• Title/Summary/Keyword: Aerosol distributions

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Characteristic of Size-Resolved Water-Soluble Organic Carbon in Atmospheric Aerosol Particles Observed during Daytime and Nighttime in an Urban Area (도시지역 낮.밤 대기에어로졸의 입경 별 수용성 유기탄소의 특성)

  • Park, Seung Shik;Shin, Dong Myung
    • Particle and aerosol research
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    • v.9 no.1
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    • pp.7-21
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    • 2013
  • Twelve-hour size-resolved atmospheric aerosols were measured to determine size distributions of water-soluble organic carbon(WSOC) during daytime and nighttime, and to investigate sources and formation pathways of WSOC in individual particle size classes. Mass, WSOC, ${NO_3}^-$, $K^+$, and $Cl^-$ at day and night showed mostly bimodal size distributions, peaking at the size range of $0.32-0.55{\mu}m$(condensation mode) and $3.1-6.2{\mu}m$(coarse mode), respectively, with a predominant condensation mode and a minor coarse mode. While ${NH_4}^+$ and ${SO_4}^{2-}$ showed unimodal size distributions which peaked between 0.32 and $0.55{\mu}m$. WSOC was enriched into nuclei mode particles(< $0.1{\mu}m$) based on the WSOC-to-mass and WSOC-to-water soluble species ratios. The sources and formation mechanisms of WSOC were inferred in reference to the size distribution characteristics of inorganic species(${SO_4}^{2-}$, ${NO_3}^-$, $K^+$, $Ca^{2+}$, $Na^+$, and $Cl^-$) and carbon monoxide. Nuclei mode WSOC was likely associated with primary combustion sources during daytime and nighttime. Among significant sources contributing to the condensation mode WSOC were homogeneous gas-phase oxidation of VOCs, primary combustion emissions, and fresh(or slightly aged) biomass burning aerosols. The droplet mode WSOC could be attributed to aqueous oxidation of VOCs in clouds, cloud-processed biomass burning aerosols, and small contributions from primary combustion sources. From the correlations between WSOC and soil-related particles, and between WSOC and sea-salt particles, it is suggested that the coarse mode WSOC during daytime is likely to condense on the soil-related particles($K^+$ and $Ca^{2+}$), while the WSOC in the coarse fraction during nighttime is likely associated with the sea-salt particles($Na^+$).

12-year LIDAR Observations of Tropospheric Aerosol over Hefei (31.9°N, 117.2°E), China

  • Wu, Decheng;Zhou, Jun;Liu, Dong;Wang, Zhenzhu;Zhong, Zhiqing;Xie, Chenbo;Qi, Fudi;Fan, Aiyuan;Wang, Yingjian
    • Journal of the Optical Society of Korea
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    • v.15 no.1
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    • pp.90-95
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    • 2011
  • 12-year LIDAR observations of tropospheric aerosol vertical distribution using a Mie scattering LIDAR in Hefei ($31.9^{\circ}N$, $117.2^{\circ}E$) from 1998 to 2009 are presented and analyzed in this paper. Characters of temporal variation and vertical distribution of tropospheric aerosol over Hefei are summarized from the LIDAR measurements. The impacts of natural source and human activities on the aerosol vertical distribution over Hefei could be seen clearly. Dust particles from the north in spring could affect the aerosol distributions below about 12 km over Hefei, and aerosol scale height in April reaches $2.29{\pm}0.68\;km$. Both LIDAR measurements and surface visibility imply that aerosols in the lower troposphere have been increasing since about 2005.

A study on Characteristics of the Liquid Atomization by Ultrasonic (초음파에 의한 액체 미립화 특성에 관한 연구)

  • 주은선;나우정;최우창
    • Transactions of the Korean Society of Automotive Engineers
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    • v.7 no.5
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    • pp.31-39
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    • 1999
  • A good atomization in uniform size brings the elevation of thermal efficiency in spray combustion, the beautiful painting on surfaces, and the economical sprinkling of chemicals. Ultrasonic atomization has been expected as a good uniform atomization mechanism due to its uniform size distribution. Influx, load, and physical properties of liquids are the effecting factors to atomize liquids. In this study, distilled water and city water are selected as reference liquids and gasoline, kerosene, and petroleum as fuel liquids. Characteristics and affinity to get the maximum effect for the ultrasonic atomization are observed by using the two ultrasonic transducers with 28kHz and 2MHz. Results show that the size distributions of liquid spray dorplet by the direct vibration method prevail over those by the aerosol method in uniform droplet size and as a whole, sizes of spray liquid droplets are increased slightly according to increasing influx in the direct vibration method and quantities of spray droplets in the aerosol method decreasing according to increasing liquid load h.

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Aerosol Size Distribution and Composition at Kosan, Cheju Island : Measurements in April 1998 (제주도 고산에서의 에어로솔 입경분포별 조성: 1998년 4월 측정 연구)

  • 김용표;배귀남;지준호;진현철;문길주
    • Journal of Korean Society for Atmospheric Environment
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    • v.15 no.5
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    • pp.677-685
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    • 1999
  • Aerosol mass size distributions were measured at Kosan, Cheju Island in April 1998 and their compositions were analyzed. Microorifice Uniform Deposit Impactor(MOUDI) was used to collect aerosols. Sulfate and ammonium ions were predominatly present at fine mode of the aerosols while nitrate, chloride, and metal ions were mostly at coarse mode. Based on the size distribution of nitrate, it is suggested that most nitrate were from gas to particle conversion on coarse particles. Non-sea salt(nss) fraction of sulfate accounted for more than 90% of total sulfate mass concentration. In general, ion concentrations in this study are lower than those measured at the same site from the previous studies. Ion balance and chloride ion levels indicates that there had been anthropogenic chloride emission sources near to the site during the measurements.

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Mass Size Distribution of Atmospheric Aerosol Particles Collected at 865 m High of Jirisan National Park (지리산 국립공원 해발 865 m 지점에서 대기에어로졸입자의 입경별 질량농도 특성)

  • Ryu, Hye-Ji;Park, Jeong-Ho
    • Journal of Environmental Science International
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    • v.26 no.1
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    • pp.29-36
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    • 2017
  • Aerosol mass size distributions were investigated at 865 m high the of Jirisan national park. A nanosampler cascade impactor was used to collect aerosols. The atmospheric aerosol particles had a unimodal mass size distribution, which peaked at $0.5-1.0{\mu}m$, and a mass aerodynamic diameter of $1.13{\mu}m$. The annual average concentrations of TSP, $PM_{10}$, $PM_{2.5}$, $PM_1$, $PM_{0.5}$ and $PM_{0.1}$ were $20.9{\mu}g/m^3$, $19.3{\mu}g/m^3$, $14.9{\mu}g/m^3$, $10.7{\mu}g/m^3$, $5.3{\mu}g/m^3$, $1.2{\mu}g/m^3$, respectively. TSP concentrations were below $30{\mu}g/m^3$ during the sampling period. On average $PM_{10}$, $PM_{2.5}$, $PM_1$, $PM_{0.5}$ and $PM_{0.1}$ made up 0.91, 0.70, 0.41, 0.19 and 0.07 of TSP, respectively. The annual average of PM2.5/PM10 ratio was 0.77.

Preliminary analyses on decontamination factors during pool scrubbing with bubble size distributions obtained from EPRI experiments

  • Lee, Yoonhee;Cho, Yong Jin;Ryu, Inchul
    • Nuclear Engineering and Technology
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    • v.53 no.2
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    • pp.509-521
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    • 2021
  • In this paper, from a review of the size distribution of the bubbles during pool scrubbing obtained from experiments by EPRI, we apply the bubble size distributions to analyses on the decontamination factors of pool scrubbing via I-COSTA (In-Containment Source Term Analysis). We perform sensitivity studies of the bubble size on the various mechanisms of deposition of aerosol particles in pool scrubbing. We also perform sensitivity studies on the size distributions of the bubbles depending on the diameters at the nozzle exit, the molecular weights of non-condensable gases in the carrier gases, and the steam fractions of the carrier gases. We then perform analyses of LACE-ESPANA experiments and compare the numerical ~ results to those from SPARC-90 and experimental results in order to show the effect of the bubble size distributions.

Aerosol Observation with Raman LIDAR in Beijing, China

  • Xie, Chen-Bo;Zhou, Jun;Sugimoto, Nobuo;Wang, Zi-Fa
    • Journal of the Optical Society of Korea
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    • v.14 no.3
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    • pp.215-220
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    • 2010
  • Aerosol observation with Raman LIDAR in NIES (National Institute for Environmental Studies, Japan) LIDAR network was conducted from 17 April to 12 June 2008 over Beijing, China. The aerosol optical properties derived from Raman LIDAR were compared with the retrieved data from sun photometer and sky radiometer observations in the Aerosol Robotic Network (AERONET). The comparison provided the complete knowledge of aerosol optical and physical properties in Beijing, especially in pollution and Asian dust events. The averaged aerosol optical depth (AOD) at 675 nm was 0.81 and the Angstrom exponent between 440 nm and 675 nm was 0.99 during experiment. The LIDAR derived AOD at 532 nm in the planetary boundary layer (PBL) was 0.48, which implied that half of the total AOD was contributed by the aerosol in PBL. The corresponding averaged LIDAR ratio and total depolarization ratio (TDR) were 48.5sr and 8.1%. The negative correlation between LIDAR ratio and TDR indicated the LIDAR ratio decreased with aerosol size because of the high TDR associated with nonspherical and large aerosols. The typical volume size distribution of the aerosol clearly demonstrated that the coarse mode radius located near 3 ${\mu}m$ in dust case, a bi-mode with fine particle centered at 0.2 ${\mu}m$ and coarse particle at 2 ${\mu}m$ was the characteristic size distribution in the pollution and clean cases. The different size distributions of aerosol resulted in its different optical properties. The retrieved LIDAR ratio and TDR were 41.1sr and 19.5% for a dust event, 53.8sr and 6.6% for a pollution event as well as 57.3sr and 7.2% for a clean event. In conjunction with the observed surface wind field near the LIDAR site, most of the pollution aerosols were produced locally or transported from the southeast of Beijing, whereas the dust aerosols associated with the clean air mass were transported by the northwesterly or southwesterly winds.

Assessment of Long-Range Transport of Atmospheric Pollutants using a Trajectory Model with the puff Concept (퍼프 유적선모델에 의한 대기오염물질의 장거리수송량의 평가)

  • 정관영
    • Journal of Korean Society for Atmospheric Environment
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    • v.12 no.2
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    • pp.167-177
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    • 1996
  • To investigate the source-receptor relationships aerosol model has been used to simulate the distribution behavior of the yellow sand. Data for meteorological fields were obtained by Meso-scale Analysis and Prediction Model System/Seoul National University (MAPMS/SNU) for five days (10-14 April 1988). To obtain the distributions of concentration of yellow sand,the aerosol model has been modified to allow quantifications of relative concentration distributions of yellow sand. Source regions of yellow sand were delineated by soil maps of China and emission rate as a function of wind stress(Westphal et al., 1987). Using 3-dimensional wind fields the backward trajectories from 3 receptor grids at the layer of .sigma. =0.95, 0.9, 0.85, 0.8 were calculated. In order to facilitate quantitative assessment of source-receptor relationships, it was assumed that the perturbations in along-trajectory and cross-trajectory proceed linearly with time, in accord with Gaussian distribution characteristics. On the basis of this assumption, the probability fields were calculated from every grid point with source strength 1. Using these probability fields and emission retes, the potential contributions of upstream sources along the trajectories were estimated. The results of this study indicate that the application of trajectory modeling is useful in investigating the quantitative relationship between source and receptor regions.

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Characteristics of the dry deposition fluxes and ambient particl size distributions of PCBs: The measurements on fall, 1999 (입자상 PCBs 건식침적량과 입경분포 특성: 1999년 가을 측정)

  • Shin, Hye Jung;Kim, Yong Pyo;Yi, Seung Muk
    • Particle and aerosol research
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    • v.5 no.4
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    • pp.179-188
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    • 2009
  • The dry deposition fluxes of particulate polychlorinated biphenyls (PCBs) were measured along with their mass size distributions at Seoul and Incheon in fall in 1999. The dry deposition fluxes of PCBs were in the range of $16.7{\sim}62.2ng/m^2/day$. The ambient concentrations of particulate PCBs were in the range of 0.07 to $0.20ng/m^3$. Generally, the mass size distribution of particulate PCBs shows bi-modal distribution. The mass fraction of PCBs in the fine particle fraction ($D_p<2.1 {\mu}m$) was over than 55% of the total PCBs concentrations. It was found that Seoul and Incheon were not the major source of PCBs emissions in Korea. Based on the comparison with the measurement data in summer, 1999, it is likely that both the dry deposition fluxes and ambient particulate PCBs concentrations were not site-specific.

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An Analysis of Aerosol-Cloud Relationship Using MODIS and NCEP/NCAR Reanalysis Data around Korea (한반도 주변에서 MODIS와 NCEP/NCAR 재분석 자료를 이용한 에어로졸과 구름의 연관성 분석)

  • Kim, Yoo-Jun;Lee, Jin-Hwa;Kim, Byung-Gon
    • Journal of Korean Society for Atmospheric Environment
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    • v.27 no.2
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    • pp.152-167
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    • 2011
  • MODIS/Terra level 3 and NCEP/NCAR Reanalysis data from 2001 to 2008 have been analyzed to understand long-term aerosol and cloud optical properties, and their relationships around Korea. Interestingly, cloud fraction(CF) has the similar annual variation to aerosol optical depth (${\tau}_a$) without any temporal significant trend. Horizontal distributions of ${\tau}_a$ showed the substantial horizontal gradient from China to Korea, especially with the strong difference over the Yellow Sea, which could represent the evidence of the anthropogenic influence from China in the perspective of long-term average. Specifically the negative correlations between ${\tau}_a$ and liquid-phase cloud effective radius ($r_e$) were shown on the monthly-average basis, only in summer with significant associations over the Yellow Sea, but not in the other seasons and/or specific regions. Relationship between ${\tau}_a$ and CF for the low-level liquid-phase clouds exhibited the overall positive correlation, being consistent with cloud lifetime effect. Meanwhile static stability showed no deterministic relationships with ${\tau}_a$ as well as CF. The dependence of aerosol-cloud relationship on the meteorological conditions should be examined more in detail with the satellite remote sensing and reanalysis data.