• Title/Summary/Keyword: Gamma emitting nuclides

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Comparative Measurement of Radioactivity with Standard Gamma-ray Ionization Chamber System (표준 감마선 전리함 장치에 의한 방사능 비교 측정)

  • Park, Tae-Soon;Woo, Dong-Ho;Oh, Pil-Jae;Hwang, Sun-Tae
    • Journal of Radiation Protection and Research
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    • v.9 no.1
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    • pp.11-18
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    • 1984
  • A Standard gamma-ray ionization chamber system was developed with a well type ionization chamber and micro current measuring circuit. Micro current was measured by the automatic Townsend balance with stepwise compensation method. For gamma emitting nuclides such as $^{241}Am,\;^{133}Ba,\;^{60}Co,\;^{134}Cs,\;^{137}Cs,\;and\;^{22}Na$ relative calibration factors to $^{226}Ra$ reference source were calculated and detection .efficiency curve was determined as a fudnction of gamma energy.

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Improvement of internal exposure assessments of the inhalation of fuel-type hot particles during long-term outages

  • Moonhyung Cho;Hyeongjin Kim
    • Nuclear Engineering and Technology
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    • v.56 no.9
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    • pp.3925-3932
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    • 2024
  • During outages at nuclear power plants, much more care for radiation workers against internal exposure should be ensured given that more hot particles exist relative to the amount during normal operation. If fuel-type hot particles (FTHP) are inhaled, they can cause more severe health risks compared to activation-type hot particles (ATHP), which contain 60Co, due to the alpha-emitting nuclides within FTHPs. The activities of difficult-to-measure nuclides within FTHPs inhaled by workers are inferred by the age-dating technique using a141Ce/144Ce ratio as measured by whole-body counters. However, this method may be limited to outages that last for only a few months due to the short half-life (32.5 days) of 141Ce. We studied the feasibility of utilizing 241Am, a nuclide with a long half-life of 432.6 years, as an alternative to 141Ce. Additionally, we improved the performance of a stand-type whole-body counter for low-energy gamma spectroscopy to meet the criterion (RMSE ≤0.25) specified in ANSI/HPS N13.30-2011 by employing an artificial neural network (ANN). This study can contribute to more rapid and accurate internal dose assessments for workers who have inhaled FTHPs during long-term outages at nuclear power plants.

ANALYSIS OF RADIOACTIVE IMPURITIES IN ALUMINA AND SILICA USED FOR ELECTRONIC MATERIALS

  • Lee Kil-Yong;Yoon Yoon-Yeol;Cho Soo-Young;Kim Yong-Je;Chung Yong-Sam
    • Nuclear Engineering and Technology
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    • v.38 no.5
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    • pp.423-426
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    • 2006
  • A developed neutron activation analysis(NAA) and gamma-spectrometry were applied to improve the analytical sensitivity and precision of impurities in electronic-circuit raw materials. It is well known that soft errors in high precision electronic circuits can be induced by alpha particles emitted from naturally occurring radioactive impurities such as U and Th. As electronic circuits have recently become smaller in dimension and higher in density, these alpha-particle emitting radioactive impurities must be strictly controlled. Therefore, new NAA methods have been established using a HTS(Hydraulic Transfer System) irradiation facility and a background reduction method. For eliminating or stabilizing fluctuated background caused by Rn-222 and its progeny nuclides in air, a nitrogen purging system is used. Using the developed NAA and gamma-spectrometry, ultra trace amounts of U(0.1ng/g) and Th(0.01ng/g) in an alumina ball and high purity silica used for an epoxy molding compound (EMC) could be determined.

SYNTHESIS OF SILICA-COATED Au WITH Ag, Co, Cu, AND Ir BIMETALLIC RADIOISOTOPE NANOPARTICLE RADIOTRACERS

  • Jung, Jin-Hyuck;Jung, Sung-Hee;Kim, Sang-Ho;Choi, Seong-Ho
    • Nuclear Engineering and Technology
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    • v.44 no.8
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    • pp.971-976
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    • 2012
  • Silica-coated Au with Ag, Co, Cu, and Ir bimetallic radioisotope nanoparticles were synthesized by neutron irradiation, after coating $SiO_2$ onto the bimetallic particles by the sol-gel St$\ddot{o}$ber process. Bimetallic nanoparticles were synthesized by irradiating aqueous bimetallic ions at room temperature. Their shell and core diameters were recorded by TEM to be 100 - 112 nm and 20 - 50 nm, respectively. The bimetallic radioisotope nanoparticles' gamma spectra showed that they each contained two gamma-emitting nuclides. The nanoparticles could be used as radiotracers in petrochemical and refinery processes that involve temperatures that would decompose conventional organic radioactive labels.

Analysis of Gamma Radionuclides in K-MILK Certified Milk (K-MILK 인증 우유의 감마핵종 분석)

  • Hee-Jin Jang;Hyo-Jin Kim;Yong-Uk Kye;Ji Eun Lee;Dong-Yeon Lee;Yeong-Rok Kang
    • Journal of the Korean Society of Radiology
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    • v.18 no.6
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    • pp.595-603
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    • 2024
  • After the Fukushima nuclear accident, interest in radioactive intake through food has increased significantly. Radioactivity is colorless, tasteless, and odorless, making it very difficult to determine whether it is contaminated, and it is important to check the radioactive safety of food as it can lead to long-term exposure during intake and absorption. In particular, children have more active metabolic activities than adults, so the risk of absorption after intake is judged to be high, so stricter acceptance standards are applied. Nevertheless, there is not little anxiety about radioactive contamination. Therefore, this study aims to confirm radioactive safety by analyzing gamma nuclides of milk with the highest intake in infancy in all ages based on 2021 national nutrition statistics. Samples were selected from 10 domestic milk types made of 100% domestic raw materials through K-MILK certification. Sample analysis was conducted according to the radioactive test method of 'Standards and Specifications for Food'. As a result of the analysis, all 10 types of milk nuclides 131I, 134Cs, 137Cs were determined to be less than MDA(Minimum Detectable Activity) and were not detected. Therefore, it is judged that there is no contamination of 131I, 134Cs, and 137Cs nuclides in milk made from domestic raw materials, and when the annual intake dose of milk was conservatively evaluated using the measured MDA value, the radioactive safety of domestic milk was confirmed at 0.001% of the annual effective dose limit.

An Intercomparison of Counting Efficiency and the Performance of Two Whole-Body Counters According to the Type of Phantom

  • Pak, Minjung;Yoo, Jaeryong;Ha, Wi-Ho;Jin, Young-Woo
    • Journal of Radiation Protection and Research
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    • v.41 no.3
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    • pp.274-281
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    • 2016
  • Background: Whole-body counters are widely used to evaluate internal contamination of the internal presence of gamma-emitting radionuclides. In internal dosimetry, it is a basic requirement that quality control procedures be applied to verify the reliability of the measured results. The implementation of intercomparison programs plays an important role in quality control, and the accuracy of the calibration and the reliability of the results should be verified through intercomparison. In this study, we evaluated the reliability of 2 whole-body counting systems using 2 calibration methods. Materials and Methods: In this study, 2 whole-body counters were calibrated using a reference male bottle manikin absorption (BOMAB) phantom and a Radiation Management Corporation (RMC-II) phantom. The reliability of the whole-body counting systems was evaluated by performing an intercomparison with International Atomic Energy Agencyto assess counting efficiency according to the type of the phantom. Results and Discussion: In the analysis of counting efficiency using the BOMAB phantom, the performance criteria of the counters were satisfied. The relative bias of activity for all radionuclides was -0.16 to 0.01 in the Fastscan and -0.01 to 0.03 in the Accuscan. However, when counting efficiency was analyzed using the RMC- II phantom, the relative bias of $^{241}Am$ activity was -0.49 in the Fastscan and 0.55 in the Accuscan, indicating that its performance criteria was not satisfactory. Conclusion: The intercomparison process demonstrated the reliability of whole-body counting systems calibrated with a BOMAB phantom. However, when the RMC-II phantom was used, the accuracy of measurements decreased for low-energy nuclides. Therefore, it appears that the RMC-II phantom should only be used for efficiency calibration for high-energy nuclides. Moreover, a novel phantom capable of matching the efficiency of the BOMAB phantom in low-energy nuclides should be developed.

Study on the Measurement of Radon concentrations in soil samples using γ-spectrometer (γ-spectrometer를 이용한 토양시료의 라돈농도 측정법에 관한 연구)

  • Kang, Sunga;Lee, Sangsoo;Choi, Guirack;Lee, Junhaeng
    • Journal of the Korean Society of Radiology
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    • v.7 no.1
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    • pp.31-36
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    • 2013
  • The radioactive gas radon ($^{222}Rn$), which is generated from the decay process of uranium ($^{238}U$) originating from the soil of more than 85 percent higher the porosity of the soil, the soil can radiate out the possibility that many isotopes. In order to protect the human body from radon, above all, the development of accurate measurement techniques to formulate appropriate measures should be followed. This study Gamma-ray spectrometry using a high purity germanium (HPGe) detector, if you want to measure radon unstable the nature radiation of the background problems can be reduced, radium and radon daughter nuclides after radioactive equilibrium leads to Radon concentration was measured, the soil samples from the Gamma-ray emitting nuclides, and the energy spectrum is analyzed.

The Prediction Methods of Iodine-129 release rate : Model Development

  • Park, Jin-Beak;Lee, Kun-Jai;Kang, Duck-Won;Shin, Sang-Woon;Park, Kyung-Rok
    • Proceedings of the Korean Nuclear Society Conference
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    • 1995.05a
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    • pp.879-884
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    • 1995
  • The results of performance assessment analyses have shown that the long-lived radionuclides such as I-129 control the potential individual dose impact to the public. I-129 is difficult-to-measure(DTM) in low-level waste because it is non-gamma emitting radionuclides and exists at extremely low concentrations in radioactive waste generated by nuclear reactors. In this study, computer modeling technique to predict release rate of I-129 is developed to provide another tools far performance assessment of land disposal facilities and characteristics of radwaste. Model suggested in this study will give conservative values of I-129 release rate far determination of radwaste characteristics. More detailed approach is implemented to account for release conditions of fuel source-nuclides. 1-131 concentration measured from reactor coolant and released fraction from tramp fuel have dominant roles in calculating release rate of I-129 with fuel defect conditions.

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Source and LVis based coincidence summing correction in HPGe gamma-ray spectrometry

  • Lee, Jieun;Kim, HyoJin;Kye, Yong Uk;Lee, Dong Yeon;Kim, Jeung Kee;Jo, Wol Soon;Kang, Yeong-Rok
    • Nuclear Engineering and Technology
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    • v.54 no.5
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    • pp.1754-1759
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    • 2022
  • The activity of gamma-ray emitting nuclides is calculated assuming that each gamma-ray is detected individually; thus, the magnitude of the coincidence summing signal must be considered during activity calculations. Here, the correction factor for the coincidence summing effect was calculated, and the detection efficiencies of two HPGe detectors were compared. The CANBERRA Inc. GC4018 high-purity Ge detector provided an estimate for the peak-to-total ratio using a point source to determine the coincidence summing correction factor. The ORTEC Inc. GEM60 high-purity Ge detector uses EFFTRAN in LVis to obtain the parameters of the detector and source model and the gamma-gamma and gamma-X match estimates, in order to determine the coincidence summing correction factor. Nuclide analyses, radioactivity comparisons, and analyses of reference material samples were performed utilizing certified reference materials to accurately determine the detection efficiencies. For both Co-60 and Y-88, the detection efficiency for a point source increased by an average of at least 12-13%, whereas the detection efficiency determined using LVis increased by an average of at least 13-15%. The calculated radioactivity values of the certified reference material and reference material samples were accurate to within 3% and 6% of the measured values, respectively.

Optimal Monitoring Intervals and MDA Requirements for Routine Individual Monitoring of Occupational Intakes Based on the ICRP OIR

  • Ha, Wi-Ho;Kwon, Tae-Eun;Jin, Young Woo
    • Journal of Radiation Protection and Research
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    • v.45 no.2
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    • pp.88-94
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    • 2020
  • Background: The International Commission on Radiological Protection (ICRP) has recently published report series on the occupational intakes of radionuclides (OIR) for internal dosimetry of radiation workers. In this study, the optimized monitoring program including the monitoring interval and the minimum detectable activity (MDA) of major radionuclides was suggested to perform the routine individual monitoring of internal exposure based on the ICRP OIR. Materials and Methods: The derived recording levels and the critical monitoring quantities were reviewed from international standards or guidelines by the International Atomic Energy Agency (IAEA), the International Organization for Standardization (ISO), and the European Radiation Dosimetry Group (EURADOS). The OIR data viewer provided by ICRP was used to evaluate the monitoring intervals and the MDA, which are derived from the reference bioassay functions and the dose coefficients. Results and Discussion: The optimal monitoring intervals were determined taking account of two requirement conditions on the potential intake underestimation and the MDA values. The MDA requirement values of the selected radionuclides were calculated based on the committed effective dose from 0.1 mSv to 5 mSv. The optimized routine individual monitoring program was suggested including the optimal monitoring intervals and the MDA requirements. The optimal MDA values were evaluated based on the committed effective dose of 0.1 mSv. However, the MDA can be adjusted considering the practical operation of the routine individual monitoring program in the nuclear facilities. Conclusion: The monitoring intervals and the MDA as crucial factors for the routine monitoring were described to suggest the optimized routine individual monitoring program of the occupational intakes. Further study on the alpha/beta-emitting radionuclides as well as short lived gamma-emitting nuclides will be necessary in the future.