• 제목/요약/키워드: fission gas

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Advances in the understanding of molybdenum effect on iodine and caesium reactivity in condensed phase in the primary circuit in nuclear severe accident conditions

  • Gouello, Melany;Hokkinen, Jouni;Karkela, Teemu
    • Nuclear Engineering and Technology
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    • 제52권8호
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    • pp.1638-1649
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    • 2020
  • In the case of a severe accident in a Light Water Reactor, the issue of late release of fission products, from the primary circuit surfaces is of particular concern due to the direct impact on the source term. CsI is the main iodine compound present in the primary circuit and can be deposited as particles or condensed species. Its chemistry can be affected by the presence of molybdenum, and can lead to the formation of gaseous iodine. The present work studied chemical reactions on the surfaces involving gaseous iodine release. CsI and MoO3 were used to highlight the effects of carrier gas composition and oxygen partial pressure on the reactions. The results revealed a noticeable effect of the presence of molybdenum on the formation of gaseous iodine, mainly identified as molecular iodine. In addition, the oxygen partial pressure prevailing in the studied conditions was an influential parameter in the reaction.

모의 DUPIC 핵연료의 소결 특성 연구 (A Study on the Sintering of Simulated DUPIC Fuel)

  • 강권호;배기광;박희성;송기찬;문제선
    • 한국분말재료학회지
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    • 제7권3호
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    • pp.123-130
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    • 2000
  • The simulated DUPIC fuel provides a convenient way to investigate fuel properties and behaviours such as thermal conductivity, thermal expansion, fission gas release, leaching and so on. Several pellets simulating the composition and microstructure of the DUPIC fuel were fabricated from resintering powder through the OREOX process of the simulated spent fuel pellets, which were prepared from the mixture of stable forms of constituent nuclides. This study describes the powder treatment, OREOX, compaction and sintering to fabricate simulated DUPIC fuel using the simulated spent fuel. The homogeneity of additives in the powder was observed after attrition milling. The microstructure of the simulated spent fuel was in agreement with the previous studies. The densities and the grain size of simulated DUPIC fuel was pellets are higher than those of simulated spent fuel pellets. Small metallic precipitates and oxide precipitates were observed on matrix grain boundaries.

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RECENT UPDATES TO NRC FUEL PERFORMANCE CODES AND PLANS FOR FUTURE IMPROVEMENTS

  • Geelhood, Kenneth
    • Nuclear Engineering and Technology
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    • 제43권6호
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    • pp.509-522
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    • 2011
  • FRAPCON-3.4a and FRAPTRAN 1.4 are the most recent versions of the U.S. Nuclear Regulatory Commission (NRC) steady-state and transient fuel performance codes, respectively. These codes have been assessed against separate effects data and integral assessment data and have been determined to provide a best estimate calculation of fuel performance. Recent updates included in FRAPCON-3.4a include updated material properties models, models for new fuel and cladding types, cladding finite element analysis capability, and capability to perform uncertainty analyses and calculate upper tolerance limits for important outputs. Recent updates included in FRAPTRAN 1.4 include: material properties models that are consistent with FRAPCON-3.4a, cladding failure models that are applicable for loss-of coolant-accident and reactivity initiated accident modeling, and updated heat transfer models. This paper briefly describes these code updates and data assessments, highlighting the particularly important improvements and data assessments. This paper also discusses areas of improvements that will be addressed in upcoming code versions.

Initial Release of Nuclides from Spent PWR Fuels

  • Kim, S. S.;K. S. Chun;Kim, Y. B.;Park, J. W.
    • 한국방사성폐기물학회:학술대회논문집
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    • 한국방사성폐기물학회 2004년도 Proceedings of the 4th Korea-China Joint Workshop on Nuclear Waste Management
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    • pp.238-244
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    • 2004
  • The relationship between the leaching and gap inventory of spent fuel has been studied. When a specimen of J44H08 spent PWR fuel with 38 GWD/MTU has been leached in the synthetic granitic groundwater in Ar atmosphere, the released fraction of cesium was increased rapidly up to 0.7% at around 500 days and stayed below 0.8% until 3 years. This 0.7% of cesium might be released from the gap in this fuel. The measurement of gap inventory with C15I08 spent PWR fuel, having 35 GWD/MTU and 0.22% of fission gas release, was also determined near 0.6% for the cesium, which is a similar fraction of cesium released from the leaching experiment with J44H08 fuel. Its gap inventories of strontium and iodine were about 0.03 and less than 0.2% respectively. Respective fractions of cesium and strontium in grain boundary of C15I08 were 0.78, 0.09%.

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Systems Engineering Approach to the Heat Transfer Analysis of PLUS 7 Fuel Rod Using ANSYS FEM Code

  • Park, Sang-Jun;Mutembei, Mutegi Peter;Namgung, Ihn
    • 시스템엔지니어링학술지
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    • 제13권1호
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    • pp.33-39
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    • 2017
  • This paper describes the system engineering approach for the heat transfer analysis of plus7 fuel rod for APR1400 using, a commercial software, ANSYS. The fuel rod is composed of fuel pellets, fill gas, end caps, plenum spring and cladding. The heat is transferred from the pellet outward by conduction through the pellet, fill gas and cladding and further by convection from the cladding surface to the coolant in the flow channel. The goal of this paper is to demonstrate the temperature and heat flux change from the fuel centerline to the cladding surface when having maximum fuel centerline temperature at 100% power. This phenomenon is modelled using the ANSYS FEM code and analyzed for steady state temperature distribution across the fuel pellet and clad and the results were compared to the standard values given in APR1400 SSAR. Specifically the applicability of commercial software in the evaluation of nuclear fuel temperature distribution has been accounted. It is note that special codes have been used for fuel rod mechanical analysis which calculates interrelated effects of temperature, pressure, cladding elastic and plastic behavior, fission gas release, and fuel densification and swelling under the time-varying irradiation conditions. To satisfactorily meet this objective we apply system engineering methodologies to formulate the process and allow for verification and validation of the results acquired. The close proximity of the results obtained validated the accuracy of the FEM analysis of the 2D axisymmetric model and 3D model. This result demonstrated the validity of commercial software instead of proprietary in-house code that is more costly to develop and maintain.

냉각수상실 사고시 격납용기로부터 누출되는 유체유량 추산을 위한 해석적 방법 (Analytical Methods of Leakage Rate Estimation from a Containment tinder a LOCA)

  • Moon-Hyun Chun
    • Nuclear Engineering and Technology
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    • 제13권3호
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    • pp.121-129
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    • 1981
  • 많은 기존 공식중 세계의 가장 우수한 최대 유량공식을 찾아, 그 세개의 한계유량공식의 개요와, 냉각재상실사고시 격납용기격리에 실패하는 경우를 특정지을 수 있는 구멍의 크기와 격납용기의 압력 및 온도 등이 주어진 상태하에서 격납용기로부터 외부대기로 방출되는 개략적인 핵분열생성물의 양을 추정하기 위한 계산절차를 제시하였다. 이상기체의 임계유량공식과 이상유(two-phase flow)의 최대유량을 산출하기 위한 무디(Moody)의 도표를 이용하여 계산실예를 제시하였으며, 그 결과를 콘뎀프트-앨티(CONTEMPT-LT) 전산코드의 질량유출공식을 콘버징 노즐(converging nozzle)을 통과하는 음속류(sonic flow)의 경우에 적용하여 산출한 값과 비교하여 보았다. 이리하여 이상 기체의 임계유량공식은 무디(Moody)의 공식이 주는 값과 거의 비슷한 결과를 줌을 입증하였다. 또한 냉각재상실 사고시 격납용기로부터의 유출율을 추정하기 위해서는 콘템프트-앨티(CONTEMPT-LT)의 질량유출공식을 사용하는 것보다 이상 기체의 최대유량공식을 사용하는 것이 더 보수적인 방법임을 보여 주었다.

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하나로 기체시료채취계통에서 생성된 응축수 억제를 위한 CFD 해석 (CFD Analysis to Suppress Condensate Water Generated in Gas Sampling System of HANARO)

  • 조성환;이종현;김대영
    • 방사성폐기물학회지
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    • 제18권2_spc호
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    • pp.327-336
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    • 2020
  • HANARO (High-flux Advanced Neutron Application Reactor)는 우라늄의 핵분열 연쇄반응에서 생성된 중성자를 이용하여 다양한 연구개발을 수행하는 열출력 30 MW 규모의 연구용 원자로이다. 탈기탱크는 HANARO의 부속시설에 설치되어 있다. 탈기탱크는 내부환경요인으로 인해 기체오염물질을 발생시킨다. 탈기탱크는 기체오염물질을 허용 가능한 수준 이하로 유지하기위해 필요하며 기체시료채취판넬의 분석기에 의해 모니터링 된다. 응축수가 발생하여 기체시료채취판넬의 분석기 내부로 유입된다면, 분석기의 측정 챔버 내부에 부식이 발생하여 고장을 야기한다. 응축수의 생성 원인은 탈기탱크에 존재하는 기체가 분석기로 유입되는 과정에서 탈기탱크와 분석기사이 온도 차이다. 응축수 생성을 억제하고 계통 내부에 생성된 응축수를 효율적으로 제거하기 위해 탈기탱크와 기체시료채취판넬 사이에 히팅시스템이 설치되었다. 이 연구에서 우리는 히팅시스템의 효율성을 알고자 한다. 또한 Wall Condensation Model을 이용하여 유체 입구온도, 외부온도 및 히팅 케이블 설정온도 변화에 따른 파이프 온도와 평균응축량의 변화를 모델링하였다.

1D AND 3D ANALYSES OF THE ZY2 SCIP BWR RAMP TESTS WITH THE FUEL CODES METEOR AND ALCYONE

  • Sercombe, J.;Agard, M.;Struzik, C.;Michel, B.;Thouvenin, G.;Poussard, C.;Kallstrom, K.R.
    • Nuclear Engineering and Technology
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    • 제41권2호
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    • pp.187-198
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    • 2009
  • In this paper, three power ramp tests performed on high burn-up Re-crystallized Zircaloy2 - UO2 BWR fuel rods (56 to 63 MWd/kgU) within the SCIP project are simulated with METEOR and ALCYONE 3D. Two of the ramp tests are of staircase type up to Linear Heat Rates of 420 and 520 W/cm and with long holding periods. Failure of the 420 W/cm fuel rod was observed after 40 minutes. The third ramp test consisted of a more standard ramp test with a constant power rate of 80 W/cm/min up to 410 W/cm with a short holding time. The tests were first simulated with the METEOR 1D fuel rod code, which gave accurate results in terms of profilometry and fission gas releases. The behaviour of a fuel pellet fragment and of the cladding piece on top of it was then investigated with ALCYONE 3D. The size and the main characteristics of the ridges after base irradiation and power ramp testing were recovered. Finally, the failure criteria validated for PWR conditions and fuel rods with low-to-medium burn-ups were used to analyze the failure probability of the KKL rodlets during ramp testing.

연구로 해체시 발생되는 흑연폐기물의 열적 거동 (Thermal Behavior of the Nuclear Graphite Waste Generated from the Decommissioning of the Nuclear Research Reactor)

  • 양희철;은희철;이동규;조용준;강영애;이근우;오원진
    • 한국방사성폐기물학회:학술대회논문집
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    • 한국방사성폐기물학회 2004년도 학술논문집
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    • pp.105-114
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    • 2004
  • This study investigated the thermal behavior of the nuclear graphite waste generated from the decommissioning of the Korean nuclear research reactor, The first part study investigated the decomposition rate of the nuclear graphite waste up to $1000^{\circ}C$ under various oxygen partial pressures using a thermo-gravimetric analyzer (TGA). Tested graphite waste sample not easily destroyed in the oxygen-deficient condition. However, the gas-solid oxidation reaction was found to be very effective in the presence of oxygen. No significant amount of the product of incomplete combustion was formed even in the limited oxygen concentration of 4% $O_2$. The influence of temperature and oxygen partial pressure was evaluated by the theoretical model analysis of the thermo-gravimetric data. The activation energy and the reaction order of graphite oxidation were evaluated as 128 kJ/mole and 1.1, respectively. The second part of this study investigated the behavior of radioactive elements under graphite oxidation atmosphere using thermodynamic equilibrium model. $^{22}Na$, $^{134}Cs$ and $^{137}Cs$ were found be the semi-volatile elements. Since volatile uranium species can be formulated at high temperatures above $1050^{\circ}C$, the temperature of incinerator furnace should be minimized. Other corrosion/activation products, fission products and uranium were found to be the non-volatile species.

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CANDU형 핵연료거동에 관한 계산모형의 검토 및 거동특성에 관한 변수적 연구 (Review of Calculational Model for the Performance of CANDU-Type Nuclear Development and Parametric Study on the Fuel Performance)

  • Man Sung Yim;Un Chul Lee;Ho Chun Suk
    • Nuclear Engineering and Technology
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    • 제15권1호
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    • pp.57-69
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    • 1983
  • 경수형원자로 핵연료봉의 거동분석을 위한 전산코드인 FRAPCON-1 코드가 월성 1호기에 장전되는 CANDU형 핵연료봉의 거동분석을 위해 적절한지를 평가하였다. 연료내의 중성자속의 감소와 연료피복재간 열전달을 계산하는 FRAPCON-1 코드의 모형들을 수정하였으며 핵분열 기체방출모형의 CANDU 핵연료에 대한 타당성여부를 검토하였고 피복재와 냉각수간의 열전달 계수 계산을 위해 중수특성을 사용하였다. 수정된 코드 FRAPCON-1-CSK를 사용하여 월성 1호기 핵연료의 각 설계변수들에 대한 민감도 분석을 수행하였다. 아울러 월성 1호기 핵연료봉의 거동특성분석도 수행하였는데 계산된 결과들은 CANDU 핵연료봉에 대한 설계기준이 알러져 있지 않는 관계로 경수로 핵연료봉 설계기준의 입장에서 검토되었다.

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