• 제목/요약/키워드: gamma-spectrometer

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Energy Calibration for Neutron Capture Resonance of Natural Sm by Using 46-MeV Electron Linear Accelerator

  • Lee, Jae-Hong;Lee, Sam-Yol
    • Journal of the Korean Society of Radiology
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    • v.1 no.2
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    • pp.31-35
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    • 2007
  • Energy calibration is important to identify accurate neutron capture resonance energy in the neutron TOF (Time-of-Flight) experiment. In present study, the accurate neutron capture resonance energies of natural Sm were measured by using a 46-MeV electron linear accelerator (linac) at the Research Reactor Institute, Kyoto University(KURRI). The BGO spectrometer were adopted for measurement the prompt capture gamma-ray of the sample. To obtain energy calibration curve, resonance energy of a gold sample used as standard resonance energy Mughabghab's data (From neutron resonance parameters data). Previous data (by Mughabghab) of natural Sm sample have been compared with the present result.

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Assessment of Nuclear Characteristics of NAA #1 Irradiation Hole in HANARO Research Reactor for Application of the $K_0$-NAA Methodology

  • Moon, Jong-Hwa;Kim, Sun-Ha;Chung, Yong-Sam;Dung, Ho-Mahn
    • Nuclear Engineering and Technology
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    • v.34 no.6
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    • pp.566-573
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    • 2002
  • Neutron activation analysis based on $textsc{k}$$_{o}$-standardization method# ($textsc{k}$o-NAA) is Com as one of the most remarkable progresses of the NAA with advantages of experimental simplicity, high accuracy, excellent flexibility with respect to irradiation and counting conditions, and suitability for computerization. This study was carried out to determine the reactor neutron spectrum parameters, i.e. $\alpha$ and f as the main factors of irradiation quality at NAA #1 irradiation hole on HANARO research reactor, to evaluate peak detection efficiency of the gamma-ray spectrometer for the use in the $textsc{k}$$_{o}$ experiments and to compare the measured concentration results with the certified values of some SRMs applying the experimentally determined to-parameters.ers.

A Study on Neutron Resonance Energy of 180Ta below 1eV Energy (1 eV 이하 에너지 영역에서의 180Ta 동위원소의 중성자공명에 대한 연구)

  • Lee, Samyol
    • Journal of the Korean Society of Radiology
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    • v.8 no.6
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    • pp.287-292
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    • 2014
  • In this study, the neutron capture cross section of $^{180}Ta$(natural existence ratio: 0.012 %) obtain by measuring has been compared with the evaluated data for the capture data. In generally, the neutron capture resonance is defined as Breit-Wigner formula. The formula consists of the resonance parameters such as neutron width, total width and neutron width. However in the case of $^{180}Ta$, these are very poor experimental neutron capture cross section data and resonance information in below 10 eV. Therefore, in the study, we analyzed the neutron resonance of $^{180}Ta$ with the measuring the prompt gamma-ray from the sample. And the resonance was compared with the evaluated data by Mughabghab, ENDF/B-VII, JEFF-3.1 and TENDL 2012. Neutron sources from photonuclear reaction with 46-MeV electron linear accelerator at Research Reactor Institute, Kyoto University used for cross section measurement of $^{180}Ta(n,{\gamma})^{181}Ta$ reaction. $BGO(Bi_4Ge_3O_{12})$ scintillation detectors used for measurement of the prompt gamma ray from the $^{180}Ta(n,{\gamma})^{181}Ta$ reaction. The BGO spectrometer was composed geometrically as total energy absorption detector.

A Study on Neutron Resonance Energy of Tantalum by 46-MeV Electron Linac TOF Method (46-MeV 전자선형가속기의 TOF 방법을 이용한 탄탈의 중성자 공명 에너지 분석에 관한 연구)

  • Lee, Samyol
    • Journal of the Korean Society of Radiology
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    • v.7 no.3
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    • pp.245-249
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    • 2013
  • Neutron sources from photonuclear reaction with 46-MeV electron linear accelerator at Research Reactor Institute, Kyoto University used for resonance energy measurement of natural tantalum. BGO($Bi_4Ge_3O_{12}$) scintillation detectors used for measurement of the prompt gamma ray from the natural tantalum sample. The BGO spectrometer was composed geometrically as total energy absorption detector. The electric signal from the spectrometer was analyzed for TOF(Time-of-Flight) spectrum which is used identification of neutron capture resonance energy. In this study, the neutron energy region is from 1 to 200 eV, because of strong X-ray effect produced photonuclear reaction in Ta target, the measurement was performed to below 1 keV energy region. The resonance energy was compared with the evaluated values(ENDF/B-VI, Mughabghab). All of the resonances from 4.28 ~ 200 eV were seen in the present measurement except 144.3 eV resonance.

Separation and Recovery for the Analysis of Radioiodine in RI Wastes (RI 폐기물 내 방사성요오드 분석을 위한 분리 및 회수)

  • Kang, Sang-Hoon;Han, Sun-Ho;Lee, Heung-N.;Jee, Kwang-Yong;Lee, In-Koo
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.5 no.4
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    • pp.267-272
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    • 2007
  • Various kinds of RI wastes are discharged from licensed organizations of radioisotopes les such as hospitals and clinic organizations, educational organizations, research institutions, and public organizations. Radioiodines such as $^{125}I\;and\;^{131}I$ are radioisotopes mainly used in nuclear medicine and industry. A method for the determination of radioiodines in RI wastes has been applied to measure low level activity using acid decomposition method and HPGe gamma ray spectrometer. Prior to analysis of real samples, $^{131}I$ reference solution and 10 g of yellow tissue paper was added to flask in mantle and was heated in 100 mL of 0.4 N $K_2Cr_2O_7$ and 100 mL of 9 M $H_2SO_4$, and then distilled after adding 10 mL of 30% $H_2PO_3$ and 1 mL of 30% $H_2O_2$. The condensed iodine by circulator was extracted into $CCl_4$, then back-extracted into the aqueous phase with 10 mL of 5% $K_2SO_2$ solution. Finally, $^{131}I$ was measured at 364.48 keV using HPGe gamma ray spectrometer after precipitation and filtration. Chemical yield of three steps such as acid decomposition process, chemical separation process, and precipitation and filtration process was more han 94% respectively, MDA(Minimum Detectable Activity) of $^{131}I$ at this analytical condition was 0.6 Bq/g.

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Changes of Free Radical Concentrations with Irradiation Dose and Storage Time in Gamma-Irradiated Sesame and Perilla Seeds (감마선 조사된 참깨, 들깨의 조사선량과 저장기간에 따른 free radical 농도의 변화)

  • Lee, Eun-Jeong;Yang, Jae-Seung
    • Korean Journal of Food Science and Technology
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    • v.34 no.3
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    • pp.396-399
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    • 2002
  • Electron spin resonance (ESR) spectroscopy was used to investigate the effect of irradiation dose and storage time on the free radical concentrations in gamma-irradiated sesame (Korean and Sudan) and perilla seeds (Korea). The samples were sealed with packed pyrex tube (50 g respectively) and then irradiated with doses of 0, 1, 5 and 10 kGy at room temperature using a Co-60 irradiator. Each sample in ESR quartz tube were calculated with ESR signals by Bruker-EPR spectrometer for 4 weeks. Free radicals detected for irradiated and unirradiated samples were higher than those of unirradiated ones. Since the free radical concentrations linearly incresed with the applied doses $(1{\sim}10\;kGy)$, highly positive correlation coefficients $(R^2=0.9926{\sim}0.9994)$ were obtained between irradiation doses and free radical concentrations right after irradiation. Although the free radical concentrations decreased with storage time, the signals of free radical in irradiated samples were observed even after 4 weeks of storage at room temperature.

PRELIMINARY FEASIBILITY STUDY OF THE SOLAR OBSERVATION PAYLOADS FOR STSAT-CLASS SATELLITES

  • Moon, Yong-Jae;Cho, Kyung-Seok;Jin, Ho;Chae, Jong-Chul;Lee, Sung-Ho;Seon, Kwang-Il;Kim, Yeon-Han;Park, Young-Deuk
    • Journal of Astronomy and Space Sciences
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    • v.21 no.4
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    • pp.329-342
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    • 2004
  • In this paper, we present preliminary feasibility studies on three types of solar observation payloads for future Korean Science and Technology Satellite (STSAT) programs. The three candidates are (1) an UV imaging telescope, (2) an UV spectrograph, and (3) an X-ray spectrometer. In the case of UV imaging telescope, the most important constraint seems to be the control stability of a satellite in order to obtain a reasonably good spatial resolution. Considering that the current pointing stability estimated from the data of the Far ultraviolet Imaging Spectrograph (FIMS) onboard the Korean STSAT-1, is around 1 arc minutes/sec, we think that it is hard to obtain a spatial resolution sufficient for scientific research by such an UV Imaging Telescope. For solar imaging missions, we realize that an image stabilization system, which is composed of a small guide telescope with limb sensor and a servo controller of secondary mirror, is quite essential for a very good pointing stability of about 0.1 arcsec. An UV spectrograph covering the solar full disk seems to be a good choice in that there is no risk due to poor pointing stability as well as that it can provide us with valuable UV spectral irradiance data valuable for studying their effects on the Earth's atmosphere and satellites. The heritage of the FIMS can be a great advantage of developing the UV spectrograph. Its main disadvantage is that two major missions are in operation or scheduled. Our preliminary investigations show that an X-ray spectrometer for the full disk Sun seems to be the best choice among the three candidates. The reasons are : (1) high temporal and spectral X-ray data are very essential for studying the acceleration process of energetic particles associated with solar flares, (2) we have a good heritage of X-ray detectors including a rocket-borne X-ray detector, (3) in the case of developing countries such as India and Czech, solar X-ray spectrometers were selected as their early stage satellite missions due to their poor pointing stabilities, and (4) there is no planned major mission after currently operating Reuven Ramaty High-Energy Solar Spectroscopic Imager (RHESSI) mission. Finally, we present a preliminary design of a solar X-ray spectrometer covering soft X-ray (2 keV) to gamma ray (10 MeV).

Radiation Field in PWR Plants (PWR 발전소에서의 방사선장 특성)

  • Song, Myung-Jae;Kim, Hee-Keun;Kim, Bong-Hwan;Chang, Si-Young
    • Journal of Radiation Protection and Research
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    • v.17 no.2
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    • pp.61-70
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    • 1992
  • Photon, neutron and beta radiation fields were measured at PWR plants which are the representative types of nuclear power plant operated in Korea. The photon energy spectra were measured at locations in the auxiliary building during operation period and in the containment vessel(C/V) during shutdown period using a portable gamma spectrometer with a HPGe detector. The distribution of average energy was found to range from 440 to 780 keV in the C/V and from 280 keV to 760 keV in the auxiliary building, respectively. The average neutron energy measured at the five locations around the operation deck in the C/V in operation using a BMSS (Bonner Multi-Sphere Spectrometer) ranged from 20 keV to 210 keV. A computer code, BUNKI was used to unfold the spectrum. The beta energy spectra in the C/V and in the auxiliary building in annual outage were determined using 14 smear samples taken from the highly contaminated areas. The analysis showed that the representative corrosion product, $^{60}Co$ made main contribution to the beta energy field.

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ESR Study of Paramagnetic Defects of the ${\gamma}$-irradiated Potassium Sulfate Single Crystal (${\gamma}$-선에 조사된 황산칼륨 단결정의 상자성 결함에 관한 전자스핀공명 연구)

  • Yo Chul Hyun;Chung Won Yang;Jong In Hong;Eun Ok Kim;Jung Sung Yang
    • Journal of the Korean Chemical Society
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    • v.25 no.6
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    • pp.367-375
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    • 1981
  • Single crystals of Potassium Sulfate ($K_2SO_4$) have been grown from the saturated solution by the evaporation method at the optimum conditions. Radiation damages in the crystal by ${\gamma}$-irradiation of about $12{\times}10^6$ Roentgen have given rise to paramagnetic centers or paramagnetic defects. Electron spin resonance (ESR) spectra of the centers are obtained with the X-band EPR spectrometer at room temperature. The ESR peaks of the paramagnetic species are found to be anisotropic but the peak of $SO_3-$ radical is an isotropic of Gaussian shape at g = 2.0036. A number of ESR spectra of the crystal for angular variation of the anisotropic peaks are recorded at various orientations of rotation about a, b and c crystallographic axes respectively. The g-values are calculated from the line position between anisotropic peaks and the isotropic one and then principal g-values and its direction cosines of the species are obtained by diagonalization of 9 matrix elements of the corresponding g-values. All the paramagnetic defects are identified by the characteristic principal g-values and its direction cosines.

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Determination of Radiolysis Produce of DHOA by GC/MS (GC/MS를 이용한 DHOA의 방사선 분해생성물 분석)

  • Yang, Han-Beom;Lee, Eil-Hee;Lim, Jae-Kwan;Chung, Dong-Yong;Kim, Kwang-Wook;Kim, Jong-Seung
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.7 no.1
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    • pp.17-23
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    • 2009
  • Dihexyloctanamide(DHOA) was used as an extractant or phase modifier with the diamide extractants in a solvent extraction process for a radioactive liquid waste treatment. The degradation compounds of the DHOA extractant, irradiated with $^{60}Co$ gamma ray, were octanoic acid and dihexylamine which are identified by a Fourier transform infrared(FT-IR) and gas chromatograph/mass spectrometer(GC/MS) analysis, and determined by the GC/MS with selected ion monitoring(SIM) mode. Retention behavior of octanoic acid, tridecane (internal standard) and dihexylamine in total ion chromatogram (TIC) were 8.65 min., 9.79 min., and 10.27 min., respectively. With increasing the absorbed dose of the $\gamma$-ray irradiated DHOA, the concentration of octanoic acid was decreased and that of dihexylamine was increased.

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