• Title/Summary/Keyword: $^{137}Cs$ 농도

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선택성 이온교환수지에 의한 Cs 함유 토양 제염폐액 정화

  • 원휘준;김계남;오원진;정종헌
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2004.06a
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    • pp.131-132
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    • 2004
  • 원자력연구소에 보관 중인 오염 토양폐기물을 토양 세척법으로 제염하여 비 방사성폐기물화 한다면 그 부피를 10% 이하로 저감시킬 수 있으며 연구소의 고체 방사성폐기물 저장 용량을 크게 늘릴 수 있다. 1988년 발견 당시 오염 토양 폐기물의 주요 방사성 핵종은 Co-60 이었는데 시간경과에 따라 Cs-134, 137 이 주요 방사성 핵종이 되었다. 오염토양 폐기물의 60 % 이상은 방사능 농도가 극히 낮아 물리적으로 입도를 분리하거나 수 세척에 의해 비 방사성폐기물화 할 수 있음을 파악하였다.(중략)

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Trial Burns of Low-Level Radioactive Wastes the Demonstration-Scale Incineration Plant at KAERI (한국원자력 연구소 실증소각시설에서의 저준위방사성폐기물 시험소각)

  • Yang, Hee-Chul;Kim, In-Tae;Kim, Jeong-Guk;Kim, Joon-Hyung;Seo, Yong-Chil
    • Nuclear Engineering and Technology
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    • v.27 no.5
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    • pp.767-774
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    • 1995
  • Behavior of radionuclides such $^{60}$ Co, $^{54}$ Mn and $^{137}$ Cs in the incineration Process was Studied by trial burns of simulated wastes with radio-isotope tracers. Behavior of nonvolatiles, $^{60}$ Co and $^{54}$ Mn, was similar to that of particulate matters in the process. Decontamination factors(DFs) for $^{60}$ Co and $^{54}$ Mn were 4.7$\times$10$^{5}$ and 6.2$\times$10$^{5}$ , respectively. Behavior of semivolatile radio-isotope, $^{137}$ Cs, was temperature dependent. DFs for $^{l37}$Cs at In different incineration temperature of 85$0^{\circ}C$ and $700^{\circ}C$ were 2.8$\times$10$^3$ and 2.6$\times$10$^4$, respectively. Trial bums of dry active waste(DAW) transported from nuclear power station(NPS) Kori 3,4 were also performed. DF for gross $\beta$/${\gamma}$ radioactivity in DAW was 1.1$\times$10$^{5}$ . This was a little higher than the estimated value, which was calculated from the tracer test results and nuclides distribution in the DAW. Average emission concentration was 0.019 Bq/N $m^3$, which could meet the maximal permissible concentration(MPC) in stack emission.n.

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Treatment of Radioactive Liquid Waste Using Natural Evaporator and Resulted Exposure Dose Assessment (증발을 이용한 방사성 액체폐기물의 처리와 피폭선량평가)

  • Jeong, Gyeong-Hwan;Park, Seung-Kook;Kim, Eun-Han;Jung, Ki-Jung;Park, Hyun-Soo
    • Journal of Radiation Protection and Research
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    • v.24 no.2
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    • pp.101-108
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    • 1999
  • The influence of the relative humidity, the temperature and the velocity of supply air on evaporation rate has been studied with non-boiling forced evaporation system in order to treat very low level radioactive liquid wastes produced from the decontamination and decommissioning activities. Experimental data on the evaporation rate have been obtained with the divers variables and experimental equation of air velocity was also obtained by the correlation of those data. The decontamination factor of this system was also obtained by the experimental data from a simulated liquid waste containing Cs-137 radio isotope ; $DF=10^4$. Since the commercial system will be operated for the treatment of the very low level radioactive liquid waste produced from decontamination & decommissioning of TRIGA Mark-II&III research reactor, the environmental assessment has been conducted to improve the operational safety. Exposure dose rate for an individual member of general public was assessed, and it showed that it was very lower than individual dose limits. The release of radioactivity of radioisotope material (Cs-137) to the environment was assessed, and result showed that it was $4.637{\times}10^{-14}\;{\mu}Ci/cc$.

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Variations in Soil-to-Red Pepper Transfer Factors of Radionuclides with Time of Their Application and Fruit Harvest (고추 재배시 방사성 핵종 처리 및 열매수확 시기에 따른 토양-작물체간 전이계수의 변이)

  • Choi, Yong-Ho;Lee, Won-Yun;Lim, Kwang-Muk;Park, Doo-Won;Lee, Myung-Ho;Lee, Chang-Woo;Lee, Hyun-Duk;Lee, Jeong-Ho
    • Journal of Radiation Protection and Research
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    • v.22 no.3
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    • pp.171-181
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    • 1997
  • A mixed solution of $^{54}Mn$, $^{60}Co$, $^{85}Sr$ and $^{137}Cs$ was applied to the soil of culture boxes in a greenhouse 2 days before transplanting red pepper and at 3 different times during its growth for investigating transfer factors ($m^2/kg-dry$) for its green and red fruits. Transfer factors varied with radionuclide, application time and harvest time by factors of about $20{\sim}100$. They decreased mostly in the order of $^{85}Sr>^{54}Min>^{60}Co>^{137}Cs$ while $^{54}Mn$ and $^{60}Co$ was higher than $^{85}Sr$ when time lapse between application and harvest was short. Transfer factors of $^{85}Sr$ and $^{137}Cs$ at the last application were lower than those at the previous one by factors of $3{\sim}20$ depending on harvest time. Variations in $^{54}Mn$ and $^{60}Co$ transfer factors with application time after transplanting were comparatively low. Transfer factors of $^{54}Mn$, $^{60}Co$ and $^{85}Sr$ mixed with topsoil before transplanting were up to $3{\sim}9$ times higher than those for the application onto soil surface 2 days after transplanting while there was no difference in $^{137}Cs$. The present results can be referred to in estimating root-uptake concentrations of the radionuclides in red pepper fruit and taking proper measures for its harvest and consumption at the event of an accidental release during the growing season of red pepper.

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Scintillation Characteristics of CsI(Li) Single Crystals (CsI(Li) 단결정의 섬광특성)

  • Lee, W.G.;Doh, S.H.;Ro, T.I.;Kim, W.;Kang, H.D.;Moon, B.S.
    • Journal of Sensor Science and Technology
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    • v.8 no.5
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    • pp.359-367
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    • 1999
  • CsI(Li) single crystals doped with 0.02, 0.1, 0.2 and 0.3 mole% lithium as an activator were grown by Czochralski method. The lattice structure of grown CsI(Li) single crystal was bcc, its lattice constant was $4.568\;{\AA}$. The absorption edge of CsI(Li) single crystal was 245 nm, and the spectral range of luminescence was $300{\sim}600\;nm$, its maximum luminescence intensity appeared at 425 nm. The energy resolutions of CsI(Li) single crystal doped with 0.2 mole% lithium were 14.5% for $^{137}Cs$(662 keV), 11.4% for $^{54}Mn$(835 keV) and 17.7% and 7.9% for $^{22}Na$(511 keV and 1275 keV), respectively. The relation formula of $\gamma$-ray energy versus energy resolution was ln (FWHM%) = -0.893lnE + 8.456 and energy calibration formula was ${\log}E_r=1.455\;{\log}(ch.)-1.277$. The phosphorescence decay time of CsI(Li) crystal doped with 0.2 mole% lithium was 0.51 s at room temperature, and its time resolution measured by CFT(constant-fraction timing method) was 9.0 ns.

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Radioactivity Analysis for Reliability Assessment in the Environmental Samples (환경 시료 중 신뢰도 검증을 위한 방사능 분석)

  • Kang, Tae-Woo;Hong, Kyung-Ae
    • Korean Journal of Environmental Agriculture
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    • v.26 no.2
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    • pp.186-191
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    • 2007
  • The objective of this research was to assess the reliability of data and to improve nuclear analytical techniques concerning the Domestic Radioactivity Intercomparison program for environmental radioactivity monitoring of Jeju from 1998 to 2006. Gross beta for filter papers and water samples was determined, and gamma nuclides for natural and artificial nuclides in soil and water samples were analyzed. The gross beta activity of all samples except for the water samples of 1998 and 1999 showed a good agreement within the confidence intervals. In gamma nuclides, $^{40}K$ and $^{137}Cs$ of soil samples and most nuclides in the water samples, with the exception of several nuclides, were evaluated to be reliable. Based on these results, it is considered that a reliable method for the analysis and monitoring of environmental radioactivity were established, which may play an important role in case of emergency radiation accident.

고순도게르마늄(HPGe) 검출기를 이용한 방사성폐기물 드럼의 핵종농도 평가

  • 박경록;강덕원
    • Proceedings of the Korean Nuclear Society Conference
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    • 1996.11b
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    • pp.583-589
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    • 1996
  • 원자력발전소에서 발생되는 방사성폐기물들은 폐기물형태 및 방사능 농도가 다양하며 영구처분장으로 이송전까지는 발전소내의 임시 저장고에 안전하게 보관, 관리하고 있다. 생성된 폐기물드럼내에는 감마방출핵종을 비롯하여 알파 및 베타방출 핵종들이 균질 또는 비균질하게 존재하고 있으며 방사능의 세기나 폐기물의 특성에 따라 안정화시키거나 압축처리하여 드럼에 담겨져 있기 때문에 일반적인 파괴분석에 의한 화학분석법으로는 작업자의 피폭, 시료의 대표성 선정 및 장시간의 화학처리 시간소요 등으로 핵종분석이 곤란하다. 따라서 본 논문은 일반적으로 감마핵종분석시 흔히 사용하고 있는 고순도게르마늄(HPGe) 검출기를 이용하여 드럼의 감마핵종농도를 분석하는 방법과 장치의 개발에 대해 언급하였으며 알파나 베타핵종과 같이 직접 분석이 곤란한 핵종들은 각 폐기물드럼내에 존재하는 Co-60이나 Cs-137과의 상관관계를 미리 예측한 척도인자 (scaling factor)를 이용하여 간접적으로 구하는 방법을 사용하고 있으나 본 논문에서는 드럼으로부터 감마핵종만을 분석하는 방법에 대해서만 언급하였다. 또한 핵종분석시스템의 최적 운전조건을 도출하기 위해 드럼회전테이블의 속도결정 및 모의드럼을 이용한 방사능측정 등을 통해 핵종 농도 분석시의 오차를 30% 이내로 유지할 수 있었다.

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Improvement on the Method of Estimating Radionuclide Concentrations in Agricultural Products for the Off-Site Internal Dose Calculation for Operating Nuclear Facilities (가동중 원자력 시설 주변 주민의 내부피폭선량 계산을 위한 농산물내 핵종 농도 평가법 개선)

  • Choi, Y.H.;Lim, K.M.;Hwang, W.T.;Choi, G.S.;Choi, H.J.;Lee, C.W.
    • Journal of Radiation Protection and Research
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    • v.29 no.2
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    • pp.73-90
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    • 2004
  • The Reg. Guide 1.109 model was reviewed against its applicability to calculating radionuclide concentrations in agricultural products for operating nuclear facilities and an improved method was proposed. The model was so modified that the radionuclides deposited since the start of operation could be considered in assessing the root uptake. Translocation factors were introduced in the equation for calculating the concentrations in edible parts due to direct plant deposition. Values specific to Korea were set up for the input parameters of the modified model. The concentrations of $^{54}Mn,\;^{60}Co,\;^{90}Sr\;and\;^{137}Cs$ in rice seeds, Chinese cabbage and radish root were calculated for various hypothetical deposition histories using the Reg. Guide 1.109 model and the modified model with parameter values in the guide and those specific to Korea put in alternately. Through comparisons among the results, it could be expected that the use of the modified model with the input of parameter values specific to Korea would result In a more resonable and realistic assessment.

Radionuclides in Environmental Samples and Sample Concentration of Land in the Analysis in the Method of Direct (직접법에서 환경시료중 육상시료의 방사성 핵종 및 농도 분석)

  • Jang, Eun-Sung;Kim, Jin-Seop
    • Journal of Environmental Science International
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    • v.24 no.3
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    • pp.275-280
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    • 2015
  • In order to measure the Radionuclides and Concentration, the directly grinded land samples (river soil, pine leaves and mugwort) among the environment samples around the nuclear power plant were filled in a 450 mL Marinelli beaker and weighed to obtain the dry mass ratio of the samples. Then the background and land samples were measured for 80,000 sec. The analysis of the collected land samples showed that most of them contained less radiation nuclide than the detection minimum limit in the 'Ministry of Education, Science and Technology Public Notice No. 2010-32.'In others, the natural radionuclides $^{40}K$ were detected. Of the products of nuclear reaction discharged by a nuclear reaction, $^{134}Cs$ and $^{137}Cs$ are more easily detected, and their discharge sources can be traced using the relative ratio. Although the radioactive concentration in the vicinity of Kori Nuclear Power Plant, which is more than 1,100km away from Fukushima, the Japanese nuclear accident site, continuous monitoring is needed as the radionuclides can still be accumulated in the soil or animals and plants.

Modeling Study on Nuclide Transport in Ocean - an Ocean Compartment Model (해양에서의 핵종이동 모델링 - 해양구획 모델)

  • Lee, Youn-Myoung;Suh, Kyung-Suk;Han, Kyong-Won
    • Nuclear Engineering and Technology
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    • v.23 no.4
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    • pp.387-400
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    • 1991
  • An ocean compartment model simulating transport of nuclides by advection due to ocean circulation and intertaction with suspended sediments is developed, by which concentration breakthrough curves of nuclides can be calculated as a function of time. Dividing ocean into arbitrary number of characteristic compartments and performing a balance of mass of nuclides in each ocean compartment, the governing equation for the concentration in the ocean is obtained and a solution by the numerical integration is obtained. The integration method is specially useful for general stiff systems. For transfer coefficients describing advective transport between adjacent compartments by ocean circulation, the ocean turnover time is calculated by a two-dimensional numerical ocean model. To exemplify the compartment model, a reference case calculation for breakthrough curves of three nuclides in low-level radioactive wastes, Tc-99, Cs-137, and Pu-238 released from hypothetical repository under the seabed is carried out with five ocean compartments. Sensitivity analysis studies for some parameters to the concentration breakthrough curves are also made, which indicates that parameters such as ocean turnover time and ocean water volume of compartments have an important effect on the breakthrough curves.

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