• Title/Summary/Keyword: aerosol extinction coefficient

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Aerosol Measurement and Property Analysis Based on Data Collected by a Micro-pulse LIDAR over Shanghai, China

  • Huang, Xingyou;Yang, Xiaowu;Geng, Fuhai;Zhang, Hua;He, Qianshan;Bu, Lingbing
    • Journal of the Optical Society of Korea
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    • v.14 no.3
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    • pp.185-189
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    • 2010
  • A micro-pulse LIDAR system (MPL) was employed to measure the aerosol over Pudong, Shanghai from July 2008 to January 2009. Based on Fernald method, aerosol optical variables such as extinction coefficient were retrieved and analyzed. Results show that aerosol exists mainly in low layers; aerosol loading reaches its maximum in the afternoon, and then decreases with time until its minimum at night. Most of the aerosol concentrates in the layer below 3 km, and optical extinction coefficient in the layer below 2 km contributes 84.25% of that below 6 km. Two extinction coefficient peaks appear in the near surface layer up to 500 m and in the level around 1000 m. Aerosol extinction coefficient shows a seasonal downward trend from summer to winter.

Effects of Aerosol Hygroscopicity on Fine Particle Mass Concentration and Light Extinction Coefficient at Seoul and Gosan in Korea

  • Choi, Eun-Kyung;Kim, Yong-Pyo
    • Asian Journal of Atmospheric Environment
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    • v.4 no.1
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    • pp.55-61
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    • 2010
  • The sensitivity of aerosol light extinction coefficient to the aerosol chemical composition change is estimated by (1) calculating the aerosol water content and chemical concentrations by a gas/particle equilibrium model and (2) calculating the aerosol light extinction coefficient by a Mie theory based optical model. The major chemical species are total (gas and particle phase) sulfuric acid, total nitric acid, and total ammonia which are based on the measurement data at Seoul and Gosan. At Seoul, since there were enough ammonia to neutralize both total sulfuric acid and total nitric acid, the dry ionic concentration is most sensitive to the variation of the total nitric acid level, while the total mass concentration (ionic concentration plus water content) and thus, the aerosol light extinction coefficient are primarily determined by the total sulfuric acid. At Gosan, since the concentration of ambient sulfuric acid was the highest among the inorganic species, sulfate salts determined aerosol hygroscopicity. Thus, both ionic and total mass concentration, and resultant aerosol light extinction coefficient are primarily determined by the sulfuric acid level.

A Study on the Concentration and Light Extinction of Atmospheric Aerosol in Seoul (서울 대기 에어로솔의 농도와 광소산에 관한 연구)

  • 김필수;오미석;김의훈
    • Journal of Korean Society for Atmospheric Environment
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    • v.7 no.3
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    • pp.227-234
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    • 1991
  • This study deals with concentration and light extinction of atmospheric aerosol in Seoul. From the measured aerosol size distribution for particle diameter ranging from 0.01 $\mum \sim 1.0 \mum$, extinction coefficient is calculated using the Mie theory. The results show that the diurnal variation of aerosol concentration, in general, reveals the lowest concentration in early morning and afternoon, while the highest at about 8 O'clock owing to the heavy traffic and accumulation of air pollution in the low atmosphere. However, aerosol concentration and extinction coefficient on April 7 give low values due to the advective wind. On the other hand, high aerosol concentration and extinction coefficenat are recorded on April 10 although solar radiation is weak. From the distribution of extinction coefficient we can find that aerosol particles of 0.1 $\mum \sim 1.0 \mum$ in diameter are highly effective on light extinction.

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Modelling of Aerosol Vertical Distribution during a Spring Season at Gwangju, Korea

  • Shin, Sung-Kyun;Lee, Kwon-Ho
    • Asian Journal of Atmospheric Environment
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    • v.10 no.1
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    • pp.13-21
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    • 2016
  • The vertical distributions of aerosol extinction coefficient were estimated using the scaling height retrieved at Gwangju, Korea ($35.23^{\circ}N$, $126.84^{\circ}E$) during a spring season (March to May) of 2009. The aerosol scaling heights were calculated on a basis of the aerosol optical depth (AOD) and the surface visibilities. During the observation period, the scaling heights varied between 3.55 km and 0.39 km. The retrieved vertical profiles of extinction coefficient from these scaling heights were compared with extinction profile derived from the Light Detection and Ranging (LIDAR) observation. The retrieve vertical profiles of aerosol extinction coefficient were categorized into three classes according to the values of AODs and the surface visibilities: (Case I) the AODs and the surface visibilities are measured as both high, (Case II) the AODs and the surface visibilities are both lower, and (Others) the others. The averaged scaling heights for the three cases were $3.09{\pm}0.46km$, $0.82{\pm}0.27km$, and $1.46{\pm}0.57km$, respectively. For Case I, differences between the vertical profile retrieved from the scaling height and the LIDAR observation was highest. Because aerosols in Case I are considered as dust-dominant, uplifted dust above planetary boundary layer (PBL) was influenced this discrepancy. However, for the Case II and other cases, the modelled vertical aerosol extinction profiles from the scaling heights are in good agreement with the results from the LIDAR observation. Although limitation in the current modelling of vertical structure of aerosols exists for aerosol layers above PBL, the results are promising to assess aerosol profile without high-cost instruments.

Aerosol-extinction Retrieval Method at Three Effective RGB Wavelengths Using a Commercial Digital Camera (상용 디지털 카메라를 이용한 3가지 유효 RGB 파장에서의 미세먼지 소산계수 산출법)

  • Park, Sunho;Kim, Dukhyeon
    • Korean Journal of Optics and Photonics
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    • v.31 no.2
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    • pp.71-80
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    • 2020
  • In this article, we suggest a new method for measuring an aerosol's extinction coefficient using a commercial camera. For a given image, we choose three pixel-points that are imaged for the same kinds of objects located in similar directions. We suggest and calculate aerosol extinction coefficients from these RGB gray levels and the different distances of the three objects. To compare our measurement results, we also measure extinction coefficients using lidar. Finally, we find that there are meaningful and sensible correlations between these two measurements, with a correlation coefficient of 0.86. We measure the aerosol extinction coefficient at three different RGB wavelengths using the same method. From these aerosol extinction coefficients at three different wavelengths, we find that the Angstrom exponent ranges from 0.7 to 1.6 over a full daytime period. We believe that these Angstrom exponents can give important information about the size of the fine particles.

Characteristics of Visibility Impairment by Semi-Continuous Optical and Chemical Property Monitoring of Aerosols in Seoul (에어로졸의 광학 및 화학 특성 준실시간 모니터링을 통한 서울지역 시정 감쇄 분석)

  • Park, Jong-Sung;Park, Seung-Myung;Song, In-Ho;Shin, Hye-Jung;Hong, You-Deog
    • Journal of Korean Society for Atmospheric Environment
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    • v.31 no.4
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    • pp.319-329
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    • 2015
  • The characteristics of aerosol light extinction were investigated by comparing measured and calculated extinction coefficient to understand the contribution of air pollutants on visibility impairment for data during 4 months (Jan~ April), 2014. The integrated nephelometer and aethalometer system were installed to measure the scattering and absorption coefficients of aerosol as well as BAM 1020, MARGA, semi-continuous OCEC analyzer, and online-XRF to calculate the extinction coefficient. The IMPROVE_2005 equation was used to determine the contributions of different chemical components on visibility impairment in $PM_{2.5}$ and $PM_{10}$ due to highest correlation with measured data. Sulfate, nitrate, and organic mass by carbon (OMC) of fine aerosol were the major contributors affecting on visibility impairment. Total contributions to light extinction were calculated as $631.0Mm^{-1}$ for the worst-case and $64.4Mm^{-1}$ for the best-case. The concentrations of aerosol component for the worst-case were 38.4 times and 45.5 times larger than those of the best-case for $(NH_4)_2SO_4$ and $NH_4NO_3$, respectively. At lower visibility condition, in which extinction coefficient was higher than $400Mm^{-1}$, extinction coefficient varied according to the relative humidity variation regardless of $PM_{2.5}$.

Analysis of Vertical Profiles and Optical Characteristics of the Asian Dust Using Ground-based Measurements (지상관측장비를 이용하여 관측한 봄철 황사의 연직분포와 광학적 특성 분석)

  • Lee, Byung-Il;Yoon, Soon-Chang;Kim, Yoonjae
    • Atmosphere
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    • v.18 no.4
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    • pp.287-297
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    • 2008
  • The vertical profiles and optical properties of Asian dust are investigated using ground-based measurements from 1998 to 2002. Vertical profiles of aerosol extinction coefficient are evaluated using MPL (Micro Pulse Lidar) data. Optical parameters such as aerosol optical thickness ($\tau$), ${\AA}ngstr\ddot{o}m$ exponent ($\alpha$), single scattering albedo ($\omega$), refractive index, and volume size distribution are analyzed with sun/sky radiometer data for the same period. We can separate aerosol vertical profiles into three categories. First category named as 'Asian dust case', which aerosol extinction coefficient is larger than $0.15km^{-1}$ and dust layer exists from surface up to 3-4km. Second category named as 'Elevated aerosol case', which aerosol layer exists between 2 and 6km with 1-2.5km thickness, and extinction coefficient is smaller than $0.15km^{-1}$. Third category named as 'Clear sky case', which aerosol extinction coefficient appears smaller than $0.15km^{-1}$. and shows that diurnal variation of background aerosol in urban area. While optical parameters for first category indicate that $\tau$ and $\alpha$ are $0.63{\pm}0.14$, $0.48{\pm}0.19$, respectively. Also, aerosol volume concentration is increased for range of 1 and $4{\mu}m$, in coarse mode. Optical parameters for second category can be separated into two different types. Optical properties of first type are very close to Asian dust cases. Also, dust reports of source region and backward trajectory analyses assure that these type is much related with Asian dust event. However, optical properties of the other type are similar to those of urban aerosol. For clear sky case, $\tau$ is relatively smaller and $\alpha$ is larger compare with other cases. Each case shows distinct characteristics in aerosol optical parameters.

Measurements of the Lidar Ratio for Asian Dust and Pollution Aerosols with a Combined Raman and Back-scatter Lidar (라만-탄성 라이다를 이용한 황사 및 오염 에어러솔의 라이다 비 측정 연구)

  • Yoon, S.C.;Lee, Y.J.;Kim, S.W.;Kim, M.H.;Sugimoto, N.
    • Atmosphere
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    • v.20 no.4
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    • pp.483-494
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    • 2010
  • The vertical profiles of the extinction coefficient, the backscatter coefficient, and the lidar ratio (i.e., extinction-to-backscattering ratio) for Asian dust and pollution aerosols are determined from Raman (inelastic) and elastic backscatter signals. The values of lidar ratios during two polluted days is found between 52 and 82 sr (July 22, 2009) and 40~60 sr (July 31, 2009) at 52 nm, with relatively low value of particle depolarization ratio (<5%) and high value of sun photometer-derived Angstrom exponent (> 1.2). However, lidar ratios between 25 and 40 sr are found during two Asian dust periods (October 20, 2009 and March 15, 2010), with 10~20% of particle depolarization ratio and the relatively low value of sun photometer-derived Angstrom exponent (< 0.39). The lidar ratio, particle depolarization ratio and color ratio are useful optical parameter to distinguish non-spherical coarse dust and spherical fine pollution aerosols. The comparison of aerosol extinction profiles determined from inelastic-backscatter signals by the Raman method and from elastic-backscatter signals by using the Fernald method with constant value of lidar ratio (50 sr) have shown that reliable aerosol extinction coefficients cannot be determined from elastic-backscatter signals alone, because the lidar ratio varies with aerosol types. A combined Raman and elastic backscatter lidar system can provide reliable information about the aerosol extinction profile and the aerosol lidar ratio.

Multi-wavelength Raman LIDAR for Use in Determining the Microphysical, Optical, and Radiative Properties of Mixed Aerosols

  • Lee, Kwon-Ho;Noh, Young Min
    • Asian Journal of Atmospheric Environment
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    • v.9 no.1
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    • pp.91-99
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    • 2015
  • The Multi-wavelength Raman LIDAR (MRL) system was developed to enable a better understanding of the complex properties of aerosols in the atmosphere. In this study, the microphysical, optical, and radiative properties of mixed aerosols were retrieved using the discrete aerosol observation products from the MRL. The dust mixing ratio, which is the proportion of dust particles to the total mixed, was derived using the particle depolarization ratio. It was employed in the retrieval of backscattering and extinction coefficient profiles for dust and non-dust particles. The vertical profiles of aerosol optical properties were then used as input parameters in the inversion algorithm for the retrieval of microphysical parameters including the effective radius, refractive index, and the single scattering albedo (SSA). Those products were successfully applied to an analysis of radiative flux using a radiative transfer model. The relationship between the MRL derived extinction and aerosol radiative forcing (ARF) in short-wavelength was assessed over Gwangju, Korea. The results clearly demonstrate that the MRL-derived extinction profiles are a good surrogate for use in the estimation of optical, microphysical, and radiative properties of aerosols. It is considered that the analytical results shown in this study can be used to provide a better understanding of air quality and the variation of local radiative effects due to aerosols.

The Measurement of the LIDAR Ratio by Using the Rotational Raman LIDAR

  • Choi, Sung-Chul;Baik, Sung-Hoon;Park, Seung-Kyu;Cha, Hyung-Ki;Song, Im-Kang;Kim, Duk-Hyeon
    • Journal of the Optical Society of Korea
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    • v.14 no.3
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    • pp.174-177
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    • 2010
  • The rotational Raman LIDAR technique has been used to accurately measure aerosol optical properties such as backscatter coefficient, extinction coefficient, and LIDAR ratio. In the case of the vibrational Raman technique, the ${\AA}$ngstr$\ddot{o}$om exponent, which has wavelength dependence on the particle properties, is assumed to obtain the extinction coefficient. However, this assumed ${\AA}$ngstr$\ddot{o}$m exponent can cause systematic errors in retrieving aerosol optical properties. In the case of the rotational Raman technique, the aerosol optical properties can be measured without any assumptions about the ${\AA}$ngstr$\ddot{o}$m exponent. In this paper, the LIDAR ratio was measured by using the rotational Raman LIDAR and vibrational Raman LIDAR in the troposphere. And, the LIDAR ratios measured by these two methods were compared.