• Current Optics and Photonics
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• v.1 no.4
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• pp.278-283
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• 2017

We theoretically study the dynamics of water tetramer in intense femtosecond laser pulses with different frequencies. The simulations are carried out by incorporating the molecular dynamics method non-adiabatically into the time-dependent local-density approximation (TDLDA-MD). Three typical scenarios of water tetramer including the normal vibration with enlarged OH bonds, free OH bonds breaking and the pure Coulomb explosion are presented by investigating the electronic and ionic dynamics. The result indicates that the ionization is enhanced and the corresponding fragmentation effect as well as the damping of the dipole moment are found more notably when increasing the laser frequency especially when the frequency falls in the resonant region of the absorption spectra. The study of the level depletion reveals that the ratio of the emission amount from different levels can be controlled by changing the laser frequency referring to the Keldysh parameter.

• Proceedings of the Korean Vacuum Society Conference
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• 2014.02a
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• pp.199.1-199.1
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• 2014

In nonlinear optics, the properties of nonlinear optical responses such as polarization and nonlinear analysis of the nonlinear surfaces were investigated using the jellium model by optical second harmonic generation. The nonlinear response of the Al metal surfaces were calculated using TDLDA. Band structure, lattice constant and bulk modulus of the Al metal were investigated. Effective potential and electron density were compared by changing different.