• 제목/요약/키워드: Nonlinear optical properties

검색결과 157건 처리시간 0.024초

Nonlinear Optical Properties and Photoluminescence of CuCl Nanocrystals Embedded in Silica Glass

  • 이민영
    • Bulletin of the Korean Chemical Society
    • /
    • 제16권2호
    • /
    • pp.126-129
    • /
    • 1995
  • Linear and nonlinear optical properties of CuCl nanocrystals in silica glass have been studied using low temperature absorption, degenerate four wave mixing (DFWM), and time-resolved photoluminescence spectroscopy. Assuming a spherical shape, effective radius of the CuCl quantum dots was estimated to be 2.5 nm, which is obtained from low temperature absorption data. The DFWM experiment was performed in 380-386 nm wavelength region, and the diffracted signal was measured as a function of wavelength with 1.0 nm interval. Time-resolved photoluminescence measurement was also carried out at 77 K to obtain the time response of CuCl nanocrystals. The experimental results on the large third order nonlinear optical of CuCl quantum dots are explained in terms of crystal size and oscillator strength of quantum spheres.

Dispersion and Nonlinear Properties of Elliptical Air Hole Photonic Crystal Fiber

  • Rao, MP Srinivasa;Singh, Vivek
    • Current Optics and Photonics
    • /
    • 제2권6호
    • /
    • pp.525-531
    • /
    • 2018
  • The effect of eccentricity on dispersion and nonlinear properties of a photonic crystal fiber having elliptical air holes is investigated using a fully vectorial effective index method. It is found that the effective refractive index increases with increase of eccentricity. The dependence of dispersion and nonlinear properties of the PCF on the eccentricity of the air hole is investigated. It is revealed that eccentricity of the air hole affects the zero dispersion wavelength. Further, the nonlinear properties such as mode field area, nonlinear coefficient and self phase modulation of the Photonic crystal fibers are analyzed. The mode field area increases and the nonlinear coefficient decreases with increase in eccentricity. The variation of the self phase modulation with elliptical air hole is also discussed.

Extraction of Distance Information with Nonlinear Correlation of Photon-Counting Integral Imaging

  • Yeom, Seokwon
    • Journal of the Optical Society of Korea
    • /
    • 제20권5호
    • /
    • pp.579-585
    • /
    • 2016
  • Integral imaging combined with photon-counting detection has been researched for three-dimensional information sensing under low-light-level conditions. This paper addresses the extraction of distance information with photon-counting integral imaging. The longitudinal distance to the object is obtained utilizing photon-counting elemental images. The pixel disparity is estimated by maximizing the nonlinear correlation of photocounts. The first- and second-order statistical properties of the nonlinear correlation are theoretically derived. In the experiments, these properties are verified by varying the mean number of photocounts in the scene. The average distance is compared to that from the intensity information, showing the robustness of the proposed system even at low photocounts.

Electro-optic Properties of a Guest-Host System Containing a Phenothiazine-based Chromophore: Effect of the Chromophore Density on the Macroscopic Optical Nonlinearity

  • Lee, Sang-Kyu;Cho, Min-Ju;Yoon, Hyuk;Lee, Seung-Hwan;Kim, Jae-Hong;Qing Zhang;Choi, Dong-Hoon
    • Macromolecular Research
    • /
    • 제12권5호
    • /
    • pp.484-489
    • /
    • 2004
  • We have prepared a phenothiazine-based nonlinear optical (NLO) chromophore that displays a fairly high microscopic nonlinearity through intramolecular charge transfer. The phenothiazine unit plays important roles of contributing its high electron donating ability and connecting the resonance pathway through a conjugative effect in the cyclized ring adjacent to the aromatic ring. Theoretical calculations and an absorption spectroscopic study provided useful information concerning the microscopic nonlinearity of the chromophores. We investigated the electro-optic (EO) properties of the guest-host systems in amorphous polycarbonate containing the synthesized chromophores at different concentrations under different poling temperatures. A real-time pole and probe method provided a much greater amount of information regarding how the EO properties can arise and how they can be optimized.

Far-field 위상 변조량 측정법을 이용한 광학매질의 비선형 특성 측정 (Measurement of the Nonlinear Optical Properties by use of the Far-Field Phase Modulation Method)

  • 김성훈;양준목;김용평;이영우;신동주;정영붕
    • 한국광학회지
    • /
    • 제9권3호
    • /
    • pp.168-174
    • /
    • 1998
  • 본 연구에서는 광학매질의 비선형 특징을 측정하기 위해, 자체집속현상을 이용하는 기존의 측정법과는 다르게, 매질을 통과한 광원의 위상섭동으로 인하여 far-field에 발생한 공간적 광장도 분포를 이용하는 far-field 위상 변조량 측정법을 사용하였다. 미선형 매질을 통과한 조사과의 위상 변화가 far-field 영역에서 나타나는 겅간적 위상 변조량을 실험적으로 측정아였고, 이를 전산시\ulcorner을 통하여 비교분석하였다. 파장 616nm, 펄스폭 106ps의 분포궤한 섹소레이저(DFDL)와 파장 308nm인 DFDL의 제2고조파를 조사광으로 사용하였고, 매질 $CS_2$$BaF_2$의 비선형 특성을 실험적으로 측정한후 이 값을 전산시늉값과 비교하였다. 이 실험에서 파장 616nm에 대해 $CS_2$$BaF_2$의 비선형 굴절률 $1.2{\times}10^{-11}$ esu와 $1.0{\times}10^{-13}$ esu를 각각 얻었고, 파장 308nm에 대해 $BaF_2$의 비선형 흡수계수 $5.0{\times}10^{-11}$cm/W를 얻었다. 이들 값은 지금까지 발표된 값들과 잘 일치한다.

  • PDF

졸-겔법에 의한 CdS 분산$SiO_2$ Glass 박막의 비선형광학특성

  • 문종수;강종봉;김경문
    • 한국세라믹학회지
    • /
    • 제33권12호
    • /
    • pp.1353-1364
    • /
    • 1996
  • Recently semiconductor doped glasses have attracted attention as nonlinear optical materials because of their large third order nonlinear optical properties. The transparent and homogeneous CdS-doped SiO2 glass thin films were obtained by the dip=coating process of the sol-gel method. Thin films were consisted of glasses containing CdS microcrystallites which were formed by dissolved Cd2+ and S2- ions in a SiO2 matrix solutions. A subsequent thermal treatment of this samples led the formation of colloidal agglomerates and finally of microcrystallites. The size of CdS microcrystallites was about 4 to 15 nm after thermal treatments at various heating conditions. From the optical absorption spectra of the CdS-doped SiO2 glass films it was found that the absorption edge was blue-shifted compared with that of the bulk CdS crystal(~2, 4 eV) and that the amount of energy shift was inversely proportional to the crystal size. And the band gap energy increased with the decrease in crystallite size indicating that the quantum size effects occured.

  • PDF