• 한국방사성폐기물학회:학술대회논문집
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• 한국방사성폐기물학회 2018년도 추계학술논문요약집
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• pp.379-379
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• 2018

MXenes are a new family of 2D transition metal carbide nanosheets analogous to graphene (Lv et al., 2017; Sun et al., 2018). Due to the easy availability, hydrophilic behavior, and tunable chemistry of MXenes, their use in applications for environmental pollution remediation such as heavy metal adsorption has recently been explored (Li et al., 2017). In this study, three-dimensional (3D) MXene ($Ti_3C_2T_x$) films with high adsorption capacity, good mechanical strength, and high selectivity for specific radionuclide from aquose solution were successfully fabricated by a polymeric precursor method using vacuum-assisted filtration. The highest removal efficiency on the films was 99.54%, 95.61%, and 82.79% for $Sr^{2+}$, $Co^{2+}$, and $Cs^+$, respectively, using a film dosage of 0.06 g/ L in the initial radionuclide solution (each radionuclide concentration = 1 mg/L and pH = 7.0). Especially, the adsorption process reached an equilibrium within 30 min. The expanded interlayer spacing of $Ti_3C_2T_x$ sheets in MXene films showed excellent radionuclide selectivity ($Cs^+$ and/or $Sr^{2+}/Co^{2+}$) (Simon, 2017). Besides, the MXene films was not only able to be easily retrieved from an aqueous solution by filtration after decontamination processes, but also to selectively separate desired target radionuclides in the solutions. Therefore, the newly developed MXene ($Ti_3C_2T_x$) films has a great potential for radionuclide removal from aqueous solution.

• 대한자원환경지질학회:학술대회논문집
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• 대한자원환경지질학회 1999년도 춘계 공동학술발표회
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• pp.4-4
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• 1999

• 한국환경과학회지
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• 제27권6호
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• pp.425-436
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• 2018

To establish initial response scenarios for nuclear accidents around the Kori nuclear power plants, the potential for radionuclide diffusion was estimated using numerical experiments and statistical techniques. This study used the numerical model WRF (Weather Research and Forecasting) and FLEXPART (Flexible Particle dispersion model) to calculate the three-dimensional wind field and radionuclide dispersion, respectively. The wind patterns observed at Gijang, near the plants, and at meteorological sites in Busan, were reproduced and applied to estimates of seasonally averaged wind fields. The distribution of emitted radionuclides are strongly associated with characteristics of topography and synoptic wind patterns over nuclear power plants. Since the terrain around the power plants is complex, estimates of radionuclide distribution often produce unexpected results when wind data from different sites are used in statistical calculations. It is highly probable that in the summer and autumn, radionuclides move south-west, towards the downtown metropolitan area. This study has clear limitations in that it uses the seasonal wind field rather than the daily wind field.

• Nuclear Engineering and Technology
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• 제54권3호
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• pp.1003-1015
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• 2022

The new methodologies to derive discharge limits considering operational flexibility according to international safety standards were developed to help reduce the environmental releases of radioactive effluents from nuclear power plants (NPPs). To overcome the limitations of the two existing methods to set up discharge limits assuming a specific statistical distribution of the effluent discharge, two modified equations were newly proposed to directly derive a particular discharge limits corresponding to the target 'compliance probability' based on the actual annual discharge data for a specific NPP and radionuclide groups. By applying these to the actual yearly discharge data of 14 Korean NPPs for 7 radionuclide groups for the past 20 years, the applicability of two new methodologies to actual cases was demonstrated. The 'characteristic value' with approximately a 90% compliance probability for each Korean NPP and radionuclide group was proposed based on the results. The new approaches for setting up the discharge limits and the characteristic values developed in this study are expected to be effectively utilized to foster operator's efforts to progressively reduce the environmental releases of radioactive effluents of NPPs relative to the previous discharge data considering operational flexibilities.

• Nuclear Engineering and Technology
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• 제50권8호
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• pp.1355-1363
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• 2018

Many radionuclides exist in normal environment and artificial radionuclides also can be detected. The radionuclides ($^{131}I$) are widely used for labeling compounds and radiation therapy. In Korea, the radionuclide ($^{131}I$) is produced at the Radioisotope Production Facility (RIPF) at the Korea Atomic Energy Research Institute in Daejeon. The residents around the RIPF assume that $^{131}I$ detected in environmental samples is produced from RIPF. To ensure the safety of the residents, the radioactive concentration of $^{131}I$ near the RIPF was investigated by monitoring environmental samples along the Gap River. The selected geographical places are near the nuclear installation, another possible location for $^{131}I$ detection, and downstream of the Gap River. The first selected places are the "front gate of KAERI", and the "Donghwa bridge". The second selected place is the sewage treatment plant. Therefore, the Wonchon bridge is selected for the upstream of the plant and the sewage treatment plant is selected for the downstream of the plant. The last selected places are the downstream where the two paths converged, which is Yongshin bridge (in front of the cogeneration plant). In these places, environmental samples, including sediment, fish, surface water, and aquatic plants, were collected. In this study, the radioactive iodine ($^{131}I$) detection along the Gap River will be investigated.

• 해양환경안전학회지
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• 제27권5호
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• pp.618-629
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• 2021

2011년 동일본대지진에 의해 발생한 후쿠시마 원자력 발전소 사고와 최근 국내 지진 발생 빈도의 증가는 원자력 발전소의 지진 안전성에 대한 불안감을 야기하였다. 더불어 최근(2021년) 일본 동경전력은 후쿠시마 원전 오염수의 태평양 방류를 결정하였으며, 이로 인해 국내외 수산물을 통한 방사능 오염 가능성이 높아지면서 국민들의 우려가 급증하고 있다. 후쿠시마 원전사고 이후 해양으로의 인공방사능 유입에 관한 연구는 국제적으로 많이 이루어졌으나, 한국인의 주요 식재료인 동아시아 연근해의 수산물에서 인공방사능의 분포 현황 및 축적에 대한 연구는 상대적으로 부족한 실정이다. 따라서 이 논문에서는 후쿠시마 원전사고 이후, 국내산 수산물에서의 원전 기원 인공방사능(예, ¹³⁷Cs, ^239+240Pu, ⁹⁰Sr 등)의 분포 특성과 관련한 최근 연구 사례들을 소개하고자 한다. 또한, 후쿠시마 원전오염수의 방류와 더불어 2030년까지 계획된 중국의 신규 원전 시설로 인한 향후 한반도 주변해역의 방사능 유출 영향에 대한 대비 및 사전 연구가 필요한 시점이기에 향후 연구 방향들을 제안하고자 한다.

• Nuclear Engineering and Technology
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• 제52권6호
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• pp.1289-1296
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• 2020

The estimation of radioactivity level is vital for population health risk assessment and geological point of view and can be evaluated as rate of exhalation and source concentration (²²⁶Ra, ²³²Th and ⁴⁰K). The present study deals with the soil samples for investigation of radionuclides content and exhalation rates of radon -thoron gas from different sites in northern Haryana, India. Absorbed dose and associated index estimated in the present study are the measures of environmental radioactivity to inhalation dose. Effective doses received by different tissues and organs by considering different occupancy and conditions are also measured. Exhalation rates of radon and thoron are measured with active scintillation monitors based on alpha spectroscopy namely scintillation radon (SRM) and thoron (STM) monitors respectively. Sample height was optimized before measurement of thoron exhalation rate using STM. Average values of radon and thoron exhalation are found 16.6 ± 0.7 mBqkg^-1h^-1 and 132.1 ± 2.6 mBqm^-2s^-1 respectively. Also, a simple approach was also adopted, to evaluate the thoron exhalation which accomplished a lot of challenges, the results are compared with the data obtained experimentally. The study is useful in the nationwide mapping of radon and thoron exhalation rates for understanding the environmental radioactivity status.

• Nuclear Engineering and Technology
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• 제53권3호
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• pp.960-966
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• 2021

A technical approach to design and carry out an experiment to determine the uptake of selected radionuclides in site-specific conditions in Kuwait was developed and successfully executed for developing a radioecological decision support system. The radionuclides from soil-to-plant transfer factors have been obtained for leafy and non-leafy vegetables, and root crops cultivated in Kuwait. Two types of vegetated soils were selected and spiked with high concentrations of three relatively short-lived selected radionuclides (⁸⁵Sr, ¹³⁴Cs, and ¹³³Ba). The highest strontium and barium transfer factors were found in the order: leafy vegetables > root crops > non-leafy vegetables. The approximate range of radiocesium transfer factor was found to be low in all plant groups and was comparable to those reported elsewhere in different soil types of temperate and tropical environments. A strong negative correlation between the obtained transfer factors and the distribution coefficient of the radionuclide in soil was found. It is recommended to adopt the newly derived parameters for the sensitive areas in Kuwait and other Gulf countries instead of using the generic parameters, whenever dose calculation codes are used. This will help to more accurately assess and predict the end results of the committed effective dose equivalent through ingestion pathway.

• 한국환경농학회지
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• 제16권4호
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• pp.304-310
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• 1997

오이의 파종 2일전 및 파종후 네 차례에 걸쳐 Mn-54, Co-60, Sr-85, Cs-137의 혼합용액을 온실내 재배상자의 토양에 처리하고 처리시기별 및 수확시기별 열매에 대한 전이계수($m^2$/㎏-fresh)를 측정하였다. 전이계수는 핵종, 처리시기 및 수확시기에 따라 최고 약 60배의 변이를 보였다. 처리시기에 따른 전이계수의 변화양상은 핵종간 및 수확시기간에 차이가 있었다. 핵종간에 전이계수는 대체로 Sr-85 > Mn-54 > Co-60 > Cs-137의 순이었다. 파종전 토양과의 혼합처리시 전이계수는 생육초기 토양표면 처리에 비해 Mn-54, Co-60, Cs-137의 경우 다소 높았으나 Sr-85의 경우 차이가 없었다. 생육초기 토양표면에 처리된 방사성 핵종의 토양층위별 농도는 재배종료후 토양 깊이에 따라 지수함수적으로 감소하고 처리량의 $80{\sim}99%$가 토심 3cm 이내에 분포하는 것으로 나타났다.핵종의 토양 침투성은 Sr-85 > Mn-54 > Co-60 > Cs-137의 순이었다. 본 연구결과는 오이의 재배기간중 토양의 방사능 오염시 열매내 방사성 핵종의 농도예측, 오이의 수확,소비 및 오이밭 제염 대책수립에 활용될 수 있다.

• Asian Pacific Journal of Cancer Prevention
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• 제15권1호
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• pp.375-380
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• 2014

This study examined the incidence rates of cancer cases (averages for 2006-2010) and relationships with environmental radioactivity levels. Soil and water samples were collected from provincial and district centers of Van city and the outdoor gamma doses were determined using a portable gamma scintillation detector. Gross alpha and beta, (226)Ra, (232)Th, and (40)K activities were measured in both tap water and soil samples. Although high rates of stomach and esophagus cancers have been reported previously in Van the underlying reasons have not hitherto been defined. Incidences of cancers were highest in the Gurpmar (326.0) and Ozalp (377.1) counties (p<0.001). As to the results of the gross alpha and gross beta radioactivity measurements in the drinking water, these two counties also had high beta radionuclide levels: Gurpmar ($140mBq/dm^3$) and Ozalp ($206mBq/dm^3$). Even if within the normal range, a relation between the higher rate of the incidence of stomach and esophagus cancers with that of the higher rate of beta radionuclide activity was clear. On Spearman correlation analysis, the relation between higher beta radionuclide levels and cancer incidence was found to be statistically significant (p<0.01). According to the results of the analysis, Van residents receive an average 1.86 mSv/y annual dose from outdoor gamma radiation, ingestion of radionuclides in the drinking water, and indoor $^{222}Rn$ activity. Moreover, gross alpha and beta activities were found to be extremely high in all of the lakes around the city of Van, Turkey. Further investigations with long-term detailed environmental radiation measurements are needed regarding the relationship between cancer cases and environmental radioactivity in the city of Van.