• Title/Summary/Keyword: Aerosol size distribution

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Development of Aerosol Model Using Moment Method and Validation by Experiments (모멘트 방법을 이용한 에어로즐 모델의 개발과 실험을 통한 검증)

  • Kim Gyeong-A;Kim Dae-Seong;Park Seong-Hun;Gwon Sun-Park;Lee Gyu-Won
    • Proceedings of the Korea Air Pollution Research Association Conference
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    • 2002.11a
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    • pp.385-386
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    • 2002
  • Many important physical properties of natural or man-made aerosol particles such as light scattering, electrostatics charges, and toxicity, as well as their behavior involving physical processes like diffusion and thermophoresis depend strongly on their size distribution. Important aerosol behavior mechanisms affecting the size distribution of aerosol particles include condensation, deposition, and coagulation. (omitted)

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Formation and Hygroscopic Growth Properties of Ultrafine Particles in College Station, Texas, in 2003 (2003년 미국 텍사스 칼리지스테이션에서 관측된 초미세입자의 형성과 흡습 성장 특성)

  • Lee, Yong-Seob;Collins, Don R.
    • Journal of Environmental Science International
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    • v.16 no.7
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    • pp.793-798
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    • 2007
  • During May of 2003, smoke from fires in the Yucatan Peninsula was transported across the Gulf of Mexico and into Texas where it caused significant enhancement in measured aerosol concentrations and reduced visibility. During this event, the formation and growth of aerosol particles has been observed by a differential mobility analyzer (DMA) / tandem differential mobility analyzer (TDMA) system to characterize the size distribution and size-resolved hygroscopicity of the aerosol. The most number concentration is by the particles smaller than 100 nm, but the integrated number concentrations for over 100 nm increased due to the aerosol growth. Hygroscopic growth factor increase from 1.2 to 1.4 for 25, 50, and 100 nm particles during the nucleating period. This distribution and the aerosol properties derived from the TDMA data were used to calculate the growth rate. Particle growth rates were in the range 1-12 nm/hr.

Aerosol Size Distributions and Optical Properties during Severe Asian Dust Episodes Measured over South Korea in Spring of 2009-2010 (2009-2010년 봄철 심한 황사 사례에 대한 에어러솔 크기 분포와 광학적 특성)

  • Kang, Dong-Hun;Kim, Jiyoung;Kim, Kyung-Eak;Lim, Byung-Sook
    • Atmosphere
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    • v.22 no.3
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    • pp.367-379
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    • 2012
  • Measurements of $PM_{10}$ mass concentration, aerosol light scattering and absorption coefficients as well as aerosol size distribution were made to characterize the aerosol physical and optical properties at the two Korean WMO/GAW regional stations, Anmyeondo and Gosan. Episodic cases of the severe Asian dust events occurred in spring of 2009-2010 were studied. Results in this study show that the aerosol size distributions and optical properties at both stations are closely associated with the dust source regions and the transport routes. According to the comparison of the $PM_{10}$ mass concentration at both stations, the aerosol concentrations at Anmyeondo are not always higher than those at Gosan although the distance from the dust source region to Anmyeondo is closer than that of Gosan. The result shows that the aerosol concentrations depend on the transport routes of the dust-containing airmass. The range of mass scattering efficiencies at Anmyeon and Gosan was 0.50~1.45 and $0.62{\sim}1.51m^2g^{-1}$, respectively. The mass scattering efficiencies are comparable to those of the previous studies by Clarke et al. (2004) and Lee (2009). It is noted that anthropogenic fine particles scatter more effectively the sunlight than coarse dust particles. Finally, we found that the aerosol size distribution and optical properties at Anmyeondo and Gosan show somewhat different properties although the samples for the same dust_episodic events are compared.

Development and Performance Evaluation of Radial Exhaust Multi-port System for Real-time Particle Size Distribution Measurement (실시간 입자분포 측정을 위한 Radial Exhaust Multi-port System의 개발 및 성능평가)

  • Lee, Hong Ku;Lee, Yang-Woo;Jeon, Ki Soo;Ahn, Kang-Ho
    • Particle and aerosol research
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    • v.9 no.3
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    • pp.133-137
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    • 2013
  • Measuring particle size distribution is one of the primary concerns in aerosol studies. For a nano-particle size distribution measurement, many scientists use a combination of a differential mobility analyzer (DMA) and a condensation particle counter (CPC) system, which is a called scanning mobility particle sizer (SMPS). Although it has a very high particle size resolution, some issues still remain. These problems include residence time between a DMA and a CPC, discontinuity of a CPC, and disturbance due to long scanning time during the precise measurement of particles. In particular, long scanning time is not adequate for measuring particle size distribution since the particle concentration is changing during the measurement. In this study, we developed radial exhaust multi-port system (REM-system) with no scanning time and high resolution to measure real-time particle size distribution. As a result of the REM-system performed using mono-disperse particle, it is expected that this system will be suitable for measuring continuously changing aerosol. If the counting efficiency of multi-condensation particle counter (M-CPC) and data inversion matrix are completed, REM-system will be a very adequate system for unsteady aerosol, which changes for SMPS scanning time.

Characteristics of Aerosol Size Distribution from OPC Measurement in Seoul, 2001 (OPC(광학적 입자 계수기)로 측정한 2001년 서울지역 에어로졸의 입경 분포)

  • 정창훈;전영신;최병철
    • Journal of Korean Society for Atmospheric Environment
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    • v.19 no.5
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    • pp.515-528
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    • 2003
  • The characteristics of one year observation aerosol data in Seoul, 200 I was studied using an OPC (Optical Particle Counter). The size resolved aerosol number concentrations of 0.3 ∼ 25 11m were measured. The results were compared with PM$_{10}$ mass concentration data under various meteorological conditions including dust and precipitation events. For fine particles whose diameter is less than 2.23 ${\mu}{\textrm}{m}$, the number concentration increases in the early morning which is considered due to transportation. while the coarse mode particles increase during daytime. This increase can be explained as local sources and human activities near sampling site. Hourly averaged data show that there exists diurnal variation. Generally, PM$_{10}$ data showed a similar tendency with OPC data. The size resolved OPC data showed that the particles of 0.5 ∼ 3.67 ${\mu}{\textrm}{m}$ are positively correlated with PM$_{10}$ data. The accumulated volume fraction of size resolved aerosol concentration in 0.5 ∼ 10 ${\mu}{\textrm}{m}$ showed that 0.5 ∼ 2.23 ${\mu}{\textrm}{m}$ particles occupied 59.2% of total aerosol volume of 0.5 ∼ 10 ${\mu}{\textrm}{m}$./TEX>.

Major factors determining the size distributions of atmospheric water-soluble aerosol particles at an urban site during winter (겨울철 도시지역 대기 수용성 에어로졸 입자의 크기 분포를 결정하는 주요 인자)

  • Park, Seungshik
    • Particle and aerosol research
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    • v.17 no.3
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    • pp.43-54
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    • 2021
  • Size distributions of atmospheric particulate matter (PM) and its water-soluble organic and inorganic components were measured between January and February 2021 at an urban site in Gwangju in order to identify the major factors that determine their size distributions. Their size distributions during the study period were mainly divided into two groups. In the first group, PM, NO3-, SO42-, NH4+ and water-soluble organic carbon (WSOC) exhibited bi-modal size distributions with a dominant condensation mode at a particle size of 0.32 ㎛. This group was dominated by local production of secondary water-soluble components under atmospheric stagnation and low relative humidity (RH) conditions, rather than long-range transportation of aerosol particles from China. On the other hand, in the second group, they showed tri-modal size distributions with a very pronounced droplet mode at a diameter of 1.0 ㎛. These size distributions were attributable to the local generation and accumulation of secondary aerosol particles under atmospheric conditions such as atmospheric stagnation and high RH, and an increase in the influx of atmospheric aerosol particles by long-distance transportation abroad. Contributions of droplet mode NO3-, SO42-, NH4+ and WSOC to fine particles in the second group were significantly higher than those in the first group period. However, their condensation mode contributions were about two-fold higher in the first group than in the second group. The significant difference in the size distribution of the accumulation mode of the WSOC and secondary ionic components between the two groups was due to the influx of aerosol particles with a long residence time by long-distance transport from China and local weather conditions (e.g., RH).

A Study of Size Distribution of Sulfate and Nitrate in Urban Air (都市大氣中 黃酸鹽과 窒酸鹽 關한 硏究)

  • 신상은;김승학;김희강
    • Journal of Korean Society for Atmospheric Environment
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    • v.2 no.1
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    • pp.33-39
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    • 1986
  • Particulate matter was collected by Andersen Air Sampler in the Seoul area during February-October, 1985, in order to investigate size distribution of sulfate and nitrate in aerosol, and conversion of sulfur dioxide to sulfate and that of nitrogen dioxide to nitrate. The size distribution of sulfate and nitrate had fine mode. The ratio of fine sulfate to total sulfate in aerosol and that of fine nitrate to total nitrate showed between 54.6% and 86%, and 55.7% and 95%, respectively, which presumably originated from gaseous reaction of sulfur dioxide and nitrogen dioxide in the atmosphere.

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Continuous Measurements of Size Separated Atmospheric Aerosol Number Concentration in Background Area (대기배경지역 에어로졸의 입경별 수농도 연속 측정)

  • Kang, Chang-Hee;Hu, Chul-Goo
    • Journal of Environmental Science International
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    • v.21 no.4
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    • pp.535-543
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    • 2012
  • The aerosol number concentration have measured with an aerodynamic particle sizer spectrometer(APS) at Gosan site, which is known as background area in Korea, from January to September 2011. The temporal variation and the size distribution of aerosol number concentration have been investigated. The entire averaged aerosol number concentration in the size range 0.25~32.0 ${\mu}m$ is about 252 particles/$cm^3$. The number concentration in small size ranges(${\leq}0.5{\mu}m$) are very higher than those in large size ranges, such as, the number concentration in range of larger than 6.5 ${\mu}m$ are almost zero particles/$cm^3$. The contributions of the number concentration to PM10 and/or PM2.5 are about 34%, 20.1% and 20.4% in the size range 0.25~0.28 ${\mu}m$, 0.28~0.30 ${\mu}m$ and 0.30~0.35 ${\mu}m$, respectively, however, the contributions are below 1% in range of larger than 0.58 ${\mu}m$. The monthly variations in the number concentration in smaller size range(<1.0 ${\mu}m$) are evidently different from the variations in range of larger than 1.0 ${\mu}m$, but the variations are appeared similar patterns in smaller size range(<1.0 ${\mu}m$), also the variations in range of larger than 1.0 ${\mu}m$ are similar too. The diurnal variations in the number concentration for smaller particle(<1.0 ${\mu}m$) are not much, but the variations for larger particle are very evident. Size-fractioned aerosol number concentrations are dramatically decreased with increased particle size. The monthly differences in the size-fractioned number concentrations for smaller size range(<0.7 ${\mu}m$) are not observed, however, the remarkable monthly differences are observed for larger size than 0.7 ${\mu}m$.

Aerosol Size Distribution and Composition at Kosan, Cheju Island : Measurements in April 1998 (제주도 고산에서의 에어로솔 입경분포별 조성: 1998년 4월 측정 연구)

  • 김용표;배귀남;지준호;진현철;문길주
    • Journal of Korean Society for Atmospheric Environment
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    • v.15 no.5
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    • pp.677-685
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    • 1999
  • Aerosol mass size distributions were measured at Kosan, Cheju Island in April 1998 and their compositions were analyzed. Microorifice Uniform Deposit Impactor(MOUDI) was used to collect aerosols. Sulfate and ammonium ions were predominatly present at fine mode of the aerosols while nitrate, chloride, and metal ions were mostly at coarse mode. Based on the size distribution of nitrate, it is suggested that most nitrate were from gas to particle conversion on coarse particles. Non-sea salt(nss) fraction of sulfate accounted for more than 90% of total sulfate mass concentration. In general, ion concentrations in this study are lower than those measured at the same site from the previous studies. Ion balance and chloride ion levels indicates that there had been anthropogenic chloride emission sources near to the site during the measurements.

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Physical, Chemical and Optical Properties of Fine Aerosol as a Function of Relative Humidity at Gosan, Korea during ABC-EAREX 2005

  • Moon, Kwang-Joo;Han, Jin-Seok;Cho, Seog-Yeon
    • Asian Journal of Atmospheric Environment
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    • v.7 no.3
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    • pp.129-138
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    • 2013
  • The water uptake by fine aerosol in the atmosphere has been investigated at Gosan, Korea during ABC-EAREX 2005. The concentration of inorganic ion and carbon components, size distribution, and light scattering coefficients in normal and dry conditions were simultaneously measured for $PM_{2.5}$ by using a parallel integrated monitoring system. The result of this study shows that ambient fine particles collected at Gosan were dominated by water-soluble ionic species (35%) and carbonaceous materials (18%). In addition, it shows the large growth of aerosol in the droplet mode when RH is higher than 70%. Size distribution of the particulate surface area in a wider size range ($0.07-17{\mu}m$) shows that the elevation of RH make ambient aerosol grow to be the droplet mode one around $0.6{\mu}m$ or the coarse mode one, larger than $2.5{\mu}m$. Hygroscopic factor data calculated from the ratio of aerosol scattering coefficients at a given ambient RH and a reference RH (25%) show that water uptake began at the intermediate RH range, from 40% to 60%, with the average hygroscopic factor of 1.10 for 40% RH, 1.11 for 50% RH, and 1.17 for 60% RH, respectively. Finally, average chemical composition and the corresponding growth curves were analyzed in order to investigate the relationship between carbonaceous material fraction and hygroscopicity. As a result, the aerosol growth curve shows that inorganic salts such as sulphate and nitrate as well as carbonaceous materials including OC largely contribute to the aerosol water uptake.