• Title/Summary/Keyword: Measurement of Radioactivity

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Optimization of $CO_2$ Direct Absorption Method for the Determination of Carbon-14 in Environmental Samples (환경시료중의 방사성탄소 측정을 위한 $CO_2$ 직접흡수법의 최적화 연구)

  • Cho, Soo-Young;Woo, Hyung-Joo;Chun, Sang-Ki
    • Journal of Radiation Protection and Research
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    • v.23 no.4
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    • pp.237-242
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    • 1998
  • The goal of this work was to optimize the liquid scintillation counting techniques for the determination of C-14 in environmental samples such as biological and air samples. Carbon-14 activities in most environmental samples were measured with direct $CO_2$ absorption method. The highest figure of merit was found through the variation of Carbosorb $E^{TM}$ and Permatluor $V^{TM}$ ratio, in the measurement windows. The best condition was 1:1 volume ratio. Average 2.35 g of $CO_2$ was reproducibly absorbed in the 20 ml mixture within 40 min. The counting efficiency determined by repeated analysis of NIST oxalic acid standard and the background count rate were measured to be $58.8{\pm}1.4%$ and $1.88{\pm}0.06\;cpm$, respectively in case of saturated solution. The correction curves of counting efficiency for partially saturated solutions and for saturated solutions with quenching were prepared, respectively. The overall uncertainty of the sample specific activity for near background levels was estimated to be about 7 % for 4 hours counting at 95 % confidence level. The long-term stability of samples has been checked for all the counting techniques over a two week periods, and no apparent change in counting efficiency and background level was found at that time.

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Absorbed Dose Measurement by the MIRD System in the $^{131}I$ Treated Thyroid Cancer Patients (갑상선 암 환자에서 $^{131}I$ 치료시 MIRD Schema에 의한 흡수선량의 평가)

  • Lim, Sang-Moo;Woo, Kwang-Sun;Chung, Wee-Sup;Hong, Sang-Woon;Kim, Jang-Hee;Kim, Ki-Sup
    • The Korean Journal of Nuclear Medicine
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    • v.29 no.1
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    • pp.54-60
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    • 1995
  • Medical Internal Radiation Dose(MIRD) schema was developed for calculating the absorbed dose from the administered radiopharmaceuticals. With the biological distribution data and the physical properties of the radionuclide we can estimate the absorbed dose by the MIRD schema. For the thyroid cancer patients received $^{131}I$ therapy, the absorbed dose to the bone marrow is the limiting factor to the administered dose, and the duration of admission is deter-mined by the retained activity in the whole body. To monitor the whole body radioactivity, we used Eberline Smart 200 system using ionization chamber as a detector. With the time activity curve of the whole body, total body residence time was obtained. From the ICRP publication 53, the residence times of the source organs, such as kidney, urinary bladder content and stomach, were used to calculate the absorbed doses of the target organs, such as stomach, red marrow, bladder wall and remaineder total body. In 8 thyroid cancer patients with 175 mci of $^{131}I$ administered orally, the mean absorbed dose in the bladder wall was 375.1, in the stomach 285.1, red marrow 25.4 and total body 22.4 rad respectively. For the monitoring of the large administered activity, this method seemed to be quite useful.

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A Study on the Measurement of the Relative Nuclear Reaction Cross-Section of the natW(p,xn)176Re Reaction using 100 MeV Proton (100 MeV 양성자를 이용한 natW(p,xn)176Re 핵반응의 상대 핵반응단면적 측정에 대한 연구)

  • Lee, Samyol
    • Journal of the Korean Society of Radiology
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    • v.15 no.2
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    • pp.257-263
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    • 2021
  • This study derives the relative cross-section for the natW(p,xn)176Re nuclear reaction by measuring the gamma rays generated from the nuclear reaction with natural tungsten using a 100 MeV linear accelerator of the Korea Multi-purpose Accelerator Complex in the Korea Atomic Energy Research Institute. In general, research on isotopes with a short half-life always shows a tendency that the intensity of radioactivity decreases rapidly within a short period of time, making it very difficult to measure itself. In particular, 176Re is one of the relatively short radionuclides with a half-life of 5.3 minutes. In this study, 109.08 keV gamma rays generated from the 176Re isotope having such a short half-life were measured using a high-purity Ge detector(HPGe detector). The obtained relative measurements were the results in the 8 to 14 MeV proton energy domain published by Richard G. in 1967, and the TENDL-2019 value, which was the result of A. J. Koning in 2019, which evaluated the nuclear reaction cross-section by calculation based on this comparative analysis was performed. The results of this study are expected to be usefully applied to the design of nuclear fusion reactor which is known as future energy sources, elements ratio for the nuclear synthesis of astrophysics.

Marinelli Beaker Measurement and Self Absorption Correction and Application for Various Environmental Samples in Monte Carlo Simulation (몬테카를로 시뮬레이션에서의 다양한 환경 샘플에 대한 Marinelli 비이커 측정 및 자기 흡수 보정과 적용)

  • Jang, Eun-Sung;Gim, Yang-Soo;Lee, Sun-Young
    • Journal of radiological science and technology
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    • v.40 no.4
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    • pp.605-611
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    • 2017
  • The structure of the actual detector was computed using the code of the PENELOPE. Using the standard mixed sources (450, 1,000 ml), compare the effectiveness of each energy according to various densities and height of the PENELOPE computer simulation, and calculate the effectiveness of the various environmental specimens and apply them to various environmental specimens to determine the lower limit. The values obtained by the obtained value were obtained by applying the obtained efficiency to the actual environmental specimens and obtaining the lower limit values. The density correction factor is 1.155 g of the density correction factor of $0.4g/cm^3$ (59.54keV), 1.153 (661 keV), $1.06g/cm^3$ 1.064 (1,836.04keV), 1.03, and 1.033. It was confirmed that the radioactivity concentration of environmental samples decreased as the amount of specimen was measured increases, and the MDA value decreased as time measured increases.

MDA Assessment of NaI(Tl), LaBr3(Ce), and CeBr3 Detectors for Freshly Deposited Radionuclides on the Soil (지표면 침적 방사성핵종에 대한 NaI(Tl), LaBr3(Ce) 및 CeBr3 검출기의 MDA 비교 평가)

  • Lee, Jun-Ho;Kim, Bong-Gi;Lee, Dong Myung;Byun, Jong-In
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.17 no.3
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    • pp.321-328
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    • 2019
  • The detection performances of the NaI(Tl), $LaBr_3$(Ce) and $CeBr_3$ scintillation detectors, which can be used to rapidly evaluate the major artificial radionuclides deposited on the soil surface in a nuclear accident or radiological emergency, were compared. Detection performance was assessed by calculating the minimum detectable activity (MDA). The detection efficiency of each detector for artificial radionuclides was semi-empirically determined using mathematical modelling and point-like sources having certified radioactivity. The background gamma-ray energy spectrum for MDA evaluation was obtained from relatively wide and flat grassland, and the MDA values of each detector for the major artificial radionuclides that could be released in nuclear accidents were calculated. As a result, the relative MDA values of each detector regarding surface deposition distribution at normal environmental radiation level were evaluated as high in the order of the NaI(Tl), $LaBr_3$(Ce), and $CeBr_3$ detectors. These results were compared based on each detector's intrinsic and measurement environment background, detection efficiency, and energy resolution for the gamma-ray energy region of the radionuclide of interest.

Separation for the Determination of $^{59/63}Ni$ in Radioactive Wastes (방사성 폐기물 내 $^{59/63}Ni$ 정량을 위한 분리)

  • Lee, Chang-Heon;Jung, Kie-Chul;Choi, Kwang-Soon;Jee, Kwang-Young;Kim, Won-Ho
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.3 no.4
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    • pp.309-317
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    • 2005
  • A study on the separation of $^{99}Tc,\;^{94}Nb,\;^{55}Fe,\;^{90}Sr\;and\;^{59/63}Ni$ in various radioactive wastes discharged from nuclear power plants has been performed for a use in their quantification which is indispensible for the evaluation of the radionuclide inventory Ni was recovered along with Ca, Mg, Al, Cr, Ti, Mn, Ce, Na, K, and Cu through the sequential separation procedure of Re(as a surrogate of $^{99}Tc$), Nb, Fe and Sr by anion exchange and Sr-Spec extraction chromatography. In this research, chemical separation of Ni from the co-existing elements was investigated by cation exchange and Ni-Spec extraction chromatography. Precipitation behaviour of Ni and the co-existing elements with dimethylglyoxime(DMG) was investigated in ammonium $citrate/ethanol-H_2O$ and tartaric $acid/acetone-H_2O$ in order to purify separated Ni fractions and to prepare $^{59/63}Ni$ source for the radioactivity measurement using a gas proportional counter. Recovery of Ni separated through ion exchange chromatographic separation procedure was $92.1\%$ with relative standard deviation of $0.9\%$. In addition, recovery of Ni with DMG in the tartaric $acid/acetone-H_2O$ was $85.6\%$ with relative standard deviation of $1.9\%$.

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Quality Control of Dose Calibrator using 3D Printery (3D 프린터를 이용한 Dose Calibrator의 품질관리)

  • Ryu, Chan-Ju
    • Journal of the Korean Society of Radiology
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    • v.15 no.3
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    • pp.307-312
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    • 2021
  • In nuclear medicine, radioactive isotope tracers are administered to the human body to obtain and evaluate disease morphological information and biological function information. Dose calibrator is a device used to measure the radioactivity of a single nuclide in medical institutions. Administration of the correct dose to the human body acts as an important factor in diagnosis and treatment, and measurement through a dose calibrator before administration is the most important factor. Dose calibrator performs daily quality control after installation in each medical institution. Quality control is a means of guaranteeing quality control after installation, and is essential for improving the quality of treatment and promoting patient safety. Therefore, accurate and standardized performance evaluation methods should be established. In this study, 3D printing was used for quantitative evaluation of quality control by increasing the accuracy and standardization of quality control. When the 3D printer was installed and reproducibility was tested, the error range of the expected value and reading value decreased by 0.302% in the F-18 nuclide and 0.09% in the 99mTc-pertechnate nuclide than when the 3D printer was installed. The error rate for other nuclides was also found to have a low error rate for reproducibility tests when 3D printing was installed.

Research on Measurement Condition Establishment of a Liquid Scintillation Counter System (액체섬광계수기 장비의 계측조건 확립에 관한 연구)

  • Park, Eung-Seop;Han, Sang-Jun;Lee, Seung-Jin;Kim, Hee-Gang;Lee, Na-Young;Mun, Ji-Yeon
    • Journal of Radiation Protection and Research
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    • v.31 no.3
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    • pp.155-164
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    • 2006
  • It is judged that there could be certainty in every process of analyzing environmental samples using Liquid Scintillation Counter. Therefore, this study focuses on quantitative evaluation on uncertainty in an effort to analyze comparatively accurately environmental samples. For this, after parameters which can have an effect on uncertainty was derived, the evaluation on each parameter was tamed out. The results of analysis of each parameter showed that the effect according to the weight difference of Teflon vial did not appear, and that standard deviations of SQP(E) averages reached saturation point at $75{\sim}90$ sec at the result of making increases step by step the irradiation time of External standard, and that values measured by repeat method produces good results compared with replicate. Also, conclusion was derived that analysis on sample after it is left in cold and dark room at least above 1,000 minutes have to be carried out, and the result of carrying out verification on results measured as well as equipment itself using radioactivity-error-analysis and chi-square test, resonable result was derived.

Photostimulated Luminescence-Thermoluminescence Application to Detection of Irradiated White Ginseng Powder (방사선 조사 백삼분말의 PSL-TL 다중검지법)

  • Chung, Hyung-Wook;Delincee, Henry;Kwon, Joong-Ho
    • Korean Journal of Food Science and Technology
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    • v.32 no.2
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    • pp.265-270
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    • 2000
  • White ginseng powder, permitted to be irradiated in Korea for the purpose of microbial decontamination, was treated with electron beam at doses of $0{\sim}15\;kGy$ for a detection trial whether it is irradiated or not by measuring photostimulated luminescence for whole samples first and then (TL) for the mineral adhering to the samples. PSL values were less than threshold value (700, $T_{1}$) and were negative for nonirradiated samples but more than 5000 $(T_2)$ and were positive for irradiated ones. After PSL measurement mineral was separated from the whole samples using density separation. Mineral of nonirradiated samples was characterized by glow curves which have low intensity and were situated at the high temperature region (about $300^{\circ}C$) by the low level of natural radioactivity. Glow curves of minerals for all irradiated samples were observed at about $200^{\circ}C$. TL ratio by normalization was 0.01 for nonirradiated sample and more than 0.78 for irradiated samples, and it was possible to detect whether white ginseng powders were irradiated or not.

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Preparation of polymeric composites for surface contamination measurement in order to characterize nuclear facilities decommissioning (원자력시설 해체 시 특성평가를 위한 표면오염 탐지 이중구조 고분자 복합체의 제조)

  • 한명진;서범경;우주희;이근우
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2004.06a
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    • pp.97-104
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    • 2004
  • Double-layered polysulfone composite films, containing cerium activated yttrium silicate (CAYS) as a flour, were prepared from double casting of two polymeric solutions, and their morphology and physical strength were superior to those of single-layered composites. The prepared polymeric films consist of a dense bottom layer and a CAYS-holding top layer. The former is made of coagulating the polysulfone and methylene chloride binary solution and works as a supporter to improve the composite's physical strength, while the latter holding the inorganic fluor plays a role as an active site to detect the radioactive contamination. The prepared films revealed two distinguished, but tightly attached, double layers, their attachment being identified by morphology of the interface between two layers. As prepared by water immersion coagulation, the films have highly developed macropores, compared with a dense structure in the film prepared by evaporation. In the radionuclide detection test of the CAYS-impregnated composites, the films have reliable detection capacity at a radionuclide spotting test. The double-layered composites with the dense support layer show a better stability in holding the radionuclides spotted on the surface as well as an improvement in physical strength, compared with the single-layer composites having shortcomings such as being too porous or being brittle.

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