• Proceedings of the Korea Water Resources Association Conference
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• 2022.05a
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• pp.383-383
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• 2022

기존 큰 지진을 대상으로 한 많은 연구결과들을 살펴보면, 큰 지진이 발생하기 전에 토양 속에 존재하는 다양한 인자들 중에 라돈(²²²Rn, 반감기=3.82일) 농도가 비정상적으로 증가하는 현상을 나타낸다. 이러한 결과들은 라돈발생의 경향성을 분석한다면, 지진발생에 대한 전조증상이나 예측이 가능함을 나타낸다. 본 연구에서는 포항지역을 중심으로 지진발생에 대한 전조증상이나 모니터링을 분석하기 위해 지하수 관측소에 설치된 라돈 관측기기에서 라돈 관측자료를 수집하고 이를 활용하는 연구를 수행하였다. 라돈 관측자료 기간은 2019년 11월부터 2020년 9월까지의 자료이며, 라돈인자 뿐만 아니라 지하수위, 강수량, 수온인자를 같이 분석하였으며, 동일기간 동안 발생한 진도 2 이상의 지진사례 6개(E1(M_L 3.5): 2019.12.30.; E2(M_L 3.2): 2020.01.30.; E3(M_L 2.4): 2020.02.09.; E4(M_L 2.7): 2020.02.16.; E5(M_L 2.8): 2020.05.27.; E6(M_L 2.1): 2020.09.22.)를 대상으로 하였다. 지진발생의 전조증상이 나타나는 지역을 분석하기 위해 Dobrovolsky radius values (Dobrovolsky et al., 1979)와 Harversine 관계식을 적용하였다. 적용결과, 시간적 분석에서 라돈의 증감 경향성이 지진발생의 전조증상과 유의미한 상관성이 있음을 확인하였으며, 공간적인 분석에서도 유의미하지는 않으나 상관성이 나타났다. 그 외 지하수위는 상관성이 어느 정도 나타났으나 강수량은 유의미한 결과를 나타내지는 않았다. 따라서 라돈을 활용한다면 지진발생의 전조증상을 시공간적으로 파악할 수 있음을 확인하였다.

• Economic and Environmental Geology
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• v.45 no.3
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• pp.277-294
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• 2012

The characteristics of temporal spacial radon variation in soil according to parent rock type and affecting factors were studied in Busan, Korea. The concentration of $^{222}Rn$ in soils and their parent elements ($^{226}Ra$,$^{228}Ra$, U and Th) in rocks and soils were measured at 24 sites in Busan area. The distribution and transportation behavior of these parent elements were analyzed and their correlations to radon concentration in soil were determined. Topographic effects were also evaluated. Two in-situ radon measurement (soil probe and buried tube) methods were applied to measure radon concentration in soil and their accuracies were evaluated. The spatial variation of radon in soil generally reflected U concentration in the parent rock. Average radon concentrations were higher in plutonic rocks than in volcanic rocks and were decreased in the order of felsic>intermediate>mafic rock. However, the radon concentrations were significantly varied in soils developed from same parent rocks due to the disequilibrium of U and $^{226}Ra$ between rock and soil. As results, the correlation of these element concentrations between rocks and soils was very low and radon concentrations in soils had highly co-related to the concentrations of these elements in soils. Th and $^{228}Ra$ show complex enrichment characteristics, differing significantly with U, in soils developed from same parent rock because the geochemical behavior of these elements during weathering and soil developing process was different with U. The radon concentrations in the same depth of soil in slope area were also different according to positions. The radon concentrations in soils developed from same parent rocks (19 sites at Pusan National University) varied 6.8~29.8Bq/L range because of small scale topographic variation. The opposite seasonal variation pattern of radon were observed according to soil properties. It was determined that buried tube method is more accurate method than soil probe method and was very advantageous application for the analysis for the characteristics of temporal spacial radon variation in soil.

• Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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• v.15 no.1
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• pp.35-44
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• 2017

A gamma-ray peak of $^{226}Ra$ (186.2 keV) overlaps with one of $^{235}U$ (185.7 keV) in a gamma-ray spectrometry system. Though reference peaks of $^{235}U$ can be used to correct the peak interference of $^{235}U$ in the analysis of $^{226}Ra$, this requires a complicated calculation process and a high limit of quantitation. On the other hand, evaluating $^{226}Ra$ using the correction constant in the overlapped peak can make a rapid measurement of $^{226}Ra$ without the complicated calculation process as well as overcome the disadvantage in the indirect measurement of $^{214}Bi$, which means the confinement of $^{222}Rn$ gas in a sample container and a time period to recover the secular equilibrium. About 93 samples with 6 species for raw-materials and by-products were prepared to evaluate the activity of $^{226}Ra$ using the correction constant. The results were compared with the activity of $^{214}Bi$, which means the indirect measurement of $^{226}Ra$, to validate the method of the direct measurement of $^{226}Ra$ using the correction constant. The difference between the direct and indirect measurement of $^{226}Ra$ was generally below about ${\pm}20%$. However, in the case of the phospho gypsum, a large error of about 50% was found in the comparison results, which indicates the disequilibrium between $^{238}U$ and $^{226}Ra$ in the materials. Application results of the contribution ratio of $^{226}Ra$ were below about ${\pm}10%$. The direct measurement of $^{226}Ra$ using the correction constant can be an effective method for its rapid measurement of raw materials and by-products because the activity of $^{226}Ra$ can be produced with a simple calculation without the consideration of the integrity of a sample container and the time period to recover the secular equilibrium.

• Journal of Radiation Protection and Research
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• v.33 no.4
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• pp.173-181
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• 2008

To ensure the performance of radon detectors, three passive radon detectors ($RadTrak^{(R)}$, $Radopot^{(R)}$, and $E-PERM^{(R)}$)have been reviewed. The difference ratios of RadTrak and Radopot tested in the radon standard chamber were -13.2% and -6.0%, respectively, which were in good accordance within 20% of the value measured by $AlphaGUARD^{(R)}$. To ensure the performance of the long term measurement, the 3 detectors were installed at the same position of approximately one hundred of dwellings for one year. The correlation curve between RadTrak and Radopot shows good agreement with a correlation coefficient ($R^2$) of 0.91. However, The correlation curve between E-PERM and Radopot shows bad agreement ($R^2$ = 0.021). In addition, the distribution map of annual mean indoor gamma dose rate measured with E-PERM was not in accordance with the distribution map of outdoor gamma dose rate measured by Portable Ion Chamber. According to the results, some requisites for the selection of the radon passive detectors in the large-scale indoor radon survey were discussed.

• Journal of the Korean Society of Radiology
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• v.5 no.5
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• pp.231-235
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• 2011

Radium is rock or soil of crust or uranium of building materials and thorium after radioactivity collapse process are created colorless and odorless inert gas that accrue well in sealed space like mine or basement. It inflow to lung circulate respiratory organ and caused lung cancer because of deposition of lung or bronchial tubes. Radium sheath of medical institution treat person's life is possible big danger to professional regarding radioactivity who has much amount exposed radioactivity and weaker immune patient. so we do this test. Using measuring instrument at test is real time radium measuring instrument, Professional Continuous Radon monitor, and measuring places are basement first floor and second floor of two hospitals and measure from 10 a.m to 3 p.m. Measurement result of Professional Continuous Radon monitor is minimum 14.8 Bq/$m^3$ to maximum 70.3 Bq/$m^3$ and show domestic baseline below 148 Bq/$m^3$, effective dose-rate is minimum 0.296 mSv to maximum 1.406 mSv that show 2.4 mSv, 10~58.3% level, exposed radiation amount from nature radiation one year.

• Analytical Science and Technology
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• v.29 no.2
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• pp.65-72
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• 2016

This study presented an analytical method for detecting radium in soils using a liquid scintillation counter (LSC). The isotope ²²⁶Ra was extracted from soil using the fusion method and then separated from interfering radionuclides using the precipitation method. Radium was coprecipitated as sulfate salts with barium (Ba) and then converted into Ba(Ra)CO₃, which is soluble in an acidic solution. The isotope ²²²Rn, the decay progeny of ²²⁶Ra, was trapped in a water immiscible cocktail and analyzed by LSC. The pulse shape analysis (PSA) level was estimated using ⁹⁰Sr and ²²⁶Ra standard solutions. The figure of merit was the highest at PSA 80, while the alpha spillover was the lowest at PSA 80. The counting efficiency was 243 ± 2% in a glass vial. This analytical method was verified with International Atomic Energy Agency (IAEA) reference materials, including IAEA-312, IAEA-314, and IAEA-315. The recovery ranged from 60–82%, while the relative bias between the measured value and the recommended value was less than 10%. The minimum detectable activity was 2.1 Bq kg⁻¹ with dry mass 1 g, the background count rate of 0.02 cpm, the recovery rate of 70% and counting time of 30 min.

• Asian Pacific Journal of Cancer Prevention
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• v.15 no.1
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• pp.375-380
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• 2014

This study examined the incidence rates of cancer cases (averages for 2006-2010) and relationships with environmental radioactivity levels. Soil and water samples were collected from provincial and district centers of Van city and the outdoor gamma doses were determined using a portable gamma scintillation detector. Gross alpha and beta, (226)Ra, (232)Th, and (40)K activities were measured in both tap water and soil samples. Although high rates of stomach and esophagus cancers have been reported previously in Van the underlying reasons have not hitherto been defined. Incidences of cancers were highest in the Gurpmar (326.0) and Ozalp (377.1) counties (p<0.001). As to the results of the gross alpha and gross beta radioactivity measurements in the drinking water, these two counties also had high beta radionuclide levels: Gurpmar ($140mBq/dm^3$) and Ozalp ($206mBq/dm^3$). Even if within the normal range, a relation between the higher rate of the incidence of stomach and esophagus cancers with that of the higher rate of beta radionuclide activity was clear. On Spearman correlation analysis, the relation between higher beta radionuclide levels and cancer incidence was found to be statistically significant (p<0.01). According to the results of the analysis, Van residents receive an average 1.86 mSv/y annual dose from outdoor gamma radiation, ingestion of radionuclides in the drinking water, and indoor $^{222}Rn$ activity. Moreover, gross alpha and beta activities were found to be extremely high in all of the lakes around the city of Van, Turkey. Further investigations with long-term detailed environmental radiation measurements are needed regarding the relationship between cancer cases and environmental radioactivity in the city of Van.

• Journal of Korean Society for Atmospheric Environment
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• v.29 no.1
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• pp.86-96
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• 2013

The realtime monitoring of radon ($^{222}Rn$) concentrations has been carried out from Gosan site, Jeju Island for three years of 2006~2008, in order to evaluate the background level and timely variational characteristics of atmospheric radon. The mean concentration of radon measured during the studying period was $2965mBq/m^3$ with its annual mean values in the range of $2768{\sim}3124mBq/m^3$. The relative ordering of the seasonal mean concentrations was seemed to vary such as winter ($3578mBq/m^3$) > fall ($3351mBq/m^3$) > spring ($2832mBq/m^3$) > summer ($2073mBq/m^3$). The monthly mean concentrations were in the order of Jan>Feb>Oct>Nov>Dec>Mar> Sep>Apr>May>Jun>Aug>Jul, so that the highest January value ($3713mBq/m^3$) exceeded almost twice as the July minimum ($1946mBq/m^3$). The hourly concentrations in a day showed the highest level ($3356mBq/m^3$) at around 7 a.m., increasing during nighttime, while reaching the lowest ($2574mBq/m^3$) at around 3 p.m. From the backward trajectory analysis for a continental fetch of radon, the high concentrations (10%) of radon matched with the air mass moving from the Asia continent to Jeju area. In contrast, the low concentrations (10%) of radon were generally correlated with the air mass of the North Pacific Ocean. In comparison by sectional inflow pathways of air mass, the radon concentrations were relatively high from the north China and the Korean peninsula.

• Journal of Korean Society for Atmospheric Environment
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• v.34 no.2
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• pp.321-330
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• 2018

Concentrations of the atmospheric radon and gaseous pollutants were measured at the Gosan site on Jeju Island from 2010 to 2015, in order to observe their time-series variation characteristics and examine the concentration change related to the airflow transport pathways. Based on the realtime monitoring of the atmospheric radon and gaseous pollutants, the daily mean concentrations of radon ($^{222}Rn$) and gaseous pollutants($SO_2$, CO, $O_3$, $NO_x$) were $2,400mBq\;m^{-3}$ and 1.3, 377.6, 41.1, 3.9 ppb, respectively. On monthly variations of radon, the mean concentration in October was the highest as $3,033mBq\;m^{-3}$, almost twice as that in July ($1,452mBq\;m^{-3}$). The diurnal variation of radon concentration shows bimodal curves at early morning (around 7 a.m.) and near midnight, whereas its lowest concentration was recorded at around 3 p.m. Several gaseous pollutants($SO_2$, CO, $NO_x$) showed a similar seasonal variation with radon concentration as high in winter and low in summer, whereas the $O_3$ concentrations had a bit different seasonal trend. According to the cluster back trajectory analysis, the frequencies of airflow pathways moving from continental North China, East China, Japan and the East Sea, the Korean Peninsula, and North Pacific Ocean routes were 36, 37, 10, 13, and 4%, respectively. When the airflow were moved to Jeju Island from continental China, the concentrations of radon and gaseous pollutants were relatively high. On the other hand, when the airflows were moved from North Pacific Ocean and East Sea, their concentrations were much lower than those from continental China.

• Economic and Environmental Geology
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• v.30 no.1
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• pp.51-60
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• 1997

The high radon (Rn222) potentials of soil, groundwater, hotspring and indoor environments in the Taejon city area were delineated by use of an EDA RDA-200 radon detector. The U and Th contents were also analysed using a Multi Channel Analyzer to illustrate the sources of the radon potentials. The average U concentrations in Taejon vary according to the type of granites such as $4.14{\pm}2.36ppm$ in schistose granite (SG), $3.13{\pm}1.70ppm$ in biotite granite (BG) and $3.01{\pm}1.95ppm$ in two mica granite (TG). The U contents in the granites are closely related with the amounts of uraniferous minerals. However, the U contents in the soil are found to be $5.05{\pm}4.75ppm$ in TG, $4.07{\pm}1.69ppm$ in BG and $3.87{\pm}1.91ppm$ in SG which are mainly explained by the different cation exchange capacities (CEC) of the soils from various granites. The levels of soil radon are $552{\pm}656pCi/l$ in SG, in which levels at two locations exceed the level of 1,350 pCi/l established as guideline for follow-up action by the U.S. Environmental Protection Agency (EPA), $443{\pm}284pCi/l$ in TG and $224{\pm}115pCi/l$ in the BG. The soil radon concentrations are found to be proportional to the U content and hardness of the soils. The groundwater radon concentrations in the domestic wells of - 30~-100 m depth show that $6,907{\pm}4,665pCi/l$ in TG, $5,503{\pm}6,551pCi/l$ in SG and $2,104{\pm}1,157pCi/l$ in BG which are positively related with U contents in soils. The radon levels of six groundwater wells in TG and two in SG are greater than guideline for drinking water level, 10,000 pCi/l by EPA (1986). Average radon contents of hotsprings and public bathes in the TG area are $7,071{\pm}1,942pCi/l$ and $1,638{\pm}709pCi/l$, respectively, which are below the EPA standard for remedial action value of the 10,000 pCi/l. The mean indoor radon concentrations of the TG and SG areas are $1.60{\pm}1.20pCi/l$ and $1.60{\pm}0.70pCi/l$, respectively. The elevated indoor radon levels of 5.6 pCi/l and 6.7 pCi/l are found to be particularly in TG area, which exceeds 4 pCi/i guideline, correlating positively with the U contents in the soil and radon concentration in the groundwater.