• Journal of Korean Society for Atmospheric Environment
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• v.22 no.2
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• pp.235-247
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• 2006

Aerosol indirect radiative forcing of climate change is considered the most uncertain forcing of climate change over the industrial period, despite numerous studies demonstrating such modification of cloud properties and several studies quantifying resulting changes in shortwave radiative fluxes. Detection of this effect is made difficult by the large inherent variability in cloud liquid water path (LWP): the dominant controlling influence of LWP on optical depth and albedo masks any aerosol influences. Here we have used ground-based remote sensing of cloud optical depth (${\tau}_c$) by narrowband radiometry and LWP by microwave radiometry to determine the dependence of optical depth on LWP, thereby permitting examination of aerosol influence. The method is limited to complete overcast conditions with liquid-phase single layer clouds, as determined mainly by millimeter wave cloud radar. The results demonstrate substantial (factor of 2) day-to-day variation in cloud drop effective radius at the ARM Southern Great Plains site that is weakly associated with variation in aerosol loading as characterized by light-scattering coefficient at the surface. The substantial scatter suggests the importance of meteorological influences on cloud drop size as well, which should be analyzed in the further intensive studies. Meanwhile, it is notable that the decrease in cloud drop effective radius results in marked increase in cloud albedo.

• Journal of Korean Society for Atmospheric Environment
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• v.12 no.4
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• pp.389-398
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• 1996

In order to understand the relative importance of various pathways leading to the production and transformation of aerosols under different atmospheric conditions, the behavior of atmospheric aerosols have been investigated using a high volume tape sample in Seoul for a week period during August 1990. The concentrations of anion $(SO^{2-}_4, NO^-_3, CI^-)$ and cation $(Ca^{2+}, Na^+, NH^+_4)$ species of aerosol samples were analyzed to identify the ionic composition of aerosols and to estimate their relative contributions to aerosol formation. The concentrations of aerosol species were calculated by a multiple regression model. The results of our calculations indicate the existence of various chemical species such as $(NH_4)_2SO_4, Na_2SO_4, CaSO_4, NH_4NO_3, NaNO_3, Ca(NO_3)_2, NH_4Cl$, and NaCl salts. According to our calculations, the most dominant species of aerosol was $(NH_4)_2SO_4$ with the mean concentration of 23.3 $/mu g/m^3$ (66.9%). The proportion of different componts with aerosol (e.g., $NH_4NO_3$ and $NH_4Cl$) was strongly affected by temperature, relative humidity, and partial presure of gases.

• Asian Journal of Atmospheric Environment
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• v.12 no.3
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• pp.193-203
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• 2018

The operational aerosol retrieval algorithm for the Moderate Resolution Imaging Spectroradiometer (MODIS) measurements was recently updated and named collection 6 (C6). The C6 MODIS aerosol algorithm, a substantially improved version of the collection 5 (C5) algorithm, uses an enhanced aerosol optical thickness(AOT) retrieval process consisting of new surface reflection and aerosol models. This study reports on the estimation and validation of the two latest versions, the C5 and C6 MODIS aerosol products over the East Asian region covering $20^{\circ}N$ to $56^{\circ}N$ and $80^{\circ}E$ to $150^{\circ}E$. This study also presents a comparative validation of the two versions(C5 and C6) of algorithms with different methods(Dark Target(DT) and Deep Blue (DB) retrieval methods) from the Terra and Aqua platforms to make use of the Aerosol Robotic Network (AERONET) sites for the years 2000-2016. Over the study region, the spatially averaged annual mean AOT retrieved from C6 AOT is about 0.035 (5%) less than the C5 counterparts. The linear correlations between MODIS and AERONET AOT are R = 0.89 (slope = 0.86) for C5 and R = 0.95 (slope = 1.00) for C6. Moreover, the magnitude of the mean error in C6 AOT-the difference between MODIS AOT and AERONET AOT-is 40% less than that in C5 AOT.

• Journal of Korean Society for Atmospheric Environment
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• v.15 no.1
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• pp.1-11
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• 1999

In this work, a theoretical model has been formulated which allows the study of the scavenging efficiencies of aerosol particles by the rain drops. Aerosol particles are scavenged by the simultaneous brownian diffusion, interception and inertial impaction force. In addition the calculations based on the collision efficiency model are carried out for the collision of aerosol particles with diameter range 0.01~30 $mu extrm{m}$ and rain drops with diameter 0.02$\times$$2^{n/3}$(n=1, 2, …, 17)cm. The results indicate that: (1) the below-cloud scavenging affects mainly the coarse particles (＞3 ${\mu}{\textrm}{m}$), the fine particles remaining almost unchanged; (2) the scavenging efficiencies by below-cloud in the heavy rain (rain intensity, 10 mm/hr) surpass the efficiency found in the drizzle rain (rain intensity, 1 mm/hr).

• Proceedings of the Korean Environmental Sciences Society Conference
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• 2019.10a
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• pp.87-87
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• 2019

• Journal of Korean Society for Atmospheric Environment
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• v.16 no.2
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• pp.113-120
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• 2000

Effects of sea-salts on the properties of aerosol collected in a coastal region were studied by applying a gas-particle equilibrium model SCAPE to the measurement data from Korea Cheju Island in summer 1994. It was found that the observed higher ammonium concentrations in fine particles (PM2.5) than in TSP were caused by forced evaporation of ammonium in coarse fraction of aerosol by sea-salts and the degree of evaporation was quantified through an application of SCAPE. By subtracting the sea-salt fraction from the measured concentra-tions the changes of aerosol property were also studied. The concentrations of nitrate at both TSP and PM2.5 decreased when alkaline sea-salt fraction was removed from the measured data. Estimates of aerosol acidity increased for most samples with sea salt loadings, However in some cases with high mass fractions of sea-salt components the aerosol acidity of PM2.5 decreased slightly. This is though to be related with the formation of solid salt with the removal of sea-salts.

• Journal of Korean Society for Atmospheric Environment
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• v.16 no.1
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• pp.1-10
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• 2000

The behavior of aerosos due to gravitational coagulation was studied experimentally and numerically. In experimental study, the geometric mean particel size increased as time elapsed in a vertical tube column, while the size decreased when the tube was set horizontally. The particle size distribution was observed to maintain the lognormal form during the coagulation process. Separately, numerical calculations were performed for studying the aerosol behavior under gravitational and Brownian coagulation using the moment method. By comparing the expeimented results with the numerical predictions, the governing mechanism of the aerosol behavior proved to be gravitational coagulation.

• Journal of Korean Society for Atmospheric Environment
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• v.19 no.2
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• pp.191-204
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• 2003

A one dimensional time dependent acid rain model considering size distribution of aerosols and hydrometeors is developed to predict observed chemical and physical properties of precipitation. Temporal variations of anions and cations observed are predicted fairly well with acid rain model simulations. It is found that aerosol depletion rates are highly dependent on aerosol sizes under the assumption of Marshall - Palmer raindrop size distribution. Also, the aerosol depletion during the initial rain event largely influences on ion concentrations in rainwaters.

• Journal of Environmental Science International
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• v.18 no.7
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• pp.721-733
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• 2009

To examine the fluctuations of aerosol number concentration with different size in the boundary layer of marine area during summer season, aerosol particles were assayed in the Ieodo Ocean Research Station, which is located 419 km southwest of Marado, the southernmost island of Korea, from 24 June to 4 July, 2008. The Laser Particle Counter (LPC) was used to measure the size of aerosol particles and NCEP/NCAR reanalysis data and sounding data were used to analyze the synoptic condition. The distribution of aerosol number concentration had a large variation from bigger particles more than 3 ${\mu}m$ in diameter to smaller particles more than 1 ${\mu}m$ in diameter with wind direction during precipitation. The aerosol number concentration decreased with increasing temperature. An increase (decrease) of small size of aerosol (0.3${\sim}$0.5 ${\mu}m$ in diameter) number concentration was induced by convergence (divergence) of the wind fields. The aerosol number concentration of bigger size more than 3 ${\mu}m$ in diameter after precipitation was removed as much as 89${\sim}$94% compared with aerosol number concentration before precipitation. It is considered that the larger aerosol particles would be more efficient for scavenging at marine boundary layer. In addition, the aerosol number concentration with divergence and convergence could be related with the occurrence and mechanism of aerosol in marine boundary layer.

• Journal of Korean Society for Atmospheric Environment
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• v.34 no.5
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• pp.668-676
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• 2018

This study has developed a technique to divide the aerosol optical depth of the entire aerosol (${\tau}_{total}$) into the dust optical depth (${\tau}_D$) and the pollution particle optical depth (${\tau}_P$) using the AERONET sun/sky radiometer data provided in Version 3. This method was applied to the analysis of AERONET data observed from 2006 to 2016 in Beijing, China, Seoul and Gosan, Korea and Osaka, Japan and the aerosol optical depth trends of different types of atmospheric aerosols in Northeast Asia were analyzed. The annual variation of ${\tau}_{total}$ showed a tendency to decrease except for Seoul where observation data were limited. However, ${\tau}_D$ tended to decrease when ${\tau}_{total}$ were separated as ${\tau}_D$ and ${\tau}_P$, but ${\tau}_P$ tended to increase except for Osaka. This is because the concentration of airborne aerosols, represented by Asian dust in Northeast Asia, is decreased in both mass concentration and optical concentration. However, even though the mass concentration of pollution particles generated by human activity tends to decrease, Which means that the optical concentration represented as aerosol optical depth is increasing in Northeast Asia.