate the effectiveness of PPS. Our quantification method for PI considers the variability and uncertainty of PD and PC value by Monte Carlo simulation. We converted the 2-D scheme of the nuclear facility into an Adversary Sequence Diagram (ASD). We used ASD to find the adversary path with the lowest probability of interruption as the most vulnerable paths (MVP). We examined a hypothetical facility (Hypothetical National Nuclear Research Facility - HNNRF) to confirm our code compared with EASI. The results show that implementing the variability extension can estimate the PI value and its associated uncertainty. The multi-path analysis code allows the analyst to make it easier to assess PPS with more extensive facilities with more complex adversary paths. However, the variability of the PD value in each protection element allows a significant decrease in the PI value. The possibility of this decrease needs to be an important concern for PPS designers to determine the PD value correctly or set a higher standard for PPS performance that remains reliable.

Design and Optimization for the Windowless Target of the China Nuclear Waste Transmutation Reactor

  • Cheng, Desheng;Wang, Weihua;Yang, Shijun;Deng, Haifei;Wang, Rongfei;Wang, Binjun
    • Nuclear Engineering and Technology
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    • 제48권2호
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    • pp.360-367
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    • 2016
  • A windowless spallation target can provide a neutron source and maintain neutron chain reaction for a subcritical reactor, and is a key component of China's nuclear waste transmutation of coupling accelerator and subcritical reactor. The main issue of the windowless target design is to form a stable and controllable free surface that can ensure that energy spectrum distribution is acquired for the neutron physical design when the high energy proton beam beats the lead-bismuth eutectic in the spallation target area. In this study, morphology and flow characteristics of the free surface of the windowless target were analyzed through the volume of fluid model using computational fluid dynamics simulation, and the results show that the outlet cross section size of the target is the key to form a stable and controllable free surface, as well as the outlet with an arc transition. The optimization parameter of the target design, in which the radius of outlet cross section is $60{\pm}1mm$, is verified to form a stable and controllable free surface and to reduce the formation of air bubbles. This work can function as a reference for carrying out engineering design of windowless target and for verification experiments.

FAST REACTOR PHYSICS AND COMPUTATIONAL METHODS

  • Yang, W.S.
    • Nuclear Engineering and Technology
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    • 제44권2호
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    • pp.177-198
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    • 2012
  • This paper reviews the fast reactor physics and computational methods. The basic reactor physics specific to fast spectrum reactors are briefly reviewed, focused on fissile material breeding and actinide burning. Design implications and reactivity feedback characteristics are compared between breeder and burner reactors. Some discussions are given to the distinct nuclear characteristics of fast reactors that make the assumptions employed in traditional LWR analysis methods not applicable. Reactor physics analysis codes used for the modeling of fast reactor designs in the U.S. are reviewed. This review covers cross-section generation capabilities, whole-core deterministic (diffusion and transport) and Monte Carlo calculation tools, depletion and fuel cycle analysis codes, perturbation theory codes for reactivity coefficient calculation and cross section sensitivity analysis, and uncertainty analysis codes.

Application of Economic Risk Measures for a Comparative Evaluation of Less and More Mature Nuclear Reactor Technologies

  • Andrianov, A.A.;Andrianova, O.N.;Kuptsov, I.S.;Svetlichny, L.I.;Utianskaya, T.V.
    • 방사성폐기물학회지
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    • 제16권4호
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    • pp.431-439
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    • 2018
  • Less mature nuclear reactor technologies are characterized by a greater uncertainty due to insufficient detailed design information, operational data, cost information, etc., but the expected performance characteristics of less mature options are usually more attractive in comparison with more mature ones. The greater uncertainty is, the higher economic risks associated with the project realization will be. Within a comparative evaluation of less and more mature nuclear reactor technologies, it is necessary to apply economic risk measures to balance judgments regarding the economic performance of less and more mature options. Assessments of any risk metrics involve calculating different characteristics of probability distributions of associated economic performance indicators and applying the Monte-Carlo method. This paper considers the applicability of statistical risk measures for different economic performance indicators within a trial case study on a comparative evaluation of less and more mature unspecified LWRs. The presented case study demonstrates the main trends associated with the incorporation of economic risk metrics into a comparative evaluation of less and more mature nuclear reactor technologies.

Neutronic optimization of thorium-based fuel configurations for minimizing slightly used nuclear fuel and radiotoxicity in small modular reactors

  • Nur Anis Zulaikha Kamarudin;Aznan Fazli Ismail;Mohamad Hairie Rabir;Khoo Kok Siong
    • Nuclear Engineering and Technology
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    • 제56권7호
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    • pp.2641-2649
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    • 2024
  • Effective management of slightly used nuclear fuel (SUNF) is crucial for both technical and public acceptance reasons. SUNF management, radiotoxicity risk, and associated financial investment and technological capabilities are major concerns in nuclear power production. Reducing the volume of SUNF can simplify its management, and one possible solution is utilizing small modular reactors (SMR) and advanced fuel designs like those with thorium. This research focuses on studying the neutronic performance and radionuclide inventory of three different thorium fuel configurations. The mass of fissile material in thorium-based fuel significantly impacts Kinf, burn-up, and neutron energy spectrum. Compared to uranium, thorium as a fuel produces far fewer transuranic elements and less long-lived fission products (LLFPs) at the end of the core cycle (EOC). However, certain fission product elements produced from thorium-based fuel exhibit higher radioactivity at the beginning of the core cycle (BOC). Physical separation of thorium and uranium in the fuel block, like seed-and-blanket units (SBU) and duplex fuel designs, generate less radioactive waste with lower radioactivity and longer cycle lengths than homogeneous or mixed thorium-uranium fuel. Furthermore, the SBU and duplex feel designs exhibit comparable neutron spectra, leading to negligible differences in SUNF production between the two.

Design and fabrication of an optimized Rogowski coil for plasma current sensing and the operation confidence of Alvand tokamak

  • Eydan, Anna;Shirani, Babak;Sadeghi, Yahya;Asgarian, Mohammad Ali;Noori, Ehsanollah
    • Nuclear Engineering and Technology
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    • 제52권11호
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    • pp.2535-2542
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    • 2020
  • To understand the fundamental parameters of Alvand tokamak, A Rogowski coil with an active integrator was designed and constructed. Considering the characteristics of the Alvand tokamak, the structural and electrical parameters affecting the sensor function, were designed. Calibration was performed directly in the presence of plasma. The sensor has a high resistance against interference of external magnetic fields. Plasma current was measured in various experiments. Based on the plasma current profile and loop voltage signal, the time evolution of plasma discharge was investigated and plasma behavior was analyzed. Alvand tokamak discharge was divided into several regions that represents different physical phenomena in the plasma. During the plasma discharge time, plasma had significant changes and its characteristic was not uniform. To understand the plasma behavior in each of the phases, the Rogowski sensor should have sufficient time resolution. The Rogowski sensor with a frequency up to 15 kHz was appropriate for this purpose.

ADVANCES IN MULTI-PHYSICS AND HIGH PERFORMANCE COMPUTING IN SUPPORT OF NUCLEAR REACTOR POWER SYSTEMS MODELING AND SIMULATION

  • Turinsky, Paul J.
    • Nuclear Engineering and Technology
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    • 제44권2호
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    • pp.103-122
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    • 2012
  • Significant advances in computational performance have occurred over the past two decades, achieved not only by the introduction of more powerful processors but the incorporation of parallelism in computer hardware at all levels. Simultaneous with these hardware and associated system software advances have been advances in modeling physical phenomena and the numerical algorithms to allow their usage in simulation. This paper presents a review of the advances in computer performance, discusses the modeling and simulation capabilities required to address the multi-physics and multi-scale phenomena applicable to a nuclear reactor core simulator, and present examples of relevant physics simulation codes' performances on high performance computers.

Research on the calculation method of sensitivity coefficients of reactor power to material density based on Monte Carlo perturbation theory

  • Wu Wang;Kaiwen Li;Yuchuan Guo;Conglong Jia;Zeguang Li;Kan Wang
    • Nuclear Engineering and Technology
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    • 제55권12호
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    • pp.4685-4694
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    • 2023
  • The ability to calculate the material density sensitivity coefficients of power with respect to the material density has broad application prospects for accelerating Monte Carlo-Thermal Hydraulics iterations. The second-order material density sensitivity coefficients for the general Monte Carlo score have been derived based on the differential operator sampling method in this paper, and the calculation of the sensitivity coefficients of cell power scores with respect to the material density has been realized in continuous-energy Monte Carlo code RMC. Based on the power-density sensitivity coefficients, the sensitivity coefficients of power scores to some other physical quantities, such as power-boron concentration coefficients and power-temperature coefficients considering only the thermal expansion, were subsequently calculated. The effectiveness of the proposed method is demonstrated in the power-density coefficients problems of the pressurized water reactor (PWR) moderator and the heat pipe reactor (HPR) reflectors. The calculations were carried out using RMC and the ENDF/B-VII.1 neutron nuclear data. It is shown that the calculated sensitivity coefficients can be used to predict the power scores accurately over a wide range of boron concentration of the PWR moderator and a wide range of temperature of HPR reflectors.